Regular fastener detection is necessary to ensure the safety of railways.However,the number of abnormal fasteners is significantly lower than the number of normal fasteners in real railways.Existing supervised inspect...Regular fastener detection is necessary to ensure the safety of railways.However,the number of abnormal fasteners is significantly lower than the number of normal fasteners in real railways.Existing supervised inspectionmethods have insufficient detection ability in cases of imbalanced samples.To solve this problem,we propose an approach based on deep convolutional neural networks(DCNNs),which consists of three stages:fastener localization,abnormal fastener sample generation based on saliency detection,and fastener state inspection.First,a lightweight YOLOv5s is designed to achieve fast and precise localization of fastener regions.Then,the foreground clip region of a fastener image is extracted by the designed fastener saliency detection network(F-SDNet),combined with data augmentation to generate a large number of abnormal fastener samples and balance the number of abnormal and normal samples.Finally,a fastener inspection model called Fastener ResNet-8 is constructed by being trained with the augmented fastener dataset.Results show the effectiveness of our proposed method in solving the problem of sample imbalance in fastener detection.Qualitative and quantitative comparisons show that the proposed F-SDNet outperforms other state-of-the-art methods in clip region extraction,reaching MAE and max F-measure of 0.0215 and 0.9635,respectively.In addition,the FPS of the fastener state inspection model reached 86.2,and the average accuracy reached 98.7%on 614 augmented fastener test sets and 99.9%on 7505 real fastener datasets.展开更多
Measurement of bloodflow velocity is key to understanding physiology and pathology in vivo.While most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the in...Measurement of bloodflow velocity is key to understanding physiology and pathology in vivo.While most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the instantaneous bloodflow velocity distribution.This is mainly due to the lack of measurement technology with high spatial and temporal resolution.Here,we tackle this problem with our recently developed dual-wavelength line-scan third-harmonic generation(THG)imaging technology.Simultaneous acquisition of dual-wavelength THG line-scanning signals enables measurement of bloodflow velocities at two radially symmetric positions in both venules and arterioles in mouse brain in vivo.Our results clearly show that the instantaneous bloodflow velocity is not symmetric under general conditions.展开更多
Both analyzing a large amount of space weather observed data and alleviating personal experience bias are significant challenges in generating artificial space weather forecast products.With the use of natural languag...Both analyzing a large amount of space weather observed data and alleviating personal experience bias are significant challenges in generating artificial space weather forecast products.With the use of natural language generation methods based on the sequence-to-sequence model,space weather forecast texts can be automatically generated.To conduct our generation tasks at a fine-grained level,a taxonomy of space weather phenomena based on descriptions is presented.Then,our MDH(Multi-Domain Hybrid)model is proposed for generating space weather summaries in two stages.This model is composed of three sequence-to-sequence-based deep neural network sub-models(one Bidirectional Auto-Regressive Transformers pre-trained model and two Transformer models).Then,to evaluate how well MDH performs,quality evaluation metrics based on two prevalent automatic metrics and our innovative human metric are presented.The comprehensive scores of the three summaries generating tasks on testing datasets are 70.87,93.50,and 92.69,respectively.The results suggest that MDH can generate space weather summaries with high accuracy and coherence,as well as suitable length,which can assist forecasters in generating high-quality space weather forecast products,despite the data being starved.展开更多
The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water resources.At present,many kinds of photothermal conversion materials have been developed and ...The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water resources.At present,many kinds of photothermal conversion materials have been developed and used as evaporators in seawater desalination.However,some evaporators need additional thermal insulation or water supply devices to achieve efficient photothermal conversion.In addition,their complex,time consuming and no scalable preparation process,high cost of raw materials and poor salt resistance hinder the practical application of these evaporator.Owing to its distinctive nanoporous structure,diatomite as fossilized single-cells algae diatoms is a promising natural silica-based material for seawater desalination.They are taken from sea and that makes true sense to use them in the sea.Herein,we report the first example of synthesis robust three-dimensional(3D)natural-diatomite composite by assembling polyaniline nanoparticles covered diatomite into the polyvinyl alcohol pre-treated melamine foam frameworks and demonstrate its application as new evaporator for seawater desalination.The porous framework does not only improve the sunlight scattering efficiency,but also offer large network of channels for water transportation.The inherent mechanism behind salt desalination process involves the absorption of water molecules on the surface of the internal silica micro-nano pores,and evaporation under the heat induced by the polyaniline absorbed sunlight.Meanwhile,the metal ions are segregated by many available pores and channels to achieve the self-desalting effect.The developed evaporator possesses the superiority of multi-stage pore structure,strong hydrophilicity,low thermal conductivity,excellent light absorption,fast water transportation and salt-resistant crystallization as well as good durability.The evaporation rate without an additional device is found to be 1.689 kg m^(-2)h^(-1)under 1-Sun irradiation,and the energy conversion efficiency is as high as 95%.This work creates a platform and develops the prospect of employing green and sustainable natural-diatomite composite evaporator for practical applications of seawater desalination.展开更多
In this study,numerical simulations of the pinching-off phenomena displayed by the dispersed phase in a continuous phase have been conducted using COMSOL Multiphysics(level-set method).Four flow patterns,namely“drop ...In this study,numerical simulations of the pinching-off phenomena displayed by the dispersed phase in a continuous phase have been conducted using COMSOL Multiphysics(level-set method).Four flow patterns,namely“drop flow”,“jet flow”,“squeeze flow”,and“co-flow”,have been obtained for different flow velocity ratios,channel diameter ratios,density ratios,viscosity ratios,and surface tension.The flow pattern map of two-phase flow in coaxial microchannels has been obtained accordingly,and the associated droplet generation process has been critically discussed considering the related frequency,diameter,and pinch-off length.In particular,it is shown that the larger the flow velocity ratio,the smaller the diameter of generated droplets and the shorter the pinch-off length.The pinch-off length of a droplet is influenced by the channel diameter ratio and density ratio.The changes in viscosity ratio have a negligible influence on the droplet generation pinching frequency.With an increase in surface tension,the frequency of generation and pinch-off length of droplets decrease,but for small surface tension the generation diameter of droplet increases.展开更多
