The caesium atomic fountain clock is a primary frequency standard.During its operation,a Majorana transition frequency shift will occur once a magnetic field at some special locations along the atomic trajectory is si...The caesium atomic fountain clock is a primary frequency standard.During its operation,a Majorana transition frequency shift will occur once a magnetic field at some special locations along the atomic trajectory is singular.In this study,by developing a physical model,we analyzed the magnetic field requirements for atomic adiabatic transition and calculated the influence of the Majorana atomic transition on the atomic state via a quantum method.Based on the simulation results for the magnetic field in the fountain clock,we applied the Monte Carlo method to simulate the relationship between the Majorana transition frequency shift and the magnetic field at the entrance of the magnetic shielding,as well as the initial atomic population.Measurement of the Majorana transition frequency shift was realized by state-selecting asymmetrically populated atoms.The relationship between the Majorana transition frequency shift and the axial magnetic field at the entrance of the magnetic shielding was obtained.The measured results were essentially consistent with the calculated results.Thus,the magnetic field at the entrance of the magnetic shielding was configured,and the Majorana transition frequency shift of the fountain clock was calculated to be 4.57×10^(-18).展开更多
With a coupling laser locked to caesium 6S1/2 Fg=4-6P3/2 Fe=5 cycling transition and a co-propagating probe laser scanned across 6S1/2 Fg=4-6Pa/2 Fe=3, 4 and 5 transitions, a novel scheme for sub-Doppler spectra in Do...With a coupling laser locked to caesium 6S1/2 Fg=4-6P3/2 Fe=5 cycling transition and a co-propagating probe laser scanned across 6S1/2 Fg=4-6Pa/2 Fe=3, 4 and 5 transitions, a novel scheme for sub-Doppler spectra in Dopplerbroadened V-type three-level system is demonstrated by detecting the transmission of the coupling laser through a caesium vapour cell. The Autler-Townes doublet in the sub-Doppler spectra of the coupling laser is clearly observed. The effects of coupling laser intensity on the splitting and linewidth of the Autler-Townes doublet are experimentally investigated and the results agree well with theoretical predictions. Taking the multiple hyperfine levels of caesium atom into account, a brief analysis is presented.展开更多
The activity of caesium-137 （Bq/kg） in the crustaceous lichens and other samples was determined to prove the feasibility that crustaceous lichens work as a sensitive biology monitor to record the caesium-137 （Bq/kg...The activity of caesium-137 （Bq/kg） in the crustaceous lichens and other samples was determined to prove the feasibility that crustaceous lichens work as a sensitive biology monitor to record the caesium-137 （Bq/kg） radiation levels of terrestrial environment. The measurements were performed with GEM series HPGe （ high-purity Germanium） coaxial detector system （ADCAM -100 ） made by EC ＆ GORTEC Company in USA. It was found that the activity of caesium-137 （Bq/kg） in the crustaceous lichens was one order of magnitude higher than that found in surface soil, and was over throe orders of magnitude higher than those found in the familiar biological samples. These results proved that crustaceous lichens may be one of the most sensitive biological monitors about the remote transmission and environmental radiation levels of caesium-137.展开更多
Recently, much attention has been focused on the use of neutral carrier species as membrane components to extract ions from aqueous solution into a hydrophobic membrane phase. Some potassium-or caesium-selective elect...Recently, much attention has been focused on the use of neutral carrier species as membrane components to extract ions from aqueous solution into a hydrophobic membrane phase. Some potassium-or caesium-selective electrodes based on bis-benzo-15-crown-5 or bis-benzo-18-crown-6 containing ester or other linkage were prepared by K. Kimura and K. W. Fung. The selective coefficients K;, K;,or K;, K were 2.6×10;, 1.9×10;and 1.7×10;, respectively.展开更多
In this paper the generation of four-wave mixing （FWM） signal using a noncycling transition of caesium atoms is investigated when the pumping laser is locked to the transition 6S1/2F= 4→6P3/2^F1 = 4, and meanwhile ...In this paper the generation of four-wave mixing （FWM） signal using a noncycling transition of caesium atoms is investigated when the pumping laser is locked to the transition 6S1/2F= 4→6P3/2^F1 = 4, and meanwhile the probe frequency is scanned across the 6S1/2F = 4→6P3/2 transition. The efficiency of the four-wave mixing signal as a function of the intensity of the pumping beams and the detuning of the pumping beams is also studied. In order to increase the detection efficiency, a repumping laser which is resonant with 6S1/2F = 3→6P3/2F′= 4 transition is used. A theoretical model is also introduced, and the theoretical results are in qualitative agreement with experimental ones.展开更多
