To correct the light scattering property parameters of milk fat for improving the detection accuracy,the Mie-theory was used to establish a predictive model for light scattering properties of milk fat globule with mul...To correct the light scattering property parameters of milk fat for improving the detection accuracy,the Mie-theory was used to establish a predictive model for light scattering properties of milk fat globule with multi-diameter distributions, by means of Monte Carlo approach to simulate actual multi-diameter size distribution of milk fat globule in milk fat solution. Scattering coefficient and absorption coefficient of multidiameter distribution milk fat particles were calculated by simulating the particles size distribution in milk fat solution. And the light scattering properties of multi-diameter distribution was compared with that of volume mean diameter,Sauter mean diameter and numerical mean diameter in milk fat solution. Theoretical simulation results indicate that the scattering coefficient and absorption coefficient of milk fat particles are determined by the particle size distribution in milk fat solution. There is a distinct difference in scattering characteristics between the milk fat particles with multi-diameter distribution and that with mean diameters. Compared to that with multi-diameter distribution,the scattering coefficient of the milk fat particles with mean diameter has a maximum mean deviation of 9042 m-1. The particle size distribution is not completely determined by the mean diameters. The dependence of the light scattering properties on the particle size distribution should be considered into the model and simulation. Therefore,it is found that the particle size distribution in milk fat solution is an essential and critical factor to significantly improve the detection accuracy of milk fat content.展开更多
When a laser is transmitted in fog, and the water droplets will scatter and absorb the laser, which affects the intensity of the laser transmission and the accuracy of radar detection. Therefore, it is of great signif...When a laser is transmitted in fog, and the water droplets will scatter and absorb the laser, which affects the intensity of the laser transmission and the accuracy of radar detection. Therefore, it is of great significance to study the laser transmission in the fog. At present, the main method of calculating the scattering and attenuation characteristics of fog is based on the radiation transmission theory, which is realized by a large number of numerical calculations or physical simulation methods, which takes time and cannot meet the requirements for obtaining the fast and accurate results. Therefore, in this paper established are a new laser forward attenuation model and backward attenuation model in low visibility fog. It is found that in low visibility environments, the results calculated by the Monte Carlo method are more accurate than those from most of the existing forward attenuation models. For the cases of 0.86-μm, 1.06-μm, 1.315-μm, 10.6-μm typical lasers incident on different fogs with different visibilities, a backscatter model is established, the error between the fitting result and the calculation result is analyzed, the backward attenuation fitting parameters of the new model are tested, and a more accurate fitting result is obtained.展开更多
Localized surface electromagnetic resonances in spherical nanoparticles with gain are investigated by using the Mie theory. Due to the coupling between the gain and resonances, super scattering phenomenon is raised an...Localized surface electromagnetic resonances in spherical nanoparticles with gain are investigated by using the Mie theory. Due to the coupling between the gain and resonances, super scattering phenomenon is raised and the total scattering efficiency is increased by over six orders of magnitude. The dual frequency resonance induced by the electric dipole term of the particle is observed. The distributions of electromagnetic field and the Poynting vector around nanoparticles are provided for better understanding different multipole resonances. Finally, the scattering properties of active spherical nanoparticles are investigated when the sizes of nanoparticles are beyond the quasi-static limit. It is noticed that more highorder multipole resonances can be excited with the increase of the radius. Besides, all resonances dominated by multipole magnetic terms can only appear in dielectric materials.展开更多
This paper proposes a method for predicting the reduced scattering coefficients of tissuesimulating phantoms or the desired amount of scatters for producing phantoms according to Mie scattering theory without measurem...This paper proposes a method for predicting the reduced scattering coefficients of tissuesimulating phantoms or the desired amount of scatters for producing phantoms according to Mie scattering theory without measurements with other instruments.The concentration of the scatters TiO2 particles is determined according to Mie theory calculation and added to transparent host epoxy resin to produce phantoms with different reduced scattering coefficients.Black India Ink is added to alter the absorption coefficients of the phantoms.The reduced scattering coefficients of phantoms are measured with single integrating sphere system.The results show that the measurements are in direct proportion to the concentration of TiO2 and have identical with Mie theory calculation at multiple wavelengths.The method proposed can accurately determine the concentration of scatters in the phantoms to ensure the phantoms are qualified with desired reduced scattering coefficients at specified wavelength.This investigation should be possible to manufacture the phantom simply in reasonably accurate for evaluation of biomedical optical imaging systems.展开更多