The automatic stealth task of military time-sensitive targets plays a crucial role in maintaining national military security and mastering battlefield dynamics in military applications.We propose a novel Military Time...The automatic stealth task of military time-sensitive targets plays a crucial role in maintaining national military security and mastering battlefield dynamics in military applications.We propose a novel Military Time-sensitive Targets Stealth Network via Real-time Mask Generation(MTTSNet).According to our knowledge,this is the first technology to automatically remove military targets in real-time from videos.The critical steps of MTTSNet are as follows:First,we designed a real-time mask generation network based on the encoder-decoder framework,combined with the domain expansion structure,to effectively extract mask images.Specifically,the ASPP structure in the encoder could achieve advanced semantic feature fusion.The decoder stacked high-dimensional information with low-dimensional information to obtain an effective mask layer.Subsequently,the domain expansion module guided the adaptive expansion of mask images.Second,a context adversarial generation network based on gated convolution was constructed to achieve background restoration of mask positions in the original image.In addition,our method worked in an end-to-end manner.A particular semantic segmentation dataset for military time-sensitive targets has been constructed,called the Military Time-sensitive Target Masking Dataset(MTMD).The MTMD dataset experiment successfully demonstrated that this method could create a mask that completely occludes the target and that the target could be hidden in real time using this mask.We demonstrated the concealment performance of our proposed method by comparing it to a number of well-known and highly optimized baselines.展开更多
The investigation endorsed the convective flow of Carreau nanofluid over a stretched surface in presence of entropy generation optimization.The novel dynamic of viscous dissipation is utilized to analyze the thermal m...The investigation endorsed the convective flow of Carreau nanofluid over a stretched surface in presence of entropy generation optimization.The novel dynamic of viscous dissipation is utilized to analyze the thermal mechanism of magnetized flow.The convective boundary assumptions are directed in order to examine the heat and mass transportation of nanofluid.The thermal concept of thermophoresis and Brownian movements has been re-called with the help of Buongiorno model.The problem formulated in dimensionless form is solved by NDSolve MATHEMATICA.The graphical analysis for parameters governed by the problem is performed with physical applications.The affiliation of entropy generation and Bejan number for different parameters is inspected in detail.The numerical data for illustrating skin friction,heat and mass transfer rate is also reported.The motion of the fluid is highest for the viscosity ratio parameter.The temperature of the fluid rises via thermal Biot number.Entropy generation rises for greater Brinkman number and diffusion parameter.展开更多
High harmonic generation in ZnO crystals under chirped single-color field and static electric field are investigated by solving the semiconductor Bloch equation(SBE). It is found that when the chirp pulse is introduce...High harmonic generation in ZnO crystals under chirped single-color field and static electric field are investigated by solving the semiconductor Bloch equation(SBE). It is found that when the chirp pulse is introduced, the interference structure becomes obvious while the harmonic cutoff is not extended. Furthermore, the harmonic efficiency is improved when the static electric field is included. These phenomena are demonstrated by the classical recollision model in real space affected by the waveform of laser field and inversion symmetry. Specifically, the electron motion in k-space shows that the change of waveform and the destruction of the symmetry of the laser field lead to the incomplete X-structure of the crystal-momentum-resolved(k-resolved) inter-band harmonic spectrum. Furthermore, a pre-acceleration process in the solid four-step model is confirmed.展开更多
There is a growing need to explore the potential of coal-fired power plants(CFPPs)to enhance the utilization rate of wind power(wind)and photovoltaic power(PV)in the green energy field.This study developed a load regu...There is a growing need to explore the potential of coal-fired power plants(CFPPs)to enhance the utilization rate of wind power(wind)and photovoltaic power(PV)in the green energy field.This study developed a load regulation model for a multi-power generation system comprising wind,PV,and coal energy storage using realworld data.The power supply process was divided into eight fundamental load regulation scenarios,elucidating the influence of each scenario on load regulation.Within the framework of the multi-power generation system with the wind(50 MW)and PV(50 MW)alongside a CFPP(330 MW),a lithium-iron phosphate energy storage system(LIPBESS)was integrated to improve the system’s load regulation flexibility.The energy storage operation strategy was formulated based on the charging and discharging priority of the LIPBESS for each basic scenario and the charging and discharging load calculation method of LIPBESS auxiliary regulation.Through optimization using the particle swarm algorithm,the optimal capacity of LIPBESS was determined to be within the 5.24-4.88 MWh range.From an economic perspective,the LIPBESS operating with CFPP as the regulating power source was 49.1% lower in capacity compared to the renewable energy-based storage mode.展开更多
Sodium borohydride(NaBH_(4)) is considered as the most potential hydrogen storage material for portable proton exchange membrane fuel cells(PEMFC)because of its high theoretical hydrogen capacity.However,the slow and ...Sodium borohydride(NaBH_(4)) is considered as the most potential hydrogen storage material for portable proton exchange membrane fuel cells(PEMFC)because of its high theoretical hydrogen capacity.However,the slow and poor kinetic stability of hydrogen generation from NaBH_(4) hydrolysis limits its application.There are two main factors influencing the kinetics stability of hydrogen generation from NaBH_(4).One factor is that the alkaline byproducts(NaBO_(2)) of the hydrolysis reaction can increase the pH of the solution,thus inhibiting the reaction process.It mainly happens in the NaBH_(4) solution hydrolysis system.Another factor is that the monotonous increase in reaction temperature leads to uncontrollable and unpredictable hydrolysis rates in the solid NaBH_(4) hydrolysis system.This is due to the excess heat generated from this exothermic reaction in the initial reaction of NaBH_(4) hydrolysis.In this perspective,we summarize the latest research progress in hydrogen generation from NaBH_(4) and emphasize the design principles of catalysts for hydrogen generation from NaBH_(4) solution and solid state NaBH_(4).The importance of carbon as catalyst support material for NaBH_(4) hydrolysis is also highlighted.展开更多
Partial shading conditions(PSCs)caused by uneven illumination become one of the most common problems in photovoltaic(PV)systems,which can make the PV power-voltage(P-V)characteristics curve show multi-peaks.Traditiona...Partial shading conditions(PSCs)caused by uneven illumination become one of the most common problems in photovoltaic(PV)systems,which can make the PV power-voltage(P-V)characteristics curve show multi-peaks.Traditional maximum power point tracking(MPPT)methods have shortcomings in tracking to the global maximum power point(GMPP),resulting in a dramatic decrease in output power.In order to solve the above problems,intelligent algorithms are used in MPPT.However,the existing intelligent algorithms have some disadvantages,such as slow convergence speed and large search oscillation.Therefore,an improved whale algorithm(IWOA)combined with the P&O(IWOA-P&O)is proposed for the MPPT of PV power generation in this paper.Firstly,IWOA is used to track the range interval of the GMPP,and then P&O is used to accurately find the MPP in that interval.Compared with other algorithms,simulation results show that this method has an average tracking efficiency of 99.79%and an average tracking time of 0.16 s when tracking GMPP.Finally,experimental verification is conducted,and the results show that the proposed algorithm has better MPPT performance compared to popular particle swarm optimization(PSO)and PSO-P&O algorithms.展开更多
