In order to understand the recycling and emission processes of hydrogen atoms in HT 7, spectral profiles of the Dα(Hα) line emitted in front of the limiter have been observed with a high-resolution spectrometer an...In order to understand the recycling and emission processes of hydrogen atoms in HT 7, spectral profiles of the Dα(Hα) line emitted in front of the limiter have been observed with a high-resolution spectrometer and simulated by using the neutral particle transport code DEGAS 2. The results show that four processes are necessary to interpret the Dα(Hα) line shape: 1) atom desorption, 2) molecular dissociation, 3) particle reflection, and 4) charge-exchange. The products of the first two processes are cold atoms which emit photons near the peak of Dα(Hα) line shape, and those from the last two are warm atoms contributing to the blue side of the spectrum. For a typical ohmic discharge (shot 68520 ne(0) ≈ 3× 10^19 m^-3. these components contribute 32%, 15%, 32% and 21%, respectively. Dα(Hα) line shapes under different plasma parameters are also discussed in this paper.展开更多
Hα(Balmer-alpha), Hβ (Balmer-beta) and Hγ (Balmer-gamma) spectral line inten- sities in atomic hydrogen plasma are investigated by using a high-power RF source. The intensities of the Hα, Hβ and Hγ spectra...Hα(Balmer-alpha), Hβ (Balmer-beta) and Hγ (Balmer-gamma) spectral line inten- sities in atomic hydrogen plasma are investigated by using a high-power RF source. The intensities of the Hα, Hβ and Hγ spectral lines are detected by increasing the input power (0-6 kW) of ICPs (inductively coupled plasmas). With the increase of net input power, the intensity of Hα im- proves rapidly (0-2 kW), and then reaches its dynamic equilibrium; the intensities of Hβ can be divided into three processes: obvious increase (0-2 kW), rapid increase (2-4 kW), almost constant (4-6 kW); while the intensities of Hγ increase very slowly. The energy levels of the excited hydro- gen atoms and the splitting energy levels produced by an obvious Stark effect play an important role in the results.展开更多
The electron density and temperature of the laser induced silicon plasma were measured using two different methods. The plasma was produced via the interaction of high peak power Nd-YAG laser at the fundamental wavele...The electron density and temperature of the laser induced silicon plasma were measured using two different methods. The plasma was produced via the interaction of high peak power Nd-YAG laser at the fundamental wavelength of 1064 nm with a plane solid iron target contain small traces of silicon as an element of minor concentration. The lines from the Si I at 288.15 nm and Si II-ionic lines at 413.08 and 634.71 nm were utilized to evaluate the plasma parameters. The reference plasma parameters were measured utilizing the Hα-line at 656.27 nm appeared in the spectra under the same condition. The electron density was measured utilizing the Stark broadening of the silicon lines and the temperature from the standard Saha-Boltzmann plot method. The comparison between electron densities from different silicon lines to that from the Hα-line reveals that the Si I-line at 288.15 nm contain some optical thickness while the Si II-ionic lines were found to be free from this effect. The measurements were repeated at different delay times between the laser and the camera in the range from 1 - 5 μsec. The electron density was found decreases from 2 × 1018 down to 4 × 1017 cm–3. After correcting the spectral intensity at the Si I-line at 288.15 nm, the temperatures evaluated from the different methods were found in an excellent agreement and decreases from 1.25 down to 0.95 eV with delay time.展开更多
In this article, we will report an experimental evidence of enhanced LIBS emission upon replacing a Bulk-Based ZnO target by the corresponding Nano-Based target. The plasma was initiated via interaction of a Nd:YAG la...In this article, we will report an experimental evidence of enhanced LIBS emission upon replacing a Bulk-Based ZnO target by the corresponding Nano-Based target. The plasma was initiated via interaction of a Nd:YAG laser at the fundamental wavelength with both targets in open air under the same experimental conditions. The measurements show an enhanced emission from the Zn I-lines at the wavelengths of 328.26, 330.29, 334.55, 468.06, 472.2, 481.01, 636.38 nm. The measurements were repeated at different delay times in the range from 1 to 5 μs at constant irradiation level and fixed gate time of 1 μs. The average enhancement over the different Zn I-lines was found increases exponentially up to 8-fold with delay time. The electron density to each plasma was measured utilizing the Hα-line appeared in the emitted spectra from each plasma and was found to give similar values. The electron temperatures were measured via Boltzmann plot method utilizing the relative intensities of the Zn I-lines and were found to give very close values. Moreover, the relative population density of the ground state of the zinc atoms (relative concentration) was measured spectroscopically utilizing the Boltzmann plot method and was found to increase in a very similar trend to that of enhancement. The results of the spectroscopic analysis conclude that these signal enhancements can be attributed to the higher concentration of neutral atoms in the Nano-Based material plasma with respect to the corresponding Bulk-based ZnO material.展开更多
