There are significant differences in the extent of impurity incorporation on different crystallographic directions of GaN microstructures,and the impurity-related deep energy level behavior will have a significant imp...There are significant differences in the extent of impurity incorporation on different crystallographic directions of GaN microstructures,and the impurity-related deep energy level behavior will have a significant impact on device performance.However,a comprehensive understanding of the effect of lateral growth on device performance has not been achieved due to the lack of comprehensive spatial distribution characterization of the optical behavior and impurity incorporation in GaN microstructures.We present a comprehensive study of the optical behavior and growth mechanism of self-assembled GaN microdisks using nanoscale spatially resolved cathodoluminescence(CL)mapping.We have found a clear growth orientation-dependent optical behavior of the lateral and vertical growth sectors of self-assembled GaN microcrystals.The lateral growth sector,i.e.,the{101¯1}-growth sector,forms six side facets of the microdisk and shows significant near-bandgap emission(NBE)and weak deep energy level luminescence.Cavity effect enhanced emission was found for the first time in such a truncated hexagonal Na-flux GaN microdisk system with an ultra-smooth surface(Ra<0.7 nm)and low stress.The self-assembled microdisk shows significant ultraviolet(UV)lasing action(main lasing peak wavelength 370.9 nm,quality factor 1278,threshold 6×10^(4)μJ/cm^(2))under pulsed optical pumping.We believe that the appearance of UV lasing action may be related to the light limitation on the six side facets of the lateral growth of the GaN microdisk,the high structural quality,the low content of deep energy level defects,the low surface roughness,and the low stress.展开更多
The III-nitride semiconductor microdisk laser exhibits high quality factor and low excitation threshold with broad development potential in the field of nanophotonics such as nanoscale light-emitting devices and on-ch...The III-nitride semiconductor microdisk laser exhibits high quality factor and low excitation threshold with broad development potential in the field of nanophotonics such as nanoscale light-emitting devices and on-chip optical integration.So far,many works have been focused on process synthesis and nanostructural design of microdisk lasers.Nevertheless,there are still some limitations in the existing optical resonance mode which is an important internal influence factor for lasing characteristics.In this work,a new double-triangular whispering-gallery mode(D3-WGM)lasing from a hexagonal GaN microdisk with a high quality(Q)factor of 3049 and an excitation threshold of around 11.5μW has been experimentally demonstrated.In addition,the optical properties of hexagonal-WGM(6-WGM),triangular-WGM(3-WGM)and D3-WGM lasing from microdisk are explored by numerical calculation and Comsol simulation.These results confirm that the D3-WGM lasing has its own significant performance advantages,namely high Q factor and easy light emission.Based on this novel laser mode characteristic,microcavity lasers are expected to be further developed and applied in the field of nanophotonics.展开更多
基金This work was supported by the National Key R&D Program of China(No.2021YFB3602000)the Fundamental Research Funds for the Central Universities(No.WK5290000003).
文摘There are significant differences in the extent of impurity incorporation on different crystallographic directions of GaN microstructures,and the impurity-related deep energy level behavior will have a significant impact on device performance.However,a comprehensive understanding of the effect of lateral growth on device performance has not been achieved due to the lack of comprehensive spatial distribution characterization of the optical behavior and impurity incorporation in GaN microstructures.We present a comprehensive study of the optical behavior and growth mechanism of self-assembled GaN microdisks using nanoscale spatially resolved cathodoluminescence(CL)mapping.We have found a clear growth orientation-dependent optical behavior of the lateral and vertical growth sectors of self-assembled GaN microcrystals.The lateral growth sector,i.e.,the{101¯1}-growth sector,forms six side facets of the microdisk and shows significant near-bandgap emission(NBE)and weak deep energy level luminescence.Cavity effect enhanced emission was found for the first time in such a truncated hexagonal Na-flux GaN microdisk system with an ultra-smooth surface(Ra<0.7 nm)and low stress.The self-assembled microdisk shows significant ultraviolet(UV)lasing action(main lasing peak wavelength 370.9 nm,quality factor 1278,threshold 6×10^(4)μJ/cm^(2))under pulsed optical pumping.We believe that the appearance of UV lasing action may be related to the light limitation on the six side facets of the lateral growth of the GaN microdisk,the high structural quality,the low content of deep energy level defects,the low surface roughness,and the low stress.
基金supported financially by the State Key Program of National Natural Science Foundation of China(No.61734008)the National Natural Science Foundation of China(Nos.61574097,61604170 and 61604169)+1 种基金the National Key Research and Development Program of China(Nos.2016YFA0201101 and 2017YFB0404100)the National Key Scientific Instrument and Equipment Development Project(No.11327804)。
文摘The III-nitride semiconductor microdisk laser exhibits high quality factor and low excitation threshold with broad development potential in the field of nanophotonics such as nanoscale light-emitting devices and on-chip optical integration.So far,many works have been focused on process synthesis and nanostructural design of microdisk lasers.Nevertheless,there are still some limitations in the existing optical resonance mode which is an important internal influence factor for lasing characteristics.In this work,a new double-triangular whispering-gallery mode(D3-WGM)lasing from a hexagonal GaN microdisk with a high quality(Q)factor of 3049 and an excitation threshold of around 11.5μW has been experimentally demonstrated.In addition,the optical properties of hexagonal-WGM(6-WGM),triangular-WGM(3-WGM)and D3-WGM lasing from microdisk are explored by numerical calculation and Comsol simulation.These results confirm that the D3-WGM lasing has its own significant performance advantages,namely high Q factor and easy light emission.Based on this novel laser mode characteristic,microcavity lasers are expected to be further developed and applied in the field of nanophotonics.