Phase matching or quasi-phase matching(QPM)is of significant importance to the conversion efficiency of second harmonic generation(SHG)in artificial nonlinear crystals like lithium niobate(LN)crystal or microstructure...Phase matching or quasi-phase matching(QPM)is of significant importance to the conversion efficiency of second harmonic generation(SHG)in artificial nonlinear crystals like lithium niobate(LN)crystal or microstructured nonlinear crystals like periodic-poled lithium niobate(PPLN)crystals.In this paper,we propose and show that the incident angle of pump laser light can be harnessed as an alternative versatile tool to engineer QPM for high-efficiency SHG in a PPLN crystal,in addition to conventional means of period adjusting or temperature tuning.A rigorous model is established and analytical solution of the nonlinear conversion efficiency under the small and large signal approximation theory is obtained at different incident angles.The variation of phase mismatching and walk-off length with incident angle or incident wavelength are also explored.Numerical simulations for a PPLN crystal with first order QPM structure are used to confirm our theoretical predictions based on the exact analytical solution of the general large-signal theory.The results show that the narrow-band tunable SHG output covers a range of 532 nm–552.8 nm at the ideal incident angle from 0°to 90°.This theoretical scheme,fully considering the reflection and transmission at the air-crystal interface,would offer an efficient theoretical system to evaluate the nonlinear frequency conversion and help to obtain the maximum SHG conversion efficiency by selecting an optimum incident wavelength and incident angle in a specially designed PPLN crystal,which would be very helpful for the design of tunable narrow-band pulse nanosecond,picosecond,and femtosecond laser devices via PPLN and other microstructured LN crystals.展开更多
Combining a Ti-diffusion periodically poled lithium niobate(PPLN)waveguide with a Sagnac interferometer,two opposite directions type-II spontaneous parametric down conversions(SPDC)occur coherently and yield a high br...Combining a Ti-diffusion periodically poled lithium niobate(PPLN)waveguide with a Sagnac interferometer,two opposite directions type-II spontaneous parametric down conversions(SPDC)occur coherently and yield a high brightness,high stability polarization entanglement source.The source produces degenerate photon pairs at 1540.4 nm with a brightness of B=(1.36±0.03)×10^(6) pairs/(s·nm·m W).We perform quantum state tomography to reconstruct the density matrix of the output state and obtain a fidelity of F=0.983±0.001.The high brightness and phase stability of our waveguide source enable a wide range of quantum information experiments operating at a low pump power as well as hold the advantage in mass production which can promote the practical applications of quantum technologies.展开更多
Generation of hyperentangled photon pairs is investigated based on the lithium niobate straight waveguide.We propose to use the nonlinear optical process of spontaneous parametric down-conversion(SPDC)and a well-desig...Generation of hyperentangled photon pairs is investigated based on the lithium niobate straight waveguide.We propose to use the nonlinear optical process of spontaneous parametric down-conversion(SPDC)and a well-designed lithium niobate waveguide structure to generate a hyperentangled(in the polarization dimension and the energy-time dimension)two-photon state.By performing numerical simulations of the waveguide structure and calculating the possible polarization states,joint spectral amplitudes(JSA),and joint temporal amplitudes(JTA)of the generated photon pair,we show that the generated photon pair is indeed hyperentangled in both the polarization dimension and the energy-time dimension.展开更多
In this contribution,we simulate,design,and experimentally demonstrate an integrated optical isolator based on spatiotemporal modulation in the thin-film lithium niobate on an insulator waveguide platform.We used two ...In this contribution,we simulate,design,and experimentally demonstrate an integrated optical isolator based on spatiotemporal modulation in the thin-film lithium niobate on an insulator waveguide platform.We used two cascaded travelling wave phase modulators for spatiotemporal modulation and a racetrack resonator as a wavelength filter to suppress the sidebands of the reverse propagating light.This enabled us to achieve an isolation of 27 dB.The demonstrated suppression of the reverse propagating light makes such isolators suitable for the integration with III-V laser diodes and Erbium doped gain sections in the thin-film lithium niobate on the insulator waveguide platform.展开更多
This paper reports a continuous-wave (CW) mid-infrared intracavity singly resonant optical parametric oscillator based on periodically poled lithium niobate (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. C...This paper reports a continuous-wave (CW) mid-infrared intracavity singly resonant optical parametric oscillator based on periodically poled lithium niobate (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. Considering the thermal lens effects, it adopted an optical ballast lens and the near-concentric cavity for better operation. At the PPLN's grating period of 28.5 μm and the temperature of 140℃, the maximum idler output power of 155 mW at 3.86 μm has been achieved when the 808 nm pump power is 8.5 W, leading to an optical-to-optical conversion efficiency of 1.82%.展开更多
