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SOME FEATURES OF CARBON CYCLES IN KARST SYSTEM AND THE IMPLICATION FOR EPIKARSTIFICATION —An Example of Yaji Karst Experimental Site in Guilin,China 被引量:15
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作者 Pan Genxing Tao Yuxiang Shun Yuhua Teng Yongzhong Han Fushun College of Resource & Environment Science,Nanjing Agricultural Univ.,Nanjing, 210095 People’s Republic of China 《Journal of Geographical Sciences》 SCIE CSCD 1997年第3期48-57,共10页
The carbon pools of biomass,littering,and SOC wre studied with regards to carbon cycles in epikarst zone,taking an example of Yaji Karst Experiemnt Site in Guilin.This study was focused on SOC and its lability,SOC dec... The carbon pools of biomass,littering,and SOC wre studied with regards to carbon cycles in epikarst zone,taking an example of Yaji Karst Experiemnt Site in Guilin.This study was focused on SOC and its lability,SOC decomposition rate,CO 2 regime in the soils. 13 ctracing was used to persua the relation of bicarbonate in karst water to soil carbon.The results indicated sufficient carbon pool in SOC for the driveing CO 2 in the karst system.It was revealed that about 60percent of carbon in epi-karst springs resulted from SOC during spring and summer.Thus,the CO 2,driving the karstification,was not simply due to adsorption of atmospheric CO 2 but due to carbon transfer through the pathway of air-plant-soil-water.The driving force should not be overlooked for the epi-karst formation by soil as an interface of carbon environmental geochemistry. 展开更多
关键词 carbon cycle carbon transfer EPIKARST SOC.
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Three-step modernization of the ocean:Modeling of carbon cycles and the revolution of ecological systems in the Ediacaran/Cambrian periods
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作者 Miyuki Tahata Yusuke Sawaki +5 位作者 Yuichiro Ueno Manabu Nishizawa Naohiro Yoshida Toshikazu Ebisuzaki Tsuyoshi Komiya Shigenori Maruyama 《Geoscience Frontiers》 SCIE CAS CSCD 2015年第1期121-136,共16页
Important ecological changes of the Earth (oxidization of the atmosphere and the ocean) increase in nutrient supply due to the break-up of the super continent (Rodinia) and the appearance of multi-cellular organis... Important ecological changes of the Earth (oxidization of the atmosphere and the ocean) increase in nutrient supply due to the break-up of the super continent (Rodinia) and the appearance of multi-cellular organisms (macroscopic algae and metazoan) took place in the Ediacaran period, priming the Cambrian explosion. The strong perturbations in carbon cycles in the ocean are recorded as excursions in carbonate and organic carbon isotope ratio (δ13Ccarb and δ13Corg) from the Ediacaran through early Cambrian periods. The Ediacaran-early Cambrian sediment records of δ13Ccarb and δ13Corg, obtained from the drill-core samples in Three Gorges in South China, are compared with the results of numerical simulation of a sim- ple one-zone model of the carbon cycle of the ocean, which has two reservoirs (i.e., dissolved organic carbon (DOC) and dissolved inorganic carbon (DIC). The fluxes from the reservoirs are assumed to be proportional to the mass of the carbon reservoirs. We constructed a model, referred to here as the Best Fit Model (BFM), which reproduce δ13Ccarb and δ13Corg records in the Ediacaran-early Cambrian period noted above. BFM reveals that the Shuram excursion is related to three major changes in the carbon cycle or the global ecological system of the Earth: (1) an increase in the coefficient of remineralization by a factor of ca. 100, possibly corresponding to a change in the dominant metabolism from anaerobic respiration to aerobic respiration, (2) an increase of carbon fractionation index from 25‰, to 33‰, possibly corresponding to the change in the primary producer from rock-living cyanobacteria to free-living macro algae, and (3) an in- crease in the coefficient of the organic carbon burial by a factor of ca. 100, possibly corresponding to the onset of a biological pump driven by the flourishing metazoan and zooplankton. The former two changes took place at the start of the Shuram excursion, while the third occurred at the end of the Shuram excursion. The other two excursions are explained by the tentative decrease in primary production due to cold periods, which correspond to the Gaskiers (ca. 580 Ma) and Bikonor (ca. 542 Ma) glaciations. 展开更多
关键词 carbon cycle change carbon isotope ratio Ediacaran to Cambrian Oxygen level Evolution of life
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Global Carbon Project (GCP) Beijing Office:a new bridge for understanding regional carbon cycles
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作者 TAO Bo CAO Mingkui YU Guirui LIU Jiyuan WANG Shaoqiang YAN Huimin 《Journal of Geographical Sciences》 SCIE CSCD 2006年第3期375-377,共3页
