Analyzing the surface passivity effect of germanium oxynitride:a comprehensive approach through first principles simulation and interface state density

High-purity germanium(HPGe)detectors,which are used for direct dark matter detection,have the advantages of a low threshold and excellent energy resolution.The surface passivation of HPGe has become crucial for achieving an extremely low energy threshold.In this study,first-principles simulations,passivation film preparation,and metal oxide semiconductor(MOS)capacitor characterization were combined to study surface passivation.Theoretical calculations of the energy band structure of the -H,-OH,and -NH_(2) passivation groups on the surface of Ge were performed,and the interface state density and potential with five different passivation groups with N/O atomic ratios were accurately analyzed to obtain a stable surface state.Based on the theoretical calculation results,the surface passivation layers of the Ge_(2)ON_(2) film were prepared via magnetron sputtering in accordance with the optimum atomic ratio structure.The microstructure,C-V,and I-V electrical properties of the layers,and the passivation effect of the Al/Ge_(2)ON_(2)/Ge MOS were characterized to test the interface state density.The mean interface state density obtained by the Terman method was 8.4×10^(11) cm^(-2) eV^(-1).The processing of germanium oxynitrogen passivation films is expected to be used in direct dark matter detection of the HPGe detector surface passivation technology to reduce the detector leakage currents.

Assessment of Modeling Collimator Designs for Gamma-Ray Transmission of Uranium Oxide Spectrometry Using HPGe Detectors

Many scientific domains use gamma-ray spectrometry, but non-destructive gamma scanning and gamma emission tomography of radioactive fuel in particular. In the experimental setting, a collimator is frequently employed to focus on a particular location of interest in the fuel. Predictive models for the transmitted gamma-ray intensity through the collimator are required for both the optimization of instrument design and the planning of measurement campaigns. Gamma-ray transport accuracy is frequently predicted using Monte Carlo radiation transport methods, but using these tools in low-efficiency experimental setups is challenging due to the lengthy computation times needed. This study focused on the full-energy peak intensity that was transmitted through several collimator designs, including rectangle and cylinder. The rate of photons arriving at a detector on the other side of the collimator was calculated for anisotropic source of SNM (U3O8). Some geometrical assumptions that depended on the source-to-collimator distance and collimator dimensions (length, radius or length, height, and width) were applied to achieve precise findings.

Measurement of the Energy Spectrum of a 6 MV Linear Accelerator Using Compton Scattering Spectroscopy and Monte Carlo-Generated Corrections

Purpose: The energy spectrum of a linear accelerator used for dose calculations is determined during beam commissioning by iteratively adjusting the spectrum and comparing calculated and measured percent depth-dose curves. Direct measurement of the energy spectrum using pulse mode detectors is particularly challenging because of the high-energy, high fluence nature of these beams and limitations of the detector systems. This work implements a Compton scattering (CS) spectroscopy setup and presents detector corrections and spectral unfolding techniques to measure the spectrum of a 6 MV linear accelerator using a pulse mode detector. Methods: Spectral measurements were performed using a Varian Clinac 21EX linear accelerator and a high-purity germanium (HPGe) detector. To reduce fluence to the detector, a custom-built lead shield and a CS spectrometry setup were used. The detector was placed at CS angles of 46°, 89°, and 125°. At each of these locations, a detector response function was generated to account for photon interactions within the experimental geometry. Gold’s deconvolution algorithm was used to unfold the energy spectrum. The measured spectra were compared to simulated spectra, which were obtained using an experimentally benchmarked model of the Clinac 21EX in MCNP6. Results: Measurements were acquired and detector response corrections were calculated for all three CS angles. A comparison of spectra for all CS angles showed good agreement with one another. The spectra for all three angles were averaged and showed good agreement with the MCNP6 simulated spectrum, with all points above 400 keV falling within 4%, which was within the uncertainty of the measurement and statistical uncertainty. Conclusions: The measurement of the energy spectrum of a 6 MV linear accelerator using a pulse-mode detector is presented in this work. For accurate spectrum determination, great care must be taken to optimize the detector setup, determine proper corrections, and to unfold the spectrum.