Based on fundamental research, we developed the basic scheme of a decontamination setup to remove acid gases (HCl, SO2, NOx) from steam-air flows with simultaneous localization of radioactive aerosols, including aeros...Based on fundamental research, we developed the basic scheme of a decontamination setup to remove acid gases (HCl, SO2, NOx) from steam-air flows with simultaneous localization of radioactive aerosols, including aerosols with a particle size of less than 0.1 μm and volatile radioactive iodine compounds. The decontamination process is based on the method of the agglomeration cocrystallization of finely dispersed and other aerosols in the gas phase by including the aerosols in the inner structure of large-particle non-radioactive aerosols of ammonium salts, for example, NH4Cl or (NH4)2SO3. For 137Cs, the most ecologically dangerous long-lived radionuclide, the setup ensures a decontamination factor of 102 to 103 in one decontamination stage. Because the setup consists of three consecutive stages of the same type, the cumulative decontamination factor can reach to 106 - 107. To localize radioactive iodine as I2, HI, HOI, HIO3, and CH3I from vapor-air flows, the setup uses a unit containing special granulated sorbents based on inorganic compounds. Developed at the Institute of Physical Chemistry, Russian Academy of Sciences, these sorbents effectively remove various radioactive iodine species (inorganic species and methyl iodide) from steam-air flows, ensuring decontamination factors of at least 104. The proposed technological scheme will allow vapor-gas flows to be cleaned of radioaerosols and all volatile radioactive iodine species at decontamination factors of not less than 104.展开更多
The existing traditional methods of assessing the rates of soil loss have many limitations and are difficult to apply in the karst areas of Southwest China. Karst depressions comprise geomorphologically important sour...The existing traditional methods of assessing the rates of soil loss have many limitations and are difficult to apply in the karst areas of Southwest China. Karst depressions comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of many depressions is not well understood. In this paper, the 137Cs technique was employed to investigate recent sedimentation rates in a Chinese polygonal karst depression. The results indicated that the sediment deposition rates ranged from 0.91 to 1.97 mm?a?1 in the period from 1963 to 2007, and the average sediment deposition rate and specific deposit yield of the catchment were estimated to be 1.47 mm?a?1 and 20 t?km?2?a?1, respectively. The results obtained were consistent with the local monitoring data of runoff plots, confirming the validity of the overall approach. It was shown that soil loss rates were very low in some karst areas of Southwest China. Above all, the approach appears to offer valuable potential to study surface erosion by estimating sediment deposition rates of karst depressions, rather than the assessment of complicated soil erosion in stony soils of carbonate rock slopes. In addition, the spacial distribution of surface soil and 137Cs inventories was affected remarkably by the inhomogeneous dissolution of limestone under the soil. It may be an important phenomenon which exists widely in the karst areas and is significantly different from other places.展开更多
After the damage of Fukushima Daiichi Nuclear Power Plant, a great number of radioactive materials were released into the Pacific Ocean. Therefore, it is necessary to research on the temporal and spatial distribution ...After the damage of Fukushima Daiichi Nuclear Power Plant, a great number of radioactive materials were released into the Pacific Ocean. Therefore, it is necessary to research on the temporal and spatial distribution of these radionuclides. We use Princeton Ocean Model to simulate the circulation of the coast water of Fukushima NPP and obtain the concentration of caesium-137 by solving the diffusion equations. We employ the Monte Carlo N-particle(MCNP) code to assess the external doses caused by these contaminated sea water. To improve the efficiency and effectiveness of volume source in MCNP code, we establish a transformation method between spot source and volume source, and determine an appropriate range of volume source. Finally, we calculate the absorbed doses of every organ/tissue and the effective dose of a human body.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.12173044)Research and Development Project of Scientific Research Instruments and Equipment of Chinese Academy of Sciences(Grant No.YJKYYQ20200020)+1 种基金Large Research Infrastructures Improvement Funds of Chinese Academy of Sciences(Grant No.DSS-WXGZ-2020-0005)Chinese Academy of Sciences for Western Young Scholars(Grant Nos.XAB2018A06,XAB2019A07,and XAB2018B16)。