It has been widely accepted that human activities, especially burning fossil fuels and land use change, have altered the climate on earth and anthropogenic carbon fluxes have become comparable in magnitude with the na... It has been widely accepted that human activities, especially burning fossil fuels and land use change, have altered the climate on earth and anthropogenic carbon fluxes have become comparable in magnitude with the natural fluxes in the global carbon cycle. The present and potential threat of adverse consequences has focused the attention of the scientists, policy makers and general public on the interaction among carbon cycle, climate change and human system. Asia is a hot spot from environmental change and sustainable development perspectives. The development pathways and environmental changes in the region have obvious consequences for the regional carbon cycle, even for global carbon budget, and the complex, diverse social, economic and environmental conditions make it highly diffficult to understand and quantify these consequences. The GCP Beijing Office "will have a supporting and coordinating role and will provide coordination, leadership and capacity building on carbon cycle sciences in China and to the larger region of Asia" and "liaise with the two International Project Offices based in Canberra and Tsukuba to coordinate a regional and global strategy consistent with the GCP Science and Implementation Framework". 展开更多
关键词 GCP regional office carbon cycle China
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Summary of Recent Climate Change Studies on the Carbon and Nitrogen Cycles in the Terrestrial Ecosystem and Ocean in China 被引量:2
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作者 徐永福 黄耀 李阳春 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2012年第5期1027-1047,共21页
This article reviews recent advances over the past and their relationship to climate change in China. The was 0.19-0.26 Pg C yr-1 for the 1980s and 1990s. 4 years in the study of the carbon-nitrogen cycling net carbon... This article reviews recent advances over the past and their relationship to climate change in China. The was 0.19-0.26 Pg C yr-1 for the 1980s and 1990s. 4 years in the study of the carbon-nitrogen cycling net carbon sink in the Chinese terrestrial ecosystem Both natural wetlands and the rice-paddy regions emitted 1.76 Tg and 6.62 Tg of CH4 per year for the periods 1995 2004 and 2005 2009, respectively. China emitted -1.1 Tg N20-N yr-1 to the atmosphere in 2004. Land soil contained -8.3 Pg N. The excess nitrogen stored in farmland of the Yangtze River basin reached 1.51 Tg N and 2.67 Tg N in 1980 and 1990, respectively. The outer Yangtze Estuary served as a moderate or significant sink of atmospheric CO2 except in autumn. Phytoplankton could take up carbon at a rate of 6.4 ×1011 kg yr-1 in the China Sea. The global ocean absorbed anthropogenic CO2 at the rates of 1.64 and 1.73 Pg C yr-1 for two sinmlations in the 1990s. Land net ecosystem production in China would increase until the mid-21st century then would decrease gradually under future climate change scenarios. This research should be strengthened in the future, including collection of more observation data, measurement of the soil organic carbon (SOC) loss and sequestration, evaluation of changes in SOC in deep soil layers, and the impacts of grassland management, carbon-nitrogen coupled effects, and development and improvement of various component models and of the coupled carbon cycle-climate model. 展开更多
关键词 carbon cycle nitrogen cycle climate change Chinese terrestrial ecosystem China Sea
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Effects and underlying mechanisms of damming on carbon and nitrogen cycles and transport in rivers of Southwest China:project introduction 被引量:2
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作者 Hua-Yun Xiao 《Acta Geochimica》 EI CAS CSCD 2017年第4期577-580,共4页
Southwest China is the primary area for damming rivers to produce hydroelectric energy and store water.River damming has changed hydrodynamic,chemical,and biological processes,which are related to sinks and sources of... Southwest China is the primary area for damming rivers to produce hydroelectric energy and store water.River damming has changed hydrodynamic,chemical,and biological processes,which are related to sinks and sources of greenhouse gases and carbon and nitrogen fluxes of different interfaces.Here,I provide an introduction to a river damming-related foundation,the National Key R&D Program of China(2016YTA0601000).Supported by the foundation,we carried out research on multiprocesses/multi-interfaces of carbon and nitrogen biogeochemical cycles in a dammed river system and have produced important results,as presented in this issue of the journal. 展开更多
关键词 Damming carbon and nitrogen cycles Southwest Chinese rivers
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Effect of Carbonation and Drying-Wetting Cycles on Chloride Diffusion Behavior of Coral Aggregate Seawater Concrete 被引量:2
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作者 DA Bo LI Yipeng +4 位作者 YU Hongfa MA Haiyan CHEN Haoyu DOU Xuemei WU Zhangyu 《Journal of Ocean University of China》 SCIE CAS CSCD 2022年第1期113-123,共11页
