The photochemical vibrational reaction of UF_6+HCl was investigated by exciting the ternary overtone of 3ν_3 of UF_6 in an intracavity CO laser system.It was found that the rate of the laser-driven reaction was much ...The photochemical vibrational reaction of UF_6+HCl was investigated by exciting the ternary overtone of 3ν_3 of UF_6 in an intracavity CO laser system.It was found that the rate of the laser-driven reaction was much greater than that of the thermal reaction and this photochemical process had an isotopic selectivity.The uranium isotope enrichment factors measured in experiments wore around 1,007 in a single step.展开更多
文摘The photochemical vibrational reaction of UF_6+HCl was investigated by exciting the ternary overtone of 3ν_3 of UF_6 in an intracavity CO laser system.It was found that the rate of the laser-driven reaction was much greater than that of the thermal reaction and this photochemical process had an isotopic selectivity.The uranium isotope enrichment factors measured in experiments wore around 1,007 in a single step.