Two assumptions are typically made when radar echo signals from precipitation are analyzed to determine the micro-physical parameters of raindrops:(1) the raindrops are assumed to be spherical;(2) multiple scattering ...Two assumptions are typically made when radar echo signals from precipitation are analyzed to determine the micro-physical parameters of raindrops:(1) the raindrops are assumed to be spherical;(2) multiple scattering effects are ignored. Radar cross sections(RCS) are usually calculated using Rayleigh's scattering equation with the simple addition method in the radar meteorological equation.We investigate the extent to which consideration of the effects of multiple scattering and of the non-spherical shapes within actual raindrop swarms would result in RCS values significantly different from those obtained by conventional analytical methods. First, we establish spherical and non-spherical raindrop models, with Gamma, JD, JT, and MP size distributions, respectively. We then use XFDTD software to calculate the radar cross sections of the above raindrop models at the S, C, X and Ku radar bands. Our XFDTD results are then compared to RCS values calculated by the Rayleigh approximation with simple addition methods. We find that:(1) RCS values calculated using multiple scattering XFDTD software differ significantly from those calculated by the simple addition method at the same band for the same model. In particular, for the spherical raindrop models, the relative differences in RCS values between the methods range from a maximum of 89.649% to a minimum of 43.701%; for the non-spherical raindrop models, the relative differences range from a maximum of 85.868% to a minimum of 11.875%.(2) Our multiple scattering XFDTD results, compared to those obtained from the Rayleigh formula,again differ at all four size distributions, by relative errors of 169.522%, 37.176%, 216.455%, and 63.428%, respectively. When nonspherical effects are considered, differences in RCS values between our XFDTD calculations and Rayleigh calculations are smaller; at the above four size distributions the relative errors are 0.213%, 0.171%, 7.683%, and 44.514%, respectively. RCS values computed by considering multiple scattering and non-spherical particle shapes are larger than Rayleigh RCS results, at all of the above four size distributions; the relative errors between the two methods are 220.673%, 129.320%, 387.240%, and 186.613%, respectively. After changing the arrangement of particles at four size distributions in the case of multiple scattering effect and non-spherical effect, the RCS values of Arrangement 2 are smaller than those of Arrangement 1; the relative errors for Arrangement 2, compared to Rayleigh, are 60.558%, 76.263%, 85.941%,64.852%, respectively. We have demonstrated that multiple scattering, non-spherical particle shapes, and the arrangement within particle swarms all affect the calculation of RCS values. The largest influence appears to be that of the multiple scattering effect.Consideration of particle shapes appears to have the least influence on computed RCS values. We conclude that multiple scattering effects must be considered in practical meteorological detection.展开更多
Some field experimental results have shown that the moving sands or dust aerosols in nature are usually electrified,and those charged particles also produce a strong electric field in air, which is named as wind-blown...Some field experimental results have shown that the moving sands or dust aerosols in nature are usually electrified,and those charged particles also produce a strong electric field in air, which is named as wind-blown sand electric field.Some scholars have pointed out that the net charge on the particle significantly enhances its electromagnetic(EM) extinction properties, but up to now, there is no conclusive research on the effect of the environmental electric field. Based on the extended Mie theory, the effect of the electric field in a sandstorm on the EM attenuation properties of the charged larger dust particle is studied. The numerical results indicate that the environmental electric field also has a great influence on the particle's optical properties, and the stronger the electric field, the bigger the effect. In addition, the charged angle, the charge density, and the particle radius all have a specific impact on the charged particle's optical properties.展开更多
