Correction of intense laser–plasma interactions by QED vacuum polarization in collision of laser beams

The influence of vacuum polarization effects on the interactions of multiple ultra-intense lasers with plasmas is discussed. The nonlinear paraxial monochromatic model of the interactions has been improved by considering the Heisenberg–Euler Lagrangian density of two laser processes. Comparing the corrections of vacuum polarization effects in the collision of laser beams with one generated by a single intense laser, we find that the former has a higher order of magnitude correction. The laser collision also produces variations in the propagation direction and polarization direction of the lasers propagating in the plasma. In addition, the strong-field quantum electrodynamic(QED) effects can be enhanced by increasing the laser intensity or frequency difference, or by adjusting the incident angles of the two laser beams.

Backward scattering of laser plasma interactions from hundreds-of-joules broadband laser on thick target

The use of broadband laser technology is a novel approach for inhibiting processes related to laser plasma interactions(LPIs).In this study,several preliminary experiments into broadband-laser-driven LPIs are carried out using a newly established hundreds-of-joules broadband second-harmonic-generation laser facility.Through direct comparison with LPI results for a traditional narrowband laser,the actual LPI-suppression effect of the broadband laser is shown.The broadband laser had a clear suppressive effect on both back-stimulated Raman scattering and back-stimulated Brillouin scattering at laser intensities below 1×10^(15) W cm^(−2).An abnormal hot-electron phenomenon is also investigated,using targets of different thicknesses.

Characterization of bright betatron radiation generated by direct laser acceleration of electrons in plasma of near critical density

Directed x-rays produced in the interaction of sub-picosecond laser pulses of moderate relativistic intensity with plasma of near-critical density are investigated. Synchrotron-like (betatron) radiation occurs in the process of direct laser acceleration (DLA) of electrons in a relativisticlaser channel when the electrons undergo transverse betatron oscillations in self-generated quasi-static electric and magnetic fields. In anexperiment at the PHELIX laser system, high-current directed beams of DLA electrons with a mean energy ten times higher than the ponderomotive potential and maximum energy up to 100 MeV were measured at 10^(19) W/cm^(2)laser intensity. The spectrum of directed x-raysin the range of 5–60 keV was evaluated using two sets of Ross filters placed at 0°and 10°to the laser pulse propagation axis. The differential x-ray absorption method allowed for absolute measurements of the angular-dependent photon fluence. We report 10^(13) photons/sr withenergies >5 keV measured at 0°to the laser axis and a brilliance of 10^(21) photons s^(−1) mm^(−2) mrad−2(0.1%BW)−1. The angular distributionof the emission has an FWHM of 14°–16°. Thanks to the ultra-high photon fluence, point-like radiation source, and ultra-short emissiontime, DLA-based keV backlighters are promising for various applications in high-energy-density research with kilojoule petawatt-class laserfacilities.

Laser-induced plasma formation in water with up to 400 mJ double-pulse LIBS

Double-pulse LIBS is a promising technique for deep-sea applications.LIBS measurements in shallow water with up to 400 mJ each pulse were done to select laser parameters which promote optimized spectral line emission from plasma even at elevated pressures,where line broadening until loss of most of the spectral information can occur.Optical emission spectroscopy,using a Czerny-Turner spectrometer,has been applied to investigate the dependence of the emitted radiation on laser parameters and hydrostatic pressure.It has been found,that higher laser pulse energies,especially with short pulse delay as required in high water pressure,can also have an adverse effect on the measured spectrum.

Intense low-noise terahertz generation by relativistic laser irradiating near-critical-density plasma

Low-noise terahertz(THz)radiation over 100 MV/cm generation by a linearly-polarized relativistic laser pulse interacting with a near-critical-density(NCD)plasma slab is studied by theory and particle-in-cell(PIC)simulations.A theoretical model is established to examine the dipole-like radiation emission.The THz radiation is attributed to the singlecycle low-frequency surface current,which is longitudinally constrained by the quasi-equilibrium established by the laser ponderomotive force and the ponderomotively induced electrostatic force.Through theoretical analysis,the spatiotemporal characteristics,polarization property of the THz radiation,and the relation between the radiation strength with the initial parameters of driving laser and plasma are obtained,which are in good consistence with the PIC simulation results.Furthermore,it is found by PIC simulations that the generation of thermal electrons can be suppressed within the appropriate parameter regime,resulting in a clear THz radiation waveform.The appropriate parameter region is given for generating a low-noise intense THz radiation with peak strength reaching 100 MV/cm,which could find potential applications in nonlinear THz physics.