Based on seawater immersion,drying-wetting cycles,carbonation and drying-wetting cycles for coral aggregate sea-water concrete(CASC)with different strength grades,the effect of carbonation and drying-wetting cycles on... Based on seawater immersion,drying-wetting cycles,carbonation and drying-wetting cycles for coral aggregate sea-water concrete(CASC)with different strength grades,the effect of carbonation and drying-wetting cycles on chloride diffusion be-havior of CASC is studied.The results show that the free surface chloride concentration(Cs),free chloride diffusion coefficient(Df)and time-dependent index(m)of CASC in the drying-wetting cycles is obviously higher than that in seawater immersion.The Df and m of CASC of carbonation and drying-wetting cycles is higher than that in the drying-wetting cycles.Carbonation increases the Df and m of CASC,which is against CASC to resist chloride corrosion.The corrosion possibility of CASC structures in different ex-posed areas is as follows:splash zone(carbonation and drying-wetting cycles)>tidal zone(drying-wetting cycles)>underwater zone(seawater immersion).Besides,the chloride diffusion rate of C65-CASC is 17.8%-63.4%higher than that of C65-ordinary aggre-gate concrete(OAC)in seawater immersion(underwater zone).Therefore,anti-corrosion measures should be adopted to improve the service life of CASC structure in the oceanic environment. 展开更多
关键词 coral aggregate seawater concrete chloride diffusion seawater immersion drying-wetting cycles carbonation and drying-wetting cycles
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Coral reef ecological pump for gathering and retaining nutrients and exporting carbon:a review and perspectives 被引量:1
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作者 Linbin Zhou Yehui Tan Liangmin Huang 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2023年第6期1-15,共15页
How coral reefs with high productivity and biodiversity can flourish in oligotrophic tropical oceans has inspired substantial research on coral reef ecosystems.Increasing evidence shows that similar to water in an oas... How coral reefs with high productivity and biodiversity can flourish in oligotrophic tropical oceans has inspired substantial research on coral reef ecosystems.Increasing evidence shows that similar to water in an oasis in the desert,there are stable nutrient supplies to coral reefs in oligotrophic oceans.Here,with emphasis on the fluxes of organic matter,we summarize at the ecosystem level(1)the multiple input pathways of external nutrients,(2)the storage of nutrients in reef organisms,(3)the efficient retaining and recycling of dissolved and particulate organic matter within coral reef ecosystems,(4)the distinctly high phytoplankton productivity and biomass inside and near oceanic coral reefs,and(5)the export of reef-related organic carbon to adjacent open oceans.These properties enable coral reefs to function as ecological“pumps”for gathering nutrients across ecosystems and space,retaining and recycling nutrients within the ecosystem,supporting high phytoplankton productivity,and exporting organic carbon to adjacent open oceans.Particularly,the high phytoplankton productivity and biomass make waters around coral reefs potential hotspots of carbon export to ocean depths via the biological pump.We demonstrate that organic carbon influx is vital for coral reef ecosystems’carbon budget and carbon export.The concept of the coral reef ecological pump provides a framework to improve the understanding of the functioning of the coral reef ecosystem and its responses to disturbance.Prospects of the coral reef ecological pump in coral reef studies are discussed in changing oceans driven by human activities and global change in the Anthropocene. 展开更多
关键词 Darwin’s Paradox coral reef NUTRIENTS coral reef ecological pump carbon export ocean carbon cycle
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Thinning intensity aff ects carbon sequestration and release in seasonal freeze–thaw areas 被引量:1
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作者 Tong Gao Xinyu Song +3 位作者 Yunze Ren Hui Liu Hangfeng Qu Xibin Dong 《Journal of Forestry Research》 SCIE CAS CSCD 2023年第4期993-1006,共14页
To explore how to respond to seasonal freeze–thaw cycles on forest ecosystems in the context of climate change through thinning,we assessed the potential impact of thinning intensity on carbon cycle dynamics.By varyi... To explore how to respond to seasonal freeze–thaw cycles on forest ecosystems in the context of climate change through thinning,we assessed the potential impact of thinning intensity on carbon cycle dynamics.By varying the number of temperature cycles,the eff ects of various thinning intensities in four seasons.The rate of mass,litter organic carbon,and soil organic carbon(SOC)loss in response to temperature variations was examined in two degrees of decomposition.The unfrozen season had the highest decomposition rate of litter,followed by the frozen season.Semi-decomposed litter had a higher decomposition rate than undecomposed litter.The decomposition rate of litter was the highest when the thinning intensity was 10%,while the litter and SOC were low.Forest litter had a good carbon sequestration impact in the unfrozen and freeze–thaw seasons,while the converse was confi rmed in the frozen and thaw seasons.The best carbon sequestration impact was identifi ed in litter,and soil layers under a 20–25%thinning intensity,and the infl uence of undecomposed litter on SOC was more noticeable than that of semi-decomposed litter.Both litter and soil can store carbon:however,carbon is transported from undecomposed litter to semi-decomposed litter and to the soil over time.In summary,the best thinning intensity being 20–25%. 展开更多
