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Air–water CO2 flux in an algae bloom year for Lake Hongfeng,Southwest China:implications for the carbon cycle of global inland waters 被引量:8
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作者 Faxiang Tao 《Acta Geochimica》 EI CAS CSCD 2017年第4期658-666,共9页
The carbon cycle of global inland waters is quantitatively comparable to other components in the global carbon budget. Among inland waters, a significant part is man-made lakes formed by damming rivers. Manmade lakes ... The carbon cycle of global inland waters is quantitatively comparable to other components in the global carbon budget. Among inland waters, a significant part is man-made lakes formed by damming rivers. Manmade lakes are undergoing a rapid increase in number and size. Human impacts and frequent algae blooms lead to it necessary to make a better constraint on their carbon cycles. Here, we make a primary estimation on the air–water CO_2 transfer flux through an algae bloom year for a subtropical man-made lake—Hongfeng Lake, Southwest China. To do this a new type of glass bottles was designed for content and isotopic analysis of DIC and other environmental parameters. At the early stage of algae bloom,CO_2 was transferred from the atmosphere to the lake with a net flux of 1.770 g·C·m^(-2). Later, the partial pressure(pCO_2) of the aqueous CO_2 increased rapidly and the lake outgassed to the atmosphere with a net flux of 95.727 g·C·m^(-2). In the remaining days, the lake again took up CO_2 from the atmosphere with a net flux of 14.804 g·C·m^(-2). As a whole, Lake Hongfeng released 4527 t C to the atmosphere, accounting for one-third of the atmosphere/soil CO_2 sequestered by chemical weathering in the whole drainage. With an empirical mode decomposition method, we found air temperature plays a major role in controlling water temperature, aqueous pCO_2 and hence CO_2 flux. This work indicates a necessity to make detailed and comprehensive carbon budgets in man-made lakes. 展开更多
关键词 CO2 flux Algae bloom Carbon cycle Inland waters lake hongfeng
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7~Be: A Geochemical Tracer for Seasonal Erosion of Surface Soil in Watershed of Lake Hongfeng, Guizhou, China 被引量:10
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作者 BAI ZHANGUO WAN GUOJIANG +3 位作者 WANG CHANGSHENG WAN XI HUANGRONGGUI P.H. SANTSCHIZ and M. BASKARANZ(1 ̄State Key Lab. Of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences,Guiyang 550002 (China))(2 ̄Department Of Marine Scien 《Pedosphere》 SCIE CAS CSCD 1996年第1期23-28,共6页
e penetrative depth in undisturbed surface soil is within 4 mm.7 ̄Be activity shows exponential decrease with soil depth, which is expressed as a diffusion process.7 ̄Be penetrative depth in undisturbed surface soil i... e penetrative depth in undisturbed surface soil is within 4 mm.7 ̄Be activity shows exponential decrease with soil depth, which is expressed as a diffusion process.7 ̄Be penetrative depth in undisturbed surface soil is apparently deeper in the fall (0.22-0.37 g cm ̄(-2) than in the spring (0.11-0.28 g cm ̄(-2) at the same site; Whereas,  ̄7Be apparent activity at the top of surface soil is higher in the