The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the ...The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the DBD plasma control technology and hot-wire anemometer velocity measurements,a novel convenient method of local drag reduction(DR)measurement is proposed by measuring the single-point velocity within the linear region of the viscous sublayer.We analyze the premise of using the method,and the maximum effective measurement range of-73.1%<DR<42.2%is obtained according to the experimental environment in this work.The local drag decreases downstream of the center of two adjacent upper electrodes and increases downstream of the upper electrodes.The magnitude of the local DR increases with increasing voltage and decreases as it moves away from the actuators.For the spanwise position in between,the streamwise distribution of the local DR is very dependent on the voltage.The variable-interval time-average detection results reveal that all bursting intensities are reduced compared to the baseline,and the amount of reduction is comparable to the absolute values of the local DR.Compared with previous results,we infer that the control mechanism is that many meandering streaks are combined together into single stabilized streaks.展开更多
In this study, SiOx films were deposited by a dielectric barrier discharge (DBD) plasma gun at an atmospheric pressure. The relationship of the film structures with plasma powers was investigated by Fourier transfor...In this study, SiOx films were deposited by a dielectric barrier discharge (DBD) plasma gun at an atmospheric pressure. The relationship of the film structures with plasma powers was investigated by Fourier transform infrared spectroscopy (FTIR), and scanning electron microscope (SEM). It was shown that an uniform and cross-linking structure film was formed by the DBD gun. As an application, the SiOx films were deposited on a carbon steel surface for the anti-corrosion purpose. The experiment was carried out in a 0.1 M NaCl solution. It was found that a very good anti-corrosive property was obtained, i.e., the corrosion rate was decreased c.a. 15 times in 5% NaCl solution compared to the non-SiOx coated steel, as detected by the potentiodynamic polarization measurement.展开更多
In this work,the dielectric-barrier-discharge plasma actuator was employed to study the flow structures induced by the plasma actuator over a flat plate and a wall-mounted hump.A phenomenological dielectric-barrier-di...In this work,the dielectric-barrier-discharge plasma actuator was employed to study the flow structures induced by the plasma actuator over a flat plate and a wall-mounted hump.A phenomenological dielectric-barrier-discharge plasma model which regarded the plasma effect as the body force was implemented into the Navier–Stokes equations solved by the method of large eddy simulations.The results show that a series of vortex pairs,which indicated dipole formation and periodicity distribution were generated in the boundary layer when the plasma was applied to the flow over a flat plane.They would enhance the energy exchanged between the near wall region and the free stream.Besides,their spatial trajectories are deeply affected by the actuation strength.When the actuator was engaged in the flow over a wall-mounted hump,the vortex pairs were also produced,which was able to delay flow separation as well as to promote flow reattachment and reduce the generation of a vortex,achieving the goal of reducing dissipation and decreasing flow resistance.展开更多
The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated...The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated.Due to temperature change mainly caused through heat produced along with plasma will lead to measurement error of shear stress measured by hot-film sensor,the correction method that takes account of the change measured by another sensor is used and works well.In order to achieve the value of shear stress change,we combine computational fluid dynamics computation with experiment to calibrate the hot-film sensor.To test the stability of the hot-film sensor,seven repeated measurements of shear stress at Ma=0.3 are conducted and show that confidence interval of hot-film sensor measurement is from−0.18 to 0.18 Pa and the root mean square is 0.11 Pa giving a relative error 0.5%over all Mach numbers in this experiment.The research on the turbulent boundary layer control with DBD plasma actuators demonstrates that the control makes shear stress increase by about 6%over the three Mach numbers,which is thought to be reliable through comparing it with the relative error 0.5%,and the value is hardly affected by burst frequency and excitation voltage.展开更多
