High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs...High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs during the underwater high voltage pulse discharge process, which brings security risks to the stability of the pulse fracturing system. In order to solve this problem, an underwater pulse power discharge system was established, the circuit oscillation generation conditions were analyzed and the circuit oscillation suppression method was proposed. Firstly, the system structure was introduced and the charging model of the energy storage capacitor was established by the state space average method. Next, the electrode high-voltage breakdown model was established through COMSOL software, the electrode breakdown process was analyzed according to the electron density distribution image, and the plasma channel impedance was estimated based on the conductivity simulation results. Then the underwater pulse power discharge process and the circuit oscillation generation condition were analyzed, and the circuit oscillation suppression strategy of using the thyristor to replace the gas spark switch was proposed. Finally, laboratory experiments were carried out to verify the precision of the theoretical model and the suppression effect of circuit oscillation. The experimental results show that the voltage variation of the energy storage capacitor, the impedance change of the pulse power discharge process, and the equivalent circuit in each discharge stage were consistent with the theoretical model. The proposed oscillation suppression strategy cannot only prevent the damage caused by circuit oscillation but also reduce the damping oscillation time by77.1%, which can greatly improve the stability of the system. This research has potential application value in the field of underwater pulse power discharge for reservoir reconstruction.展开更多
High voltage pulse natural organic matter (NOM) toxic by-products. Fulvic acid discharge plasma can remove and produce no production of solution was treated by high voltage pulse discharge plasma in this paper. It w...High voltage pulse natural organic matter (NOM) toxic by-products. Fulvic acid discharge plasma can remove and produce no production of solution was treated by high voltage pulse discharge plasma in this paper. It was shown that: for the reason of thermolysis and oxidation, the pH and Oxidation Reduction Potential (ORP) of solution decreased gradually with the increase of peak voltage and fulvic acid solution concentration, meanwhile the temperature and turbidity of solution increased gradually. Adding hydrochlorid acid in the treatment could amplify the effect of plasma. When the concentration of NOM as the surrogate parameter, Ultraviolet Absorbancy Degree (UV254) increased slowly by the effect of plasma, while the degradation of Total Organic Carbon (TOC) was first-order reaction. The removal rate of TOC increased from 22.6% to 33.4% by high voltage pulse electrical field of 35 kv, and from 25.6% to 36.7% with the addition of hydrochlorid acid. This paper may provide some basis for the scale-up design of water treatment process by high voltage pulse discharge plasma with other technologies.展开更多
Organic pollutants could be degraded by using bubble discharge in water with gas aeration in the discharge reactor and more plasma can be generated in the discharge process. When pulsed high voltage was applied betwee...Organic pollutants could be degraded by using bubble discharge in water with gas aeration in the discharge reactor and more plasma can be generated in the discharge process. When pulsed high voltage was applied between electrodes with gas aerated into the reactor, it showed that bubbles were broken, which meant that breakdown took place. It could also be observed that the removal rate of phenol increased with increasing discharge voltage or pulse frequency, and with reducing initial phenol concentration or solution electric conductivity. It could remove more amount of phenol by oxygen aeration. With increasing oxygen flow rate, the removal rate increased. There was little difference with air or nitrogen aeration for phenol removal. The solution temperature after discharge increased to a great extent. However, this part of energy consumption did not contribute to the reaction, which led to a reduction in the energy utilization efficiency.展开更多
Precise control of the discharge in space and time is of great significance for better applications of discharge plasma.Here,we used a femtosecond laser filament to trigger and guide a highvoltage DC pulse discharge t...Precise control of the discharge in space and time is of great significance for better applications of discharge plasma.Here,we used a femtosecond laser filament to trigger and guide a highvoltage DC pulse discharge to achieve spatiotemporal control of the discharge plasma.In space,the discharge plasma is distributed strictly along the channel generated by the femtosecond laser filament.The breakdown voltage threshold is reduced,and the discharge length is extended.In time,the electrical parameters such as the electrode voltage and the electrode gap affect discharge delay time and jitter.By optimizing the parameters,we can achieve sub-nanosecond jitter of the discharge.Based on the spatiotemporal control of the discharge,we applied filamenttriggered discharge for one-dimensional composition measurements of the gas flow field.Besides,the technique shows great potential in studying the spatiotemporal evolution of discharge plasma.展开更多