spring (0.3-2.2 Bq g ̄(-1_) than in the fall (0.2-0.5 Bq g ̄(-1) at the same site. The  ̄7Be inventory (189-544 Bq m ̄(-2) changes with both locations and seasons. Although the  ̄7Be flux to the earth's surface increases with amount of precipitation, its maximum inventory in the soil profiles decreases to 30%-40% after the rainy period. Calculated by the diffusion equation, the erosion and accumulation rates of soil particles are agreeable with the observation in situ., which shows that the rates in fall are 1.5 times those in spring. The eroded soil particles almost all have been removed on the tablelands rather than transported into the drainage system. This indicstes that the soil erosion process in the karst region is only partial transportation within a short distance. 展开更多
关键词 e erosion trace lake hongfeng watershed surface soil
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Enzymatic and Microbial Degradation of Organic Matter in Lake Hongfeng, Guizhou Province, China 被引量:1
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作者 梁小兵 朱建明 +4 位作者 刘丛强 魏中青 汪福顺 万国江 黄荣贵 《Chinese Journal Of Geochemistry》 EI CAS 2004年第1期81-88,共8页
In this work, enzymatic and microbial degradation of organic matter in Lake Hongfeng, Guizhou Province, is described in terms of variations in DNA, α-glucosidase and sulfate-reduction bacteria (SRB). Organic matter i... In this work, enzymatic and microbial degradation of organic matter in Lake Hongfeng, Guizhou Province, is described in terms of variations in DNA, α-glucosidase and sulfate-reduction bacteria (SRB). Organic matter is degraded by microbes and extracellular enzymes excreted by the former, to a relatively low content below the 11-cm sediment depth. The distribution of DNA indicated that microbes are very active at the 9-cm sediment depth, where organic matter is degraded by microbes intensively. The contents of α-glucosidase are highest in suspend layer ({0.75} μmol·min+{-1}·g+{-1} dry sediments), showing that starch and hepatin in organic matter have been degraded intensively. α-glucosidase activity weakens with sediment depth. At the 11-cm depth where the degradation of organic matter started to slow down, α-glucosidase activity has been reduced to {0.17} μmol·min+{-1}·g+{-1} (dry sediment). Molecular biological research indicated that sulfate reduction bacteria (SRB) are distributed mainly at the upper 7-cm sediments in Lake Hongfeng. Combined with the results of research on the variations of organic matter and SO+{2-}-4, it is indicated that SO+{2-}-4 is unlikely to become an important electron acceptor and sulfate reduction is not limited by the supply of organic matter in Lake Hongfeng. 展开更多
关键词 生化酶 降解 有机物 贵州
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Analysis on the Eutrophication and Algae Blooms of Hongfeng Lake Reservoir in Guizhou 被引量:3
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作者 夏品华 张明时 李存雄 《Meteorological and Environmental Research》 CAS 2010年第12期96-98,103,共4页