RADIONUCLIDES IN NOODLES AND BREAD CONSUMED IN HONG KONG

Most of the natural occurring radionuclides in both noodles and bread are found to have specific activities below the detectable limit of the high purity germanium (n-type) spectrometer system of the EG&G Ortec Company. For dried bread, 40K,137Cs and 60Co are found to be 44.45￣84.52, < 0.012 ￣0.052, < 0.018 ￣0.054 Bq/kg;for noodles, to be 29.55￣64.54, < 0.01 ￣0.069 and < 9.8× 10-3 ￣ 0.074 Bq/kg,respectively. The weighted committed dose equivalents due to the ingestion of 137Csfrom noodles and bread for a male and female adults have been estimated to be 0.5and 0.6μSv, respectively, being less than the values recommended by ICRP.

Simulation of Gamma-Ray and Neutron Spectrometers for Microsatellite Missions

Microsatellites have recently opened windows of frequent and low cost missions for planetary exploration. The performance of gamma-ray and neutron spectrometers on future microsatellite missions is simulated to assess the possibility of observation of hydrogen and major elements, given their concentration on the observation target. The measured elemental abundance will provide important geological constraints, and some of them may serve as space resources. Four different types of target bodies with various hydrogen concentrations in the range of 0 - 20,000 ppm are assumed as target compositions;Earth’s core, C-type, S-type and Martian meteorites. Gamma-ray and neutron emission rates show unique footprints that are related to the different elemental compositions. The starting point is the solid angle subtended between observation target and spectrometers that allow estimating the gamma-ray and neutron count rates emitted by the celestial bodies. In this work, three types of gamma-ray detectors;high-purity germanium (HPGe), CeBr3 and LaBr3(Ce), a neutron spectrometer combining a lithium glass scintillator with a boron loaded plastic scintillator and a dual mode spectrometer Cs2LiYCl6(Ce) (CLYC) are simulated, focusing on their observation backgrounds as a model case for microsatellite based measurements. The background count level of both gamma-ray (except for the LaBr3 detector) and neutron count rates was negligible under these particular conditions. The gamma-ray detectors were compared by the figure of merit, which was determined by their efficiency and energy resolution. It was found that each detector has unique advantages. The HPGe detector has the highest figure of merit due to its excellent energy resolution, whereas the CLYC detector is low in weight and power consumption due to its dual sensitivity to gamma-ray and neutron. The CeBr3 detector is an intermediate choice. The neutron count rates are calculated separately in three energy ranges, i.e. , thermal (<0.5 eV), epithermal (0.5 eV - 500 keV), and fast (>500 keV), as a function of the hydrogen concentration in the 0 - 20,000 ppm range. The thermal and epithermal neutron count rates are found to decrease with hydrogen concentration, while the fast neutron count rate increases with the target average atomic mass. The optimal detector should be decided by the mission restraints on mass, power consumption, and heat thermal design.

Probing dark matter particles from evaporating primordial black holes via electron scattering in the CDEX-10 experiment

Dark matter(DM)is a major constituent of the Universe.However,no definite evidence of DM particles(denoted as“χ”)has been found in DM direct detection(DD)experiments to date.There is a novel concept of detectingχfrom evaporating primordial black holes(PBHs).We search forχemitted from PBHs by investigating their interaction with target electrons.The examined PBH masses range from 1×10^(15)to 7×10^(16)g under the current limits of PBH abundance fPBH.Using 205.4 kg·day data obtained from the CDEX-10 experiment conducted in the China Jinping Underground Laboratory,we exclude theχ-electron(χ-e)elastic-scattering cross sectionσ_(χe)~5×10^(-29)cm^(2)forχwith a mass■keV from our results.With the higher radiation background but lower energy threshold(160 eV),CDEX-10 fills a part of the gap in the previous work.If(m_(χ),σ_(χe))can be determined in the future,DD experiments are expected to impose strong constraints on fPBHfor large MPBHs.