In the present paper, latent track formation in yttrium iron garnet (YIG) produced by high energy Ar ions is briefly reported at first. Then, in the framework of thermal spike model, a phenomenological parameter descr...In the present paper, latent track formation in yttrium iron garnet (YIG) produced by high energy Ar ions is briefly reported at first. Then, in the framework of thermal spike model, a phenomenological parameter describing the effective energy transfer from excited electrons to lattice atoms, effective energy deposition Qeff, is deduced. Qeff is a function of ion velocity, electronic energy loss (Se) and mean free path λ of excited electrons in the matter, and is a time moderate term initialized by Waligorski’s function of spatial energy deposition of secondary electrons ejected by incident ions. Size of ion latent track is proportional to Qeff value. From Qeff obtained by use of realistic λ values, the sizes of latent tracks in SiO2, YIG, Ti and Zr produced by given swift heavy ion irradiations are deduced and com- pared with experimental results. It is found that, from the fits to experimental results, the best λ values for SiO2, YIG, Ti and Zr are (6±1), (8±2), (6.1±1.0) and (9.6±1.0) nm, respectively. Moreover, the relationship between experimental damage and Qeff is discussed.展开更多
The primary motivation for studying how irradiation modifies the structures and properties of solid materials involves the understanding of undesirable phenomena,including irradiation-induced degradation of components...The primary motivation for studying how irradiation modifies the structures and properties of solid materials involves the understanding of undesirable phenomena,including irradiation-induced degradation of components in nuclear reactors and space exploration,and beneficial applications,including material performance tailoring through ion beam modification and defect engineering.In this work,the formation mechanism of latent tracks with different damage morphologies in LiNbO_(3)crystals under 0.09-6.17 Me V/u ion irradiation with an electronic energy loss from 2.6-13.2 ke V/nm is analyzed by experimental characterizations and numerical calculations.Irradiation-induced damage is preliminarily evaluated via the prism coupling technique to analyze the correlation between the dark-mode spectra and energy loss profiles of irradiated regions.Under the irradiation conditions of different ion velocities and electronic energy losses,different damage morphologies,from individual spherical defects to discontinuous and continuous tracks,are experimentally characterized.During ion penetration process,the ion velocity determines the spatiotemporal distribution of deposited irradiation energy induced by electronic energy loss,meaning that the two essential factors including electronic energy loss and ion velocity coaffect the track damage.The inelastic thermal spike model is used to numerically calculate the spatiotemporal evolutions of energy deposition and the corresponding atomic temperature under different irradiation conditions,and a quantitative relationship is proposed by comparison with corresponding experimentally observed track damage morphologies.The obtained quantitative relationship between irradiation conditions and track damage provides deep insight and guidance for understanding the damage behavior of crystal materials in extreme radiation environments and selecting irradiation parameters,including ion species and energies,for ion beam technique application in atomic-level defect manipulation,material modification,and micro/nanofabrication.展开更多
A comparative analysis is performed on the structural damage response and associated mechanisms in lanthanum aluminate and yttrium aluminate crystals under various irradiation conditions by a combination of experiment...A comparative analysis is performed on the structural damage response and associated mechanisms in lanthanum aluminate and yttrium aluminate crystals under various irradiation conditions by a combination of experimental and theoretical approaches.Under low-energy Au~+irradiation,the damage accumulation curve shows a higher damage rate for LaAlO_(3)crystals than YAlO_(3)crystals.The relatively low irradiation tolerance of LaAlO_(3)to the action of nuclear collisions is ascribed to the large amorphization cross-section and effective cross-section for defect-stimulated amorphization.Under swift Ar^(12+),Ni^(19+)and Kr^(17+)irradiation with different ion energies and velocities,the formed highly-disordered/amorphous latent tracks with different morphologies in pristine and predamaged crystals are discussed,and the corresponding electronic energy loss and lattice temperature thresholds are quantitatively determined.Compared to YAlO_(3),LaAlO_(3)exhibits lower sensitivity and higher damage tolerance to the electronic energy loss process,attributing to its relatively high recrystallization efficiency during the rapid quenching process.Furthermore,the introduction of lattice defects into LaAlO_(3)and YAlO_(3)crystals considerably enhances the sensitivity and intensity of thermal spike response to the electronic energy loss,and the induced effective modification of track morphologies demonstrates the synergistic effect between the electronic energy loss and pre-existing defects created by nuclear collisions.In this case,even under the action of electronic energy loss below the threshold,the lattice temperature in the nuclear-collision damaged crystalline system could still meet the criterion for track production.The irradiation energy deposited to atoms and induced lattice temperature evolution discussed in this work provide a deeper insight into the complex processes involved in irradiation-induced latent track behaviors.展开更多
基金Supported by NSFC (Projects 10125522 10175084 10475102) and the Chinese Academy of Sciences.