[Objective] The research aimed to know the ecological environment pollution characteristics of Hongfeng Lake water area and the evolution rule,which provided the theory basis for improving the water quality condition.... [Objective] The research aimed to know the ecological environment pollution characteristics of Hongfeng Lake water area and the evolution rule,which provided the theory basis for improving the water quality condition.[Method] Based on the investigation and research of indoor and outdoor,the water quality,aquatic ecosystem,pollution characteristic of sediment and occurrence law of algae blooms in Hongfeng Lake were comprehensively analyzed by combining with the relevant literatures.[Result] Hongfeng Lake was in moderate-heavy eutrophication situation,and the water quality was V-bad V class.The sediment accumulated a lot of nutrient salt,which was the important pollution source of eutrophication in Hongfeng Lake Reservoir.The aquatic ecosystem degraded,and it was easy to form the algae blooms.[Conclusion] The pollution treatment of Hongfeng Lake was extremely urgent. 展开更多
关键词 EUTROPHICATION Algae blooms hongfeng lake China
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Relationship between Water Quality and Stream Grade,Landscape Background of Hongfeng Lake Watershed in Guizhou Province 被引量:1
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作者 邹光城 杨实钦 +3 位作者 李阳兵 牛晓宁 李晶晶 周盈 《Journal of Landscape Research》 2009年第10期42-46,共5页
Xiayun Township watershed in the upper reaches of Hongfeng Lake is selected to study the relationship between stream grade and water quality.Turbidity and ammonium nitrogen concentration are obviously related to the s... Xiayun Township watershed in the upper reaches of Hongfeng Lake is selected to study the relationship between stream grade and water quality.Turbidity and ammonium nitrogen concentration are obviously related to the stream grade,generally speaking,are positively correlated,and the water quality is degrading from the upper reaches to the lower reaches.In the future,the influence of different land use types on the water quality should be fully analyzed on the basis of enhancing the water quality monitoring to provide supports for effectively controlling non-point source pollutions and treating the water environment of Hongfeng Lake. 展开更多
关键词 hongfeng lake WATERSHED STREAM GRADE Water quality
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The oxygen isotopic composition of phosphate as an effective tracer for phosphate sources in Hongfeng Lake 被引量:2
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作者 Yongxue Ji Jingan Chen +2 位作者 Runyu Zhang Yong Liu Jingfu Wang 《Acta Geochimica》 EI CAS CSCD 2017年第4期619-625,共7页
In order to characterize the oxygen isotopic composition of internal phosphate and explore the possibility of using these data to identify phosphate sources, we measured oxygen isotopic compositions of phosphate(δ^(1... In order to characterize the oxygen isotopic composition of internal phosphate and explore the possibility of using these data to identify phosphate sources, we measured oxygen isotopic compositions of phosphate(δ^(18)O_p) in sediment pore water in Hongfeng Lake, a typical deep-water lake in a mountainous area. These data, in combination with δ^(18)O_p in surface water samples and water column samples, were successfully used to identify phosphate sources. The δ^(18)O_p value of sediment pore water ranged from 15.2% to 