In the increasingly decentralized energy environment,economical power dispatching from distributed generations(DGs)is crucial to minimizing operating costs,optimizing resource utilization,and guaranteeing a consistent...In the increasingly decentralized energy environment,economical power dispatching from distributed generations(DGs)is crucial to minimizing operating costs,optimizing resource utilization,and guaranteeing a consistent and sustainable supply of electricity.A comprehensive review of optimization techniques for economic power dispatching from distributed generations is imperative to identify the most effective strategies for minimizing operational costs while maintaining grid stability and sustainability.The choice of optimization technique for economic power dispatching from DGs depends on a number of factors,such as the size and complexity of the power system,the availability of computational resources,and the specific requirements of the application.Optimization techniques for economic power dispatching from distributed generations(DGs)can be classified into two main categories:(i)Classical optimization techniques,(ii)Heuristic optimization techniques.In classical optimization techniques,the linear programming(LP)model is one of the most popular optimization methods.Utilizing the LP model,power demand and network constraints are met while minimizing the overall cost of generating electricity from DGs.This approach is efficient in determining the best DGs dispatch and is capable of handling challenging optimization issues in the large-scale system including renewables.The quadratic programming(QP)model,a classical optimization technique,is a further popular optimization method,to consider non-linearity.The QP model can take into account the quadratic cost of energy production,with consideration constraints like network capacity,voltage,and frequency.The metaheuristic optimization techniques are also used for economic power dispatching from DGs,which include genetic algorithms(GA),particle swarm optimization(PSO),and ant colony optimization(ACO).Also,Some researchers are developing hybrid optimization techniques that combine elements of classical and heuristic optimization techniques with the incorporation of droop control,predictive control,and fuzzy-based methods.These methods can deal with large-scale systems with many objectives and non-linear,non-convex optimization issues.The most popular approaches are the LP and QP models,while more difficult problems are handled using metaheuristic optimization techniques.In summary,in order to increase efficiency,reduce costs,and ensure a consistent supply of electricity,optimization techniques are essential tools used in economic power dispatching from DGs.展开更多
The supercritical CO_(2) Brayton cycle is considered a promising energy conversion system for Generation IV reactors for its simple layout,compact structure,and high cycle efficiency.Mathematical models of four Brayto...The supercritical CO_(2) Brayton cycle is considered a promising energy conversion system for Generation IV reactors for its simple layout,compact structure,and high cycle efficiency.Mathematical models of four Brayton cycle layouts are developed in this study for different reactors to reduce the cost and increase the thermohydraulic performance of nuclear power generation to promote the commercialization of nuclear energy.Parametric analysis,multi-objective optimizations,and four decision-making methods are applied to obtain each Brayton scheme’s optimal thermohydraulic and economic indexes.Results show that for the same design thermal power scale of reactors,the higher the core’s exit temperature,the better the Brayton cycle’s thermo-economic performance.Among the four-cycle layouts,the recompression cycle(RC)has the best overall performance,followed by the simple recuperation cycle(SR)and the intercooling cycle(IC),and the worst is the reheating cycle(RH).However,RH has the lowest total cost of investment(C_(tot))of$1619.85 million,and IC has the lowest levelized cost of energy(LCOE)of 0.012$/(kWh).The nuclear Brayton cycle system’s overall performance has been improved due to optimization.The performance of the molten salt reactor combined with the intercooling cycle(MSR-IC)scheme has the greatest improvement,with the net output power(W_(net)),thermal efficiencyη_(t),and exergy efficiency(η_(e))improved by 8.58%,8.58%,and 11.21%,respectively.The performance of the lead-cooled fast reactor combined with the simple recuperation cycle scheme was optimized to increase C_(tot) by 27.78%.In comparison,the internal rate of return(IRR)increased by only 7.8%,which is not friendly to investors with limited funds.For the nuclear Brayton cycle,the molten salt reactor combined with the recompression cycle scheme should receive priority,and the gas-cooled fast reactor combined with the reheating cycle scheme should be considered carefully.展开更多
The understanding of how genetic and epigenetic factors influence tumorigenesis, progression and invasion, is vastly growing since new technologies allow the analysis of the functional genome namely the exome, the tra...The understanding of how genetic and epigenetic factors influence tumorigenesis, progression and invasion, is vastly growing since new technologies allow the analysis of the functional genome namely the exome, the transcriptome and the epigenome, besides enabling genome-wide assessment of genetic variations. With the advent of new drugs that are indicated tissue agnostic, depending on certain mutations, there is a growing demand for fast and cost-effective genetic diagnosis. The method in focus that already became an indispensable tool in viral diagnosis is next-generation sequencing (NGS). This approach allows sequencing of literally every DNA molecule in the sample and can either be used to assess numerous genetic markers of one patient at a time, or to assess fewer markers of many patients in parallel, which reduces costs. We submitted 23 samples of different tumor entities to four diagnostic companies with different analysis profiles. The results as disclosed and discussed in this report indicate that so far, the main application of NGS is rather in cancer research than in diagnosis, as none of the reports had a real impact on the therapeutic scheme. We are perfectly aware that such a small cohort cannot be generalized, but considering the costs vs. benefits, NGS should be engaged upon a very stringent evaluation only. However, in cases where obtaining a tissue biopsy is impossible or unfavorable, analysis of liquid biopsy by NGS provides a vital alternative.展开更多
With the current integration of distributed energy resources into the grid,the structure of distribution networks is becoming more complex.This complexity significantly expands the solution space in the optimization p...With the current integration of distributed energy resources into the grid,the structure of distribution networks is becoming more complex.This complexity significantly expands the solution space in the optimization process for network reconstruction using intelligent algorithms.Consequently,traditional intelligent algorithms frequently encounter insufficient search accuracy and become trapped in local optima.To tackle this issue,a more advanced particle swarm optimization algorithm is proposed.To address the varying emphases at different stages of the optimization process,a dynamic strategy is implemented to regulate the social and self-learning factors.The Metropolis criterion is introduced into the simulated annealing algorithm to occasionally accept suboptimal solutions,thereby mitigating premature convergence in the population optimization process.The inertia weight is adjusted using the logistic mapping technique to maintain a balance between the algorithm’s global and local search abilities.The incorporation of the Pareto principle involves the consideration of network losses and voltage deviations as objective functions.A fuzzy membership function is employed for selecting the results.Simulation analysis is carried out on the restructuring of the distribution network,using the IEEE-33 node system and the IEEE-69 node system as examples,in conjunction with the integration of distributed energy resources.The findings demonstrate that,in comparison to other intelligent optimization algorithms,the proposed enhanced algorithm demonstrates a shorter convergence time and effectively reduces active power losses within the network.Furthermore,it enhances the amplitude of node voltages,thereby improving the stability of distribution network operations and power supply quality.Additionally,the algorithm exhibits a high level of generality and applicability.展开更多