To improve the‘detonation-supporting’performance of fuel-rich catalytic combustion products,DBD plasma,stimulated by adjustable nanosecond pulse power supply,was used to further regulate the components and concentra...To improve the‘detonation-supporting’performance of fuel-rich catalytic combustion products,DBD plasma,stimulated by adjustable nanosecond pulse power supply,was used to further regulate the components and concentrations of the hydrocarbon blends.In this paper,the parameters including load voltage,frequency,rising(falling)edge,pulse width and feeding flow rate were changed respectively,and the corresponding concentration and proportion change of the components in blend gas were investigated.According to the experiment result,it was found that when the discharge frequency is low,the plasma mainly promotes the transformation of light gaseous substances,while it mainly promotes the conversion to heavy hydrocarbons when the frequency is larger.Increasing load voltage will strengthen this trend.The controlling and reforming effect of plasma on the blend gas will decrease with the increase of voltage rising(falling)edge and the feeding flow rate.The regulation effect will be strengthened with the increase of pulse width under 200 ns.With the increase of discharge intensity,the‘carbon’settles on the walls of the reactor,which will change the dielectric constant,leading to the loss of control of the discharge.展开更多
Using a plexiglas plate model, the performance of peristaltic flow acceleration in- duced by multiple DBD (dielectric barrier discharge) plasma actuators was studied based on PIV (particle image velocimetry). The ...Using a plexiglas plate model, the performance of peristaltic flow acceleration in- duced by multiple DBD (dielectric barrier discharge) plasma actuators was studied based on PIV (particle image velocimetry). The asynchronous and the duty cycle pulsed actuation modes were proposed and tested. The velocity fields induced by multiple DBD plasma actuators with different phase angles and duty cycle ratios were acquired and the momentum transfer characteristics of the flow field were discussed. Consequently, the mechanism of the peristalsis-acceleration multi- ple DBD plasma actuation was analyzed. The results show that the peristaltic flow acceleration effect of multiple plasma actuators occurs mainly in paraelectric direction, and the mechanism of peristaltic flow acceleration is ejection pushing effect rather than injection pumping effect. The asynchronous and the duty cycle pulsed actuation modes can, with energy consumption increase of merely 10%, achieve 65% and 42% increase of downstream velocity, and thus are promising in velocity improvement and energy saving.展开更多
In this paper, the effect of dielectric-barrier discharge plasma excitation characteristics on turbulent boundary layer separation over a hump is investigated using computational fluid dynamics. Four different turbule...In this paper, the effect of dielectric-barrier discharge plasma excitation characteristics on turbulent boundary layer separation over a hump is investigated using computational fluid dynamics. Four different turbulence models were used for verification. The Reynolds stress model showed the best agreement with the experimental data, in general. Based on the verification and validation, the effect of duty cycle and excitation frequency on the turbulent flow separation were investigated. The results showed that the pulsed plasma excitation could effectively suppress the flow separation by mixing augmentation. With increasing duty cycle and excitation frequency, the flow separation first increased, then decreased again. The optimal duty cycle was 0.75 and the optimal excitation frequency was 50 Hz.展开更多
Perturbation is generally considered as the flow noise,and its energy can gain transient growth in the separation bubble.The amplified perturbations may cause unstable Kelvin–Helmohltz vortices which induce the three...Perturbation is generally considered as the flow noise,and its energy can gain transient growth in the separation bubble.The amplified perturbations may cause unstable Kelvin–Helmohltz vortices which induce the three-dimensional transition.Active control of noise amplification via dielectric barrier discharge plasma actuator in the flow over a square leading-edge flat plate is numerically studied.The actuator is installed near the plate leading-edge where the separation bubble is formed.The maximum energy amplification of perturbations is positively correlated with the separation bubble scale which decreases with the increasing control parameters.As the magnitude of noise amplification is reduced,the laminar-turbulent transition is successfully suppressed.展开更多