Divergence angle consideration in energy spread measurement for high-quality relativistic electron beam in laser wakefield acceleration

The thorough exploration of the transverse quality represented by divergence angle has been lacking yet in the energy spread measurement of the relativistic electron beam for laser wakefield acceleration(LWFA). In this work, we fill this gap by numerical simulations based on the experimental data, which indicate that in a C-shape magnet, magnetic field possesses the beam focusing effect, considering that the divergence angle will result in an increase in the full width at half maxima(FWHM) of the electron density distribution in a uniformly isotropic manner, while the length-to-width ratio decreases. This indicates that the energy spread obtained from the electron deflection distance is smaller than the actual value, regardless of the divergence angle. A promising and efficient way to accurately correct the value is presented by considering the divergence angle(for instance, for an electron beam with a length-to-width ratio of 1.12, the energy spread correct from 1.2% to 1.5%), providing a reference for developing the high-quality electron beam source.

High-resolution x-ray monochromatic imaging for laser plasma diagnostics based on toroidal crystal

Monochromatic x-ray imaging is an essential method for plasma diagnostics related to density information.Large-field high-resolution monochromatic imaging of a He-like iron(Fe XXV)Kαcharacteristic line(6.701 keV)for laser plasma diagnostics was achieved using a developed toroidal crystal x-ray imager.A high-index crystal orientation Ge(531)wafer with a Bragg angle of 75.37°and the toroidal substrate were selected to obtain sufficient diffraction efficiency and compensate for astigmatism under oblique incidence.A precise offline assembly method of the toroidal crystal imager based on energy substitution was proposed,and a spatial resolution of 3-7μm was obtained by toroidal crystal imaging of a 600 line-pairs/inch Au grid within an object field of view larger than 1.0 mm.The toroidal crystal x-ray imager has been successfully tested via side-on backlight imaging experiments of the sinusoidal modulation target and a 1000 line-pairs/inch Au grid with a linewidth of 5μm using an online alignment method based on dual positioning balls to indicate the target and backlighter.This paper describes the optical design,adjustment method,and experimental results of a toroidal crystal system in a laboratory and laser facility.

Extremely powerful and frequency-tunable terahertz pulses from a table-top laser–plasma wiggler

The production of broadband,terawatt terahertz(THz) pulses has been demonstrated by irradiating relativistic lasers on solid targets.However,the generation of extremely powerful,narrow-band and frequency-tunable THz pulses remains a challenge.Here,we present a novel approach for such THz pulses,in which a plasma wiggler is elaborated by a table-top laser and a near-critical density plasma.In such a wiggler,the laser-accelerated electrons emit THz radiations with a period closely related to the plasma thickness.The theoretical model and numerical simulations predict that a THz pulse with a laser-THz energy conversion of over 2.0%,an ultra-strong field exceeding 80 GV/m,a divergence angle of approximately 200 and a center frequency tunable from 4.4 to 1.5 THz can be generated from a laser of 430 mJ.Furthermore,we demonstrate that this method can work across a wide range of laser and plasma parameters,offering potential for future applications with extremely powerful THz pulses.

Transmission effects of high energy nanosecond lasers in laser-induced air plasma under different pressures

When a high energy nanosecond(ns)laser induces breakdown in the air,the plasma density generated in the rarefied atmosphere is much smaller than that at normal pressure.It is associated with a relatively lower absorption coefficient and reduces energy loss of the laser beam at low pressure.In this paper,the general transmission characterizations of a Joule level 10 ns 1064 nm focused laser beam are investigated both theoretically and experimentally under different pressures.The evolution of the electron density(n_(e)),the changes in electron temperature(T_(e))and the variation of laser intensity(I)are employed for numerical analyses in the simulation model.For experiments,four optical image transfer systems with focal length(f)of 200 mm are placed in a chamber and employed to focus the laser beam and produce plasmas at the focus.The results suggest that the transmittance increases obviously with the decreasing pressure and the plasma channels on the transmission path can be observed by the self-illumination.The simulation results agree well with the experimental data.The numerical model presents that the maximum n_e at the focus can reach 10^(19)cm^(-3),which is far below the critical density(n_(c)).As a result,the laser beam is not completely shielded by the plasmas.