In this paper we report on a continuous-wave (CW) intracavity singly resonant optical parametric oscillator (ICSRO) based on periodically poled LiNbO3 (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. Consi...In this paper we report on a continuous-wave (CW) intracavity singly resonant optical parametric oscillator (ICSRO) based on periodically poled LiNbO3 (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. Considering the thermal lens effects and diffraction loss, an optical ballast lens and a near-concentric cavity are adopted for better operation. Through varying the grating period and the temperature, the tunable signal output from 1406 nm to 1513 nm is obtained. At a PPLN grating period of 29 pm and a temperature of 413 K, a maximum signal output power of 820 mW at 1500 nm is achieved when the 808 nm pump power is 10.9 W, leading to an optical-to-optical conversion efficiency of 7.51%.展开更多
Tunable coherent emission is generated in a single-pass, cascaded wavelength conversion process from mode-locked laser-pumped monolithic periodically poled lithium niobate(PPLN). Three ranges of wavelength, includin...Tunable coherent emission is generated in a single-pass, cascaded wavelength conversion process from mode-locked laser-pumped monolithic periodically poled lithium niobate(PPLN). Three ranges of wavelength, including visible output from 628 nm to 639 nm, near-infrared output from 797 nm to 816 nm, and mid-infrared output from 3167 nm to 3459 nm,were obtained from the monolithic PPLN, which consists of a 10-mm section for 532-nm-pumped optical parametric generation(OPG) and a 7-mm section for 1064-nm-pumped sum frequency generation(SFG). A pump-to-signal conversion efficiency of 23.4% for OPG at 50°C and a quantum efficiency of 26.2% for SFG at 200°C were obtained.展开更多
Lithium niobate on insulator(LNOI)is rising as one of the most promising platforms for integrated photonics due to the high-index-contrast and excellent material properties of lithium niobate,such as wideband transpar...Lithium niobate on insulator(LNOI)is rising as one of the most promising platforms for integrated photonics due to the high-index-contrast and excellent material properties of lithium niobate,such as wideband transparency from visible to mid-infrared,large electro-optic,piezoelectric,and second-order harmonic coefficients.The fast-developing micro-and nanostructuring techniques on LNOI have enabled various structure,devices,systems,and applications.In this contribution,we review the latest developments in this platform,including ultra-high speed electro-optic modulators,optical frequency combs,opto-electro-mechanical system on chip,second-harmonic generation in periodically poled LN waveguides,and efficient edge coupling for LNOI.展开更多
The holographic storage properties of Fe (0.03% (mass fraction) Fe2O3):LiNbO3 doped with Sc at different levels (0, 1%, 2%, 3%) were investigated. The Sc threshold concentration in Fe:LiNbO3 was implied to be ...The holographic storage properties of Fe (0.03% (mass fraction) Fe2O3):LiNbO3 doped with Sc at different levels (0, 1%, 2%, 3%) were investigated. The Sc threshold concentration in Fe:LiNbO3 was implied to be about 3% (mole fraction) because O-H vibration absorption peak of Sc (3%):Fe:LiNbO3 was at 3508 cm^-1, compared with 3484 cm^-1 of crystals with lower Sc doping level. Sc(3%):Fe:LiNbO3 exhibited higher optical damage resistance ability. The threshold intensity (wavelength 488 nm) of Sc (3%):Fe:LiNbO3 was 2.2 ×10^2 W ·cm^-2, two orders of masnitude higher than that of Fe:LiNbO3. Holographic storage properties of the crystals were determined in an extraordinary polarized laser of wavelength 632.8 nm by a two-wave coupling method. It was found that in terms of holographic storage properties, the optimal doping concentration of Sc was 2% (mole fraction) among this crystal series.展开更多
This paper investigates the photorefractive properties of iron doped lithium niobate with different [Li]/[Nb] ratios The experimental results show two photorefractive centres for iron doped near-stoichiometric lithium...This paper investigates the photorefractive properties of iron doped lithium niobate with different [Li]/[Nb] ratios The experimental results show two photorefractive centres for iron doped near-stoichiometric lithium niobate crystal Besides Fe^2+ and Fe^3+ ions, small polarons and bipolarons are considered as another photoactive centre.展开更多