The ε-Fe3N-based magnetic lubricant which is stable and high saturation magnetization has been prepared by a homemade DBD device under the atmospheric pressure. The results show that the NH3 flow rate, the applied pe...The ε-Fe3N-based magnetic lubricant which is stable and high saturation magnetization has been prepared by a homemade DBD device under the atmospheric pressure. The results show that the NH3 flow rate, the applied peak-to-peak voltage and the mass ratio of surfactant and carrier lubricant have important effects on the phase structure, the magnetic properties, the size of ferroparticles and the stability of the ε-Fe3N-based magnetic lubricant. TEM images show the e-Fe3N ferroparticles are dispersed in the carrier lubricant homogeneously, and the cluster phenomenon is not observed. The stable e-Fe3N-based magnetic lubricant with the saturation magnetization of 50.11 mT and the mean ferroparticle size of 11 nm is prepared successfully. The main particles of the atmospheric-pressure Ar/NH3/Fe(CO)5 DBD plasma are NH, N, N+, Fe, N2, Ar, Ha, and CO; NH is a decomposition product of NH3. Fe and N active radicals are two elementary species in the preparation of the c-Fe3N-based magnetic lubricant in the atmospheric-pressure DBD plasma. There are two discharge modes for DBD plasma, namely, multi-pulse APGD and filamentary discharge. By increasing the applied peak-to-peak voltage from 4600 to 7800 V, the discharge mode is changed from single-pulse APGD with filamentary discharge to two-pulse APGD with filamentary discharge, and the Lissajous figure also converts from a quadrilateral with one step to two steps on the right-hand side.展开更多
Plasma treatment has been known as an effective way to improve the surface bonding between the reinforcement material and the matrix, by modifying the surface morphology and the chemical composes of the material. In o...Plasma treatment has been known as an effective way to improve the surface bonding between the reinforcement material and the matrix, by modifying the surface morphology and the chemical composes of the material. In order to investigate the effects of atmospheric dielectric barrier discharge (DBD) plasma treatment on the surface properties of polyacrylonitrile-based (PAN-based) carbon fiber, atomic force microscope(AFM), X-ray photoelectron spectroscopy(XPS), and contact angle test were introduced to compare different treatment duration. The interfacial adhesion of carbon fiber/epoxy (CF/EP) composites were analyzed by a single fiber composite (SFC) for filament fragmentation test. And the tensile strength test and Weibull analysis were carried out to observe whether the etching could affect the strength. The results prove that the DBD plasma improves the surface properties of the carbon fiber. Further, when the treatment time was around 90 s, the roughness and oxygen containing group of the carbon fiber reached the peak values. Also, the fiber showed the best adhesion to the polymer in contact angle test and the optimum interfacial shear strength (IFSS) in fragmentation test. The Weibull analyses of the tensile data revealed no substantial changes in the tensile strength within the treatment time of 180 s.展开更多
A new method for liquefying coal using dielectric barrier discharge plasma has been studied.By utilizing waste oil as the solvent and processing coal nano powder in the plasma for 10 min,we have attained a liquid yiel...A new method for liquefying coal using dielectric barrier discharge plasma has been studied.By utilizing waste oil as the solvent and processing coal nano powder in the plasma for 10 min,we have attained a liquid yield of more than 80%.The experiment shows that not only the coal nanopowder promoted the liquefaction process,but hydrogen radicals improved the liquid yield effectively.In the plasma processing,the phenomenon of the changing color of the nanopowder solution and not producing a solid residue has been obviously observed.The rational parameters that affected the liquefaction of coal nanopowder have been achieved through the experiment,and the liquefied products have been analyzed.展开更多
A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-li...A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-like discharge was achieved. Two kinds of typical bacteria, i.e., the Staphylococcus aureus (S. aureus) and Escherichia coil (E. coil), were employed to study the bacterial inactivation mechanism by means of the non-thermal plasma. The killing log value (KLV) of S. aureus reached up to 5.38 with a treatment time of 90 s and that of E. coil up to 5.36 with 60 s, respectively. According to the argon emission spectra of the plasma jet and the scanning electron microscope (SEM) images of the two bacteria before and after the plasma treatment, it is concluded that the reactive species in the argon plasma played a major role in the bacterial inactivation, while the heat, electric field and UV photons had little effect.展开更多
In this study,Ag/γ-Al_(2)O_(3)catalysts were synthesized by an Ar dielectric barrier discharge plasma using silver nitrate as the Ag source andγ-alumina(γ-Al_(2)O_(3))as the support.It is revealed that plasma can r...In this study,Ag/γ-Al_(2)O_(3)catalysts were synthesized by an Ar dielectric barrier discharge plasma using silver nitrate as the Ag source andγ-alumina(γ-Al_(2)O_(3))as the support.It is revealed that plasma can reduce silver ions to generate crystalline silver nanoparticles(Ag NPs)of good dispersion and uniformity on the alumina surface,leading to the formation of Ag/γ-Al_(2)O_(3)catalysts in a green manner without traditional chemical reductants.Ag/γ-Al_(2)O_(3)exhibited good catalytic activity and stability in CO oxidation reactions,and the activity increased with increase in the Ag content.For catalysts with more than 2 wt%Ag,100%CO conversion can be achieved at 300°C.The catalytic activity of the Ag/γ-Al_(2)O_(3)catalysts is also closely related to the size of theγ-alumina,where Ag/nano-γ-Al_(2)O_(3)catalysts demonstrate better performance than Ag/micro-γ-Al_(2)O_(3)catalysts with the same Ag content.In addition,the catalytic properties of plasma-generated Ag/nano-γ-Al_(2)O_(3)(Ag/γ-Al_(2)O_(3)-P)catalysts were compared with those of Ag/nano-γ-Al_(2)O_(3)catalysts prepared by the traditional calcination approach(Ag/γ-Al_(2)O_(3)-C),with the plasma-generated samples demonstrating better overall performance.This simple,rapid and green plasma process is considered to be applicable for the synthesis of diverse noble metal-based catalysts.展开更多