关键词 Forest carbon cycle Seasonal freeze–thaw THINNING Climate change
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Lateral downslope transport and tentative sedimentary organic carbon box model in the southern Yap Trench,western Pacific Ocean 被引量:1
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作者 Dong Li Jun Zhao +2 位作者 Chenggang Liu Jianming Pan Ji Hu 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2023年第1期61-74,共14页
Sediment collapse and subsequent lateral downslope migration play important roles in shaping the habitats and regulating sedimentary organic carbon(SOC)cycling in hadal trenches.In this study,three sediment cores were... Sediment collapse and subsequent lateral downslope migration play important roles in shaping the habitats and regulating sedimentary organic carbon(SOC)cycling in hadal trenches.In this study,three sediment cores were collected using a human-occupied vehicle across the axis of the southern Yap Trench(SYT).The total organic carbon(TOC)and total nitrogen(TN)contents,δ13C,radiocarbon ages,specific surface areas,and grain size compositions of sediments from three cores were measured.We explored the influence of the lateral downslope transport on the dispersal of the sediments and established a tentative box model for the SOC balance.In the SYT,the surface TOC content decreased with water depth and was decoupled by the funneling effect of the V-shaped hadal trench.However,the sedimentation(0.0025 cm/a)and SOC accumulation rates(∼0.038 g/(m^(2)·a)(in terms of OC))were approximately 50%higher in the deeper hadal region than in the abyssal region(0.0016 cm/a and∼0.026 g/(m^(2)·a)(in terms of OC),respectively),indicating the occurrence of lateral downslope transport.The fluctuating variations in the prokaryotic abundances and the SOC accumulation rate suggest the periodic input of surficial sediments from the shallow region.The similar average TOC(0.31%–0.38%),TN(0.06%–0.07%)contents,and SOC compositions(terrestrial OC(11%–18%),marine phytoplanktonic OC(45%–53%),and microbial OC(32%–44%))of the three sites indicate that the lateral downslope transport has a significant mixing effect on the SOC composition.The output fluxes of the laterally transported SOC(0.44–0.56 g/(m^(2)·a)(in terms of OC))contributed approximately(47%–73%)of the total SOC input,and this proportion increased with water depth.The results of this study demonstrate the importance of lateral downslope transport in the spatial distribution and development of biomes. 展开更多
关键词 southern Yap Trench sedimentary organic carbon cycling lateral downslope transport diluting effect box model
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Effects of Spin Transition and Cation Substitution on the Optical Properties and Iron Partitioning in Carbonate Minerals
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作者 HU Jun XU Liangxu +1 位作者 LIU Jin YUE Donghui 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2023年第1期350-357,共8页
The high-pressure behavior of deep carbonate dictates the state and dynamics of oxidized carbon in the Earth's mantle,playing a vital role in the global carbon cycle and potentially influencing long-term climate c... The high-pressure behavior of deep carbonate dictates the state and dynamics of oxidized carbon in the Earth's mantle,playing a vital role in the global carbon cycle and potentially influencing long-term climate change.Optical absorption and Raman spectroscopic measurements were carried out on two natural carbonate samples in diamond-anvil cells up to 60 GPa.Mg-substitution in high-spin siderite FeCO_(3)increases the crystal field absorption band position by approximately 1000 cm^(-1),but such an effect is marginal at>40 GPa when entering the low-spin state.The crystal field absorption band of dolomite cannot be recognized upon compression to 45.8 GPa at room temperature but,in contrast,the high-pressure polymorph of dolomite exhibits a strong absorption band at frequencies higher than(Mg,Fe)CO_(3)in the lowspin state by 2000–2500 cm^(-1).Additionally,these carbonate minerals show more complicated features for the absorption edge,decreasing with pressure and undergoing a dramatic change through the spin crossover.The optical and vibrational properties of carbonate minerals are highly correlated with iron content and spin transition,indicating that iron is preferentially partitioned into low-spin carbonates.These results shed new light on how carbonate minerals evolve in the mantle,which is crucial to decode the deep carbon cycle. 展开更多
关键词 carbonate petrology/mineralogy MANTLE high pressure diamond-anvil cell iron spin transition iron partitioning deep carbon cycle
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The Paleoproterozoic and Neoproterozoic Carbon Cycle Promoted the Evolution of a Habitable Earth
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作者 LIU Zhicheng ZHANG Lifei 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2023年第1期316-326,共11页