We report on the fabrication of the lO-mm-long lithium niobate ridge waveguide and its supercontinuum gen- eration at near-visible wavelengths (around 800hm). The waveguides are fabricated by a combination of MeV co...We report on the fabrication of the lO-mm-long lithium niobate ridge waveguide and its supercontinuum gen- eration at near-visible wavelengths (around 800hm). The waveguides are fabricated by a combination of MeV copper ion implantation followed by wet etching in a proton exchanged lithium niobate planar waveguide. Using a mode-locked Ti:sapphire laser with a central wavelength of 800nm, the generated broadest supereontinuum through the ridge waveguides spans 302 nm (at -30 dB points), from 693 to 995 nm. Temporal coherence proper- ties of the supercontinuum are experimentally studied by a Michelson interferometer and the coherence length of the broadest supercontinuum is measured to be 5.2 μm. Our results offer potential for a compact and integrated supercontinuum source for applications including bio-imaging, spectroscopy and optical communication.展开更多
We study the effect of waveguide thickness variations on the frequency spectrum of spontaneous parametric downconversion in the periodically-poled lithium niobate on insulator(LNOI)waveguide.We analyze several variati...We study the effect of waveguide thickness variations on the frequency spectrum of spontaneous parametric downconversion in the periodically-poled lithium niobate on insulator(LNOI)waveguide.We analyze several variation models and our simulation results show that thickness variations in several nanometers can induce distinct effects on the central peak of the spectrum,such as narrowing,broadening,and splitting.We also prove that the effects of positive and negative variations can be canceled and thus lead to a variation-robust feature and an ultra-broad bandwidth.Our study may promote the development of on-chip photon sources in the LNOI platform,as well as opens up a way to engineer photon frequency state.展开更多
Multi-lane integrated transmitter chips are key components in future compact optical modules to realize high-speed optical interconnects.Thin-film lithium niobate(TFLN)photonics have emerged as a promising platform fo...Multi-lane integrated transmitter chips are key components in future compact optical modules to realize high-speed optical interconnects.Thin-film lithium niobate(TFLN)photonics have emerged as a promising platform for achieving high-performance chip-scale optical systems.Combining a coarse wavelength-division multiplexing(CWDM)devices using fabrication-tolerant angled multimode interferometer structure and high-performance electro-optical modulators,we demonstrate monolithic on-chip four-channel CWDM transmitter on the TFLN platform for the first time.The four-channel CWDM transmitter enables high-speed transmissions of 100 Gb/s data rate per wavelength channel(i.e.,an aggregated date rate of 400 Gb/s).展开更多
The molecular dynamic simulation of lithium niobate thin films deposited on silicon substrate is carried out by using the dissipative particle dynamics method. The simulation results show that the Si (111) surface i...The molecular dynamic simulation of lithium niobate thin films deposited on silicon substrate is carried out by using the dissipative particle dynamics method. The simulation results show that the Si (111) surface is more suitable for the growth of smooth LiNbO3 thin films compared to the Si(100) surface, and the optimal deposition temperature is around 873 K, which is consistent with the atomic force microscope results. In addition, the calculation molecular number is increased to take the electron spins and other molecular details into account.展开更多
We report the formation of two waveguide layers in a lithium niobate crystal by irradiation with swift heavy Kr ions with high (GeV) energies and ultralow fluences. The micro-Raman spectra are measured at different ...We report the formation of two waveguide layers in a lithium niobate crystal by irradiation with swift heavy Kr ions with high (GeV) energies and ultralow fluences. The micro-Raman spectra are measured at different depths in the irradiated layer and show that the high electronic energy loss can cause lattice damage along the ion trajectory, while the nuclear energy loss causes damage at the end of the ion track. Two waveguide layers are formed by confinement with two barriers associated with decreases in the refractive index that are caused by electronic and nuclear energy losses, respectively.展开更多
The temperature dependency of a 5-mo1% MgO-doped periodically poled lithium niobate waveguide was investi- gated in this paper. We started with the temperature-dependent refractive index equation for the waveguide. Se...The temperature dependency of a 5-mo1% MgO-doped periodically poled lithium niobate waveguide was investi- gated in this paper. We started with the temperature-dependent refractive index equation for the waveguide. Secondly, the temperature dependency of the second harmonic generation effect was experimentally researched under different temperatures and pump powers. The quasi-phase matched wavelengths, efficiency bandwidths and peak efficiencies of the waveguide were measured. The experimental results agreed with theoretical simulations, which are indispensable in the following all-optical sampling studies based on the cascaded second harmonic generation/difference-frequency generation process in the current device.展开更多