While dielectric-barrier-discharge(DBD)based plasma actuation systems have been successfully demonstrated to suppress massive flow separation over wind turbine blades to reduce the transient aerodynamic loadings actin...While dielectric-barrier-discharge(DBD)based plasma actuation systems have been successfully demonstrated to suppress massive flow separation over wind turbine blades to reduce the transient aerodynamic loadings acting on the turbine blades,it is still a non-trivial task to establish a best combination of various operating parameters for a DBD plasma actuation system to achieve the optimized flow control effectiveness.In the present study,a regression Kriging based metamodeling technique is developed to optimize the operating parameters of a DBD plasma actuation system for suppressing deep stall over the surface of a wind turbine blade section/airfoil model.The data points were experimentally obtained by embedding a nanosecond-pulsed DBD(NS-DBD)plasma actuator at the leading edge of the airfoil model.The applied voltage and frequency for the NS-DBD plasma actuation were used as the design variables to demonstrate the optimization procedure.The highest possible lift coefficient of the turbine airfoil model at deep stalled angles of attack(i.e.,α?=?22°and 24°)were selected as the objective function for the optimization.It was found that,while the metamodeling-based procedure could accurately predict the objective function within the bounds of the design variables with an uncertainty~?2%,a global accuracy level of~?97%was achieved within the whole design space.展开更多
Cold plasma generated by dielectric barrier discharge (DBD) at atmospheric pressure was adopted for preparation of commercial TiO2 Degussa P25 supported Au catalysts (Au/P25- P) with the assistance of the depositi...Cold plasma generated by dielectric barrier discharge (DBD) at atmospheric pressure was adopted for preparation of commercial TiO2 Degussa P25 supported Au catalysts (Au/P25- P) with the assistance of the deposition-precipitation procedure. The influences of the plasma reduction time and calcination on the performance of the Au/P25-P catalysts were investigated. CO oxidation was performed to investigate the catalytic activity of the Au/P25 catalysts. The results show that DBD cold plasma for the fabrication of Au/P25-P catalysts is a fast process, and Au/P25-P (4 min) exhibited the highest CO oxidation activity due to the complete reduction of Au compounds and less consumption of oxygen vacancies. In order to form more oxygen vacancies active species, Au/P25-P was calcined to obtain Au/P25-PC catalysts. Interestingly, Au/P25- PC exhibited the highest activity for CO oxidation among the Au/P25 samples. The results of transmission electron microscopy (TEM) indicated that the smaller size and high distribution of Au nanoparticles are the mean reasons for a high performance of Au/P25-PC. Atmospheric- pressure DBD cold plasma was proved to be of great efficiency in preparing high performance supported Au catalysts.展开更多
基金the financial support received from the National Science Fund for Distinguished Young Scholars(No.12102359)。
文摘The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the DBD plasma control technology and hot-wire anemometer velocity measurements,a novel convenient method of local drag reduction(DR)measurement is proposed by measuring the single-point velocity within the linear region of the viscous sublayer.We analyze the premise of using the method,and the maximum effective measurement range of-73.1%<DR<42.2%is obtained according to the experimental environment in this work.The local drag decreases downstream of the center of two adjacent upper electrodes and increases downstream of the upper electrodes.The magnitude of the local DR increases with increasing voltage and decreases as it moves away from the actuators.For the spanwise position in between,the streamwise distribution of the local DR is very dependent on the voltage.The variable-interval time-average detection results reveal that all bursting intensities are reduced compared to the baseline,and the amount of reduction is comparable to the absolute values of the local DR.Compared with previous results,we infer that the control mechanism is that many meandering streaks are combined together into single stabilized streaks.