Current therapeutic approaches for volumetric muscle loss(VML)face challenges due to limited graft availability and insufficient bioactivities.To overcome these limitations,tissue-engineered scaffolds have emerged as ...Current therapeutic approaches for volumetric muscle loss(VML)face challenges due to limited graft availability and insufficient bioactivities.To overcome these limitations,tissue-engineered scaffolds have emerged as a promising alternative.In this study,we developed aligned ternary nanofibrous matrices comprised of poly(lactide-co-ε-caprolactone)integrated with collagen and Ti_(3)C_(2)T_(x)MXene nanoparticles(NPs)(PCM matrices),and explored their myogenic potential for skeletal muscle tissue regeneration.The PCM matrices demonstrated favorable physicochemical properties,including structural uniformity,alignment,microporosity,and hydrophilicity.In vitro assays revealed that the PCM matrices promoted cellular behaviors and myogenic differentiation of C2C12 myoblasts.Moreover,in vivo experiments demonstrated enhanced muscle remodeling and recovery in mice treated with PCM matrices following VML injury.Mechanistic insights from next-generation sequencing revealed that MXene NPs facilitated protein and ion availability within PCM matrices,leading to elevated intracellular Ca^(2+)levels in myoblasts through the activation of inducible nitric oxide synthase(i NOS)and serum/glucocorticoid regulated kinase 1(SGK1),ultimately promoting myogenic differentiation via the m TOR-AKT pathway.Additionally,upregulated i NOS and increased NO–contributed to myoblast proliferation and fiber fusion,thereby facilitating overall myoblast maturation.These findings underscore the potential of MXene NPs loaded within highly aligned matrices as therapeutic agents to promote skeletal muscle tissue recovery.展开更多
With the introduction of the“dual carbon goals,”there has been a robust development of distributed photovoltaic power generation projects in the promotion of their construction.As part of this initiative,a comprehen...With the introduction of the“dual carbon goals,”there has been a robust development of distributed photovoltaic power generation projects in the promotion of their construction.As part of this initiative,a comprehensive and systematic analysis has been conducted to study the overall benefits of photovoltaic power generation projects.The evaluation process encompasses economic,technical,environmental,and social aspects,providing corresponding analysis methods and data references.Furthermore,targeted countermeasures and suggestions are proposed,signifying the research’s importance for the construction and development of subsequent distributed photovoltaic power generation projects.展开更多
Decarbonization of the power sector in China is an essential aspect of the energy transition process to achieve carbon neutrality.The power sector accounts for approximately 40%of China’s total CO_(2) emissions.Accor...Decarbonization of the power sector in China is an essential aspect of the energy transition process to achieve carbon neutrality.The power sector accounts for approximately 40%of China’s total CO_(2) emissions.Accordingly,collaborative optimization in power generation expansion planning(GEP)simultaneously considering economic,environmental,and technological concerns as carbon emissions is necessary.This paper proposes a collaborative mixedinteger linear programming optimization approach for GEP.This minimizes the power system’s operating cost to resolve emission concerns considering energy development strategies,flexible generation,and resource limitations constraints.This research further analyzes the advantages and disadvantages of current GEP techniques.Results show that the main determinants of new investment decisions are carbon emissions,reserve margins,resource availability,fuel consumption,and fuel price.The proposed optimization method is simulated and validated based on China’s power system data.Finally,this study provides policy recommendations on the flexible management of traditional power sources,the market-oriented mechanism of new energy sources,and the integration of new technology to support the attainment of carbon-neutral targets in the current energy transition process.展开更多
Hydrogen peroxide(H_(2)O_(2)) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently,the prominent method for the preparation of H_(2)O_(2) is the anthr...Hydrogen peroxide(H_(2)O_(2)) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently,the prominent method for the preparation of H_(2)O_(2) is the anthraquinone oxidation.Unfortunately, it is not conducive to economic and sustainable development since it is a complex process and involves unfriendly environment and potential hazards. In this context, numerous approaches have been developed to synthesize H_(2)O_(2). Among them, photo/electro-catalytic ones are considered as two of the most promising manners for on-site synthesis of H_(2)O_(2). These alternatives are sustainable in that only water or O_(2) is required. Namely, water oxidation(WOR) or oxygen reduction(ORR)reactions can be further coupled with clean and sustainable energy. For photo/electro-catalytic reactions for H_(2)O_(2) generation, the design of the catalysts is extremely important and has been extensively conducted with an aim to obtain ultimate catalytic performance. This article overviews the basic principles of WOR and ORR,followed by the summary of recent progresses and achievements on the design and performance of various photo/electro-catalysts for H_(2)O_(2) generation. The related mechanisms for these approaches are highlighted from theoretical and experimental aspects. Scientific challenges and opportunities of engineering photo/electro-catalysts for H_(2)O_(2) generation are also outlined and discussed.展开更多
Accurate insight into the heat generation rate(HGR) of lithium-ion batteries(LIBs) is one of key issues for battery management systems to formulate thermal safety warning strategies in advance.For this reason,this pap...Accurate insight into the heat generation rate(HGR) of lithium-ion batteries(LIBs) is one of key issues for battery management systems to formulate thermal safety warning strategies in advance.For this reason,this paper proposes a novel physics-informed neural network(PINN) approach for HGR estimation of LIBs under various driving conditions.Specifically,a single particle model with thermodynamics(SPMT) is first constructed for extracting the critical physical knowledge related with battery HGR.Subsequently,the surface concentrations of positive and negative electrodes in battery SPMT model are integrated into the bidirectional long short-term memory(BiLSTM) networks as physical information.And combined with other feature variables,a novel PINN approach to achieve HGR estimation of LIBs with higher accuracy is constituted.Additionally,some critical hyperparameters of BiLSTM used in PINN approach are determined through Bayesian optimization algorithm(BOA) and the results of BOA-based BiLSTM are compared with other traditional BiLSTM/LSTM networks.Eventually,combined with the HGR data generated from the validated virtual battery,it is proved that the proposed approach can well predict the battery HGR under the dynamic stress test(DST) and worldwide light vehicles test procedure(WLTP),the mean absolute error under DST is 0.542 kW/m^(3),and the root mean square error under WLTP is1.428 kW/m^(3)at 25℃.Lastly,the investigation results of this paper also show a new perspective in the application of the PINN approach in battery HGR estimation.展开更多
基金supported in part by the National Natural Science Foundation of China (Grant Nos.51975347 and 51907117)in part by the Shanghai Science and Technology Program (Grant No.22010501600).