Efficient ion acceleration driven by a Laguerre–Gaussian laser in near-critical-density plasma

Laser-driven ion accelerators have the advantages of compact size,high density,and short bunch duration over conventional accelerators.Nevertheless,it is still challenging to generate ion beams with quasi-monoenergetic peak and low divergence in experiments with the current ultrahigh intensity laser and thin target technologies.Here we propose a scheme that a Laguerre–Gaussian laser irradiates a near-critical-density(NCD)plasma to generate a quasi-monoenergetic and low-divergence proton beam.The Laguerre–Gaussian laser pulse in an NCD plasma excites a moving longitudinal electrostatic field with a large amplitude,and it maintains the inward bowl-shape for dozens of laser durations.This special distribution of the longitudinal electrostatic field can simultaneously accelerate and converge the protons.Our particle-in-cell(PIC)simulation shows that the efficient proton acceleration can be realized with the Laguerre–Gaussian laser intensity ranging from 3.9×10^(21)W·cm^(-2)–1.6×10^(22)W·cm^(-2)available in the near future,e.g.,a quasi-monoenergetic proton beam with peak energy~115 MeV and divergence angles less than 5°can be generated by a 5.3×10^(21)W·cm^(-2)pulse.This work could provide a reference for the high-quality ion beam generation with PWclass laser systems available recently.

Diagnostics of laser-induced plasma on carbon-based polymer material using atomic and molecular emission spectra

Time-integrated optical emission analysis of laser-induced plasma on Teflon is presented.Plasma was induced under atmospheric pressure air using transversely excited atmospheric CO_(2) laser pulses.Teflon is a C-based polymer that is,among other things,interesting as a substrate for laser-induced breakdown spectroscopy analysis of liquid samples.This study aimed to determine the optimal experimental conditions for obtaining neutral and ionized C spectral lines and C2 and CN molecular band emission suitable for spectrochemical purposes.Evaluation of plasma parameters was done using several spectroscopic techniques.Stark profiles of appropriate C ionic lines were used to determine electron number density.The ratio of the integral intensity of ionic-to-atomic C spectral lines was used to determine the ionization temperature.A spectral emission of C2 Swan and CN violet bands system was used to determine the temperature of the colder,peripheral parts of plasma.We critically analyzed the use of molecular emission bands as a tool for plasma diagnostics and suggested methods for possible improvements.

Time-resolved K-shell x-ray spectra of nanosecond laser-produced titanium tracer in gold plasmas

A study of a nanosecond laser irradiation on the titanium-layer-buried gold planar target is presented. The timeresolved x-ray emission spectra of titanium tracer are measured by a streaked crystal spectrometer. By comparing the simulated spectra obtained by using the FLYCHK code with the measured titanium spectra, the temporal plasma states, i.e.,the electron temperatures and densities, are deduced. To evaluate the feasibility of using the method for the characterization of Au plasma states, the deduced plasma states from the measured titanium spectra are compared with the Multi-1D hydrodynamic simulations of laser-produced Au plasmas. By comparing the measured and simulated results, an overall agreement for the electron temperatures is found, whereas there are deviations in the electron densities. The experiment–theory discrepancy may suggest that the plasma state could not be well reproduced by the Multi-1D hydrodynamic simulation, in which the radial gradient is not taken into account. Further investigations on the spectral characterization and hydrodynamic simulations of the plasma states are needed. All the measured and FLYCHK simulated spectra are given in this paper as datasets. The datasets are openly available at http://www.doi.org/10.57760/sciencedb.j00113.00032.

