The physicochemical properties of plasma-activated water(PAW)generated under different process conditions were investigated,and their changes under different storage conditions were also studied.The results showed tha...The physicochemical properties of plasma-activated water(PAW)generated under different process conditions were investigated,and their changes under different storage conditions were also studied.The results showed that increasing the processing time and power,and decreasing generated water volume,could cause an increase in the redox potential,conductivity,and temperature of PAW,and a decrease in its pH.A slower dissipation of the reactive oxygen and nitrogen species in PAW was found on storage at 4℃in a sealed conical flask than on storage at room temperature.The inactivation ability of plasma-activated lactic acid(LA)to Listeria monocytogenes(L.monocytogenes)and Pseudomonas aeruginosa(P.aeruginosa)was higher than that of PAW or LA alone under the same experimental conditions.The results of this study may provide theoretical information for the application of PAW as a potential antimicrobial agent in the future.展开更多
The pulsed corona discharge(CD)generated in contact with water and directly in water,and high-power air plasma jet(APJ)were studied for production of plasma activated water(PAW).The changes of physical(pH,redox potent...The pulsed corona discharge(CD)generated in contact with water and directly in water,and high-power air plasma jet(APJ)were studied for production of plasma activated water(PAW).The changes of physical(pH,redox potential,conductivity,temperature)and chemical(peroxides,nitrites,nitrates concentrations)properties of treated water were investigated.The comparison of CD generated in gas/water interface and underwater configuration in the same system showed that the interaction of reactive oxygen and nitrogen species formed in ambient air in gas/water system induces different chemical processes,leading to lower pH,higher oxidation-reduction potential(ORP)and higher conductivity of PAW than in underwater discharge.High yield of peroxide was observed in both configurations.The PAW prepared by APJ exhibits high concentration of nitrites and nitrates according to supplied energy,and related significant decrease of pH and increase of ORP and conductivity after treatment.The antimicrobial effect of PAW prepared by CD and plasma jet on lentils sprouts was studied in different treatment and washing times.The APJ appears to have great efficacy on water activation resulted in strong decontamination effect.The PAW treated by APJ for 10 min led to bacterial reduction from initial 8.3 to 5.9 and 4.0 log10 CFU g^(-1)after 10 and 30 min of washing,respectively.展开更多
An exploratory study was conducted in the coastal plantation （12- and 17-year-old Sonneratia apetala） of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of N...An exploratory study was conducted in the coastal plantation （12- and 17-year-old Sonneratia apetala） of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of Noakhali district, in Bangladesh to determine afforestation effects on soil properties. At soil depths of 0-10, 10-30 and 30-40 cm across three different land strips viz. inland, middle and sea side in 12- and 17-year-old keora （Sonneratia apetala） plantations, soil moisture, particle density, organic matter and C, total N, pH, available P, K, Na, Ca and Mg were significantly （p≤0.05, p≤0.01, p≤0.001） higher, and soil salinity significantly （p〈0.001） lower than that in their adjacent barren lands. Soil moisture, particle density, organic matter and C, total N, pH, soil salinity, available P, K, Na, Ca and Mg of surface soil in Char Alim plantation at inland were 31.09%, 2.24 g.cm^-3, 2.41%, 4.14%, 0.58%, 7.07, 0.09 dS＇cm^-1, 28.06 mg.L^-1, 0.50 mg-L^- 1 11.5 mg-L^-1, 3.30 mg·L^-1 and 2.7 mmol.kg^-1, respectively. Their corresponding values for the same depth and land position at adjacent Char Rehania barren land were 16.69%, 1.25g.cm^-3, 0.43%, 0.74%, 0.25%, 6.57, 0.13 dS.cm^-1, 13.07mg-L^-1, 0.30 mg.L^-1, 1.4 mg.L^-1, 0.30 mmol·kg^-1 and 0.50 mg.L^-1, respectively. Soil moisture, particle density, organic matter and C, total N, pH, available P, K and Ca decreased, and soil salinity, available Na and Mg increased from inland towards sea side in the plantations. Although soil texture did not differ in most soil depths between plantation and adjacent barren land, proportion of sand particle was significantly （p≤0.01） lower and silt particle significantly （p〈0.001） in the plantations higher than that in their adjacent barren lands. In the study, evaluation of all the parameters was also done for the other pair of lands.展开更多
