In this article,an efficient,simple and environmentally friendly approach to the synthesis of diacetals(diketals) pentaerythritol using SOH-functionalized ionic liquids(ILs) as catalysts was reported.The ILs show high...In this article,an efficient,simple and environmentally friendly approach to the synthesis of diacetals(diketals) pentaerythritol using SOH-functionalized ionic liquids(ILs) as catalysts was reported.The ILs show high catalytic activity and reusability with good to excellent yields of the desired products.Hammett method has been used to determine the acidity order of these ionic liquids and the results are consistent with the catalytic activities observed in acetalization reaction.Maximum product yield of 93%was observed on using[PSPy][OTf]as catalyst and it can be reused at least 8 times without obvious activity loss.展开更多
The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-fun...The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-function, Appell function F3 and a general class of poly- nomials. The results obtained provide unification and extension of the results given by Saxena et al. [13], Srivastava and Grag [17], Srivastava et al. [20], and etc. The results are obtained in compact form and are useful in preparing some tables of operators of fractional calculus. On account of the general nature of the Saigo-Maeda operators, R-function, and a general class of polynomials a large number of new and known results involving Saigo fractional calculus operators and several special functions notably H-function, /-function, Mittag-Leffier function, generalized Wright hypergeometric function, generalized Bessel-Maitland function follow as special cases of our main findings.展开更多
针对目标函数中包含耦合函数H(x,y)的非凸非光滑极小化问题,提出了一种线性惯性交替乘子方向法(Linear Inertial Alternating Direction Method of Multipliers,LIADMM)。为了方便子问题的求解,对目标函数中的耦合函数H(x,y)进行线性化...针对目标函数中包含耦合函数H(x,y)的非凸非光滑极小化问题,提出了一种线性惯性交替乘子方向法(Linear Inertial Alternating Direction Method of Multipliers,LIADMM)。为了方便子问题的求解,对目标函数中的耦合函数H(x,y)进行线性化处理,并在x-子问题中引入惯性效应。在适当的假设条件下,建立了算法的全局收敛性;同时引入满足Kurdyka-Lojasiewicz不等式的辅助函数,验证了算法的强收敛性。通过两个数值实验表明,引入惯性效应的算法比没有惯性效应的算法收敛性能更好。展开更多
基金supported by National 863 High-Tech Research and Development Program of China(No. 2007AA05Z101)
文摘In this article,an efficient,simple and environmentally friendly approach to the synthesis of diacetals(diketals) pentaerythritol using SOH-functionalized ionic liquids(ILs) as catalysts was reported.The ILs show high catalytic activity and reusability with good to excellent yields of the desired products.Hammett method has been used to determine the acidity order of these ionic liquids and the results are consistent with the catalytic activities observed in acetalization reaction.Maximum product yield of 93%was observed on using[PSPy][OTf]as catalyst and it can be reused at least 8 times without obvious activity loss.
基金NBHM Department of Atomic Energy,Government of India,Mumbai for the finanicai assistance under PDF sanction no.2/40(37)/2014/R&D-II/14131
文摘The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-function, Appell function F3 and a general class of poly- nomials. The results obtained provide unification and extension of the results given by Saxena et al. [13], Srivastava and Grag [17], Srivastava et al. [20], and etc. The results are obtained in compact form and are useful in preparing some tables of operators of fractional calculus. On account of the general nature of the Saigo-Maeda operators, R-function, and a general class of polynomials a large number of new and known results involving Saigo fractional calculus operators and several special functions notably H-function, /-function, Mittag-Leffier function, generalized Wright hypergeometric function, generalized Bessel-Maitland function follow as special cases of our main findings.
文摘针对目标函数中包含耦合函数H(x,y)的非凸非光滑极小化问题,提出了一种线性惯性交替乘子方向法(Linear Inertial Alternating Direction Method of Multipliers,LIADMM)。为了方便子问题的求解,对目标函数中的耦合函数H(x,y)进行线性化处理,并在x-子问题中引入惯性效应。在适当的假设条件下,建立了算法的全局收敛性;同时引入满足Kurdyka-Lojasiewicz不等式的辅助函数,验证了算法的强收敛性。通过两个数值实验表明,引入惯性效应的算法比没有惯性效应的算法收敛性能更好。