文摘The caesium atomic fountain clock is a primary frequency standard.During its operation,a Majorana transition frequency shift will occur once a magnetic field at some special locations along the atomic trajectory is singular.In this study,by developing a physical model,we analyzed the magnetic field requirements for atomic adiabatic transition and calculated the influence of the Majorana atomic transition on the atomic state via a quantum method.Based on the simulation results for the magnetic field in the fountain clock,we applied the Monte Carlo method to simulate the relationship between the Majorana transition frequency shift and the magnetic field at the entrance of the magnetic shielding,as well as the initial atomic population.Measurement of the Majorana transition frequency shift was realized by state-selecting asymmetrically populated atoms.The relationship between the Majorana transition frequency shift and the axial magnetic field at the entrance of the magnetic shielding was obtained.The measured results were essentially consistent with the calculated results.Thus,the magnetic field at the entrance of the magnetic shielding was configured,and the Majorana transition frequency shift of the fountain clock was calculated to be 4.57×10^(-18).
基金Project supported by the National Natural Science Foundation of China （Grant Nos 60578018, 10434080 and 10374062）, by the Key Scientific Program of Education Ministry of China （Grant No 204019）, and by the Research Funds for Youth Academic Leaders of Shanxi Province, China.
文摘With a coupling laser locked to caesium 6S1/2 Fg=4-6P3/2 Fe=5 cycling transition and a co-propagating probe laser scanned across 6S1/2 Fg=4-6Pa/2 Fe=3, 4 and 5 transitions, a novel scheme for sub-Doppler spectra in Dopplerbroadened V-type three-level system is demonstrated by detecting the transmission of the coupling laser through a caesium vapour cell. The Autler-Townes doublet in the sub-Doppler spectra of the coupling laser is clearly observed. The effects of coupling laser intensity on the splitting and linewidth of the Autler-Townes doublet are experimentally investigated and the results agree well with theoretical predictions. Taking the multiple hyperfine levels of caesium atom into account, a brief analysis is presented.
文摘The activity of caesium-137 （Bq/kg） in the crustaceous lichens and other samples was determined to prove the feasibility that crustaceous lichens work as a sensitive biology monitor to record the caesium-137 （Bq/kg） radiation levels of terrestrial environment. The measurements were performed with GEM series HPGe （ high-purity Germanium） coaxial detector system （ADCAM -100 ） made by EC ＆ GORTEC Company in USA. It was found that the activity of caesium-137 （Bq/kg） in the crustaceous lichens was one order of magnitude higher than that found in surface soil, and was over throe orders of magnitude higher than those found in the familiar biological samples. These results proved that crustaceous lichens may be one of the most sensitive biological monitors about the remote transmission and environmental radiation levels of caesium-137.
基金Supported by the National Natural Science Foundation of China
文摘Recently, much attention has been focused on the use of neutral carrier species as membrane components to extract ions from aqueous solution into a hydrophobic membrane phase. Some potassium-or caesium-selective electrodes based on bis-benzo-15-crown-5 or bis-benzo-18-crown-6 containing ester or other linkage were prepared by K. Kimura and K. W. Fung. The selective coefficients K;, K;,or K;, K were 2.6×10;, 1.9×10;and 1.7×10;, respectively.
基金Project supported by the National Natural Science Foundation of China （Grant No 60378004） and the Youth Science Foundation of Shanxi Province,China （Grant Nos 20031004 and 20041013）.
文摘In this paper the generation of four-wave mixing （FWM） signal using a noncycling transition of caesium atoms is investigated when the pumping laser is locked to the transition 6S1/2F= 4→6P3/2^F1 = 4, and meanwhile the probe frequency is scanned across the 6S1/2F = 4→6P3/2 transition. The efficiency of the four-wave mixing signal as a function of the intensity of the pumping beams and the detuning of the pumping beams is also studied. In order to increase the detection efficiency, a repumping laser which is resonant with 6S1/2F = 3→6P3/2F′= 4 transition is used. A theoretical model is also introduced, and the theoretical results are in qualitative agreement with experimental ones.