An exploratory study was conducted in the coastal plantation (12-and 17-year-old Sonneratia apetala) of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of Noak...An exploratory study was conducted in the coastal plantation (12-and 17-year-old Sonneratia apetala) of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of Noakhali district, in Bangladesh to determine afforestation effects on soil properties. At soil depths of 0-10, 10-30 and 30-40 cm across three different land strips viz. inland, middle and sea side in 12-and 17-year-old keora (Sonneratia apetala) plantations, soil moisture, particle density, organic matter and C, total N, pH, available P, K, Na, Ca and Mg were significantly (p≤0.05, p≤0.01, p≤0.001) higher, and soil salinity significantly (p≤0.001) lower than that in their adjacent barren lands. Soil moisture, particle density, organic matter and C, total N, pH, soil salinity, available P, K, Na, Ca and Mg of surface soil in Char Alim plantation at inland were 31.09%, 2.24 g·cm-3, 2.41%, 4.14%, 0.58%, 7.07, 0.09 dS·cm-1, 28.06 mg·L-1, 0.50 mg·L-1 11.5 mg·L-1, 3.30 mg·L-1 and 2.7 mmol·kg-1, respectively. Their corresponding values for the same depth and land position at adjacent Char Rehania barren land were 16.69%, 1.25g·cm-3, 0.43%, 0.74%, 0.25%, 6.57, 0.13 dS·cm-1, 13.07mg·L-1, 0.30 mg·L-1, 1.4 mg·L-1, 0.30 mmol·kg-1 and 0.50 mg·L-1, respectively. Soil moisture, particle density, organic matter and C, total N, pH, available P, K and Ca decreased, and soil salinity, available Na and Mg increased from inland towards sea side in the plantations. Although soil texture did not differ in most soil depths between plantation and adjacent barren land, proportion of sand particle was significantly (p≤0.01) lower and silt particle significantly (p≤0.001) in the plantations higher than that in their adjacent barren lands. In the study, evaluation of all the parameters was also done for the other pair of lands.展开更多
Nanoparticles are thought to induce more severe health impacts than larger particles. The nanoparticles from coal-fired boilers are classified into three size fractions with a 13-stage low pressure impactor. Their phy...Nanoparticles are thought to induce more severe health impacts than larger particles. The nanoparticles from coal-fired boilers are classified into three size fractions with a 13-stage low pressure impactor. Their physicochemical properties are characterized by the high-resolution field emission scanning electron microscope and X-ray fluorescence spectrometer (XRF). The results show that coal-derived nanoparticles mainly consist of individual primary particles of 20―150 nm and their aggregates. Inor-ganic nanoparticles primarily contain ash-forming elements and their aggregates have a dense struc-ture. Organic nanoparticles are dominated by the element carbon and their aggregates have a loose structure. Nanoparticles from the same boiler have a similar composition and are primarily composed of sulfur, refractory elements and alkali/alkaline elements. Some transition and heavy metals are also detected. For different boilers, greater differences are observed in the production of the nanoparticles and their composition, possibly due to the use of low-NOx burners. Coal-derived nanoparticles have a small size, large specific surface area and complicated chemical composition, and thus are potentially more harmful to human health.展开更多
基金National Natural Science Foundation of China(No.32260643)for financial support of this study。
文摘The physicochemical properties of plasma-activated water(PAW)generated under different process conditions were investigated,and their changes under different storage conditions were also studied.The results showed that increasing the processing time and power,and decreasing generated water volume,could cause an increase in the redox potential,conductivity,and temperature of PAW,and a decrease in its pH.A slower dissipation of the reactive oxygen and nitrogen species in PAW was found on storage at 4℃in a sealed conical flask than on storage at room temperature.The inactivation ability of plasma-activated lactic acid(LA)to Listeria monocytogenes(L.monocytogenes)and Pseudomonas aeruginosa(P.aeruginosa)was higher than that of PAW or LA alone under the same experimental conditions.The results of this study may provide theoretical information for the application of PAW as a potential antimicrobial agent in the future.
基金supported by the Slovak Research and Development Agency under the contract Nos.APVV-16-0216,APVV-19-0386 and Slovak Grant Agency No.1/0782/19。
文摘The pulsed corona discharge(CD)generated in contact with water and directly in water,and high-power air plasma jet(APJ)were studied for production of plasma activated water(PAW).The changes of physical(pH,redox potential,conductivity,temperature)and chemical(peroxides,nitrites,nitrates concentrations)properties of treated water were investigated.The comparison of CD generated in gas/water interface and underwater configuration in the same system showed that the interaction of reactive oxygen and nitrogen species formed in ambient air in gas/water system induces different chemical processes,leading to lower pH,higher oxidation-reduction potential(ORP)and higher conductivity of PAW than in underwater discharge.High yield of peroxide was observed in both configurations.The PAW prepared by APJ exhibits high concentration of nitrites and nitrates according to supplied energy,and related significant decrease of pH and increase of ORP and conductivity after treatment.The antimicrobial effect of PAW prepared by CD and plasma jet on lentils sprouts was studied in different treatment and washing times.The APJ appears to have great efficacy on water activation resulted in strong decontamination effect.The PAW treated by APJ for 10 min led to bacterial reduction from initial 8.3 to 5.9 and 4.0 log10 CFU g^(-1)after 10 and 30 min of washing,respectively.