The carbon cycle is an important process that regulates Earth's evolution.We compare two typical periods,in the Paleoproterozoic and Neoproterozoic,in which many geological events occurred.It remains an open quest... The carbon cycle is an important process that regulates Earth's evolution.We compare two typical periods,in the Paleoproterozoic and Neoproterozoic,in which many geological events occurred.It remains an open question when modern plate tectonics started on Earth and how it has influenced the carbon cycle through time.In the Paleoproterozoic,intense weathering in a highly CO_(2)and CH_(4)rich atmosphere caused more nutritional elements to be carried into the ocean.Terrestrial input boosted high biological productivity,deposition of sediments and the formation of an altered oceanic crust,which may have promoted an increase in the oxygen content.Sediment lubrication and a decrease in mantle potential temperature made cold and deep subduction possible,which carried more carbon into the deep mantle.Carbon can be stored in the mantle as diamond and carbonated mantle rocks,being released by arc and mid-ocean ridge outgassing at widely different times.From the Paleoproterozoic through the Neoproterozoic to the Phanerozoic,the carbon cycle has promoted the evolution of a habitable Earth. 展开更多
关键词 carbon cycle great oxidation event modern subduction PALEOPROTEROZOIC NEOPROTEROZOIC
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δ^(13)C_(org) perturbations preserved by the interglacial Datangpo Formation in South China with implications for stratigraphic correlation and carbon cycle
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作者 Xian-yin An Yu-jie Zhang +5 位作者 Li Tian Shi-lei Liu Qi-yu Wang Yong Du Hu-yue Song Jun Hu 《China Geology》 CAS CSCD 2023年第3期420-428,共9页
Palaeoclimatic and palaeoenvironmental reconstructions of the Cryogenian Period have attracted attention in relation to the debated“Snowball Earth”hypothesis and the early evolution of metazoan life.The carbon cycle... Palaeoclimatic and palaeoenvironmental reconstructions of the Cryogenian Period have attracted attention in relation to the debated“Snowball Earth”hypothesis and the early evolution of metazoan life.The carbon cycle and redox conditions of the Sturtian-Marinoan non-glacial interval have been subjected to much controversy in the past decades because of the lack of a high-resolution stratigraphic correlation scheme.As one of the typical Sturtian-Marinoan interglacial deposits,the Datangpo Formation was widely distributed in South China with shales continuously deposited.The previous zircon dating data of the Datangpo Formation provide important ages for global constrain of the Sturtian-Marinoan non-glacial interval.Here we present a high-resolution straitigraphic study of the organic carbon isotopes of the Datangpo Formation from a drill core section in northern Guizhou Province.Based on measured episodicδ^(13)C_(org) perturbations,three positive shifts and three negative excursions are identified.Aδ^(13)C_(org)-based chemostratigraphic correlation scheme is proposed herein that works well for the Datangpo Formation regionally.Meanwhile,theδ^(13)C_(org) vertical gradients changed dynamically throughout the formation.This discovery implies that a significant ocean circulation overturn might have occurred in the upper Datangpo Formation,coinciding with the potential oxygenation. 展开更多
关键词 Organic carbon isotope carbon cycle INTERGLACIAL Palaeoenvironmental reconstruction Cryogenian Period Snowball Earth Neoproterozoic Era Datangpo Formation Geological survey engineering South China Plate
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Estimating Carbon Capture Potential of Fallow Weeds in Rice Cropping Systems
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作者 Ge Chen Yuling Kang +2 位作者 Fangbo Cao Jiana Chen Min Huang 《Phyton-International Journal of Experimental Botany》 SCIE 2023年第1期71-77,共7页
Weeds occurred during the fallow season can well perform the function of carbon(C)capture due to receiving little human disturbance.This study aimed to evaluate the C capture potential of fallow weeds in rice(Oryza sa... Weeds occurred during the fallow season can well perform the function of carbon(C)capture due to receiving little human disturbance.This study aimed to evaluate the C capture potential of fallow weeds in rice(Oryza sativa L.)cropping systems.A six-region,two-year on-farm investigation and a three-year tillage experiment were conducted to estimate C capture in fallow weeds in rice cropping systems.The on-farm investigation showed that the average mean C capture by fallow weeds across six regions and two years reached 112 g m^(-2).The tillage experiment indicated that no-tillage practices increased C capture by fallow weeds by 80%on average as compared with conventional tillage.The results of this study not only contribute to an understanding of C capture potential of fallow weeds in rice cropping systems,but also provide a reference for including fallow weeds in the estimation of vegetative C sink. 展开更多
关键词 carbon cycling fallow weeds NO-TILLAGE rice cropping system vegetative carbon sink
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Effects of Anthropogenic CO2 and Thermally-Induced CO2 on Global Warming
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作者 Masaharu Nishioka 《Atmospheric and Climate Sciences》 2024年第3期317-327,共11页