The relationship between temperature and oxygen vacancy concentration is deduced in this paper. Based on the data of thermal weight-loss experiment, the formation enthalpies of congruent and several doped LN crystals ...The relationship between temperature and oxygen vacancy concentration is deduced in this paper. Based on the data of thermal weight-loss experiment, the formation enthalpies of congruent and several doped LN crystals have been calculated. It was found that the formation enthalpy of oxygen vacancies can be decreased evidently by doping valence-changeable ions. The experimental results were discussed and a new reduction process of the photorefractive LN crystal at a relatively low temperature was proposed, and the reduced crystals showed a good effect in practical use.展开更多
Recently,Mach–Zehnder modulators based on thin-film lithium niobate have attracted broad interest for their potential for high modulation bandwidth,low insertion loss,high extinction ratio,and high modulation efficie...Recently,Mach–Zehnder modulators based on thin-film lithium niobate have attracted broad interest for their potential for high modulation bandwidth,low insertion loss,high extinction ratio,and high modulation efficiency.The periodic capacitively loaded traveling-wave electrode is optimally adopted for ultimate high-performances in this type of modulator.However,such an electrode structure on a silicon substrate still suffers from the velocity mismatch and substrate leakage loss for microwave signals.Here,we introduce a thin-film lithium niobate modulator structure using this periodic capacitively loaded electrode on a silicon substrate.Backside holes in the silicon substrate are prepared to solve robustly the above difficulties.The fabricated device exhibits an insertion loss of 0.9 dB,a halfwave-voltage–length product of 2.18 V·cm,and an ultra-wide bandwidth well exceeding 67 GHz for a 10-mm-long device.Data transmissions with rates up to 112 Gb/s are demonstrated.The proposed structure and fabrication strategy are compatible for other types of monolithic and heterogeneous integrated thin-film lithium niobate modulators on a silicon substrate.展开更多
Whispering-gallery-mode(WGM)microresonators can greatly enhance light-matter interaction,making them indispensable units for frequency conversion in nonlinear optics.Efficient nonlinear wave mixing in microresonators ...Whispering-gallery-mode(WGM)microresonators can greatly enhance light-matter interaction,making them indispensable units for frequency conversion in nonlinear optics.Efficient nonlinear wave mixing in microresonators requires stringent simultaneous optical resonance and phase-matching conditions.Thus,it is challenging to achieve efficient frequency conversion over a broad bandwidth.Here,we demonstrate broadband second-harmonic generation(SHG)in the x-cut thinfilm lithium niobate(TFLN)microdisk with a quality factor above 107by applying the cyclic quasi-phase-matching(CQPM)mechanism,which is intrinsically applicable for broadband operation.Broadband SHG of continuous-wave laser with a maximum normalized conversion efficiency of~15%/m W is achieved with a bandwidth spanning over 100 nm in the telecommunication band.Furthermore,broadband SHG of femtosecond lasers,supercontinuum lasers,and amplified spontaneous emission in the telecommunication band is also experimentally observed.The work is beneficial for integrated nonlinear photonics devices like frequency converters and optical frequency comb generator based on second-order nonlinearity on the TFLN platform.展开更多
We demonstrate single-mode microdisk lasers in the telecom band with ultralow thresholds on erbium-ytterbium co-doped thin-film lithium niobate(TFLN).The active microdisk was fabricated with high-Q factors by photolit...We demonstrate single-mode microdisk lasers in the telecom band with ultralow thresholds on erbium-ytterbium co-doped thin-film lithium niobate(TFLN).The active microdisk was fabricated with high-Q factors by photolithography-assisted chemomechanical etching.Thanks to the erbium-ytterbium co-doping providing high optical gain,the ultralow loss nanostructuring,and the excitation of high-Q coherent polygon modes,which suppresses multimode lasing and allows high spatial mode overlap between pump and lasing modes,single-mode laser emission operating at 1530 nm wavelength was observed with an ultralow threshold,under a 980-nm-band optical pump.The threshold was measured as low as 1μW,which is one order of magnitude smaller than the best results previously reported in single-mode active TFLN microlasers.The conversion efficiency reaches 4.06×10^(-3),which is also the highest value reported in single-mode active TFLN microlasers.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.11974119)the Science and Technology Project of Guangdong Province,China(Grant No.2020B010190001)+2 种基金the Guangdong Innovative and Entrepreneurial Research Team Program(Grant No.2016ZT06C594)the National Key Research and Development Program of China(Grant Nos.2018YFA,0306200,and 2019YFB2203500)the Science and Technology Program of Guangzhou City(Grant No.2023A04J1309).
