Considering that KBe2BO3F2(KBBF) is an outstanding deep ultraviolet crystal which can generate the shortest wavelengths in second harmonic generation and sum-frequency generation,we report the determination of the non...Considering that KBe2BO3F2(KBBF) is an outstanding deep ultraviolet crystal which can generate the shortest wavelengths in second harmonic generation and sum-frequency generation,we report the determination of the nonlinear optical coefficients of the KBBF crystal.The d11 coefficient was determined to be 0.49pm/V by the Maker fringes method at the wavelength 1064nm,which is in agreement well with the theoretical value.展开更多
We report that a deep ultraviolet （DUV） laser from the sixth harmonic of a 1064nm laser has been firstly used as light source in an ultrahigh energy-resolution angle-resolved photoemission spectroscopy （ARPES）. Th...We report that a deep ultraviolet （DUV） laser from the sixth harmonic of a 1064nm laser has been firstly used as light source in an ultrahigh energy-resolution angle-resolved photoemission spectroscopy （ARPES）. The wavelength is 177.3nm obtained by using the second harmonic KBe2BO3F2 crystal with a frequency tripled 1064nm Nd：YVO4 laser. The large flux （10^14 - 10^15 photons/s） and narrow line width （0.26 meV） are suitable for the ultrahigh-energy resolution ARPES. The laser-ARPES can be a powerful tool to study the electronic structure at and near the Fermi level of the superconductor and correlated materials. The laser-ARPES has worked more than 500 h already.展开更多
We briefly review recent results on photoemission spectroscopy based on the deep and vacuum ultraviolet diode pumped solid-state lasers which we have developed.Cascaded second harmonic generation with the nonlinear cr...We briefly review recent results on photoemission spectroscopy based on the deep and vacuum ultraviolet diode pumped solid-state lasers which we have developed.Cascaded second harmonic generation with the nonlinear crystal KBe2BO3F2(KBBF)is used to generate deep ultraviolet and vacuum ultraviolet laser radiation,which complements traditional incoherent light sources such as gas discharge lamps and synchrotron radiation,and has greatly improved resolution with respect to energy,momentum,and spin of photoemission spectroscopy.Many new functions have been developed with the advantages of high photon energy,narrow linewidth,high photon flux density,and so on.These have led to the observation of various new phenomena and the amassment of new data in the fields of high temperature superconductivity,topological electronics,Fermi semi-metals,and so forth.These laser systems have revived the field of photoemission spectroscopy and provided a new platform in this frontier research field.展开更多
文摘Considering that KBe2BO3F2(KBBF) is an outstanding deep ultraviolet crystal which can generate the shortest wavelengths in second harmonic generation and sum-frequency generation,we report the determination of the nonlinear optical coefficients of the KBBF crystal.The d11 coefficient was determined to be 0.49pm/V by the Maker fringes method at the wavelength 1064nm,which is in agreement well with the theoretical value.
基金Supported by the National Basic Research Programme of China under Grant No 2004CB619006, and the National Natural Science Foundation of China under Grant Nos 60578030 and 50590404.
文摘We report that a deep ultraviolet （DUV） laser from the sixth harmonic of a 1064nm laser has been firstly used as light source in an ultrahigh energy-resolution angle-resolved photoemission spectroscopy （ARPES）. The wavelength is 177.3nm obtained by using the second harmonic KBe2BO3F2 crystal with a frequency tripled 1064nm Nd：YVO4 laser. The large flux （10^14 - 10^15 photons/s） and narrow line width （0.26 meV） are suitable for the ultrahigh-energy resolution ARPES. The laser-ARPES can be a powerful tool to study the electronic structure at and near the Fermi level of the superconductor and correlated materials. The laser-ARPES has worked more than 500 h already.
基金Project supported by the National Development Project for Major Scientific Research Facility(No.ZDYZ2012-2)the National Instrumentation Program(No.2012YQ120048)
文摘We briefly review recent results on photoemission spectroscopy based on the deep and vacuum ultraviolet diode pumped solid-state lasers which we have developed.Cascaded second harmonic generation with the nonlinear crystal KBe2BO3F2(KBBF)is used to generate deep ultraviolet and vacuum ultraviolet laser radiation,which complements traditional incoherent light sources such as gas discharge lamps and synchrotron radiation,and has greatly improved resolution with respect to energy,momentum,and spin of photoemission spectroscopy.Many new functions have been developed with the advantages of high photon energy,narrow linewidth,high photon flux density,and so on.These have led to the observation of various new phenomena and the amassment of new data in the fields of high temperature superconductivity,topological electronics,Fermi semi-metals,and so forth.These laser systems have revived the field of photoemission spectroscopy and provided a new platform in this frontier research field.