文摘Regular fastener detection is necessary to ensure the safety of railways.However,the number of abnormal fasteners is significantly lower than the number of normal fasteners in real railways.Existing supervised inspectionmethods have insufficient detection ability in cases of imbalanced samples.To solve this problem,we propose an approach based on deep convolutional neural networks(DCNNs),which consists of three stages:fastener localization,abnormal fastener sample generation based on saliency detection,and fastener state inspection.First,a lightweight YOLOv5s is designed to achieve fast and precise localization of fastener regions.Then,the foreground clip region of a fastener image is extracted by the designed fastener saliency detection network(F-SDNet),combined with data augmentation to generate a large number of abnormal fastener samples and balance the number of abnormal and normal samples.Finally,a fastener inspection model called Fastener ResNet-8 is constructed by being trained with the augmented fastener dataset.Results show the effectiveness of our proposed method in solving the problem of sample imbalance in fastener detection.Qualitative and quantitative comparisons show that the proposed F-SDNet outperforms other state-of-the-art methods in clip region extraction,reaching MAE and max F-measure of 0.0215 and 0.9635,respectively.In addition,the FPS of the fastener state inspection model reached 86.2,and the average accuracy reached 98.7%on 614 augmented fastener test sets and 99.9%on 7505 real fastener datasets.
基金funded by the National Natural Science Foundation of China(Grant/Award Numbers 62075135 and 61975126)the Science and Technology Innovation Commission of Shenzhen(Grant/Award Numbers JCYJ20190808174819083 and JCYJ20190808175201640)Shenzhen Science and Technology Planning Project(ZDSYS 20210623092006020).
文摘Measurement of bloodflow velocity is key to understanding physiology and pathology in vivo.While most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the instantaneous bloodflow velocity distribution.This is mainly due to the lack of measurement technology with high spatial and temporal resolution.Here,we tackle this problem with our recently developed dual-wavelength line-scan third-harmonic generation(THG)imaging technology.Simultaneous acquisition of dual-wavelength THG line-scanning signals enables measurement of bloodflow velocities at two radially symmetric positions in both venules and arterioles in mouse brain in vivo.Our results clearly show that the instantaneous bloodflow velocity is not symmetric under general conditions.
基金Supported by the Key Research Program of the Chinese Academy of Sciences(ZDRE-KT-2021-3)。
文摘Both analyzing a large amount of space weather observed data and alleviating personal experience bias are significant challenges in generating artificial space weather forecast products.With the use of natural language generation methods based on the sequence-to-sequence model,space weather forecast texts can be automatically generated.To conduct our generation tasks at a fine-grained level,a taxonomy of space weather phenomena based on descriptions is presented.Then,our MDH(Multi-Domain Hybrid)model is proposed for generating space weather summaries in two stages.This model is composed of three sequence-to-sequence-based deep neural network sub-models(one Bidirectional Auto-Regressive Transformers pre-trained model and two Transformer models).Then,to evaluate how well MDH performs,quality evaluation metrics based on two prevalent automatic metrics and our innovative human metric are presented.The comprehensive scores of the three summaries generating tasks on testing datasets are 70.87,93.50,and 92.69,respectively.The results suggest that MDH can generate space weather summaries with high accuracy and coherence,as well as suitable length,which can assist forecasters in generating high-quality space weather forecast products,despite the data being starved.
基金the Qingdao Innovation Leading Talent Program,National Natural Science Foundation of China(21805124)Natural Science Foundation of Shandong Province(ZR2018BEM020).
文摘The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water resources.At present,many kinds of photothermal conversion materials have been developed and used as evaporators in seawater desalination.However,some evaporators need additional thermal insulation or water supply devices to achieve efficient photothermal conversion.In addition,their complex,time consuming and no scalable preparation process,high cost of raw materials and poor salt resistance hinder the practical application of these evaporator.Owing to its distinctive nanoporous structure,diatomite as fossilized single-cells algae diatoms is a promising natural silica-based material for seawater desalination.They are taken from sea and that makes true sense to use them in the sea.Herein,we report the first example of synthesis robust three-dimensional(3D)natural-diatomite composite by assembling polyaniline nanoparticles covered diatomite into the polyvinyl alcohol pre-treated melamine foam frameworks and demonstrate its application as new evaporator for seawater desalination.The porous framework does not only improve the sunlight scattering efficiency,but also offer large network of channels for water transportation.The inherent mechanism behind salt desalination process involves the absorption of water molecules on the surface of the internal silica micro-nano pores,and evaporation under the heat induced by the polyaniline absorbed sunlight.Meanwhile,the metal ions are segregated by many available pores and channels to achieve the self-desalting effect.The developed evaporator possesses the superiority of multi-stage pore structure,strong hydrophilicity,low thermal conductivity,excellent light absorption,fast water transportation and salt-resistant crystallization as well as good durability.The evaporation rate without an additional device is found to be 1.689 kg m^(-2)h^(-1)under 1-Sun irradiation,and the energy conversion efficiency is as high as 95%.This work creates a platform and develops the prospect of employing green and sustainable natural-diatomite composite evaporator for practical applications of seawater desalination.
基金funded by University Natural Science Research Project of Anhui Province,Grant Numbers (KJ2020A0826,2022AH051885,2022AH051891,2022AH030160,62303231)Intelligent Detection Research Team Funds for the Anhui Institute of Information Technology,Grant Number (AXG2023_kjc_5004).
文摘In this study,numerical simulations of the pinching-off phenomena displayed by the dispersed phase in a continuous phase have been conducted using COMSOL Multiphysics(level-set method).Four flow patterns,namely“drop flow”,“jet flow”,“squeeze flow”,and“co-flow”,have been obtained for different flow velocity ratios,channel diameter ratios,density ratios,viscosity ratios,and surface tension.The flow pattern map of two-phase flow in coaxial microchannels has been obtained accordingly,and the associated droplet generation process has been critically discussed considering the related frequency,diameter,and pinch-off length.In particular,it is shown that the larger the flow velocity ratio,the smaller the diameter of generated droplets and the shorter the pinch-off length.The pinch-off length of a droplet is influenced by the channel diameter ratio and density ratio.The changes in viscosity ratio have a negligible influence on the droplet generation pinching frequency.With an increase in surface tension,the frequency of generation and pinch-off length of droplets decrease,but for small surface tension the generation diameter of droplet increases.