文摘Phase matching or quasi-phase matching(QPM)is of significant importance to the conversion efficiency of second harmonic generation(SHG)in artificial nonlinear crystals like lithium niobate(LN)crystal or microstructured nonlinear crystals like periodic-poled lithium niobate(PPLN)crystals.In this paper,we propose and show that the incident angle of pump laser light can be harnessed as an alternative versatile tool to engineer QPM for high-efficiency SHG in a PPLN crystal,in addition to conventional means of period adjusting or temperature tuning.A rigorous model is established and analytical solution of the nonlinear conversion efficiency under the small and large signal approximation theory is obtained at different incident angles.The variation of phase mismatching and walk-off length with incident angle or incident wavelength are also explored.Numerical simulations for a PPLN crystal with first order QPM structure are used to confirm our theoretical predictions based on the exact analytical solution of the general large-signal theory.The results show that the narrow-band tunable SHG output covers a range of 532 nm–552.8 nm at the ideal incident angle from 0°to 90°.This theoretical scheme,fully considering the reflection and transmission at the air-crystal interface,would offer an efficient theoretical system to evaluate the nonlinear frequency conversion and help to obtain the maximum SHG conversion efficiency by selecting an optimum incident wavelength and incident angle in a specially designed PPLN crystal,which would be very helpful for the design of tunable narrow-band pulse nanosecond,picosecond,and femtosecond laser devices via PPLN and other microstructured LN crystals.
基金Project supported by the National Key R&D Program of China(Grant Nos.2022YFF0712800 and 2019YFA0308700)。
文摘Combining a Ti-diffusion periodically poled lithium niobate(PPLN)waveguide with a Sagnac interferometer,two opposite directions type-II spontaneous parametric down conversions(SPDC)occur coherently and yield a high brightness,high stability polarization entanglement source.The source produces degenerate photon pairs at 1540.4 nm with a brightness of B=(1.36±0.03)×10^(6) pairs/(s·nm·m W).We perform quantum state tomography to reconstruct the density matrix of the output state and obtain a fidelity of F=0.983±0.001.The high brightness and phase stability of our waveguide source enable a wide range of quantum information experiments operating at a low pump power as well as hold the advantage in mass production which can promote the practical applications of quantum technologies.
基金the Key-Area Research and Development Program of Guangdong Province of China(Grant No.2018B030325002)the National Natural Science Foundation of China(Grant No.62075129)+1 种基金the Open Project Program of SJTU-Pinghu Institute of Intelligent Optoelectronics(Grant No.2022SPIOE204)the Science and Technology on Metrology and Calibration Laboratory(Grant No.JLJK2022001B002)。
文摘Generation of hyperentangled photon pairs is investigated based on the lithium niobate straight waveguide.We propose to use the nonlinear optical process of spontaneous parametric down-conversion(SPDC)and a well-designed lithium niobate waveguide structure to generate a hyperentangled(in the polarization dimension and the energy-time dimension)two-photon state.By performing numerical simulations of the waveguide structure and calculating the possible polarization states,joint spectral amplitudes(JSA),and joint temporal amplitudes(JTA)of the generated photon pair,we show that the generated photon pair is indeed hyperentangled in both the polarization dimension and the energy-time dimension.
基金This work was supported by the Australian Research Council(ARC)grants DP190102773,DP190101576,DP220100488.
文摘In this contribution,we simulate,design,and experimentally demonstrate an integrated optical isolator based on spatiotemporal modulation in the thin-film lithium niobate on an insulator waveguide platform.We used two cascaded travelling wave phase modulators for spatiotemporal modulation and a racetrack resonator as a wavelength filter to suppress the sidebands of the reverse propagating light.This enabled us to achieve an isolation of 27 dB.The demonstrated suppression of the reverse propagating light makes such isolators suitable for the integration with III-V laser diodes and Erbium doped gain sections in the thin-film lithium niobate on the insulator waveguide platform.
基金Project supported in part by the National Natural Science Foundation of China (Grant Nos 10474071, 60637010, 60671036 and60278001)Tianjin Applied Fundamental Research Project, China (07JCZDJC05900)
文摘This paper reports a continuous-wave (CW) mid-infrared intracavity singly resonant optical parametric oscillator based on periodically poled lithium niobate (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. Considering the thermal lens effects, it adopted an optical ballast lens and the near-concentric cavity for better operation. At the PPLN's grating period of 28.5 μm and the temperature of 140℃, the maximum idler output power of 155 mW at 3.86 μm has been achieved when the 808 nm pump power is 8.5 W, leading to an optical-to-optical conversion efficiency of 1.82%.
