We study theoretically how to produce and detect the ultracold ground-state Cs2 molecule from Feshbach state. Nu- merical calculations are performed by solving the quantum Liouville equation based on multilevel Bloch ...We study theoretically how to produce and detect the ultracold ground-state Cs2 molecule from Feshbach state. Nu- merical calculations are performed by solving the quantum Liouville equation based on multilevel Bloch model. The producing efficiency reaches 55% and the detecting efficiency is 31%. The producing and detecting efficiencies are closely related to the Rabi frequencies of laser pulses. The decay of relevant electronic and vibrational states obviously reduces the producing and detecting efficiencies.展开更多
The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital...The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS<sub>2</sub> molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.10974024 and 11274056)
文摘We study theoretically how to produce and detect the ultracold ground-state Cs2 molecule from Feshbach state. Nu- merical calculations are performed by solving the quantum Liouville equation based on multilevel Bloch model. The producing efficiency reaches 55% and the detecting efficiency is 31%. The producing and detecting efficiencies are closely related to the Rabi frequencies of laser pulses. The decay of relevant electronic and vibrational states obviously reduces the producing and detecting efficiencies.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11574117,11271158,61575077 and 11575071
文摘The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS<sub>2</sub> molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.