15.8%, with an average value of 15.5%—the δ^(18)O_p value of internal phosphate. The δ^(18)O_p values decreased gradually through the water column from 19.4% in surface water to 16.4% in deeper water, implying that internal phosphate had more negative δ^(18)O_p values than external phosphate. This finding was substantiated by horizontal variations in δ^(18)O_p values, which decreased with increasing distance from inflowing rivers. All collected evidence suggests that external and internal phosphate have distinctly different isotopic signatures and that these signatures have not been considerably altered by biological mediation in Hongfeng Lake. Therefore, δ^(18)O_p can be used to distinguish phosphate sources. A two-endmember mixing model showed that internal phosphate had an average contribution of 40%, highlighting the influence of internal phosphorus loading on aqueous phosphate and eutrophication. This study illustrates the need to reduce the internal phosphorus load from sediment and provides guidance for nutrient management and in-lake restoration treatment in Hongfeng Lake. The data presented here are limited, but serve to highlight the great potential of δ^(18)O_p as an effective tracer for identifying phosphate sources. Systematic investigations of the oxygen isotopic compositions of external phosphate, internal phosphate, and phosphate through the water column, in combination with in-lake P biogeochemical cycle study, would be desirable in further research. 展开更多
关键词 Phosphate source δ18Op EUTROPHICATION hongfeng lake
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Purification of Eutrophic Water by Five Aqua-Cultured Plants in Lake Hongfeng, Guiyang, China 被引量:1
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作者 SUN Rongguo FAN Li 《Wuhan University Journal of Natural Sciences》 CAS CSCD 2019年第1期37-44,共8页
The purification efficiency of eutrophic water by five aqua-cultured plants(Chlorophytum comosum, Salix babylonica, Dracaena sanderiana, Myriophyllum verticillatum, Alternanthera philoxeroides) in Lake Hongfeng, China... The purification efficiency of eutrophic water by five aqua-cultured plants(Chlorophytum comosum, Salix babylonica, Dracaena sanderiana, Myriophyllum verticillatum, Alternanthera philoxeroides) in Lake Hongfeng, China, was investigated. The results indicated that the biomass of Myriophyllum verticillatum and Alternanthera philoxeroides reached the highest level in 87 days after transplant. The removal efficiencies of total nitrate(TN), total phosphorus(TP), chemical oxygen demand(CODCr), and chlorophyll(Chl-a) by the plants ranged from 44% to 96%. The Secchi depth(SD) increased from 0.08-0.1 m to 1.3-3.2 m for the experiments with five cultivars of aqua-cultured plants. Purification efficiency of eutrophic water correlated significantly, in a positive way, with biomass amount and plant productivity. The Carlson's trophic state indexes decreased from 76 to 21 when the cultivar was Myriophyllum verticillatum, suggesting that Myriophyllum verticillatum can be selected as the plant to remediate karst drainage areas of Guizhou Plateau, where the water body underwent eutrophication. The research results provided a good case for lake environmental management and recovery in karst areas of Yunnan-Guizhou Plateau, China. 展开更多