基金Project supported partly by the National Natural Science Foundation of China (Grant Nos 60637010 and 60671036)the National Basic Research Program of China (Grant No 2007CB310403)the Tianjin Applied Fundamental Research Project, China(Grant No 07JCZDJC05900)
文摘In this paper we report on a continuous-wave (CW) intracavity singly resonant optical parametric oscillator (ICSRO) based on periodically poled LiNbO3 (PPLN) pumped by a diode-end-pumped CW Nd:YVO4 laser. Considering the thermal lens effects and diffraction loss, an optical ballast lens and a near-concentric cavity are adopted for better operation. Through varying the grating period and the temperature, the tunable signal output from 1406 nm to 1513 nm is obtained. At a PPLN grating period of 29 pm and a temperature of 413 K, a maximum signal output power of 820 mW at 1500 nm is achieved when the 808 nm pump power is 10.9 W, leading to an optical-to-optical conversion efficiency of 7.51%.
基金Project supported by the National Basic Research Program of China(Grant No.2013CB632704)
文摘Tunable coherent emission is generated in a single-pass, cascaded wavelength conversion process from mode-locked laser-pumped monolithic periodically poled lithium niobate(PPLN). Three ranges of wavelength, including visible output from 628 nm to 639 nm, near-infrared output from 797 nm to 816 nm, and mid-infrared output from 3167 nm to 3459 nm,were obtained from the monolithic PPLN, which consists of a 10-mm section for 532-nm-pumped optical parametric generation(OPG) and a 7-mm section for 1064-nm-pumped sum frequency generation(SFG). A pump-to-signal conversion efficiency of 23.4% for OPG at 50°C and a quantum efficiency of 26.2% for SFG at 200°C were obtained.
基金the National Key Research and Development Program of China(2019YFB2203800)the National Natural Science Foundation of China under Grant No.61835008,61905079,and 61905084.
文摘Lithium niobate on insulator(LNOI)is rising as one of the most promising platforms for integrated photonics due to the high-index-contrast and excellent material properties of lithium niobate,such as wideband transparency from visible to mid-infrared,large electro-optic,piezoelectric,and second-order harmonic coefficients.The fast-developing micro-and nanostructuring techniques on LNOI have enabled various structure,devices,systems,and applications.In this contribution,we review the latest developments in this platform,including ultra-high speed electro-optic modulators,optical frequency combs,opto-electro-mechanical system on chip,second-harmonic generation in periodically poled LN waveguides,and efficient edge coupling for LNOI.
基金Project supported by Natural Science Foundation of Heilongjiang Province (E200512)
文摘The holographic storage properties of Fe (0.03% (mass fraction) Fe2O3):LiNbO3 doped with Sc at different levels (0, 1%, 2%, 3%) were investigated. The Sc threshold concentration in Fe:LiNbO3 was implied to be about 3% (mole fraction) because O-H vibration absorption peak of Sc (3%):Fe:LiNbO3 was at 3508 cm^-1, compared with 3484 cm^-1 of crystals with lower Sc doping level. Sc(3%):Fe:LiNbO3 exhibited higher optical damage resistance ability. The threshold intensity (wavelength 488 nm) of Sc (3%):Fe:LiNbO3 was 2.2 ×10^2 W ·cm^-2, two orders of masnitude higher than that of Fe:LiNbO3. Holographic storage properties of the crystals were determined in an extraordinary polarized laser of wavelength 632.8 nm by a two-wave coupling method. It was found that in terms of holographic storage properties, the optimal doping concentration of Sc was 2% (mole fraction) among this crystal series.
基金Project supported by the research funding via Program for Changjiang Scholars of ChinaInnovative Research Team in University,China+1 种基金the National Natural Science Foundation of China(Grant No60578019)Program for Changjiang Scholars and Innovative Research Team in University
文摘This paper investigates the photorefractive properties of iron doped lithium niobate with different [Li]/[Nb] ratios The experimental results show two photorefractive centres for iron doped near-stoichiometric lithium niobate crystal Besides Fe^2+ and Fe^3+ ions, small polarons and bipolarons are considered as another photoactive centre.
基金Supported by the National Natural Science Foundation of China under Grant Nos 61575129 and 11375105the Postdoctoral Science Foundation of China under Grant No 2016M602511+1 种基金the Shenzhen Science and Technology Planning under Grant No JCYJ20160422142912923the State Key Laboratory of Nuclear Physics and Technology,Peking University
文摘We report on the fabrication of the lO-mm-long lithium niobate ridge waveguide and its supercontinuum gen- eration at near-visible wavelengths (around 800hm). The waveguides are fabricated by a combination of MeV copper ion implantation followed by wet etching in a proton exchanged lithium niobate planar waveguide. Using a mode-locked Ti:sapphire laser with a central wavelength of 800nm, the generated broadest supereontinuum through the ridge waveguides spans 302 nm (at -30 dB points), from 693 to 995 nm. Temporal coherence proper- ties of the supercontinuum are experimentally studied by a Michelson interferometer and the coherence length of the broadest supercontinuum is measured to be 5.2 μm. Our results offer potential for a compact and integrated supercontinuum source for applications including bio-imaging, spectroscopy and optical communication.