A Software program has been developed in order to perform a fast and reliable calculation to plasma electron density in laser induced breakdown spectroscopy (LIBS) experiments. This program is based on analyzing the e...A Software program has been developed in order to perform a fast and reliable calculation to plasma electron density in laser induced breakdown spectroscopy (LIBS) experiments. This program is based on analyzing the emitted spectral line shape via utilizing facilities of the MatLab7? package to perform this task. This software can perform the following tasks;read the exported data file (*txt-format) from ICCD camera-software, specify the working wavelength of interest, removes the continuum emission component appeared under the line, calculates the spectral line intensity of the line, calculates the spectral shift of the line from the tabulated values, correct against spectral shift jitter at the peak emission, de-convoluting and extracting the different components contributing to the emitted line full width at half of the maximum (FWHM) and finally calculates the plasma electron density. In this article we shall present the results of the test measurement of the plasma electron density utilizing spectral line shape analysis to the emitted Hα-line, Si I-line at 288.15 nm and O I-line at 777.2 nm at different camera delay times ranging from 1 to 5 μs.展开更多
We compare Balmer-alpha (Ha) and Balmer-beta (Hβ) emissions from high-power (1.0-6.0 kW) hydrogen inductively coupled plasmas (ICPs), and propose region Ⅰ (0.0-2.0 kW), region Ⅱ (2.0-5.0 kW), and region...We compare Balmer-alpha (Ha) and Balmer-beta (Hβ) emissions from high-power (1.0-6.0 kW) hydrogen inductively coupled plasmas (ICPs), and propose region Ⅰ (0.0-2.0 kW), region Ⅱ (2.0-5.0 kW), and region Ⅲ (5.0-6.0 kW). In region Ⅰ, both Ha emission intensity (la) and Hβ emission intensity (1β) increase with radio frequency (RF) power, which is explained by the corona model and Boltzmann's law, etc. However, in region II, la almost remains constant while 1β rapidly achieves its maximum value. In region Ⅲ, 1α slightly increases with RF power, while 1β decreases with RF power, which deviates significantly from the theoretical explanation for the Ha and Hβ emissions in region I. It is suggested that two strong electric fields are generated in high-power (2.0-6.0 kW) hydrogen ICPs: one is due to the external electric field of high-power RF discharge, and the other one is due to the micro electric field of the ions and electrons around the exited state hydrogen atoms in ICPs. Therefore, the strong Stark effect can play an important role in explaining the experimental results.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No 10725523)
文摘In order to understand the recycling and emission processes of hydrogen atoms in HT 7, spectral profiles of the Dα(Hα) line emitted in front of the limiter have been observed with a high-resolution spectrometer and simulated by using the neutral particle transport code DEGAS 2. The results show that four processes are necessary to interpret the Dα(Hα) line shape: 1) atom desorption, 2) molecular dissociation, 3) particle reflection, and 4) charge-exchange. The products of the first two processes are cold atoms which emit photons near the peak of Dα(Hα) line shape, and those from the last two are warm atoms contributing to the blue side of the spectrum. For a typical ohmic discharge (shot 68520 ne(0) ≈ 3× 10^19 m^-3. these components contribute 32%, 15%, 32% and 21%, respectively. Dα(Hα) line shapes under different plasma parameters are also discussed in this paper.
基金supported by the National Magnetic Confinement Fusion Science Program of China(Nos.2011GB108011 and 2010GB103001)the Major International(Regional) Project Cooperation and Exchanges(No.11320101005)
文摘Hα(Balmer-alpha), Hβ (Balmer-beta) and Hγ (Balmer-gamma) spectral line inten- sities in atomic hydrogen plasma are investigated by using a high-power RF source. The intensities of the Hα, Hβ and Hγ spectral lines are detected by increasing the input power (0-6 kW) of ICPs (inductively coupled plasmas). With the increase of net input power, the intensity of Hα im- proves rapidly (0-2 kW), and then reaches its dynamic equilibrium; the intensities of Hβ can be divided into three processes: obvious increase (0-2 kW), rapid increase (2-4 kW), almost constant (4-6 kW); while the intensities of Hγ increase very slowly. The energy levels of the excited hydro- gen atoms and the splitting energy levels produced by an obvious Stark effect play an important role in the results.