Traditional extraction methods are based on high-temperature maceration with organic solvents,which are dangerous for human health.A viable alternative to overcome the issues associated with conventional extraction is...Traditional extraction methods are based on high-temperature maceration with organic solvents,which are dangerous for human health.A viable alternative to overcome the issues associated with conventional extraction is to increase cell tissue permeability by applying high voltage electrical discharge(HVED)treatments.The objective of this work was to validate the electroporation of blueberry plant cells using a new HVED generator prototype at a high frequency,investigate the effect,intensity,and duration of the applied voltage,and recover anthocyanins from its electroporated cells.The electroporation level of the HVED-treated blueberries was measured qualitatively by transmission electron microscopy(TEM)analysis.Meanwhile,it was quantitatively measured by the cell permeabilization index(Zp)and anthocyanin extraction level.Results of the micrographs(TEM)showed electroporation in all treatments in which Zp was 0.24 when applying a 2 kV treatment for 2 s,whereas a 3-fold increase in tissue damage was revealed with the most powerful treatment(10 kV voltage,30 s).In addition,anthocyanin values ranged from 83.09±1.20(control)to 136.82±0.84(HVED),which was 64.66%higher.The HVED treatment can increase mass transfer rates during conventional extraction processes.It should be noted that the validated prototype required a low specific energy requirement(31–204 kJ/kg)for proper tissue electropermeabilization.In conclusion,we demonstrated the capability of the developed HVED prototype to boost mass transfer phenomena and thus potentially increase its adaptability to assist dissimilar industrial processes or waste(e.g.,peels and seeds)such as freeze-drying operations.展开更多
基金financially supported by the National Science and Technology Major Project(No.2016ZX05034004)。
文摘High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs during the underwater high voltage pulse discharge process, which brings security risks to the stability of the pulse fracturing system. In order to solve this problem, an underwater pulse power discharge system was established, the circuit oscillation generation conditions were analyzed and the circuit oscillation suppression method was proposed. Firstly, the system structure was introduced and the charging model of the energy storage capacitor was established by the state space average method. Next, the electrode high-voltage breakdown model was established through COMSOL software, the electrode breakdown process was analyzed according to the electron density distribution image, and the plasma channel impedance was estimated based on the conductivity simulation results. Then the underwater pulse power discharge process and the circuit oscillation generation condition were analyzed, and the circuit oscillation suppression strategy of using the thyristor to replace the gas spark switch was proposed. Finally, laboratory experiments were carried out to verify the precision of the theoretical model and the suppression effect of circuit oscillation. The experimental results show that the voltage variation of the energy storage capacitor, the impedance change of the pulse power discharge process, and the equivalent circuit in each discharge stage were consistent with the theoretical model. The proposed oscillation suppression strategy cannot only prevent the damage caused by circuit oscillation but also reduce the damping oscillation time by77.1%, which can greatly improve the stability of the system. This research has potential application value in the field of underwater pulse power discharge for reservoir reconstruction.
文摘High voltage pulse natural organic matter (NOM) toxic by-products. Fulvic acid discharge plasma can remove and produce no production of solution was treated by high voltage pulse discharge plasma in this paper. It was shown that: for the reason of thermolysis and oxidation, the pH and Oxidation Reduction Potential (ORP) of solution decreased gradually with the increase of peak voltage and fulvic acid solution concentration, meanwhile the temperature and turbidity of solution increased gradually. Adding hydrochlorid acid in the treatment could amplify the effect of plasma. When the concentration of NOM as the surrogate parameter, Ultraviolet Absorbancy Degree (UV254) increased slowly by the effect of plasma, while the degradation of Total Organic Carbon (TOC) was first-order reaction. The removal rate of TOC increased from 22.6% to 33.4% by high voltage pulse electrical field of 35 kv, and from 25.6% to 36.7% with the addition of hydrochlorid acid. This paper may provide some basis for the scale-up design of water treatment process by high voltage pulse discharge plasma with other technologies.