基金supported by the National Natural Science Foundation of China(No.10475010)
文摘In this study, SiOx films were deposited by a dielectric barrier discharge (DBD) plasma gun at an atmospheric pressure. The relationship of the film structures with plasma powers was investigated by Fourier transform infrared spectroscopy (FTIR), and scanning electron microscope (SEM). It was shown that an uniform and cross-linking structure film was formed by the DBD gun. As an application, the SiOx films were deposited on a carbon steel surface for the anti-corrosion purpose. The experiment was carried out in a 0.1 M NaCl solution. It was found that a very good anti-corrosive property was obtained, i.e., the corrosion rate was decreased c.a. 15 times in 5% NaCl solution compared to the non-SiOx coated steel, as detected by the potentiodynamic polarization measurement.
基金supported by the Scientific Research Project Fund of Middle East Technical University,under project # BAP-08-11-2016-044
文摘In this work,the dielectric-barrier-discharge plasma actuator was employed to study the flow structures induced by the plasma actuator over a flat plate and a wall-mounted hump.A phenomenological dielectric-barrier-discharge plasma model which regarded the plasma effect as the body force was implemented into the Navier–Stokes equations solved by the method of large eddy simulations.The results show that a series of vortex pairs,which indicated dipole formation and periodicity distribution were generated in the boundary layer when the plasma was applied to the flow over a flat plane.They would enhance the energy exchanged between the near wall region and the free stream.Besides,their spatial trajectories are deeply affected by the actuation strength.When the actuator was engaged in the flow over a wall-mounted hump,the vortex pairs were also produced,which was able to delay flow separation as well as to promote flow reattachment and reduce the generation of a vortex,achieving the goal of reducing dissipation and decreasing flow resistance.
基金the European Commission through the Research and Innovation action DRAGY(Drag Reduction via Turbulent Boundary Layer Flow Control)under Grant No.690623+1 种基金the Ministry of Industry and Information Technology(MIIT)of the Chinese governmentsupport received from National Natural Science Foundation of China(No.11572256).
文摘The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated.Due to temperature change mainly caused through heat produced along with plasma will lead to measurement error of shear stress measured by hot-film sensor,the correction method that takes account of the change measured by another sensor is used and works well.In order to achieve the value of shear stress change,we combine computational fluid dynamics computation with experiment to calibrate the hot-film sensor.To test the stability of the hot-film sensor,seven repeated measurements of shear stress at Ma=0.3 are conducted and show that confidence interval of hot-film sensor measurement is from−0.18 to 0.18 Pa and the root mean square is 0.11 Pa giving a relative error 0.5%over all Mach numbers in this experiment.The research on the turbulent boundary layer control with DBD plasma actuators demonstrates that the control makes shear stress increase by about 6%over the three Mach numbers,which is thought to be reliable through comparing it with the relative error 0.5%,and the value is hardly affected by burst frequency and excitation voltage.