基金supported in part by the National Natural Science Foundation of China(Grant No.62276274)Shaanxi Natural Science Foundation(Grant No.2023-JC-YB-528)Chinese aeronautical establishment(Grant No.201851U8012)。
文摘The automatic stealth task of military time-sensitive targets plays a crucial role in maintaining national military security and mastering battlefield dynamics in military applications.We propose a novel Military Time-sensitive Targets Stealth Network via Real-time Mask Generation(MTTSNet).According to our knowledge,this is the first technology to automatically remove military targets in real-time from videos.The critical steps of MTTSNet are as follows:First,we designed a real-time mask generation network based on the encoder-decoder framework,combined with the domain expansion structure,to effectively extract mask images.Specifically,the ASPP structure in the encoder could achieve advanced semantic feature fusion.The decoder stacked high-dimensional information with low-dimensional information to obtain an effective mask layer.Subsequently,the domain expansion module guided the adaptive expansion of mask images.Second,a context adversarial generation network based on gated convolution was constructed to achieve background restoration of mask positions in the original image.In addition,our method worked in an end-to-end manner.A particular semantic segmentation dataset for military time-sensitive targets has been constructed,called the Military Time-sensitive Target Masking Dataset(MTMD).The MTMD dataset experiment successfully demonstrated that this method could create a mask that completely occludes the target and that the target could be hidden in real time using this mask.We demonstrated the concealment performance of our proposed method by comparing it to a number of well-known and highly optimized baselines.
文摘The investigation endorsed the convective flow of Carreau nanofluid over a stretched surface in presence of entropy generation optimization.The novel dynamic of viscous dissipation is utilized to analyze the thermal mechanism of magnetized flow.The convective boundary assumptions are directed in order to examine the heat and mass transportation of nanofluid.The thermal concept of thermophoresis and Brownian movements has been re-called with the help of Buongiorno model.The problem formulated in dimensionless form is solved by NDSolve MATHEMATICA.The graphical analysis for parameters governed by the problem is performed with physical applications.The affiliation of entropy generation and Bejan number for different parameters is inspected in detail.The numerical data for illustrating skin friction,heat and mass transfer rate is also reported.The motion of the fluid is highest for the viscosity ratio parameter.The temperature of the fluid rises via thermal Biot number.Entropy generation rises for greater Brinkman number and diffusion parameter.
基金supported by the Natural Science Foundation of Jilin Province (Grant No.20220101010JC)the National Natural Science Foundation of China (Grant No.12074146)。
文摘High harmonic generation in ZnO crystals under chirped single-color field and static electric field are investigated by solving the semiconductor Bloch equation(SBE). It is found that when the chirp pulse is introduced, the interference structure becomes obvious while the harmonic cutoff is not extended. Furthermore, the harmonic efficiency is improved when the static electric field is included. These phenomena are demonstrated by the classical recollision model in real space affected by the waveform of laser field and inversion symmetry. Specifically, the electron motion in k-space shows that the change of waveform and the destruction of the symmetry of the laser field lead to the incomplete X-structure of the crystal-momentum-resolved(k-resolved) inter-band harmonic spectrum. Furthermore, a pre-acceleration process in the solid four-step model is confirmed.
基金supported by the Natural Science Foundation of China(Grant Nos.52076079,52206010)Natural Science Foundation of Hebei Province,China(Grant No.E2020502013)the Fundamental Research Funds for the Central Universities(2021MS076,2021MS079).
文摘There is a growing need to explore the potential of coal-fired power plants(CFPPs)to enhance the utilization rate of wind power(wind)and photovoltaic power(PV)in the green energy field.This study developed a load regulation model for a multi-power generation system comprising wind,PV,and coal energy storage using realworld data.The power supply process was divided into eight fundamental load regulation scenarios,elucidating the influence of each scenario on load regulation.Within the framework of the multi-power generation system with the wind(50 MW)and PV(50 MW)alongside a CFPP(330 MW),a lithium-iron phosphate energy storage system(LIPBESS)was integrated to improve the system’s load regulation flexibility.The energy storage operation strategy was formulated based on the charging and discharging priority of the LIPBESS for each basic scenario and the charging and discharging load calculation method of LIPBESS auxiliary regulation.Through optimization using the particle swarm algorithm,the optimal capacity of LIPBESS was determined to be within the 5.24-4.88 MWh range.From an economic perspective,the LIPBESS operating with CFPP as the regulating power source was 49.1% lower in capacity compared to the renewable energy-based storage mode.
基金supported by MOST of China(No.2021YFB4000603)NSFC(No.22179002 and 51971004).
文摘Sodium borohydride(NaBH_(4)) is considered as the most potential hydrogen storage material for portable proton exchange membrane fuel cells(PEMFC)because of its high theoretical hydrogen capacity.However,the slow and poor kinetic stability of hydrogen generation from NaBH_(4) hydrolysis limits its application.There are two main factors influencing the kinetics stability of hydrogen generation from NaBH_(4).One factor is that the alkaline byproducts(NaBO_(2)) of the hydrolysis reaction can increase the pH of the solution,thus inhibiting the reaction process.It mainly happens in the NaBH_(4) solution hydrolysis system.Another factor is that the monotonous increase in reaction temperature leads to uncontrollable and unpredictable hydrolysis rates in the solid NaBH_(4) hydrolysis system.This is due to the excess heat generated from this exothermic reaction in the initial reaction of NaBH_(4) hydrolysis.In this perspective,we summarize the latest research progress in hydrogen generation from NaBH_(4) and emphasize the design principles of catalysts for hydrogen generation from NaBH_(4) solution and solid state NaBH_(4).The importance of carbon as catalyst support material for NaBH_(4) hydrolysis is also highlighted.
基金supported in part by the Natural Science Foundation of Jiangsu Province under Grant BK20200969(L.Z.,URL:http://std.jiangsu.gov.cn/)in part by Basic Science(Natural Science)Research Project of Colleges and Universities in Jiangsu Province under Grant 22KJB470025(L.R.,URL:http://jyt.jiangsu.gov.cn/)in part by Social People’s Livelihood Technology Plan General Project of Nantong under Grant MS12021015(L.Q.,URL:http://kjj.nantong.gov.cn/).
文摘Partial shading conditions(PSCs)caused by uneven illumination become one of the most common problems in photovoltaic(PV)systems,which can make the PV power-voltage(P-V)characteristics curve show multi-peaks.Traditional maximum power point tracking(MPPT)methods have shortcomings in tracking to the global maximum power point(GMPP),resulting in a dramatic decrease in output power.In order to solve the above problems,intelligent algorithms are used in MPPT.However,the existing intelligent algorithms have some disadvantages,such as slow convergence speed and large search oscillation.Therefore,an improved whale algorithm(IWOA)combined with the P&O(IWOA-P&O)is proposed for the MPPT of PV power generation in this paper.Firstly,IWOA is used to track the range interval of the GMPP,and then P&O is used to accurately find the MPP in that interval.Compared with other algorithms,simulation results show that this method has an average tracking efficiency of 99.79%and an average tracking time of 0.16 s when tracking GMPP.Finally,experimental verification is conducted,and the results show that the proposed algorithm has better MPPT performance compared to popular particle swarm optimization(PSO)and PSO-P&O algorithms.