关键词 aqua-cultured PLANTS EUTROPHIC water lake Hong feng remediation Carlson's trophic state index
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Agricultural Non-point Source Pollution in Drinking Water Conservation Area of the Hongfeng Lake in Guiyang City 被引量:1
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作者 YANG Tongquan LIU Hongyan +3 位作者 YU Yanghua CHEN Zhu RAO Cheng JIANG Chang 《Journal of Landscape Research》 2016年第5期100-104,共5页
On the basis of investigating rural population, land types, livestock and poultry breeding scale in drinking water conservation area of the Hongfeng Lake in Guiyang City, as well as the urban domestic pol utant discha... On the basis of investigating rural population, land types, livestock and poultry breeding scale in drinking water conservation area of the Hongfeng Lake in Guiyang City, as well as the urban domestic pol utant discharge coefficient, livestock and poultry excretion coefficient, nitrogen fertilizer and phosphate fertilizer loss rate in the first national pollution source survey, this paper tried to explore current situation of agricultural non-point source pollution, and provide scientific support for the pollution control. The results showed that in the drinking water conservation area of the Hongfeng lake in 2013, contribution rate of pollution sources to the water pollution in the Hongfeng Lake followed the sequence "livestock and poultry breeding > rural life > farmland fertilizer". Among all agricultural non-point source pollutants, livestock and poultry breeding pollutants were major pollution sources, with a contribution rate to CODCr, TP and NH3-N in water above 50%; rural domestic pollutants were also important pollution sources, its contribution rate to CODCr and NH3-N was 43.49% and 46.69%, respectively; contribution rate of farmland fertilizer pollutants to TN and TP was 33.76% and 27.71%, respectively, higher than that of rural domestic pollutants(25.87% and 6.75%). Therefore, the control of non-point source pollution within the drinking water conservation area should be enhanced, so as to control the pollution from the source. 展开更多
关键词 The hongfeng lake Agricultural non-point source pollution Pollutant contribution rate Control measures
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ANNUAL LAMINATIONS IN THE SEDIMENTS OF HONGFENG LAKE, CHINA
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作者 Wu Fengchang Wan Guojiang(State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, the Chinese Academy of Sciences, Guiyang 550002, PRC) 《Chinese Geographical Science》 SCIE CSCD 1996年第4期375-382,共8页
Hongfeng Lake is an eutrophic freshwater atificial reservior.It began to restore water in 1960. Three sediment cores were taken from both about 25m of water in the center of Hongfeng bake in May 1991. The stratigraphy... Hongfeng Lake is an eutrophic freshwater atificial reservior.It began to restore water in 1960. Three sediment cores were taken from both about 25m of water in the center of Hongfeng bake in May 1991. The stratigraphy of the three cores was easily matched .by using prominent marking horizons and characteristic