基金supported by National Natural Science Foundation of China(Nos.91941105,91941301,51790511)。
文摘To improve the‘detonation-supporting’performance of fuel-rich catalytic combustion products,DBD plasma,stimulated by adjustable nanosecond pulse power supply,was used to further regulate the components and concentrations of the hydrocarbon blends.In this paper,the parameters including load voltage,frequency,rising(falling)edge,pulse width and feeding flow rate were changed respectively,and the corresponding concentration and proportion change of the components in blend gas were investigated.According to the experiment result,it was found that when the discharge frequency is low,the plasma mainly promotes the transformation of light gaseous substances,while it mainly promotes the conversion to heavy hydrocarbons when the frequency is larger.Increasing load voltage will strengthen this trend.The controlling and reforming effect of plasma on the blend gas will decrease with the increase of voltage rising(falling)edge and the feeding flow rate.The regulation effect will be strengthened with the increase of pulse width under 200 ns.With the increase of discharge intensity,the‘carbon’settles on the walls of the reactor,which will change the dielectric constant,leading to the loss of control of the discharge.
基金supported by National Natural Science Foundation of China(No.51107101)the Foundation for Fundamental Research of the Northwestern Polytechnical University of China(JC201103)
文摘Using a plexiglas plate model, the performance of peristaltic flow acceleration in- duced by multiple DBD (dielectric barrier discharge) plasma actuators was studied based on PIV (particle image velocimetry). The asynchronous and the duty cycle pulsed actuation modes were proposed and tested. The velocity fields induced by multiple DBD plasma actuators with different phase angles and duty cycle ratios were acquired and the momentum transfer characteristics of the flow field were discussed. Consequently, the mechanism of the peristalsis-acceleration multi- ple DBD plasma actuation was analyzed. The results show that the peristaltic flow acceleration effect of multiple plasma actuators occurs mainly in paraelectric direction, and the mechanism of peristaltic flow acceleration is ejection pushing effect rather than injection pumping effect. The asynchronous and the duty cycle pulsed actuation modes can, with energy consumption increase of merely 10%, achieve 65% and 42% increase of downstream velocity, and thus are promising in velocity improvement and energy saving.
基金supported by National Natural Science Foundation of China (No. 51576065)the Fundamental Research Funds for the Central Universities (Nos. 2015CY05, 2018QN037, 2018ZD09)
文摘In this paper, the effect of dielectric-barrier discharge plasma excitation characteristics on turbulent boundary layer separation over a hump is investigated using computational fluid dynamics. Four different turbulence models were used for verification. The Reynolds stress model showed the best agreement with the experimental data, in general. Based on the verification and validation, the effect of duty cycle and excitation frequency on the turbulent flow separation were investigated. The results showed that the pulsed plasma excitation could effectively suppress the flow separation by mixing augmentation. With increasing duty cycle and excitation frequency, the flow separation first increased, then decreased again. The optimal duty cycle was 0.75 and the optimal excitation frequency was 50 Hz.
基金funded by the Specialized Research Fund for the Doctoral Program of Higher Education(Grant No.20133219110039)
文摘Perturbation is generally considered as the flow noise,and its energy can gain transient growth in the separation bubble.The amplified perturbations may cause unstable Kelvin–Helmohltz vortices which induce the three-dimensional transition.Active control of noise amplification via dielectric barrier discharge plasma actuator in the flow over a square leading-edge flat plate is numerically studied.The actuator is installed near the plate leading-edge where the separation bubble is formed.The maximum energy amplification of perturbations is positively correlated with the separation bubble scale which decreases with the increasing control parameters.As the magnitude of noise amplification is reduced,the laminar-turbulent transition is successfully suppressed.
基金supported by National Natural Science Foundation of China (Grant Nos. 11605020 and 21673026)by the National Natural Science Foundation of Liaoning Province, China (Grant No. 2015020585)
文摘The ε-Fe3N-based magnetic lubricant which is stable and high saturation magnetization has been prepared by a homemade DBD device under the atmospheric pressure. The results show that the NH3 flow rate, the applied peak-to-peak voltage and the mass ratio of surfactant and carrier lubricant have important effects on the phase structure, the magnetic properties, the size of ferroparticles and the stability of the ε-Fe3N-based magnetic lubricant. TEM images show the e-Fe3N ferroparticles are dispersed in the carrier lubricant homogeneously, and the cluster phenomenon is not observed. The stable e-Fe3N-based magnetic lubricant with the saturation magnetization of 50.11 mT and the mean ferroparticle size of 11 nm is prepared successfully. The main particles of the atmospheric-pressure Ar/NH3/Fe(CO)5 DBD plasma are NH, N, N+, Fe, N2, Ar, Ha, and CO; NH is a decomposition product of NH3. Fe and N active radicals are two elementary species in the preparation of the c-Fe3N-based magnetic lubricant in the atmospheric-pressure DBD plasma. There are two discharge modes for DBD plasma, namely, multi-pulse APGD and filamentary discharge. By increasing the applied peak-to-peak voltage from 4600 to 7800 V, the discharge mode is changed from single-pulse APGD with filamentary discharge to two-pulse APGD with filamentary discharge, and the Lissajous figure also converts from a quadrilateral with one step to two steps on the right-hand side.