More stable and accurate recursive formulas and a computing procedure for scat-tering coefficient calculation of a multilayered sphere are proposed, This procedure involves threelogarithmic derivatives of Ricatti-Bess...More stable and accurate recursive formulas and a computing procedure for scat-tering coefficient calculation of a multilayered sphere are proposed, This procedure involves threelogarithmic derivatives of Ricatti-Bessel function ψ_n~'(z)/ ψ_n(z), X_n~'(z)/X_n(z),ξ_n~'(z)/ ξ_n(z), as wellas the ratioψ_n(z)/X_n(z). The asymptotic behavior, stability, and accuracy of the procedureand scattering coefficients a_n and b_n are discussed for various complex refractive indices. Thisprocedure can be applied to large and small inhomogeneous spherical particles.展开更多
It is of both the theoretical and practical importance to reduce the storage andCPU time of moment methods by utilizing the geometrical and physical features of the scatterer.An unified approach based on the group the...It is of both the theoretical and practical importance to reduce the storage andCPU time of moment methods by utilizing the geometrical and physical features of the scatterer.An unified approach based on the group theory is presented to deal with the EM scattering fromsymmetric and anti-symmetric structures.展开更多
Near-infrared spectroscopy(NIRS)technology and Mie theory are utilized for fundamental research on radiofrequency ablation of biological tissue.Firstly,NIRS is utilized to monitor rats undergoing radiofrequency ablati...Near-infrared spectroscopy(NIRS)technology and Mie theory are utilized for fundamental research on radiofrequency ablation of biological tissue.Firstly,NIRS is utilized to monitor rats undergoing radiofrequency ablation surgery in real time so as to explore the relationship between reduced scattering coefficient(μ_(s)')and the degree of thermally induced tissue coagulation.Then,Mie theory is utilized to analyze the morphological structure change of biological tissue so as to explore the basic mechanism of the change of optical parameters caused by thermally induced tissue coagulation.Results show that there is a close relationship between μ_(s)' and the degree of thermally induced tissue coagulation;the degree of thermal coagulation can be obtained by the value of μ_(s)';when biological tissue thermally coagulates,the average equivalent scattering particle decreases,the particle density increases,and the anisotropy factor decreases.展开更多
The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unav...The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.展开更多
The optical absorption of semiconducting AgBr nanocubes is significantly increased by up to 5 times in the measured spectral range when they are bonded to the surface of dielectric SiO2 nanospheres through electrostat...The optical absorption of semiconducting AgBr nanocubes is significantly increased by up to 5 times in the measured spectral range when they are bonded to the surface of dielectric SiO2 nanospheres through electrostatic interaction. The absorption enhancement factor depends on the wavelength and the size of the SiO2 nanoparticles (NPs). Finite-difference time-domain calculations provide the nearfield intensity mapping of a heterostructure that is composed of a AgBr nanocube in close contact with a SiO2 nanosphere. The electric-field distributions indicate the field enhancement near the SiO2/AgBr interface due to light scattering and absorption enhancement in the AgBr nanocube, implying that the enhanced scattering nearfield increases the absorption cross section of the AgBr nanocube. The absorption cross-section spectra calculated using Mie theory agree with the experimental observations. This discovery sheds light on the utilization of dielectric spherical particles to increase the absorption in semiconductor NPs, thus improving the light-harvesting efficiency for solar-energy conversion.展开更多
Light scattering by small particles has a long and interesting history in physics.Nonetheless,it continues to surprise with new insights and applications.This includes new discoveries,such as novel plasmonic effects,a...Light scattering by small particles has a long and interesting history in physics.Nonetheless,it continues to surprise with new insights and applications.This includes new discoveries,such as novel plasmonic effects,as well as exciting theoretical and experimental developments such as optical trapping,anomalous light scattering,optical tweezers,nanospasers,and novel aspects and realizations of Fano resonances.These have led to important new applications,including several ones in the biomedical area and in sensing techniques at the single-molecule level.There are additionally many potential future applications in optical devices and solar energy technologies.Here we review the fundamental aspects of light scattering by small spherical particles,emphasizing the phenomenological treatments and new developments in this field.展开更多
基金Sponsored by the National Natural Science Foundation of China(Grant No.51206038)the Scientific Research Fund of Heilongjiang Provincial Education Department(Grant No.12521122)