基金Project supported by the National Key R&D Program of China(Grant No.2019YFA0705000)Leading-edge Technology Program of Jiangsu Natural Science Foundation,China(Grant No.BK20192001)the National Natural Science Foundation of China(Grant Nos.51890861,11690031,11974178,and 11627810).
文摘We study the effect of waveguide thickness variations on the frequency spectrum of spontaneous parametric downconversion in the periodically-poled lithium niobate on insulator(LNOI)waveguide.We analyze several variation models and our simulation results show that thickness variations in several nanometers can induce distinct effects on the central peak of the spectrum,such as narrowing,broadening,and splitting.We also prove that the effects of positive and negative variations can be canceled and thus lead to a variation-robust feature and an ultra-broad bandwidth.Our study may promote the development of on-chip photon sources in the LNOI platform,as well as opens up a way to engineer photon frequency state.
基金This work is supported partially by the National Major Research and Development Program(2019YFB1803902)National Natural Science Foundation of China(NSFC)(62135012,62105107)+3 种基金Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang(2021R01001)Guangdong Basic and Applied Basic Research Foundation(2021A 1515012215,2021B1515120057)Science and Technology Planning Project of Guangdong Province(2019A050510039)Fundamental Research Funds for the Central Universities(2021QNA5001).
文摘Multi-lane integrated transmitter chips are key components in future compact optical modules to realize high-speed optical interconnects.Thin-film lithium niobate(TFLN)photonics have emerged as a promising platform for achieving high-performance chip-scale optical systems.Combining a coarse wavelength-division multiplexing(CWDM)devices using fabrication-tolerant angled multimode interferometer structure and high-performance electro-optical modulators,we demonstrate monolithic on-chip four-channel CWDM transmitter on the TFLN platform for the first time.The four-channel CWDM transmitter enables high-speed transmissions of 100 Gb/s data rate per wavelength channel(i.e.,an aggregated date rate of 400 Gb/s).
基金supported by the National Basic Research Program of China(Grant No.2011CB922003)the International S&T Cooperation Program of China(Grant No.2013DFG52660)+1 种基金the Taishan Scholar Construction Project Special Fund,Chinathe Fundamental Research Funds for the Central Universities,China(Grant Nos.65030091 and 65010961)
文摘The molecular dynamic simulation of lithium niobate thin films deposited on silicon substrate is carried out by using the dissipative particle dynamics method. The simulation results show that the Si (111) surface is more suitable for the growth of smooth LiNbO3 thin films compared to the Si(100) surface, and the optimal deposition temperature is around 873 K, which is consistent with the atomic force microscope results. In addition, the calculation molecular number is increased to take the electron spins and other molecular details into account.
基金supported by the National Natural Science Foundation of China(Grant Nos.11275117,U1432120,and 11274188)the Heavy Ion Research Facility in Lanzhou(HIRFL),China
文摘We report the formation of two waveguide layers in a lithium niobate crystal by irradiation with swift heavy Kr ions with high (GeV) energies and ultralow fluences. The micro-Raman spectra are measured at different depths in the irradiated layer and show that the high electronic energy loss can cause lattice damage along the ion trajectory, while the nuclear energy loss causes damage at the end of the ion track. Two waveguide layers are formed by confinement with two barriers associated with decreases in the refractive index that are caused by electronic and nuclear energy losses, respectively.
基金supported by the National Natural Science Foundation of China (Grant Nos. 60777024 and 60978007)
文摘The temperature dependency of a 5-mo1% MgO-doped periodically poled lithium niobate waveguide was investi- gated in this paper. We started with the temperature-dependent refractive index equation for the waveguide. Secondly, the temperature dependency of the second harmonic generation effect was experimentally researched under different temperatures and pump powers. The quasi-phase matched wavelengths, efficiency bandwidths and peak efficiencies of the waveguide were measured. The experimental results agreed with theoretical simulations, which are indispensable in the following all-optical sampling studies based on the cascaded second harmonic generation/difference-frequency generation process in the current device.