基金the Key Laboratory Fundings of Science and Technology Commission of Shanghai Municipality,China(No. 10521100404,No.10JC1400400)Foundation of Key Laboratory of Textile Science & Technology,Ministry of Education of China(No. 11D10114)
文摘Plasma treatment has been known as an effective way to improve the surface bonding between the reinforcement material and the matrix, by modifying the surface morphology and the chemical composes of the material. In order to investigate the effects of atmospheric dielectric barrier discharge (DBD) plasma treatment on the surface properties of polyacrylonitrile-based (PAN-based) carbon fiber, atomic force microscope(AFM), X-ray photoelectron spectroscopy(XPS), and contact angle test were introduced to compare different treatment duration. The interfacial adhesion of carbon fiber/epoxy (CF/EP) composites were analyzed by a single fiber composite (SFC) for filament fragmentation test. And the tensile strength test and Weibull analysis were carried out to observe whether the etching could affect the strength. The results prove that the DBD plasma improves the surface properties of the carbon fiber. Further, when the treatment time was around 90 s, the roughness and oxygen containing group of the carbon fiber reached the peak values. Also, the fiber showed the best adhesion to the polymer in contact angle test and the optimum interfacial shear strength (IFSS) in fragmentation test. The Weibull analyses of the tensile data revealed no substantial changes in the tensile strength within the treatment time of 180 s.
文摘A new method for liquefying coal using dielectric barrier discharge plasma has been studied.By utilizing waste oil as the solvent and processing coal nano powder in the plasma for 10 min,we have attained a liquid yield of more than 80%.The experiment shows that not only the coal nanopowder promoted the liquefaction process,but hydrogen radicals improved the liquid yield effectively.In the plasma processing,the phenomenon of the changing color of the nanopowder solution and not producing a solid residue has been obviously observed.The rational parameters that affected the liquefaction of coal nanopowder have been achieved through the experiment,and the liquefied products have been analyzed.
基金supported in part by China Foundation for the Author of National Excellent Doctoral Dissertation(No.200338)New Century Excellent Talents in University(No.NCET-04-0943)
文摘A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-like discharge was achieved. Two kinds of typical bacteria, i.e., the Staphylococcus aureus (S. aureus) and Escherichia coil (E. coil), were employed to study the bacterial inactivation mechanism by means of the non-thermal plasma. The killing log value (KLV) of S. aureus reached up to 5.38 with a treatment time of 90 s and that of E. coil up to 5.36 with 60 s, respectively. According to the argon emission spectra of the plasma jet and the scanning electron microscope (SEM) images of the two bacteria before and after the plasma treatment, it is concluded that the reactive species in the argon plasma played a major role in the bacterial inactivation, while the heat, electric field and UV photons had little effect.