文摘An exploratory study was conducted in the coastal plantation （12- and 17-year-old Sonneratia apetala） of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of Noakhali district, in Bangladesh to determine afforestation effects on soil properties. At soil depths of 0-10, 10-30 and 30-40 cm across three different land strips viz. inland, middle and sea side in 12- and 17-year-old keora （Sonneratia apetala） plantations, soil moisture, particle density, organic matter and C, total N, pH, available P, K, Na, Ca and Mg were significantly （p≤0.05, p≤0.01, p≤0.001） higher, and soil salinity significantly （p〈0.001） lower than that in their adjacent barren lands. Soil moisture, particle density, organic matter and C, total N, pH, soil salinity, available P, K, Na, Ca and Mg of surface soil in Char Alim plantation at inland were 31.09%, 2.24 g.cm^-3, 2.41%, 4.14%, 0.58%, 7.07, 0.09 dS＇cm^-1, 28.06 mg.L^-1, 0.50 mg-L^- 1 11.5 mg-L^-1, 3.30 mg·L^-1 and 2.7 mmol.kg^-1, respectively. Their corresponding values for the same depth and land position at adjacent Char Rehania barren land were 16.69%, 1.25g.cm^-3, 0.43%, 0.74%, 0.25%, 6.57, 0.13 dS.cm^-1, 13.07mg-L^-1, 0.30 mg.L^-1, 1.4 mg.L^-1, 0.30 mmol·kg^-1 and 0.50 mg.L^-1, respectively. Soil moisture, particle density, organic matter and C, total N, pH, available P, K and Ca decreased, and soil salinity, available Na and Mg increased from inland towards sea side in the plantations. Although soil texture did not differ in most soil depths between plantation and adjacent barren land, proportion of sand particle was significantly （p≤0.01） lower and silt particle significantly （p〈0.001） in the plantations higher than that in their adjacent barren lands. In the study, evaluation of all the parameters was also done for the other pair of lands.
文摘An exploratory study was conducted in the coastal plantation (12-and 17-year-old Sonneratia apetala) of Char Alim and Char Piya and on their adjacent barren lands at Char Rehania and Char Nurul Islam in Hatiya of Noakhali district, in Bangladesh to determine afforestation effects on soil properties. At soil depths of 0-10, 10-30 and 30-40 cm across three different land strips viz. inland, middle and sea side in 12-and 17-year-old keora (Sonneratia apetala) plantations, soil moisture, particle density, organic matter and C, total N, pH, available P, K, Na, Ca and Mg were significantly (p≤0.05, p≤0.01, p≤0.001) higher, and soil salinity significantly (p≤0.001) lower than that in their adjacent barren lands. Soil moisture, particle density, organic matter and C, total N, pH, soil salinity, available P, K, Na, Ca and Mg of surface soil in Char Alim plantation at inland were 31.09%, 2.24 g·cm-3, 2.41%, 4.14%, 0.58%, 7.07, 0.09 dS·cm-1, 28.06 mg·L-1, 0.50 mg·L-1 11.5 mg·L-1, 3.30 mg·L-1 and 2.7 mmol·kg-1, respectively. Their corresponding values for the same depth and land position at adjacent Char Rehania barren land were 16.69%, 1.25g·cm-3, 0.43%, 0.74%, 0.25%, 6.57, 0.13 dS·cm-1, 13.07mg·L-1, 0.30 mg·L-1, 1.4 mg·L-1, 0.30 mmol·kg-1 and 0.50 mg·L-1, respectively. Soil moisture, particle density, organic matter and C, total N, pH, available P, K and Ca decreased, and soil salinity, available Na and Mg increased from inland towards sea side in the plantations. Although soil texture did not differ in most soil depths between plantation and adjacent barren land, proportion of sand particle was significantly (p≤0.01) lower and silt particle significantly (p≤0.001) in the plantations higher than that in their adjacent barren lands. In the study, evaluation of all the parameters was also done for the other pair of lands.
基金Supported by National Natural Science Foundation of China (Grant Nos. 50721005 , 50706013 and 50720145604)
文摘Nanoparticles are thought to induce more severe health impacts than larger particles. The nanoparticles from coal-fired boilers are classified into three size fractions with a 13-stage low pressure impactor. Their physicochemical properties are characterized by the high-resolution field emission scanning electron microscope and X-ray fluorescence spectrometer (XRF). The results show that coal-derived nanoparticles mainly consist of individual primary particles of 20―150 nm and their aggregates. Inor-ganic nanoparticles primarily contain ash-forming elements and their aggregates have a dense struc-ture. Organic nanoparticles are dominated by the element carbon and their aggregates have a loose structure. Nanoparticles from the same boiler have a similar composition and are primarily composed of sulfur, refractory elements and alkali/alkaline elements. Some transition and heavy metals are also detected. For different boilers, greater differences are observed in the production of the nanoparticles and their composition, possibly due to the use of low-NOx burners. Coal-derived nanoparticles have a small size, large specific surface area and complicated chemical composition, and thus are potentially more harmful to human health.