文摘The relationship between temperature and oxygen vacancy concentration is deduced in this paper. Based on the data of thermal weight-loss experiment, the formation enthalpies of congruent and several doped LN crystals have been calculated. It was found that the formation enthalpy of oxygen vacancies can be decreased evidently by doping valence-changeable ions. The experimental results were discussed and a new reduction process of the photorefractive LN crystal at a relatively low temperature was proposed, and the reduced crystals showed a good effect in practical use.
基金This work was partially supported by the National Natural Science Foundation of China(NSFC)(Nos.62135012,62105107,and 61961146003)Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang(No.2021R01001)。
文摘Recently,Mach–Zehnder modulators based on thin-film lithium niobate have attracted broad interest for their potential for high modulation bandwidth,low insertion loss,high extinction ratio,and high modulation efficiency.The periodic capacitively loaded traveling-wave electrode is optimally adopted for ultimate high-performances in this type of modulator.However,such an electrode structure on a silicon substrate still suffers from the velocity mismatch and substrate leakage loss for microwave signals.Here,we introduce a thin-film lithium niobate modulator structure using this periodic capacitively loaded electrode on a silicon substrate.Backside holes in the silicon substrate are prepared to solve robustly the above difficulties.The fabricated device exhibits an insertion loss of 0.9 dB,a halfwave-voltage–length product of 2.18 V·cm,and an ultra-wide bandwidth well exceeding 67 GHz for a 10-mm-long device.Data transmissions with rates up to 112 Gb/s are demonstrated.The proposed structure and fabrication strategy are compatible for other types of monolithic and heterogeneous integrated thin-film lithium niobate modulators on a silicon substrate.
基金supported by the National Natural Science Foundation of China(Nos.12074252,12192252,and 62022058)the National Key Research and Development Program of China(No.2022YFA1205101)+1 种基金the Shanghai Municipal Science and Technology Major Project(No.2019SHZDZX01-ZX06)and the Yangyang Development Fund。
文摘Whispering-gallery-mode(WGM)microresonators can greatly enhance light-matter interaction,making them indispensable units for frequency conversion in nonlinear optics.Efficient nonlinear wave mixing in microresonators requires stringent simultaneous optical resonance and phase-matching conditions.Thus,it is challenging to achieve efficient frequency conversion over a broad bandwidth.Here,we demonstrate broadband second-harmonic generation(SHG)in the x-cut thinfilm lithium niobate(TFLN)microdisk with a quality factor above 107by applying the cyclic quasi-phase-matching(CQPM)mechanism,which is intrinsically applicable for broadband operation.Broadband SHG of continuous-wave laser with a maximum normalized conversion efficiency of~15%/m W is achieved with a bandwidth spanning over 100 nm in the telecommunication band.Furthermore,broadband SHG of femtosecond lasers,supercontinuum lasers,and amplified spontaneous emission in the telecommunication band is also experimentally observed.The work is beneficial for integrated nonlinear photonics devices like frequency converters and optical frequency comb generator based on second-order nonlinearity on the TFLN platform.
基金supported by the National Key R&D Program of China(Nos.2019YFA0705000,2022YFA1404600,and 2022YFA1205100)the National Natural Science Foundation of China(NSFC)(Nos.62122079,12192251,62235019,12334014,12134001,12104159,and 11933005)+4 种基金the Innovation Program for Quantum Science and Technology(No.2021ZD0301403)the Shanghai Municipal Science and Technology Major Project(No.2019SHZDZX01)the Science and Technology Commission of Shanghai Municipality(Nos.21DZ1101500 and 23ZR1481800)the Youth Innovation Promotion Association of Chinese Academy of Sciences(No.2020249)the Engineering Research Center for Nanophotonics&Advanced Instrument,Ministry of Education,East China Normal University(No.2023nmc005)。
文摘We demonstrate single-mode microdisk lasers in the telecom band with ultralow thresholds on erbium-ytterbium co-doped thin-film lithium niobate(TFLN).The active microdisk was fabricated with high-Q factors by photolithography-assisted chemomechanical etching.Thanks to the erbium-ytterbium co-doping providing high optical gain,the ultralow loss nanostructuring,and the excitation of high-Q coherent polygon modes,which suppresses multimode lasing and allows high spatial mode overlap between pump and lasing modes,single-mode laser emission operating at 1530 nm wavelength was observed with an ultralow threshold,under a 980-nm-band optical pump.The threshold was measured as low as 1μW,which is one order of magnitude smaller than the best results previously reported in single-mode active TFLN microlasers.The conversion efficiency reaches 4.06×10^(-3),which is also the highest value reported in single-mode active TFLN microlasers.