Changes in CO2 and temperature are correlated, but it is difficult to observe which is the cause and which is the effect. The release of CO2 dissolved in the ocean into the atmosphere depends on the atmospheric temper... Changes in CO2 and temperature are correlated, but it is difficult to observe which is the cause and which is the effect. The release of CO2 dissolved in the ocean into the atmosphere depends on the atmospheric temperature. However, examining the relationship between changes in CO2 caused by other phenomena and temperature is difficult. Studies of soil respiration (Rs) since the late 20th century have shown that CO2 emissions from soil respiration (Rs) are overwhelmingly greater than CO2 emissions from fossil fuel combustion. This is also noted in the IPCC carbon budget assessment. In this paper, the dependences of Rs on temperature, time, latitude, precipitation, seasons, etc., were investigated using the latest NASA database. The changes in temperature and Rs correlated well. There is also a good correlation between Rs and CO2 generation. Therefore, an increase in temperature results in an increase in CO2. On the other hand, there is no evidence other than model calculations that an increase in anthropogenic CO2 is mainly linked to a rise in temperature. The idea that global warming is caused by anthropogenic CO2 production is still a hypothesis. For these reasons, the relationship between global warming and anthropogenic CO2 should be reconsidered based on physical evidence without preconceptions. . 展开更多
关键词 Global Warming Anthropogenic CO2 Thermally-Induced CO2 Soil Respiration carbon cycles
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Why Terrestrial Stable Carbon-isotope Stratigraphy Works: a Review 被引量:2
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作者 FANG Linhao LU Yuanzheng DENG Shenghui 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2014年第5期1603-1613,共11页
Carbon-isotope stratigraphy launched since the early technological development of carbon- isotope measurement in 1950s, however, the emergence and advance of terrestrial carbon-isotope stratigraphy took quite a long w... Carbon-isotope stratigraphy launched since the early technological development of carbon- isotope measurement in 1950s, however, the emergence and advance of terrestrial carbon-isotope stratigraphy took quite a long way. At early stage the exploration of carbon-isotope stratigraphy based on the marine biological shell carbonates was verified by repeatable carbon-isotope stratigraphic data, laboratory chemical experiments and the later laboratory foraminiferal culture experiments. The breakthrough for testifying the fundamentals of terrestrial carbon-isotope stratigraphy lies on the synchronous fluctuations between the carbon-isotope stratigraphic curves derived from marine biological shell carbonates and those derived from terrestrial C3 plants. The character that carbon-isotope stratigraphic curves can be globally synchronously correlated over the marine and terrestrial/atmospheric reservoir mainly excludes the potential biasing factors, such as diagenetic bias, carbon-isotope variations in intra/inter individual plant in same species or between species, ecological changes, changes in aridity, changes in source input and representative sampling. Therefore, the fundamentals of terrestrial carbon-isotope stratigraphy based on C3 plant successfully established. The terrestrial carbon-isotope stratigraphy can be used for global stratigraphic correlation, reconstructing the evolution of atmospheric CO2 and can further verify the published global carbon-cycle models. The terrestrial carbon-isotope stratigraphy based on the compound specific biomarkers and single-grained pollen may be a promising perspective in future. 展开更多
关键词 TERRESTRIAL stratigraphic correlation carbon-isotope stratigraphy DIAGENESIS carbon cycles
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Spatiotemporal Variability and Environmental Controls of Temperature Sensitivity of Ecosystem Respiration across the Tibetan Plateau
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作者 Danrui SHENG Xianhong MENG +8 位作者 Shaoying WANG Zhaoguo LI Lunyu SHANG Hao CHEN Lin ZHAO Mingshan DENG Hanlin NIU Pengfei XU Xiaohu WEN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第9期1821-1842,共22页
Warming-induced carbon loss via ecosystem respiration(R_(e))is probably intensifying in the alpine grassland ecosystem of the Tibetan Plateau owing to more accelerated warming and the higher temperature sensitivity of... Warming-induced carbon loss via ecosystem respiration(R_(e))is probably intensifying in the alpine grassland ecosystem of the Tibetan Plateau owing to more accelerated warming and the higher temperature sensitivity of R_(e)(Q_(10)).However,little is known about the patterns and controlling factors of Q_(10)on the plateau,impeding the comprehension of the intensity of terrestrial carbon-climate feedbacks for these sensitive and vulnerable ecosystems.Here,we synthesized and analyzed multiyear observations from 14 sites to systematically compare the spatiotemporal variations of Q_(10)values in diverse climate zones and ecosystems,and