文摘To correct the light scattering property parameters of milk fat for improving the detection accuracy,the Mie-theory was used to establish a predictive model for light scattering properties of milk fat globule with multi-diameter distributions, by means of Monte Carlo approach to simulate actual multi-diameter size distribution of milk fat globule in milk fat solution. Scattering coefficient and absorption coefficient of multidiameter distribution milk fat particles were calculated by simulating the particles size distribution in milk fat solution. And the light scattering properties of multi-diameter distribution was compared with that of volume mean diameter,Sauter mean diameter and numerical mean diameter in milk fat solution. Theoretical simulation results indicate that the scattering coefficient and absorption coefficient of milk fat particles are determined by the particle size distribution in milk fat solution. There is a distinct difference in scattering characteristics between the milk fat particles with multi-diameter distribution and that with mean diameters. Compared to that with multi-diameter distribution,the scattering coefficient of the milk fat particles with mean diameter has a maximum mean deviation of 9042 m-1. The particle size distribution is not completely determined by the mean diameters. The dependence of the light scattering properties on the particle size distribution should be considered into the model and simulation. Therefore,it is found that the particle size distribution in milk fat solution is an essential and critical factor to significantly improve the detection accuracy of milk fat content.
基金supported by the National Natural Science Foundation of China (Grant Nos. 61571355 and 61401342)。
文摘When a laser is transmitted in fog, and the water droplets will scatter and absorb the laser, which affects the intensity of the laser transmission and the accuracy of radar detection. Therefore, it is of great significance to study the laser transmission in the fog. At present, the main method of calculating the scattering and attenuation characteristics of fog is based on the radiation transmission theory, which is realized by a large number of numerical calculations or physical simulation methods, which takes time and cannot meet the requirements for obtaining the fast and accurate results. Therefore, in this paper established are a new laser forward attenuation model and backward attenuation model in low visibility fog. It is found that in low visibility environments, the results calculated by the Monte Carlo method are more accurate than those from most of the existing forward attenuation models. For the cases of 0.86-μm, 1.06-μm, 1.315-μm, 10.6-μm typical lasers incident on different fogs with different visibilities, a backscatter model is established, the error between the fitting result and the calculation result is analyzed, the backward attenuation fitting parameters of the new model are tested, and a more accurate fitting result is obtained.
基金supported by the National Natural Science Foundation of China(Grant Nos.11174222 and 91230203)
文摘Localized surface electromagnetic resonances in spherical nanoparticles with gain are investigated by using the Mie theory. Due to the coupling between the gain and resonances, super scattering phenomenon is raised and the total scattering efficiency is increased by over six orders of magnitude. The dual frequency resonance induced by the electric dipole term of the particle is observed. The distributions of electromagnetic field and the Poynting vector around nanoparticles are provided for better understanding different multipole resonances. Finally, the scattering properties of active spherical nanoparticles are investigated when the sizes of nanoparticles are beyond the quasi-static limit. It is noticed that more highorder multipole resonances can be excited with the increase of the radius. Besides, all resonances dominated by multipole magnetic terms can only appear in dielectric materials.
基金supported by National High-Tech Research and Development Project(863)of China(2006AA020801).
文摘This paper proposes a method for predicting the reduced scattering coefficients of tissuesimulating phantoms or the desired amount of scatters for producing phantoms according to Mie scattering theory without measurements with other instruments.The concentration of the scatters TiO2 particles is determined according to Mie theory calculation and added to transparent host epoxy resin to produce phantoms with different reduced scattering coefficients.Black India Ink is added to alter the absorption coefficients of the phantoms.The reduced scattering coefficients of phantoms are measured with single integrating sphere system.The results show that the measurements are in direct proportion to the concentration of TiO2 and have identical with Mie theory calculation at multiple wavelengths.The method proposed can accurately determine the concentration of scatters in the phantoms to ensure the phantoms are qualified with desired reduced scattering coefficients at specified wavelength.This investigation should be possible to manufacture the phantom simply in reasonably accurate for evaluation of biomedical optical imaging systems.