aqnences of laminations. In three layer Samples studied, diatom and other algae taxa appear in repeating apuences. The presence of laminations may reflect either the regular changes of physical-chemical conditions within the lake or the variation in the intensity of erosion and transport of material from the catchment, pat iculaly where instability in the lake-water system has occult as a result of human activities. The larninations were mainly cantal by seasonal variation of envionmental conditions,particularly climate.Unlike t of the previous examples, they have ben fo ̄ at most recent Sediments, in a small freshwater lake in the eastern slOPe of the QinghaiXiZang Plateau, China in a subtropical climate, which is adenly controlled by  ̄theastern and southwestern mon ̄n. It is believed that it's the first reported instanceOf laminated lake sediments from China. 展开更多
关键词 ANNUAL LAMINATIONS hongfeng lake CARBONATE GEOCHEMISTRY
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基于山水林田湖草协同/权衡的生态管控分区研究
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作者 吕思思 李威 +3 位作者 苏维词 赵卫权 罗军华 孙小琼 《灌溉排水学报》 CAS CSCD 2024年第9期88-94,共7页
【目的】厘清山、水、林、田、湖、草之间的协同和权衡关系,优化红枫湖流域的生态管控分区,制定科学的分区管理措施。【方法】以红枫湖流域为研究区,分析各子系统在全域和局部空间的协同/权衡关系,探讨基于山、水、林、田、湖、草协同... 【目的】厘清山、水、林、田、湖、草之间的协同和权衡关系,优化红枫湖流域的生态管控分区,制定科学的分区管理措施。【方法】以红枫湖流域为研究区,分析各子系统在全域和局部空间的协同/权衡关系,探讨基于山、水、林、田、湖、草协同理念的生态管控分区方案。【结果】流域内生产区与生态区的空间分异性明显,林地、草地的主要生态保护功能不同,湖面临高污染风险,除湖子系统调蓄水能力较好的区域外,其他区域农业种植依赖于降水。红枫湖流域可划分为9类生态管控区。【结论】基于协调、权衡关系的分区方法能够保证各类分区生态环境差异的最大化,各分区管理措施差异明显。 展开更多
关键词 协同/权衡 生态分区 SOFM 红枫湖流域
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基于高通量测序的红枫湖入湖口湖岸缓冲带微生物学特征分析
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作者 饶程 刘鸿雁 《环保科技》 2024年第5期6-12,64,共8页
本文选取贵阳市重要饮用水源地——红枫湖为研究对象,在不同生境下的4条主要支流入湖口缓冲带处布点采集土壤样品,采用HiSeq测序对土壤细菌16S rRNA V4区和真菌ITS1区进行测序,并结合土壤环境因子,对微生物群落组成特征与多样性进行分析... 本文选取贵阳市重要饮用水源地——红枫湖为研究对象,在不同生境下的4条主要支流入湖口缓冲带处布点采集土壤样品,采用HiSeq测序对土壤细菌16S rRNA V4区和真菌ITS1区进行测序,并结合土壤环境因子,对微生物群落组成特征与多样性进行分析,以期为恢复红枫湖湖岸缓冲带植被生态提供参考和依据。结果显示,4个缓冲带中共发现细菌种类有53个门、813属;真菌种类有6个门、406属,各缓冲带在门水平上的组成相似,共同的优势细菌门为变形菌门(Proteobacteria)、酸杆菌门(Acidobacteria)、蓝菌门(Cyanbacteria)等,优势真菌门为子囊菌门(Ascomycota)、担子菌门(Basidiomycota)和壶菌门(Chytridiomycota)。在细菌属水平上,麦翁河缓冲带土壤中的硝化与反硝化细菌含量(7.13%)高于其余三个缓冲带。4个入湖口缓冲带中土壤细菌的多样性指数排序为:HL>MX>MW>YC;真菌的多样性指数:YC>MX>HL>MW。相关分析结果显示细菌多样性指数与全氮呈显著正相关(n=12,r=0.567,p<0.05),真菌群落多样性指数与全盐量呈显著正相关(n=12,r=0.622,p<0.05)。因此,不同的植物组成对湖岸缓冲带土壤微生物的组成和多样性产生影响,同时人类垦殖活动也起着不可忽视的作用。 展开更多
关键词 红枫湖 湖岸缓冲带 高通量 微生物多样性
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贵州红枫湖沉积物磷赋存形态及沉积历史 被引量:69
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作者 王雨春 马梅 +2 位作者 万国江 刘丛强 尹澄清 《湖泊科学》 EI CAS CSCD 2004年第1期21-27,共7页
采集了云贵高原深水湖泊红枫湖现代沉积物未受扰动的柱状样品,通过分析不同形态沉积磷在沉积剖面上的分布特征,并结合沉积物样品柱的210Pb、137Cs年代学研究结果,揭示了红枫湖现代沉积过程中不同形态沉积磷的早期成岩改造的时间变化序列... 采集了云贵高原深水湖泊红枫湖现代沉积物未受扰动的柱状样品,通过分析不同形态沉积磷在沉积剖面上的分布特征,并结合沉积物样品柱的210Pb、137Cs年代学研究结果,揭示了红枫湖现代沉积过程中不同形态沉积磷的早期成岩改造的时间变化序列,以及沉积磷外源输入负荷的历史变化.采用Ruttenberg法分析沉积磷的地球化学赋存形态,研究表明,红枫湖沉积物中有机磷和铁结合态磷是沉积磷的主要赋存形态,分别占沉积全磷的60%和28%.沉积磷在垂直剖面上的分布特征显示,红枫湖现代沉积过程中,沉积磷在最终埋藏前可能发生非常剧烈的形态转化和再迁移,尤其是有机磷和铁结合态磷的成岩改造可能是湖泊系统磷循环质量平衡的重要方面.年代学数据同时表明,近年的人为活动导致湖泊系统(包括沉积物)磷负荷的显著增加. 展开更多
关键词 沉积物 赋存形态 早期成岩作用 沉积年代 红枫湖
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贵州红枫湖沉积物磷赋存形态的空间变化特征 被引量:31