further explore the relationships between Q_(10)and environmental factors.Moreover,structural equation modeling was utilized to identify the direct and indirect factors predicting Q_(10)values during the annual,growing,and non-growing seasons.The results indicated that the estimated Q_(10)values were strongly dependent on temperature,generally,with the average Q_(10)during different time periods increasing with air temperature and soil temperature at different measurement depths(5 cm,10 cm,20 cm).The Q_(10)values differentiated among ecosystems and climatic zones,with warming-induced Q_(10)declines being stronger in colder regions than elsewhere based on spatial patterns.NDVI was the most cardinal factor in predicting annual Q_(10)values,significantly and positively correlated with Q_(10).Soil temperature(Ts)was identified as the other powerful predictor for Q_(10),and the negative Q_(10)-Ts relationship demonstrates a larger terrestrial carbon loss potentiality in colder than in warmer regions in response to global warming.Note that the interpretations of the effect of soil moisture on Q_(10)were complicated,reflected in a significant positive relationship between Q_(10)and soil moisture during the growing season and a strong quadratic correlation between the two during the annual and non-growing season.These findings are conducive to improving our understanding of alpine grassland ecosystem carbon-climate feedbacks under warming climates. 展开更多
关键词 carbon cycle eddy covariance measurements ecosystem respiration Q_(10)value Tibetan Plateau climate change
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Bifunctional S-scheme g-C3N4/Bi/BiVO4 hybrid photocatalysts toward artificial carbon cycling 被引量:20
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作者 Quan Xie Wanmei He +3 位作者 Shengwei Liu Chuanhao Li Jinfeng Zhang Po Keung Wong 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2020年第1期140-153,共14页
Although both the aerobic photocatalytic oxidation of organic pollutants into CO2 and the anaerobic photocatalytic reduction of CO2 into solar fuels have been intensively studied,few efforts have been devoted to combi... Although both the aerobic photocatalytic oxidation of organic pollutants into CO2 and the anaerobic photocatalytic reduction of CO2 into solar fuels have been intensively studied,few efforts have been devoted to combining these carbon-involved photocatalytic oxidation-reduction processes together,by which an artificial photocatalytic carbon cycling process can be established.The key challenge lies in the exploitation of efficient bifunctional photocatalysts,capable of triggering both aerobic oxidation and anaerobic reduction reactions.In this work,a bifunctional ternary g-C3N4/Bi/BiVO4 hybrid photocatalyst is successfully constructed,which not only demonstrates superior aerobic photocatalytic oxidation performance in degrading an organic pollutant(using the dye,Rhodamine B as a model),but also exhibits impressive photocatalytic CO2 reduction performance under anaerobic conditions.Moreover,a direct conversion of Rhodamine B to solar fuels in a one-pot anaerobic reactor can be achieved with the as-prepared ternary g-C3N4/Bi/BiVO4 hybrid photocatalyst.The excellent bifunctional photocatalytic performance of the g-C3N4/Bi/BiVO4 photocatalyst is associated with the formation of efficient S-scheme hybrid junctions,which contribute to promoting the appropriate charge dynamics,and sustaining favorable charge potentials.The formation of the S-scheme heterojunction is supported by scavenger studies and density functional theory calculations.Moreover,the in-situ formed plasmonic metallic Bi nanoparticles in the S-scheme hybrid g-C3N4/Bi/BiVO4 photocatalyst enhances vectorial interfacial electron transfer.This novel bifunctional S-scheme g-C3N4/Bi/BiVO4 hybrid photocatalyst system provides new insights for the further development of an integrated aerobic-anaerobic reaction system for photocatalytic carbon cycling. 展开更多
关键词 S-scheme Plasmonic Bi nanoparticles Photocatalytic CO2 reduction Photocatalytic degradation of organic pollutants carbon cycling
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Black carbon and polycyclic aromatic hydrocarbons (PAHs) in surface sediments of China’s marginal seas 被引量:13
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作者 康延菊 王旭晨 +3 位作者 戴民汉 冯桓 李安春 宋茜 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2009年第2期297-308,共12页
This study investigates the distribution of black carbon (BC) and its correlation with total polycyclic aromatic hydrocarbons (EPAH) in the surface sediments of China's marginal seas. BC content ranges from 〈0.1... This study investigates the distribution of black carbon (BC) and its correlation with total polycyclic aromatic hydrocarbons (EPAH) in the surface sediments of China's marginal seas. BC content ranges from 〈0.10 to 2.45 mg/g dw (grams dry weight) in the sediments studied, and varied among the different coastal regions. The Bohai Bay sediments had the highest BC contents (average 2.18 mg/g dw), which comprises a significant fraction (27%-41%) of the total organic carbon (TOC) preserved in the sediments. In comparison, BC in the surface sediments of the North Yellow Sea, Jiaozhou