文摘The electron density and temperature of the laser induced silicon plasma were measured using two different methods. The plasma was produced via the interaction of high peak power Nd-YAG laser at the fundamental wavelength of 1064 nm with a plane solid iron target contain small traces of silicon as an element of minor concentration. The lines from the Si I at 288.15 nm and Si II-ionic lines at 413.08 and 634.71 nm were utilized to evaluate the plasma parameters. The reference plasma parameters were measured utilizing the Hα-line at 656.27 nm appeared in the spectra under the same condition. The electron density was measured utilizing the Stark broadening of the silicon lines and the temperature from the standard Saha-Boltzmann plot method. The comparison between electron densities from different silicon lines to that from the Hα-line reveals that the Si I-line at 288.15 nm contain some optical thickness while the Si II-ionic lines were found to be free from this effect. The measurements were repeated at different delay times between the laser and the camera in the range from 1 - 5 μsec. The electron density was found decreases from 2 × 1018 down to 4 × 1017 cm–3. After correcting the spectral intensity at the Si I-line at 288.15 nm, the temperatures evaluated from the different methods were found in an excellent agreement and decreases from 1.25 down to 0.95 eV with delay time.
文摘In this article, we will report an experimental evidence of enhanced LIBS emission upon replacing a Bulk-Based ZnO target by the corresponding Nano-Based target. The plasma was initiated via interaction of a Nd:YAG laser at the fundamental wavelength with both targets in open air under the same experimental conditions. The measurements show an enhanced emission from the Zn I-lines at the wavelengths of 328.26, 330.29, 334.55, 468.06, 472.2, 481.01, 636.38 nm. The measurements were repeated at different delay times in the range from 1 to 5 μs at constant irradiation level and fixed gate time of 1 μs. The average enhancement over the different Zn I-lines was found increases exponentially up to 8-fold with delay time. The electron density to each plasma was measured utilizing the Hα-line appeared in the emitted spectra from each plasma and was found to give similar values. The electron temperatures were measured via Boltzmann plot method utilizing the relative intensities of the Zn I-lines and were found to give very close values. Moreover, the relative population density of the ground state of the zinc atoms (relative concentration) was measured spectroscopically utilizing the Boltzmann plot method and was found to increase in a very similar trend to that of enhancement. The results of the spectroscopic analysis conclude that these signal enhancements can be attributed to the higher concentration of neutral atoms in the Nano-Based material plasma with respect to the corresponding Bulk-based ZnO material.
文摘A Software program has been developed in order to perform a fast and reliable calculation to plasma electron density in laser induced breakdown spectroscopy (LIBS) experiments. This program is based on analyzing the emitted spectral line shape via utilizing facilities of the MatLab7? package to perform this task. This software can perform the following tasks;read the exported data file (*txt-format) from ICCD camera-software, specify the working wavelength of interest, removes the continuum emission component appeared under the line, calculates the spectral line intensity of the line, calculates the spectral shift of the line from the tabulated values, correct against spectral shift jitter at the peak emission, de-convoluting and extracting the different components contributing to the emitted line full width at half of the maximum (FWHM) and finally calculates the plasma electron density. In this article we shall present the results of the test measurement of the plasma electron density utilizing spectral line shape analysis to the emitted Hα-line, Si I-line at 288.15 nm and O I-line at 777.2 nm at different camera delay times ranging from 1 to 5 μs.
基金supported by the National Magnetic Confinement Fusion Science Program of China(Grant Nos.2011GB108011 and 2010GB103001)the MajorInternational(Regional)Project Cooperation and Exchanges(Grant No.11320101005)
文摘We compare Balmer-alpha (Ha) and Balmer-beta (Hβ) emissions from high-power (1.0-6.0 kW) hydrogen inductively coupled plasmas (ICPs), and propose region Ⅰ (0.0-2.0 kW), region Ⅱ (2.0-5.0 kW), and region Ⅲ (5.0-6.0 kW). In region Ⅰ, both Ha emission intensity (la) and Hβ emission intensity (1β) increase with radio frequency (RF) power, which is explained by the corona model and Boltzmann's law, etc. However, in region II, la almost remains constant while 1β rapidly achieves its maximum value. In region Ⅲ, 1α slightly increases with RF power, while 1β decreases with RF power, which deviates significantly from the theoretical explanation for the Ha and Hβ emissions in region I. It is suggested that two strong electric fields are generated in high-power (2.0-6.0 kW) hydrogen ICPs: one is due to the external electric field of high-power RF discharge, and the other one is due to the micro electric field of the ions and electrons around the exited state hydrogen atoms in ICPs. Therefore, the strong Stark effect can play an important role in explaining the experimental results.