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作者 王敬富 陈敬安 +2 位作者 曾艳 杨永琼 杨海全 《湖泊科学》 CAS CSCD 北大核心 2012年第5期789-796,共8页
选取贵州省红枫湖这一典型的亚深水型人工湖泊作为对象,研究了6个代表性湖区沉积物柱芯磷的赋存形态,结合水体温度和溶解氧现场监测结果,探讨了该类型湖泊沉积物内源磷释放风险.研究结果表明,红枫湖沉积物总磷含量普遍较高,表层沉积物... 选取贵州省红枫湖这一典型的亚深水型人工湖泊作为对象,研究了6个代表性湖区沉积物柱芯磷的赋存形态,结合水体温度和溶解氧现场监测结果,探讨了该类型湖泊沉积物内源磷释放风险.研究结果表明,红枫湖沉积物总磷含量普遍较高,表层沉积物总磷含量均值大于1500 mg/kg,明显高于下部沉积物.NaOH-SRP和rest-P是沉积物磷的主要赋存形态.NH4Cl-P和BD-P含量表层最高,随深度增加明显降低,rest-P含量在垂向上变化不大.人为活动是造成沉积物总磷及赋存形态空间分布差异的主要原因,工业废水和网箱养鱼活动等大大增加了沉积物NaOH-SRP含量.红枫湖深水湖区底部水温多在14.5~23.5℃之间,随季节变化底部水温差异明显,溶解氧含量通常不高于1.5 mg/L,整体处于季节性缺氧或厌氧状态.以NaOH-SRP为主的沉积物磷赋存形态和深水缺氧环境大大增加了红枫湖沉积物内源磷释放的风险,在未来的研究中亟待加强对该类型湖泊沉积物内源磷释放机制、控制因素及治理措施的研究. 展开更多
关键词 红枫湖 沉积物 磷形态 温度 溶解氧
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红枫湖季节性热分层消亡期水体的理化特征 被引量:31
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作者 王敬富 陈敬安 +2 位作者 杨永琼 夏品华 杨海全 《环境科学研究》 EI CAS CSCD 北大核心 2012年第8期845-851,共7页
以云贵高原典型的人工河道型水库红枫湖为研究对象,对近2年来4个代表性湖区季节性热分层消亡期水体的理化特征进行了原位监测.结果表明:红枫湖水体季节性热分层历经发生、发展和消亡的周期性演化过程,对湖泊水环境的变化起着重要的控制... 以云贵高原典型的人工河道型水库红枫湖为研究对象,对近2年来4个代表性湖区季节性热分层消亡期水体的理化特征进行了原位监测.结果表明:红枫湖水体季节性热分层历经发生、发展和消亡的周期性演化过程,对湖泊水环境的变化起着重要的控制作用.秋季初期,气温骤降易于引起季节性热分层的突发性消亡,表现为水体垂向混匀.以2010年为例,分层消失使得上层水温由28.6℃降至23.0℃,ρ(DO)(溶解氧浓度)由9.6 mg/L降至4.0 mg/L,pH由8.8降至7.9,电导率由0.32 mS/cm升至0.36 mS/cm,局部湖区出现鱼类死亡现象;短时间内的剧烈垂直混合,致使沉积物营养盐扰动释放,上部水体ρ(TP)增加了约0.01 mg/L,ρ(TN)增加了0.1 mg/L.红枫湖水体垂向混合可对湖泊水环境产生重要影响,其影响的水体深度和环境效应一方面与气温变幅等因素有关,另一方面还受湖泊温跃层位置和底层水体的绝对温度等因素控制,在预测该类突发性水质恶化事件及评估其环境影响时需予以考虑. 展开更多
关键词 红枫湖 季节性热分层 缺氧 营养盐释放
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红枫湖、百花湖沉积物中磷的存在形态研究 被引量:65
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作者 王雨春 万国江 +2 位作者 王仕禄 李社红 黄荣贵 《矿物学报》 CAS CSCD 北大核心 2000年第3期273-278,共6页
湖泊沉积物中磷存在形态 ,是理解湖泊系统中磷的生物地球化学循环的重要方面 ,对研究湖泊富营养化等环境问题具有重要意义。本次工作中 ,采用连续提取化学分析技术 ,对红枫 -百花湖沉积物中磷的存在形态及其剖面变化进行了研究 ,磷的存... 湖泊沉积物中磷存在形态 ,是理解湖泊系统中磷的生物地球化学循环的重要方面 ,对研究湖泊富营养化等环境问题具有重要意义。本次工作中 ,采用连续提取化学分析技术 ,对红枫 -百花湖沉积物中磷的存在形态及其剖面变化进行了研究 ,磷的存在形态包括 :吸附态磷 (LooselysorbedP)、铁结合态磷 (Fe boundP)、钙结合态磷 (Ca boundP)、矿物晶格中结合力强的残留态磷 (Detrial P)和有机态磷 (Organic P)。研究表明 ,两湖沉积物中 ,铁结合态磷 (Fe boundP)所占比例最大。铁氧化物或铁氢氧化物矿物的早期成岩作用 ,是影响沉积物磷地球化学循环的主要方面。 展开更多
关键词 磷形态 湖泊沉积物 百花湖 红枫湖
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云贵高原湖泊颗粒有机物稳定氮同位素的季节和剖面变化特征 被引量:19
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作者 王静 吴丰昌 +4 位作者 黎文 王立英 郭建阳 傅平青 张润宇 《湖泊科学》 EI CAS CSCD 北大核心 2008年第5期571-578,共8页
以贵州省两个高原湖泊(红枫湖和百花湖)为例,利用颗粒态有机物稳定氮同位素比值(δ15NPOM)的季节及水体剖面变化反映揭示了湖泊氮源变换以及内部生物地球化学作用,为研究湖泊系统氮的循环转化提供有用信息.结果发现:红枫湖表层颗粒态有... 以贵州省两个高原湖泊(红枫湖和百花湖)为例,利用颗粒态有机物稳定氮同位素比值(δ15NPOM)的季节及水体剖面变化反映揭示了湖泊氮源变换以及内部生物地球化学作用,为研究湖泊系统氮的循环转化提供有用信息.结果发现:红枫湖表层颗粒态有机物的δ15N变化范围是3.7‰-14.9‰;百花湖表层颗粒态有机物的δ15N变化范围为1.3‰-8.7‰.红枫湖在冬季(2月)和夏末秋初(9月)出现高值;百花湖则在冬季(2月)出现最低值,夏末秋初(9月)出现高值.红枫湖δ15NPOM值的季节性变化规律恰好与无机氮源的δ15N值的变化规律一致,冬季高δ15NPOM值的原因是其枯水期受工业废水中富含15N的无机氮源的影响,而春季低δ15NPOM值的原因则是受内源硝化作用产生的富含14N的无机氮源的影响.百花湖冬季δ15NPOM值低的原因是受生活污水中具有较低δ15N值的有机颗粒的影响.同时,湖泊水体剖面δ15NPOM和C/N比值相结合可以示踪湖泊系统内部特殊的生物地球化学过程. 展开更多
关键词 颗粒态有机物 稳定氮同位素 C/N 百花湖 红枫湖
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氧化还原条件对红枫湖沉积物磷释放影响的微尺度分析 被引量:20
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作者 徐洋 陈敬安 +1 位作者 王敬富 罗婧 《湖泊科学》 EI CAS CSCD 北大核心 2016年第1期68-74,共7页