Bay, East China Sea and the South China Sea is less abundant and accounted for an average of 6%, 8%, 14% and 5%, respectively, of the sedimentary organic carbon pool. The concentration of EPAH in the surface sediments ranges from 41 to 3 667 ng/g dw and showed large spatial variations among the sampling sites of different costal regions. The Bohai Bay has the highest ZPAH values, ranging from 79 to 3 667 ng/g dw. This reflects the high anthropogenically contaminated nature of the sediments in the bay. BC is positively correlated to TOC but a strong correlation is not found between BC and ZPAH in the surface sediments studied, suggesting that BC and PAHs preserved in the sediments are derived from different sources and controlled by different biogeochemical processes. Our study suggests that the abundance of BC preserved in the sediments could represent a significant sink pool of carbon cycling in China's marginal seas. 展开更多
关键词 Black carbon PAH marine sediment carbon cycle China's marginal seas
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Estimation of soil organic carbon reservoir in China 被引量:17
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作者 WANG Shao-qiang1, ZHOU Cheng-hu1, LI Ke-rang1, ZHU Song-li2, HUANG Fang-hong1 (1.The State Key Laboratory of Resources and Environment Information System, Institute of Geographic Sciences and Natural Resources Research, CAS, Beijing 100101, China 《Journal of Geographical Sciences》 SCIE CSCD 2001年第1期3-13,共11页
The paper respectively adopted physio-chemical properties of every soil stratum from 2473 soil profiles of the second national soil survey. The corresponding carbon content of soils is estimated by utilizing conversio... The paper respectively adopted physio-chemical properties of every soil stratum from 2473 soil profiles of the second national soil survey. The corresponding carbon content of soils is estimated by utilizing conversion coefficient 0.58. In the second soil survey, the total amount of soil organic carbon is about 924.18xl08t and carbon density is about 10.53 kgC/m2 in China according to the area of 877.63x106hm2 surveyed throughout the country. The spatial distribution characteristics of soil organic carbon in China is that the carbon storage increases when latitude increases in eastern China and the carbon storage decreases when longitude reduces in northern China. A transitional zone with great variation in carbon storage exists. Moreover, there is an increasing tendency of carbon density with decrease of latitude in western China. Soil circle is of great significance to global change, but with substantial difference in soil spatial distribution throughout the country. Because the structure of soil is inhomogeneous, it could bring some mistakes in estimating soil carbon reservoirs. It is necessary to farther resolve soil respiration and organic matter conversion and other questions by developing uniform and normal methods of measurement and sampling. 展开更多
关键词 terrestrial ecosystem global change soil carbon reservoir carbon cycle
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Temporal variation of soil carbon stock and its controlling factors over the last two decades on the southern Song-nen Plain,Heilongjiang Province 被引量:19
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作者 Xueqi Xia Zhongfang Yang +2 位作者 Yan Liao Yujun Cui Yansheng Li 《Geoscience Frontiers》 SCIE CAS 2010年第1期125-132,共8页
Against the current background of global climate change, the study of variations in the soil carbon pool and its controlling factors may aid in the evaluation of soil's role in the mitigation or enhancement of greenh... Against the current background of global climate change, the study of variations in the soil carbon pool and its controlling factors may aid in the evaluation of soil's role in the mitigation or enhancement of greenhouse gas. This paper studies spatial and temporal variation in the soil carbon pool and their controlling factors in the southern Song-nen Plain in Heilongjiang Province, using soil data collected over two distinct periods by the Multi-purpose Regional Geochemical Survey in 2005-2007, and another soil survey conducted in 1982-1990. The study area is a carbon source of 1479 t/km2 and in the past 20 years, from the 1980s until 2005, the practical carbon emission from the soil was 0.12 Gt. Temperature, which has been found to be linearly correlated to soil organic carbon, is the domi- nant climatologic factor controlling soil organic carbon contents. Our study shows that in the relevant area and time period the potential loss of soil organic carbon caused by rising temperatures was 0.10 Gt, the potential soil carbon emission resulting from land-use change was 0.09 Gt, and the combined potential loss of soil carbon (0.19 Gt) caused by warming and land-use change is comparable to that of fossil fuel combustion (0.21 Gt). Due to the time delay in soil carbon pool variation, there is still 0.07 Gt in the potential emission caused by warming and land-use change that will be gradually released in the future. 展开更多
关键词 The southern Song-nen Plain in Heilongjiang Province Soil carbon pool Spatial and temporal variation carbon cycle
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