Influence of the position relationship between gas–liquid interface and laser focus on plasma evolution characteristics in jet LIBS technology

In order to understand the characteristics of breakdown process,plasma evolution and spectral emission in liquid jets laser-induced breakdown spectroscopy methods under the influence of the position variation between laser focus and gas–liquid interface,this work takes the plasma generated by laser-induced liquid jets as the object of study and discusses the changes in the spatial and temporal evolution characteristics and spectral radiation of the plasma when the position parameters between the laser focal point and the gas–liquid interface are different.The initial breakdown position is always between the front interface and the focus when the laser focus moves along the vertical direction of the interface,forming a phenomenon like’interface effect’.The relationship between laser pulse energy and breakdown probability exhibits a law similar to a‘hysteresis curve’in the study of breakdown threshold.In this work,plasma with smaller size,rounder shape,stronger radiation,higher temperature,and higher density can be produced when the focus position is in the liquid column 0.2 mm away from the front interface.Simultaneously,the spectral signal intensity and signal-to-back ratio of the characteristic peaks of target elements in water reach maximum values,and the spectral signal becomes more stable(relative standard deviation value reaches 2%).The Ca element’s ion radiation at 393.366 nm and atomic radiation at 422.673 nm are studied using narrow-band filtering imaging and time-space resolution spectroscopy.The findings demonstrate that the laws of ion and atomic radiation are not perfectly consistent in space and time.

Effect of sharp vacuum-plasma boundary on the electron injection and acceleration in a few-cycle laser driven wakefield

The electron injection and acceleration driven by a few-cycle laser with a sharp vacuum-plasma boundary have been investigated through three-dimensional(3D)particle-in-cell simulations.It is found that an isotropic boundary impact injection(BII)first occurs at the vacuum-plasma boundary,and then carrier-envelope-phase(CEP)shift causes the transverse oscillation of the plasma bubble,resulting in a periodic electron self-injection(SI)in the laser polarization direction.It shows that the electron charge of the BII only accounts for a small part of the total charge,and the CEP can effectively tune the quality of the injected electron beam.The dependences of laser intensity and electron density on the total charge and the ratio of BII charge to the total charge are studied.The results are beneficial to electron acceleration and its applications,such as betatron radiation source.

Plasma density transition-based electron injection in laser wake field acceleration driven by a flying focus laser

By using a high-intensity flying focus laser,the dephasingless[Phys.Rev.Lett.124134802(2020)]or phase-locked[Nat.Photon.14475(2020)]laser wakefield acceleration(LWFA)can be realized,which may overcome issues of laser diffraction,pump depletion,and electron dephasing which are always suffered in usual LWFA.The scheme thus has the potentiality to accelerate electrons to Te V energy in a single acceleration stage.However,the controlled electron injection has not been self-consistently included in such schemes.Only external injection was suggested in previous theoretical studies,which requires other accelerators and is relatively difficulty to operate.Here,we numerically study the actively controlled density transition injection in phase-locked LWFA to get appropriate density profiles for amount of electron injection.The study shows that compared with LWFA driven by lasers with fixed focus,a larger plasma density gradient is necessary.Electrons experience both transverse and longitudinal loss during acceleration due to the superluminal group velocity of the driver and the variation of the wakefield structure.Furthermore,the periodic deformation and fracture of the flying focus laser in the high-density plasma plateau make the final injected charge also depend on the beginning position of the density downramp.Our studies show a possible way for amount of electron injection in LWFA driven by flying focus lasers.

A laser-produced plasma source based on thin-film Gd targets for next-generation extreme ultraviolet lithography

We have studied laser-produced plasma based on mass-limited thin-film Gd targets for beyond the current extreme ultraviolet(EUV)light source of 13.5 nm wavelength based on tin.The influences of the laser intensity on the emission spectra centered around 6.7 nm from thin-film Gd targets were first investigated.It is found that the conversion efficiency of the produced plasma is saturated when the laser intensity goes beyond 2×10^(11)W cm^(-2).We have systematically compared the emission spectra of the laser-produced plasma with the changes in the thicknesses of the thin-film Gd targets.It is proved that a minimum-mass target with a thickness of 400 nm is sufficient to provide the maximum conversion efficiency,which also implies that this thickness is the ablation depth for the targets.These findings should be helpful in the exploration of next-generation EUV sources,as the thin-film Gd targets will reduce the debris during the plasma generation process compared with the bulk targets.