选取贵州红枫湖为研究对象,在实验室条件下模拟了自然、好氧和厌氧条件下沉积物内源磷的释放过程,联合应用微电极技术和沉积物磷形态分析对沉积物—水界面开展了微尺度观测与研究.结果表明,厌氧条件下红枫湖沉积物总磷含量显著降低,且... 选取贵州红枫湖为研究对象,在实验室条件下模拟了自然、好氧和厌氧条件下沉积物内源磷的释放过程,联合应用微电极技术和沉积物磷形态分析对沉积物—水界面开展了微尺度观测与研究.结果表明,厌氧条件下红枫湖沉积物总磷含量显著降低,且主要是NaOH提取态磷(NaOH-P)和残渣态磷(rest-P)含量降低所致,厌氧条件下沉积物孔隙水中磷酸盐浓度明显升高,而好氧条件下沉积物孔隙水磷酸盐浓度显著降低,反映厌氧条件显著促进了红枫湖沉积物磷释放.厌氧条件下沉积物内部溶解氧浓度下降、硫还原活动增强可能是导致NaOH-P释放的主要原因.O_2浓度的降低加速了沉积物还原作用并产生大量H2S,进而与二价铁离子形成硫化亚铁沉淀,最终导致NaOH-P(Fe-P)释放到孔隙水中.好氧条件向厌氧条件的转换可通过改变沉积物内部pH值分布和微生物活动促使rest-P释放:厌氧条件下,厌氧微生物不仅可以消耗硫酸根产生H_2S,导致pH值降低,还可消耗有机质,将有机磷转变为无机磷.上述研究结果表明,沉积物—水界面氧化还原环境可影响沉积物氧渗透深度、pH值分布、微生物活动、硫循环以及有机质降解过程,进而控制沉积物磷的形态转化与释放.联合应用微电极技术和沉积物磷形态分析对湖泊沉积物—水界面开展微尺度观测研究是揭示沉积物内源磷释放机制与控制因素的有效途径. 展开更多
关键词 氧化还原环境 微电极 微尺度 沉积物内源磷 红枫湖
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贵州红枫湖底泥磷释放的模拟实验研究 被引量:27
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作者 张红 陈敬安 +2 位作者 王敬富 杨海全 计永雪 《地球与环境》 CAS CSCD 2015年第2期243-251,共9页
在实验室条件下,模拟了温度、溶解氧(Dissolved Oxygen,DO)、pH、扰动、微生物等环境因子对红枫湖底泥磷释放的影响。实验结果表明:(1)底泥磷的释放量随温度的升高而增大,5℃时底泥磷的释放通量为0.59mg·m-2·d-1;25℃和3... 在实验室条件下,模拟了温度、溶解氧(Dissolved Oxygen,DO)、pH、扰动、微生物等环境因子对红枫湖底泥磷释放的影响。实验结果表明:(1)底泥磷的释放量随温度的升高而增大,5℃时底泥磷的释放通量为0.59mg·m-2·d-1;25℃和35℃时底泥磷的释放通量分别为1.25和3.68mg·m-2·d-1。(2)厌氧(DO〈2.0mg/L)条件下,底泥磷释放显著,释放通量在1.15~4.57mg·m-2·d-1之间;好氧(DO〉6.0mg/L)条件下,底泥磷的释放通量仅为0.82mg·m-2·d-1。(3)底泥磷的释放与上覆水pH值密切相关,且释放量随上覆水pH值的升高而增大,当pH=5.5和pH=7.5时,底泥磷的释放通量分别为1.15和1.25mg·m-2·d-1;当pH=9.5时,底泥磷的释放通量为4.57mg·m-2·d-1。(4)扰动条件下的底泥磷释放通量(2.62mg·m-2·d-1)明显大于静置条件下的底泥磷释放通量(1.25mg·m-2·d-1)。(5)微生物对底泥磷释放有明显影响,灭菌条件下的底泥磷释放量明显大于有微生物条件下的底泥磷释放量。综上所述,高温、厌氧、高pH值、强烈扰动均可促进红枫湖底泥磷的释放,微生物对底泥磷释放有明显抑制作用。基于红枫湖底泥磷释放模拟实验结果,计算了不同环境条件下红枫湖底泥磷的释放通量,在此基础上估算出红枫湖夏季热分层期间(6~9月)底泥磷释放量约为8.58t,占红枫湖水体总磷负荷(约28t)的30.6%,表明红枫湖底泥内源磷释放对水体磷负荷和富营养化有重要贡献,亟待开展底泥内源污染治理。 展开更多
关键词 红枫湖 底泥磷 释放量 释放通量
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贵州红枫湖沉积物有机质的酶及微生物降解 被引量:10
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作者 梁小兵 朱建明 +4 位作者 刘丛强 魏中青 汪福顺 万国江 黄荣贵 《第四纪研究》 CAS CSCD 北大核心 2003年第5期565-572,共8页
文章通过DNA、α 葡萄糖苷酶和硫酸盐还原菌等的变化 ,研究了贵州红枫湖沉积物中有机质的酶及微生物降解。有机质在微生物及其分泌的胞外酶的作用下被降解 ,在沉积物深度 1 1cm以下被降解到相对较低的含量。DNA的分布表明表层 9cm的沉... 文章通过DNA、α 葡萄糖苷酶和硫酸盐还原菌等的变化 ,研究了贵州红枫湖沉积物中有机质的酶及微生物降解。有机质在微生物及其分泌的胞外酶的作用下被降解 ,在沉积物深度 1 1cm以下被降解到相对较低的含量。DNA的分布表明表层 9cm的沉积物深度内微生物的活动较为强烈 ,是微生物降解有机质的主要位置。α 葡萄糖苷酶在悬浮层含量最高 ,达0 75 μmol/min·g干沉积物 ,提示有机质中的淀粉和糖原等物质在悬浮层降解较为激烈 ,被大量分解 ;随着沉积物深度的增加α 葡萄糖苷酶活性减弱 ,在有机质降解明显开始变缓的 1 1cm沉积物中 ,α 葡萄糖苷酶活性已降低到 0 1 7μmol/min·g干沉积物。分子生物学的研究表明红枫湖沉积物表层 7cm是硫酸盐还原菌的主要分布位置 ,结合有机质和SO2 -4 含量的研究结果 ,提示红枫湖沉积物中SO2 -4 不可能成为有机质氧化的主要电子受体 。 展开更多
关键词 红枫湖 沉积物 有机质 微生物 微生物降解
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贵州红枫湖沉积物生物可利用磷分布特征及其与粒径的关系 被引量:16
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作者 朱元荣 张润宇 +1 位作者 吴丰昌 傅平青 《湖泊科学》 EI CAS CSCD 北大核心 2010年第4期513-520,共8页
应用化学提取法分析了红枫湖主要出入湖河口及湖心沉积物生物可利用磷(BAP)的含量,并探讨了BAP空间分布与总磷(TP)和粒度组成之间的关系.研究结果表明,各形态BAP含量顺序为:藻类可利用磷(AAP)>NaHCO3可提取磷(Olsen-P)>水溶性磷(W... 应用化学提取法分析了红枫湖主要出入湖河口及湖心沉积物生物可利用磷(BAP)的含量,并探讨了BAP空间分布与总磷(TP)和粒度组成之间的关系.研究结果表明,各形态BAP含量顺序为:藻类可利用磷(AAP)>NaHCO3可提取磷(Olsen-P)>水溶性磷(WSP)>易解吸磷(RDP).沉积物柱芯中BAP迅速降低,剖面变化比TP更为明显.各形态BAP与TP显著相关,除RDP与AAP外,其它形态BAP之间也显著相关.Olsen-P是评价红枫湖沉积物磷的生物有效性的最佳指标.红枫湖沉积物颗粒组成以粘土及粉砂为主,湖心沉积物比河口粒度小.表层(0-5cm)沉积物中Olsen-P和AAP的含量与细组分(粘土)的比例呈正相关,而RDP、WSP与细组分呈负相关性,表明沉积物细组分对深水湖泊富营养化的重要性. 展开更多
关键词 沉积物 生物可利用磷 粒径 空间分布 深水湖泊 红枫湖
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