文摘In the increasingly decentralized energy environment,economical power dispatching from distributed generations(DGs)is crucial to minimizing operating costs,optimizing resource utilization,and guaranteeing a consistent and sustainable supply of electricity.A comprehensive review of optimization techniques for economic power dispatching from distributed generations is imperative to identify the most effective strategies for minimizing operational costs while maintaining grid stability and sustainability.The choice of optimization technique for economic power dispatching from DGs depends on a number of factors,such as the size and complexity of the power system,the availability of computational resources,and the specific requirements of the application.Optimization techniques for economic power dispatching from distributed generations(DGs)can be classified into two main categories:(i)Classical optimization techniques,(ii)Heuristic optimization techniques.In classical optimization techniques,the linear programming(LP)model is one of the most popular optimization methods.Utilizing the LP model,power demand and network constraints are met while minimizing the overall cost of generating electricity from DGs.This approach is efficient in determining the best DGs dispatch and is capable of handling challenging optimization issues in the large-scale system including renewables.The quadratic programming(QP)model,a classical optimization technique,is a further popular optimization method,to consider non-linearity.The QP model can take into account the quadratic cost of energy production,with consideration constraints like network capacity,voltage,and frequency.The metaheuristic optimization techniques are also used for economic power dispatching from DGs,which include genetic algorithms(GA),particle swarm optimization(PSO),and ant colony optimization(ACO).Also,Some researchers are developing hybrid optimization techniques that combine elements of classical and heuristic optimization techniques with the incorporation of droop control,predictive control,and fuzzy-based methods.These methods can deal with large-scale systems with many objectives and non-linear,non-convex optimization issues.The most popular approaches are the LP and QP models,while more difficult problems are handled using metaheuristic optimization techniques.In summary,in order to increase efficiency,reduce costs,and ensure a consistent supply of electricity,optimization techniques are essential tools used in economic power dispatching from DGs.
基金This work was supported of National Natural Science Foundation of China Fund(No.52306033)State Key Laboratory of Engines Fund(No.SKLE-K2022-07)the Jiangxi Provincial Postgraduate Innovation Special Fund(No.YC2022-s513).
文摘The supercritical CO_(2) Brayton cycle is considered a promising energy conversion system for Generation IV reactors for its simple layout,compact structure,and high cycle efficiency.Mathematical models of four Brayton cycle layouts are developed in this study for different reactors to reduce the cost and increase the thermohydraulic performance of nuclear power generation to promote the commercialization of nuclear energy.Parametric analysis,multi-objective optimizations,and four decision-making methods are applied to obtain each Brayton scheme’s optimal thermohydraulic and economic indexes.Results show that for the same design thermal power scale of reactors,the higher the core’s exit temperature,the better the Brayton cycle’s thermo-economic performance.Among the four-cycle layouts,the recompression cycle(RC)has the best overall performance,followed by the simple recuperation cycle(SR)and the intercooling cycle(IC),and the worst is the reheating cycle(RH).However,RH has the lowest total cost of investment(C_(tot))of$1619.85 million,and IC has the lowest levelized cost of energy(LCOE)of 0.012$/(kWh).The nuclear Brayton cycle system’s overall performance has been improved due to optimization.The performance of the molten salt reactor combined with the intercooling cycle(MSR-IC)scheme has the greatest improvement,with the net output power(W_(net)),thermal efficiencyη_(t),and exergy efficiency(η_(e))improved by 8.58%,8.58%,and 11.21%,respectively.The performance of the lead-cooled fast reactor combined with the simple recuperation cycle scheme was optimized to increase C_(tot) by 27.78%.In comparison,the internal rate of return(IRR)increased by only 7.8%,which is not friendly to investors with limited funds.For the nuclear Brayton cycle,the molten salt reactor combined with the recompression cycle scheme should receive priority,and the gas-cooled fast reactor combined with the reheating cycle scheme should be considered carefully.
文摘The understanding of how genetic and epigenetic factors influence tumorigenesis, progression and invasion, is vastly growing since new technologies allow the analysis of the functional genome namely the exome, the transcriptome and the epigenome, besides enabling genome-wide assessment of genetic variations. With the advent of new drugs that are indicated tissue agnostic, depending on certain mutations, there is a growing demand for fast and cost-effective genetic diagnosis. The method in focus that already became an indispensable tool in viral diagnosis is next-generation sequencing (NGS). This approach allows sequencing of literally every DNA molecule in the sample and can either be used to assess numerous genetic markers of one patient at a time, or to assess fewer markers of many patients in parallel, which reduces costs. We submitted 23 samples of different tumor entities to four diagnostic companies with different analysis profiles. The results as disclosed and discussed in this report indicate that so far, the main application of NGS is rather in cancer research than in diagnosis, as none of the reports had a real impact on the therapeutic scheme. We are perfectly aware that such a small cohort cannot be generalized, but considering the costs vs. benefits, NGS should be engaged upon a very stringent evaluation only. However, in cases where obtaining a tissue biopsy is impossible or unfavorable, analysis of liquid biopsy by NGS provides a vital alternative.
基金This research is supported by the Science and Technology Program of Gansu Province(No.23JRRA880).
文摘With the current integration of distributed energy resources into the grid,the structure of distribution networks is becoming more complex.This complexity significantly expands the solution space in the optimization process for network reconstruction using intelligent algorithms.Consequently,traditional intelligent algorithms frequently encounter insufficient search accuracy and become trapped in local optima.To tackle this issue,a more advanced particle swarm optimization algorithm is proposed.To address the varying emphases at different stages of the optimization process,a dynamic strategy is implemented to regulate the social and self-learning factors.The Metropolis criterion is introduced into the simulated annealing algorithm to occasionally accept suboptimal solutions,thereby mitigating premature convergence in the population optimization process.The inertia weight is adjusted using the logistic mapping technique to maintain a balance between the algorithm’s global and local search abilities.The incorporation of the Pareto principle involves the consideration of network losses and voltage deviations as objective functions.A fuzzy membership function is employed for selecting the results.Simulation analysis is carried out on the restructuring of the distribution network,using the IEEE-33 node system and the IEEE-69 node system as examples,in conjunction with the integration of distributed energy resources.The findings demonstrate that,in comparison to other intelligent optimization algorithms,the proposed enhanced algorithm demonstrates a shorter convergence time and effectively reduces active power losses within the network.Furthermore,it enhances the amplitude of node voltages,thereby improving the stability of distribution network operations and power supply quality.Additionally,the algorithm exhibits a high level of generality and applicability.
