Stabilizing global climate change to within 1.5℃requires a reduction in greenhouse gas emissions,with a primary focus on carbon dioxide(CO_(2))emissions.CO_(2)flooding in oilfields has recently been recognized as an ...Stabilizing global climate change to within 1.5℃requires a reduction in greenhouse gas emissions,with a primary focus on carbon dioxide(CO_(2))emissions.CO_(2)flooding in oilfields has recently been recognized as an important way to reduce CO_(2)emissions by storing CO_(2)in oil reservoirs.This work proposes an advanced CO_(2)enhanced oil recovery(EOR)method-namely,storage-driven CO_(2)EOR-whose main target is to realize net-zero or even negative CO_(2)emissions by sequestrating the maximum possible amount of CO_(2)in oil reservoirs while accomplishing the maximum possible oil recovery.Here,dimethyl ether(DME)is employed as an efficient agent in assisting conventional CO_(2)EOR for oil recovery while enhancing CO_(2)sequestration in reservoirs.The results show that DME improves the solubility of CO_(2)in in situ oil,which is beneficial for the solubility trapping of CO_(2)storage;furthermore,the presence of DME inhibits the"escape"of lighter hydrocarbons from crude oil due to the CO_(2)extraction effect,which is critical for sustainable oil recovery.Sto rage-driven CO_(2)EOR is superior to conventional CO_(2)EOR in improving sweeping efficiency,especially during the late oil production period.This work demonstrates that storage-driven CO_(2)EOR exhibits higher oil-in-place(OIP)recovery than conventional CO_(2)EOR.Moreover,the amount of sequestrated CO_(2)in storage-driven CO_(2)EOR exceeds the amount of emissions from burning the produced oil;that is,the sequestrated CO_(2)offsets not only current emissions but also past CO_(2)emissions.By altering developing scenarios,such as water alternating storage-driven CO_(2)EOR,more CO_(2)sequestration and higher oil recovery can be achieved.This work demonstrates the potential utilization of DME as an efficient additive to CO_(2)for enhancing oil recovery while improving CO_(2)storage in oil reservoirs.展开更多
基金financial support from the Science Foundation of China University of Petroleum,Beijing(2462021QNXZ012 and 2462021YJRC012)supported by the Fundamental Research Funds for the Central Universities。
文摘Stabilizing global climate change to within 1.5℃requires a reduction in greenhouse gas emissions,with a primary focus on carbon dioxide(CO_(2))emissions.CO_(2)flooding in oilfields has recently been recognized as an important way to reduce CO_(2)emissions by storing CO_(2)in oil reservoirs.This work proposes an advanced CO_(2)enhanced oil recovery(EOR)method-namely,storage-driven CO_(2)EOR-whose main target is to realize net-zero or even negative CO_(2)emissions by sequestrating the maximum possible amount of CO_(2)in oil reservoirs while accomplishing the maximum possible oil recovery.Here,dimethyl ether(DME)is employed as an efficient agent in assisting conventional CO_(2)EOR for oil recovery while enhancing CO_(2)sequestration in reservoirs.The results show that DME improves the solubility of CO_(2)in in situ oil,which is beneficial for the solubility trapping of CO_(2)storage;furthermore,the presence of DME inhibits the"escape"of lighter hydrocarbons from crude oil due to the CO_(2)extraction effect,which is critical for sustainable oil recovery.Sto rage-driven CO_(2)EOR is superior to conventional CO_(2)EOR in improving sweeping efficiency,especially during the late oil production period.This work demonstrates that storage-driven CO_(2)EOR exhibits higher oil-in-place(OIP)recovery than conventional CO_(2)EOR.Moreover,the amount of sequestrated CO_(2)in storage-driven CO_(2)EOR exceeds the amount of emissions from burning the produced oil;that is,the sequestrated CO_(2)offsets not only current emissions but also past CO_(2)emissions.By altering developing scenarios,such as water alternating storage-driven CO_(2)EOR,more CO_(2)sequestration and higher oil recovery can be achieved.This work demonstrates the potential utilization of DME as an efficient additive to CO_(2)for enhancing oil recovery while improving CO_(2)storage in oil reservoirs.