基金supported by the Fundamental Research Funds for the Central Universities of China(HEUCFZ1124,HEUCFR1005)the Open Research Fund Program of State Key Laboratory of Water Resources and Hydropower Engineering Science of China(2010B077)
文摘Organic pollutants could be degraded by using bubble discharge in water with gas aeration in the discharge reactor and more plasma can be generated in the discharge process. When pulsed high voltage was applied between electrodes with gas aerated into the reactor, it showed that bubbles were broken, which meant that breakdown took place. It could also be observed that the removal rate of phenol increased with increasing discharge voltage or pulse frequency, and with reducing initial phenol concentration or solution electric conductivity. It could remove more amount of phenol by oxygen aeration. With increasing oxygen flow rate, the removal rate increased. There was little difference with air or nitrogen aeration for phenol removal. The solution temperature after discharge increased to a great extent. However, this part of energy consumption did not contribute to the reaction, which led to a reduction in the energy utilization efficiency.
基金funded by National Natural Science Foundation of China(NSFC)(Nos.51806149,91741205)。
文摘Precise control of the discharge in space and time is of great significance for better applications of discharge plasma.Here,we used a femtosecond laser filament to trigger and guide a highvoltage DC pulse discharge to achieve spatiotemporal control of the discharge plasma.In space,the discharge plasma is distributed strictly along the channel generated by the femtosecond laser filament.The breakdown voltage threshold is reduced,and the discharge length is extended.In time,the electrical parameters such as the electrode voltage and the electrode gap affect discharge delay time and jitter.By optimizing the parameters,we can achieve sub-nanosecond jitter of the discharge.Based on the spatiotemporal control of the discharge,we applied filamenttriggered discharge for one-dimensional composition measurements of the gas flow field.Besides,the technique shows great potential in studying the spatiotemporal evolution of discharge plasma.
基金supported by the Universidad del Bío-Bío[Scholarship fund for postgraduate research],the INNOVA BIOBIO[16IP-65192 project].
文摘Traditional extraction methods are based on high-temperature maceration with organic solvents,which are dangerous for human health.A viable alternative to overcome the issues associated with conventional extraction is to increase cell tissue permeability by applying high voltage electrical discharge(HVED)treatments.The objective of this work was to validate the electroporation of blueberry plant cells using a new HVED generator prototype at a high frequency,investigate the effect,intensity,and duration of the applied voltage,and recover anthocyanins from its electroporated cells.The electroporation level of the HVED-treated blueberries was measured qualitatively by transmission electron microscopy(TEM)analysis.Meanwhile,it was quantitatively measured by the cell permeabilization index(Zp)and anthocyanin extraction level.Results of the micrographs(TEM)showed electroporation in all treatments in which Zp was 0.24 when applying a 2 kV treatment for 2 s,whereas a 3-fold increase in tissue damage was revealed with the most powerful treatment(10 kV voltage,30 s).In addition,anthocyanin values ranged from 83.09±1.20(control)to 136.82±0.84(HVED),which was 64.66%higher.The HVED treatment can increase mass transfer rates during conventional extraction processes.It should be noted that the validated prototype required a low specific energy requirement(31–204 kJ/kg)for proper tissue electropermeabilization.In conclusion,we demonstrated the capability of the developed HVED prototype to boost mass transfer phenomena and thus potentially increase its adaptability to assist dissimilar industrial processes or waste(e.g.,peels and seeds)such as freeze-drying operations.