基金supported by the National Research Foundation of Korea(NRF)grant funded by the Korean Government(the Ministry of Science and ICT(MSIT))(No.2021R1A2C2006013)the Bio&Medical Technology Development Program of the NRF funded by the Korean government(MSIT)(No.RS-2023-00223591)the Korea Medical Device Development Fund grant funded by the Korean government(the MSIT,the MOTIE,the Ministry of Health and Welfare,the Ministry of Food and Drug Safety)(NTIS Number:9991006781,KMDF_PR_(2)0200901_0108)。
文摘Current therapeutic approaches for volumetric muscle loss(VML)face challenges due to limited graft availability and insufficient bioactivities.To overcome these limitations,tissue-engineered scaffolds have emerged as a promising alternative.In this study,we developed aligned ternary nanofibrous matrices comprised of poly(lactide-co-ε-caprolactone)integrated with collagen and Ti_(3)C_(2)T_(x)MXene nanoparticles(NPs)(PCM matrices),and explored their myogenic potential for skeletal muscle tissue regeneration.The PCM matrices demonstrated favorable physicochemical properties,including structural uniformity,alignment,microporosity,and hydrophilicity.In vitro assays revealed that the PCM matrices promoted cellular behaviors and myogenic differentiation of C2C12 myoblasts.Moreover,in vivo experiments demonstrated enhanced muscle remodeling and recovery in mice treated with PCM matrices following VML injury.Mechanistic insights from next-generation sequencing revealed that MXene NPs facilitated protein and ion availability within PCM matrices,leading to elevated intracellular Ca^(2+)levels in myoblasts through the activation of inducible nitric oxide synthase(i NOS)and serum/glucocorticoid regulated kinase 1(SGK1),ultimately promoting myogenic differentiation via the m TOR-AKT pathway.Additionally,upregulated i NOS and increased NO–contributed to myoblast proliferation and fiber fusion,thereby facilitating overall myoblast maturation.These findings underscore the potential of MXene NPs loaded within highly aligned matrices as therapeutic agents to promote skeletal muscle tissue recovery.
文摘With the introduction of the“dual carbon goals,”there has been a robust development of distributed photovoltaic power generation projects in the promotion of their construction.As part of this initiative,a comprehensive and systematic analysis has been conducted to study the overall benefits of photovoltaic power generation projects.The evaluation process encompasses economic,technical,environmental,and social aspects,providing corresponding analysis methods and data references.Furthermore,targeted countermeasures and suggestions are proposed,signifying the research’s importance for the construction and development of subsequent distributed photovoltaic power generation projects.
基金supported by the Natural Science Foundation of Shandong Province (No.ZR2019MEE078)Education and Teaching Reform Research Project of Shandong University (“Development of an experiment platform to support the intelligent energy courses”)。
文摘Decarbonization of the power sector in China is an essential aspect of the energy transition process to achieve carbon neutrality.The power sector accounts for approximately 40%of China’s total CO_(2) emissions.Accordingly,collaborative optimization in power generation expansion planning(GEP)simultaneously considering economic,environmental,and technological concerns as carbon emissions is necessary.This paper proposes a collaborative mixedinteger linear programming optimization approach for GEP.This minimizes the power system’s operating cost to resolve emission concerns considering energy development strategies,flexible generation,and resource limitations constraints.This research further analyzes the advantages and disadvantages of current GEP techniques.Results show that the main determinants of new investment decisions are carbon emissions,reserve margins,resource availability,fuel consumption,and fuel price.The proposed optimization method is simulated and validated based on China’s power system data.Finally,this study provides policy recommendations on the flexible management of traditional power sources,the market-oriented mechanism of new energy sources,and the integration of new technology to support the attainment of carbon-neutral targets in the current energy transition process.
基金supported by Shanxi Province Science Foundation (20210302124446202102070301018)+1 种基金the National Natural Science Joint Foundation (U1710112)Basic Research Project from the Institute of Coal Chemistry, CAS (SCJC-HN-2022-17)。
文摘Hydrogen peroxide(H_(2)O_(2)) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently,the prominent method for the preparation of H_(2)O_(2) is the anthraquinone oxidation.Unfortunately, it is not conducive to economic and sustainable development since it is a complex process and involves unfriendly environment and potential hazards. In this context, numerous approaches have been developed to synthesize H_(2)O_(2). Among them, photo/electro-catalytic ones are considered as two of the most promising manners for on-site synthesis of H_(2)O_(2). These alternatives are sustainable in that only water or O_(2) is required. Namely, water oxidation(WOR) or oxygen reduction(ORR)reactions can be further coupled with clean and sustainable energy. For photo/electro-catalytic reactions for H_(2)O_(2) generation, the design of the catalysts is extremely important and has been extensively conducted with an aim to obtain ultimate catalytic performance. This article overviews the basic principles of WOR and ORR,followed by the summary of recent progresses and achievements on the design and performance of various photo/electro-catalysts for H_(2)O_(2) generation. The related mechanisms for these approaches are highlighted from theoretical and experimental aspects. Scientific challenges and opportunities of engineering photo/electro-catalysts for H_(2)O_(2) generation are also outlined and discussed.
基金funded by the Artificial Intelligence Technology Project of Xi’an Science and Technology Bureau in China(No.21RGZN0014)。
文摘Accurate insight into the heat generation rate(HGR) of lithium-ion batteries(LIBs) is one of key issues for battery management systems to formulate thermal safety warning strategies in advance.For this reason,this paper proposes a novel physics-informed neural network(PINN) approach for HGR estimation of LIBs under various driving conditions.Specifically,a single particle model with thermodynamics(SPMT) is first constructed for extracting the critical physical knowledge related with battery HGR.Subsequently,the surface concentrations of positive and negative electrodes in battery SPMT model are integrated into the bidirectional long short-term memory(BiLSTM) networks as physical information.And combined with other feature variables,a novel PINN approach to achieve HGR estimation of LIBs with higher accuracy is constituted.Additionally,some critical hyperparameters of BiLSTM used in PINN approach are determined through Bayesian optimization algorithm(BOA) and the results of BOA-based BiLSTM are compared with other traditional BiLSTM/LSTM networks.Eventually,combined with the HGR data generated from the validated virtual battery,it is proved that the proposed approach can well predict the battery HGR under the dynamic stress test(DST) and worldwide light vehicles test procedure(WLTP),the mean absolute error under DST is 0.542 kW/m^(3),and the root mean square error under WLTP is1.428 kW/m^(3)at 25℃.Lastly,the investigation results of this paper also show a new perspective in the application of the PINN approach in battery HGR estimation.