Study of the 6.x nm short wavelength radiation spectra of laser-produced erbium plasmas for BEUV lithography

Beyond extreme ultraviolet(BEUV)radiation with a wavelength of 6.x nm for lithography is responsible for reducing the source wavelength to enable continued miniaturization of semiconductor devices.In this work,the Required BEUV light at 6.x nm wavelength was generated in dense and hot Nd:YAG laser-produced Er plasmas.The spectral contributions from the 4p–4d and 4d–4f transitions of singly,doubly and triply excited states of Er XXIV–Er XXXII in the BEUV band were calculated using Cowan and the Flexible Atomic Code.It was also found that the radiative transitions between multiply excited states dominate the narrow wavelength window around 6.x nm.Under the assumption of collisional radiative equilibrium of the laser-produced Er plasmas,the relative ion abundance in the experiment was inferred.Using the Boltzmann quantum state energy level distribution and Gram–Charlier fitting function of unresolved transition arrays(UTAs),the synthetic spectrum around 6.x nm was finally obtained and compared with the experimental spectrum.The spatio-temporal distributions of electron density and electron temperature were calculated based on radiation hydrodynamic simulation in order to identify the contributions of various ionic states to the UTAs arising from the Er plasmas near 6.x nm.

Laser-assisted ablation and plasma formation of titanium explored by LIBS,QCM, optical microscopy and SEM analyses along with mechanical modifications under different pressures of Ar and Ne

This study deals with the investigation of Nd:YAG laser-assisted ablation and plasma formation of Ti at irradiance of 0.85 GW cm-2 under Ar and Ne environment at various pressures ranging from 10-120 Torr.Laser-induced breakdown spectroscopy is used to evaluate plasma parameters,whereas quartz crystal microbalance is used for ablation yield measurements.The crater depth is evaluated by optical microscopy.The surface features are explored by scanning electron microscope(SEM) analysis and the micro-hardness is measured by a Vickers hardness tester.It is observed that the plasma parameters are higher in Ar than in Ne,and are strongly correlated with the ablation yield,ablation depth,surface features and hardness of laser-ablated Ti.These parameters increase with increasing the pressure of environmental gases,attain their maxima at 40 Torr for Ar and at 60 Torr for Ne.Afterwards,they show a decreasing trend up till a maximum pressure of 120 Torr.The maximum value of the electron temperature(Te) is5480 K,number density(ne) is 1.46 × 1018 cm-3,ablation depth is 184 μm,ablation yield is3.9 × 1015 atoms/pulse and hardness is 300 HV in the case of Ar atmosphere.SEM analysis reveals the growth of surface features,such as cones,ridges and pores,whose appearance is more distinct in Ar than Ne and is attributed to temperature,pressure and density gradients along with recoil pressure of the Ti plasma.

Supersonic gas jet stabilization in laser–plasma acceleration

Supersonic gas jets generated via a conical nozzle are widely applied in the laser wakefield acceleration of electrons.The stability of the gas jet is critical to the electron injection and the reproducibility of the wakefield acceleration.Here we discussed the role of the stilling chamber in a modified converging-diverging nozzle to dissipate the turbulence and to stabilize the gas jets.By the fluid dynamics simulations and the Mach-Zehnder interferometer measurements,the instability originating from the nonlinear turbulence is studied and the mechanism to suppress the instability is proposed.Both the numerical and experimental results prove that the carefully designed nozzle with a stilling chamber is able to reduce the perturbation by more than 10% compared with a simple-conical nozzle.

Extreme ultraviolet spectral characteristic analysis of highly charged ions in laserproduced Cu plasmas

This paper reports the results of spectral measurements and a theoretical analysis of the temporal and spatial evolution of laser-produced Cu plasma in vacuum in the range of 8–14 nm.The time dependence of the extreme ultraviolet band spectrum at different positions near the target surface was obtained and found to be dominated by three broad-band features.The 3p and 3d excitations of Cu5+–Cu9+ions were calculated using the Hartree–Fock theory with configuration interactions.The characteristics of the spectral line distribution for the 3p–nd and 3d–nf transition arrays were analyzed.Based on the steady-state collisional radiation model and the normalized Boltzmann distribution,the complex spectral structure in the band of 13–14 nm is accurately explained through consistency comparisons and benchmarking between the experimental and theoretical simulation spectra,demonstrating that the structure mainly stems from the overlapping contribution of the 3d–4f and 3p–3d transition arrays for the Cu5+–Cu9+ions.These results may help in studying the radiation characteristics of isoelectronic series highly-charged ions involving the 3d excitation process.