基金supported by the Natural Science Foundation of Jiangsu Province (Grant No. BK20170945)the National Natural Science Foundation of China (Grant Nos. 41675029+6 种基金 41275004 61372066 41571348)National Key Laboratory of Disaster Weather, China Academy of Meteorological Sciences (2016LASW-B12)the Key Laboratory for Aerosol-Cloud-Precipitation of CMA-NUIST (KDW1703)the Startup Foundation for Introducing Talent of Nanjing University of Information Science and Technology (2016r028)Earth Science Virtual Simulation Experiment Teaching Course Construction Project of Nanjing University of Information Science and Technology (XNFZ2017C02)
文摘Two assumptions are typically made when radar echo signals from precipitation are analyzed to determine the micro-physical parameters of raindrops:(1) the raindrops are assumed to be spherical;(2) multiple scattering effects are ignored. Radar cross sections(RCS) are usually calculated using Rayleigh's scattering equation with the simple addition method in the radar meteorological equation.We investigate the extent to which consideration of the effects of multiple scattering and of the non-spherical shapes within actual raindrop swarms would result in RCS values significantly different from those obtained by conventional analytical methods. First, we establish spherical and non-spherical raindrop models, with Gamma, JD, JT, and MP size distributions, respectively. We then use XFDTD software to calculate the radar cross sections of the above raindrop models at the S, C, X and Ku radar bands. Our XFDTD results are then compared to RCS values calculated by the Rayleigh approximation with simple addition methods. We find that:(1) RCS values calculated using multiple scattering XFDTD software differ significantly from those calculated by the simple addition method at the same band for the same model. In particular, for the spherical raindrop models, the relative differences in RCS values between the methods range from a maximum of 89.649% to a minimum of 43.701%; for the non-spherical raindrop models, the relative differences range from a maximum of 85.868% to a minimum of 11.875%.(2) Our multiple scattering XFDTD results, compared to those obtained from the Rayleigh formula,again differ at all four size distributions, by relative errors of 169.522%, 37.176%, 216.455%, and 63.428%, respectively. When nonspherical effects are considered, differences in RCS values between our XFDTD calculations and Rayleigh calculations are smaller; at the above four size distributions the relative errors are 0.213%, 0.171%, 7.683%, and 44.514%, respectively. RCS values computed by considering multiple scattering and non-spherical particle shapes are larger than Rayleigh RCS results, at all of the above four size distributions; the relative errors between the two methods are 220.673%, 129.320%, 387.240%, and 186.613%, respectively. After changing the arrangement of particles at four size distributions in the case of multiple scattering effect and non-spherical effect, the RCS values of Arrangement 2 are smaller than those of Arrangement 1; the relative errors for Arrangement 2, compared to Rayleigh, are 60.558%, 76.263%, 85.941%,64.852%, respectively. We have demonstrated that multiple scattering, non-spherical particle shapes, and the arrangement within particle swarms all affect the calculation of RCS values. The largest influence appears to be that of the multiple scattering effect.Consideration of particle shapes appears to have the least influence on computed RCS values. We conclude that multiple scattering effects must be considered in practical meteorological detection.
基金supported by the National Natural Science Foundation of China(Grant Nos.11562017 and 11302111)the CAS "Light of West China" Program(Grant No.XAB2017AW03)the Major Innovation Projects for Building First-class Universities in China’s Western Region(Grant No.ZKZD2017006)
文摘Some field experimental results have shown that the moving sands or dust aerosols in nature are usually electrified,and those charged particles also produce a strong electric field in air, which is named as wind-blown sand electric field.Some scholars have pointed out that the net charge on the particle significantly enhances its electromagnetic(EM) extinction properties, but up to now, there is no conclusive research on the effect of the environmental electric field. Based on the extended Mie theory, the effect of the electric field in a sandstorm on the EM attenuation properties of the charged larger dust particle is studied. The numerical results indicate that the environmental electric field also has a great influence on the particle's optical properties, and the stronger the electric field, the bigger the effect. In addition, the charged angle, the charge density, and the particle radius all have a specific impact on the charged particle's optical properties.