文摘In the present paper, latent track formation in yttrium iron garnet (YIG) produced by high energy Ar ions is briefly reported at first. Then, in the framework of thermal spike model, a phenomenological parameter describing the effective energy transfer from excited electrons to lattice atoms, effective energy deposition Qeff, is deduced. Qeff is a function of ion velocity, electronic energy loss (Se) and mean free path λ of excited electrons in the matter, and is a time moderate term initialized by Waligorski’s function of spatial energy deposition of secondary electrons ejected by incident ions. Size of ion latent track is proportional to Qeff value. From Qeff obtained by use of realistic λ values, the sizes of latent tracks in SiO2, YIG, Ti and Zr produced by given swift heavy ion irradiations are deduced and com- pared with experimental results. It is found that, from the fits to experimental results, the best λ values for SiO2, YIG, Ti and Zr are (6±1), (8±2), (6.1±1.0) and (9.6±1.0) nm, respectively. Moreover, the relationship between experimental damage and Qeff is discussed.
基金supported by the National Natural Science Foundation of China(No.11875038)the National Laboratory of Heavy Ion Accelerator in Lanzhou,and the State Key Laboratory of Nuclear Physics and Technology,Peking University+2 种基金financial support from the Young Scholars Program of Shandong Universityfinancial support from the Youth Innovation Promotion Association CAS(No.2019262)supported by the U.S.Department of Energy,Office of Science,Basic Energy Sciences,Materials Sciences and Engineering Division。
文摘The primary motivation for studying how irradiation modifies the structures and properties of solid materials involves the understanding of undesirable phenomena,including irradiation-induced degradation of components in nuclear reactors and space exploration,and beneficial applications,including material performance tailoring through ion beam modification and defect engineering.In this work,the formation mechanism of latent tracks with different damage morphologies in LiNbO_(3)crystals under 0.09-6.17 Me V/u ion irradiation with an electronic energy loss from 2.6-13.2 ke V/nm is analyzed by experimental characterizations and numerical calculations.Irradiation-induced damage is preliminarily evaluated via the prism coupling technique to analyze the correlation between the dark-mode spectra and energy loss profiles of irradiated regions.Under the irradiation conditions of different ion velocities and electronic energy losses,different damage morphologies,from individual spherical defects to discontinuous and continuous tracks,are experimentally characterized.During ion penetration process,the ion velocity determines the spatiotemporal distribution of deposited irradiation energy induced by electronic energy loss,meaning that the two essential factors including electronic energy loss and ion velocity coaffect the track damage.The inelastic thermal spike model is used to numerically calculate the spatiotemporal evolutions of energy deposition and the corresponding atomic temperature under different irradiation conditions,and a quantitative relationship is proposed by comparison with corresponding experimentally observed track damage morphologies.The obtained quantitative relationship between irradiation conditions and track damage provides deep insight and guidance for understanding the damage behavior of crystal materials in extreme radiation environments and selecting irradiation parameters,including ion species and energies,for ion beam technique application in atomic-level defect manipulation,material modification,and micro/nanofabrication.
基金supported by the National Natural Science Foundation of China(Grant No.11875038 and 11775135)the National Laboratory of Heavy Ion Accelerator in Lanzhou+4 种基金the State Key Laboratory of Nuclear Physics and Technology,Peking Universityfinancial support from the Young Scholars Program of Shandong Universityfinancial support from the Youth Innovation Promotion Association CAS(Grant No.2019262)supported by the U.S.Department of Energy,Office of Science,Basic Energy Sciences,Materials Sciences and Engineering Divisionsupport from the University of Tennessee Governor’s Chair program。
文摘A comparative analysis is performed on the structural damage response and associated mechanisms in lanthanum aluminate and yttrium aluminate crystals under various irradiation conditions by a combination of experimental and theoretical approaches.Under low-energy Au~+irradiation,the damage accumulation curve shows a higher damage rate for LaAlO_(3)crystals than YAlO_(3)crystals.The relatively low irradiation tolerance of LaAlO_(3)to the action of nuclear collisions is ascribed to the large amorphization cross-section and effective cross-section for defect-stimulated amorphization.Under swift Ar^(12+),Ni^(19+)and Kr^(17+)irradiation with different ion energies and velocities,the formed highly-disordered/amorphous latent tracks with different morphologies in pristine and predamaged crystals are discussed,and the corresponding electronic energy loss and lattice temperature thresholds are quantitatively determined.Compared to YAlO_(3),LaAlO_(3)exhibits lower sensitivity and higher damage tolerance to the electronic energy loss process,attributing to its relatively high recrystallization efficiency during the rapid quenching process.Furthermore,the introduction of lattice defects into LaAlO_(3)and YAlO_(3)crystals considerably enhances the sensitivity and intensity of thermal spike response to the electronic energy loss,and the induced effective modification of track morphologies demonstrates the synergistic effect between the electronic energy loss and pre-existing defects created by nuclear collisions.In this case,even under the action of electronic energy loss below the threshold,the lattice temperature in the nuclear-collision damaged crystalline system could still meet the criterion for track production.The irradiation energy deposited to atoms and induced lattice temperature evolution discussed in this work provide a deeper insight into the complex processes involved in irradiation-induced latent track behaviors.