文摘Based on fundamental research, we developed the basic scheme of a decontamination setup to remove acid gases (HCl, SO2, NOx) from steam-air flows with simultaneous localization of radioactive aerosols, including aerosols with a particle size of less than 0.1 μm and volatile radioactive iodine compounds. The decontamination process is based on the method of the agglomeration cocrystallization of finely dispersed and other aerosols in the gas phase by including the aerosols in the inner structure of large-particle non-radioactive aerosols of ammonium salts, for example, NH4Cl or (NH4)2SO3. For 137Cs, the most ecologically dangerous long-lived radionuclide, the setup ensures a decontamination factor of 102 to 103 in one decontamination stage. Because the setup consists of three consecutive stages of the same type, the cumulative decontamination factor can reach to 106 - 107. To localize radioactive iodine as I2, HI, HOI, HIO3, and CH3I from vapor-air flows, the setup uses a unit containing special granulated sorbents based on inorganic compounds. Developed at the Institute of Physical Chemistry, Russian Academy of Sciences, these sorbents effectively remove various radioactive iodine species (inorganic species and methyl iodide) from steam-air flows, ensuring decontamination factors of at least 104. The proposed technological scheme will allow vapor-gas flows to be cleaned of radioaerosols and all volatile radioactive iodine species at decontamination factors of not less than 104.
基金supported by the National Basic Research Program of China (973 Program) (Grant No. 2006CB403200)the National Natural Science Foundation of China(Grant No. 41001162)+3 种基金Knowledge Inno-vation Project of the Chinese Academy of Sciences (Grant No. KZCX2-YW-306)Provincial Governor Foundation of GuiZhou (Grant No. 2010)Opening Fund of State Key Labo-ratory of Environmental Geochemistry(Grant No. SKLEG9008)National Key Technology R & D Program (Grant Nos. 2006BAC01A09 and 2008BAD98B07)
文摘The existing traditional methods of assessing the rates of soil loss have many limitations and are difficult to apply in the karst areas of Southwest China. Karst depressions comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of many depressions is not well understood. In this paper, the 137Cs technique was employed to investigate recent sedimentation rates in a Chinese polygonal karst depression. The results indicated that the sediment deposition rates ranged from 0.91 to 1.97 mm?a?1 in the period from 1963 to 2007, and the average sediment deposition rate and specific deposit yield of the catchment were estimated to be 1.47 mm?a?1 and 20 t?km?2?a?1, respectively. The results obtained were consistent with the local monitoring data of runoff plots, confirming the validity of the overall approach. It was shown that soil loss rates were very low in some karst areas of Southwest China. Above all, the approach appears to offer valuable potential to study surface erosion by estimating sediment deposition rates of karst depressions, rather than the assessment of complicated soil erosion in stony soils of carbonate rock slopes. In addition, the spacial distribution of surface soil and 137Cs inventories was affected remarkably by the inhomogeneous dissolution of limestone under the soil. It may be an important phenomenon which exists widely in the karst areas and is significantly different from other places.
基金supported by the National Natural Science Foundation of China(Grant No.71373140)the State Key Laboratory of NBC Protection for Civilian(Grant No.SKLNBC0308)Tsinghua University Initiative Scientific Research Program(Grant Nos.2012Z10137,2012THZ0124)
文摘After the damage of Fukushima Daiichi Nuclear Power Plant, a great number of radioactive materials were released into the Pacific Ocean. Therefore, it is necessary to research on the temporal and spatial distribution of these radionuclides. We use Princeton Ocean Model to simulate the circulation of the coast water of Fukushima NPP and obtain the concentration of caesium-137 by solving the diffusion equations. We employ the Monte Carlo N-particle(MCNP) code to assess the external doses caused by these contaminated sea water. To improve the efficiency and effectiveness of volume source in MCNP code, we establish a transformation method between spot source and volume source, and determine an appropriate range of volume source. Finally, we calculate the absorbed doses of every organ/tissue and the effective dose of a human body.