基金Supported by the National Natural Science Foundation of China
文摘More stable and accurate recursive formulas and a computing procedure for scat-tering coefficient calculation of a multilayered sphere are proposed, This procedure involves threelogarithmic derivatives of Ricatti-Bessel function ψ_n~'(z)/ ψ_n(z), X_n~'(z)/X_n(z),ξ_n~'(z)/ ξ_n(z), as wellas the ratioψ_n(z)/X_n(z). The asymptotic behavior, stability, and accuracy of the procedureand scattering coefficients a_n and b_n are discussed for various complex refractive indices. Thisprocedure can be applied to large and small inhomogeneous spherical particles.
文摘It is of both the theoretical and practical importance to reduce the storage andCPU time of moment methods by utilizing the geometrical and physical features of the scatterer.An unified approach based on the group theory is presented to deal with the EM scattering fromsymmetric and anti-symmetric structures.
基金supported by the National Natural Science Foundation(Grant No.30671997)the National High Technology Research and Development Program of China(No.2008AA02Z438).
文摘Near-infrared spectroscopy(NIRS)technology and Mie theory are utilized for fundamental research on radiofrequency ablation of biological tissue.Firstly,NIRS is utilized to monitor rats undergoing radiofrequency ablation surgery in real time so as to explore the relationship between reduced scattering coefficient(μ_(s)')and the degree of thermally induced tissue coagulation.Then,Mie theory is utilized to analyze the morphological structure change of biological tissue so as to explore the basic mechanism of the change of optical parameters caused by thermally induced tissue coagulation.Results show that there is a close relationship between μ_(s)' and the degree of thermally induced tissue coagulation;the degree of thermal coagulation can be obtained by the value of μ_(s)';when biological tissue thermally coagulates,the average equivalent scattering particle decreases,the particle density increases,and the anisotropy factor decreases.
基金support from the National Natural Science Foundation of China (No. 50876069)the Ministry of Education of the People’s Republic of China (No.208041)from the Shanghai Municipal Education Commis-sion (No. 07ZZ88)
文摘The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.
文摘The optical absorption of semiconducting AgBr nanocubes is significantly increased by up to 5 times in the measured spectral range when they are bonded to the surface of dielectric SiO2 nanospheres through electrostatic interaction. The absorption enhancement factor depends on the wavelength and the size of the SiO2 nanoparticles (NPs). Finite-difference time-domain calculations provide the nearfield intensity mapping of a heterostructure that is composed of a AgBr nanocube in close contact with a SiO2 nanosphere. The electric-field distributions indicate the field enhancement near the SiO2/AgBr interface due to light scattering and absorption enhancement in the AgBr nanocube, implying that the enhanced scattering nearfield increases the absorption cross section of the AgBr nanocube. The absorption cross-section spectra calculated using Mie theory agree with the experimental observations. This discovery sheds light on the utilization of dielectric spherical particles to increase the absorption in semiconductor NPs, thus improving the light-harvesting efficiency for solar-energy conversion.
基金Work at ORNL was supported by the United States Department of Energy,Basic Energy Sciences,Materials Sciences and Engineering Division.
文摘Light scattering by small particles has a long and interesting history in physics.Nonetheless,it continues to surprise with new insights and applications.This includes new discoveries,such as novel plasmonic effects,as well as exciting theoretical and experimental developments such as optical trapping,anomalous light scattering,optical tweezers,nanospasers,and novel aspects and realizations of Fano resonances.These have led to important new applications,including several ones in the biomedical area and in sensing techniques at the single-molecule level.There are additionally many potential future applications in optical devices and solar energy technologies.Here we review the fundamental aspects of light scattering by small spherical particles,emphasizing the phenomenological treatments and new developments in this field.