基金financial support from National Natural Science Foundation of China(Nos.52004102 and 22078125)Postdoctoral Science Foundation of China(No.2021M690068)+2 种基金Fundamental Research Funds for the Central Universities(Nos.JUSRP221018 and JUSRP622038)Key Laboratory of Green Cleaning Technology and Detergent of Zhejiang Province(No.Q202204)Open Project of Key Laboratory of Green Chemical Engineering Process of Ministry of Education(No.GCP202112)。
文摘In this study,Ag/γ-Al_(2)O_(3)catalysts were synthesized by an Ar dielectric barrier discharge plasma using silver nitrate as the Ag source andγ-alumina(γ-Al_(2)O_(3))as the support.It is revealed that plasma can reduce silver ions to generate crystalline silver nanoparticles(Ag NPs)of good dispersion and uniformity on the alumina surface,leading to the formation of Ag/γ-Al_(2)O_(3)catalysts in a green manner without traditional chemical reductants.Ag/γ-Al_(2)O_(3)exhibited good catalytic activity and stability in CO oxidation reactions,and the activity increased with increase in the Ag content.For catalysts with more than 2 wt%Ag,100%CO conversion can be achieved at 300°C.The catalytic activity of the Ag/γ-Al_(2)O_(3)catalysts is also closely related to the size of theγ-alumina,where Ag/nano-γ-Al_(2)O_(3)catalysts demonstrate better performance than Ag/micro-γ-Al_(2)O_(3)catalysts with the same Ag content.In addition,the catalytic properties of plasma-generated Ag/nano-γ-Al_(2)O_(3)(Ag/γ-Al_(2)O_(3)-P)catalysts were compared with those of Ag/nano-γ-Al_(2)O_(3)catalysts prepared by the traditional calcination approach(Ag/γ-Al_(2)O_(3)-C),with the plasma-generated samples demonstrating better overall performance.This simple,rapid and green plasma process is considered to be applicable for the synthesis of diverse noble metal-based catalysts.
基金the National Science Foundation(NSF)(Grants OISE-1826978 and CBET-1916380).
文摘While dielectric-barrier-discharge(DBD)based plasma actuation systems have been successfully demonstrated to suppress massive flow separation over wind turbine blades to reduce the transient aerodynamic loadings acting on the turbine blades,it is still a non-trivial task to establish a best combination of various operating parameters for a DBD plasma actuation system to achieve the optimized flow control effectiveness.In the present study,a regression Kriging based metamodeling technique is developed to optimize the operating parameters of a DBD plasma actuation system for suppressing deep stall over the surface of a wind turbine blade section/airfoil model.The data points were experimentally obtained by embedding a nanosecond-pulsed DBD(NS-DBD)plasma actuator at the leading edge of the airfoil model.The applied voltage and frequency for the NS-DBD plasma actuation were used as the design variables to demonstrate the optimization procedure.The highest possible lift coefficient of the turbine airfoil model at deep stalled angles of attack(i.e.,α?=?22°and 24°)were selected as the objective function for the optimization.It was found that,while the metamodeling-based procedure could accurately predict the objective function within the bounds of the design variables with an uncertainty~?2%,a global accuracy level of~?97%was achieved within the whole design space.
基金supported by National Natural Science Foundation of China(Nos.11505019,21173028)the Science and Technology Research Project of Liaoning Provincial Education Department(No.L2013464)+1 种基金the Scientific Research Foundation for the Doctor of Liaoning Province(No.20131004)the Dalian Jinzhou New District Science and Technology Plan Project(No.KJCX-ZTPY-2014-0001)
文摘Cold plasma generated by dielectric barrier discharge (DBD) at atmospheric pressure was adopted for preparation of commercial TiO2 Degussa P25 supported Au catalysts (Au/P25- P) with the assistance of the deposition-precipitation procedure. The influences of the plasma reduction time and calcination on the performance of the Au/P25-P catalysts were investigated. CO oxidation was performed to investigate the catalytic activity of the Au/P25 catalysts. The results show that DBD cold plasma for the fabrication of Au/P25-P catalysts is a fast process, and Au/P25-P (4 min) exhibited the highest CO oxidation activity due to the complete reduction of Au compounds and less consumption of oxygen vacancies. In order to form more oxygen vacancies active species, Au/P25-P was calcined to obtain Au/P25-PC catalysts. Interestingly, Au/P25- PC exhibited the highest activity for CO oxidation among the Au/P25 samples. The results of transmission electron microscopy (TEM) indicated that the smaller size and high distribution of Au nanoparticles are the mean reasons for a high performance of Au/P25-PC. Atmospheric- pressure DBD cold plasma was proved to be of great efficiency in preparing high performance supported Au catalysts.