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Realizing External Quantum Efficiency over 25% with Low Efficiency Roll-Off in Polymer-Based Light-Emitting Diodes Synergistically Utilizing Intramolecular Sensitization and Bipolar Thermally Activated Delayed Fluorescence Monomer 被引量:1
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作者 Yuchao Liu Yanchao Xie +4 位作者 Lei Hua Xingwen Tong Shian Ying Zhongjie Ren Shouke Yan 《CCS Chemistry》 CSCD 2023年第4期1005-1017,共13页
Since polymer-based light-emitting diodes(PLEDs)arewellsuited building blocks for large-area and low-cost flexible display equipment,state-of-the-art thermally activated delayed fluorescence(TADF)PLEDs are in high dem... Since polymer-based light-emitting diodes(PLEDs)arewellsuited building blocks for large-area and low-cost flexible display equipment,state-of-the-art thermally activated delayed fluorescence(TADF)PLEDs are in high demand.To respond to this demand,light-emitting TADF units have initially been modified with electron-transporting units to balance the carrier transport of regiorandom TADF polymers,and simultaneously,an intramolecular sensitizing strategy has also been employed by covalently incorporating TADF sensitizers with light-emitting TADF units and hosts in conjugated polymers to accelerate the spin-flip of triplet excitons.Superior photophysical properties have been achieved by a rational regulation of the proportions of each component,achieving a photoluminescence quantumyield of 90%,an extremely high rate of reverse intersystem crossing of 3×106 s−1,and a relatively low nonradiative decay rate of around 105 s−1.As a result,the solutionprocessed PLEDs can attain an external quantum efficiency(EQE)value of 25.4%with emission peaks of around 550 nm,representing record-high performance for PLEDs.The efficiency roll-off can also be significantly suppressed,maintaining an EQE value of 24.2%at 1000 cd/m2 with ideal efficiency roll-off of lower than 5%.Encouragingly,this work provides a valid strategy to tackle the imperative need for PLEDs with high EQE and low efficiency roll-off. 展开更多
关键词 thermally activated delayed fluorescence polymer light-emitting diodes intramolecular sensitizing strategy balanced carrier transports low efficiency roll-off
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Efficient deep blue OLEDs with extremely low efficiency roll-off at high brightness based on phenanthroimidazole derivatives
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作者 Xiang Chen Jue-Wen Zhao +5 位作者 Xu-Hui Zheng Jie-Ji Zhu Guo-Xi Yang Shan-Shun Tang Qing-Xiao Tong Si-Lu Tao 《Chinese Chemical Letters》 SCIE CAS CSCD 2019年第11期1989-1993,共5页
Phosphorescent and thermally activated delayed fluorescence(TADF)emitters can break through the spin statistics rules and achieve great success in external quantum efficiency(over 5%).However,maintaining high efficien... Phosphorescent and thermally activated delayed fluorescence(TADF)emitters can break through the spin statistics rules and achieve great success in external quantum efficiency(over 5%).However,maintaining high efficiency at high brightness is a tremendous challenge for applications of organic light emitting diodes.Hence,we reported two phenanthroimidazole derivatives PPI-An-CN and PPI-An-TP and achieved extremely low efficiency roll-off with about 99%of the maximum external quantum efficiency(EQEmax)maintained even at a high luminance of 1000 cd/cm2 based non-doped devices.When doping the two materials in CBP(4,4'-bis(N-carbazolyl)-1,1'-biphenyl),the doped devices still exhibited excellent stability at high brightness with CIEy≈0.07 and low turn-on voltage of only 2.8 V.The state-ofthe-art low efficiency roll-off makes the new materials attractive for potential applications.It is the first time that the Fragment Contribution Analysis method has been used to analyze the excited state properties of the molecules in the field of OLEDs,which helps us understand the mechanism more intuitively and deeply. 展开更多
关键词 OLED Deep blue Phenanthroimidazole low efficiency roll-off Fragment contribution analysis
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Lattice reconstruction for mixed-halide blue perovskite light-emitting diodes with high brightness,outstanding color stability and low efficiency roll-off
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作者 Jionghua Wu Renjie Wang +4 位作者 Rui Zhang Giuseppe Portale Eduardo Solano Xiaoke Liu Feng Gao 《Science China Materials》 SCIE EI CAS 2024年第11期3553-3560,共8页
We report a simple,effective,and universal lattice reconstruction approach to improve the quality of perovskite films by using nonpolar solvents with high Gutmann donor numbers(DNs).We find that high-DN nonpolar solve... We report a simple,effective,and universal lattice reconstruction approach to improve the quality of perovskite films by using nonpolar solvents with high Gutmann donor numbers(DNs).We find that high-DN nonpolar solvents,for instance,ethyl acetate,can interact with perovskite precursors.Such a solvent can make the perovskite lattice more ordered and“harder”and promote the formation of heterostructures with low-dimensional perovskite impurities and residual solvent molecules.As a result,the latticereconstructed perovskite films exhibit reduced defect densities and suppressed ion migration.The resultant mixed-halide blue perovskite light-emitting diodes(PeLEDs)show greatly enhanced tolerance to high driving current densities and voltages,demonstrating high brightness,outstanding color stability and low efficiency roll-off.Our work provides a deep understanding of the interactions between nonpolar solvents and perovskites and offers useful guidelines for further development of high-power PeLEDs. 展开更多
关键词 color stability mixed halide perovskite low efficiency roll-off high brightness ion migration
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A Solution for Scalable Routing in Depth Divisions-Based DUSNs via Adding a Scalable Parameter to Control Depth Clusters: Creating an Energy Efficient and Low Delay NI-Independent Communication Protocol 被引量:3
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作者 Mohammad Reza Khosravi Reza Salari Habib Rostami 《Journal of Computer and Communications》 2016年第7期55-61,共7页
Due to effectiveness of network layer on general performance of networks, designing routing protocols is very important for lifetime and traffic efficiency in wireless sensor networks. So in this paper, we are going t... Due to effectiveness of network layer on general performance of networks, designing routing protocols is very important for lifetime and traffic efficiency in wireless sensor networks. So in this paper, we are going to represent an efficient and scalable version of depth-based routing (DBR) protocol that is limited by depth divisions-policy. In fact the new version is a network information independent routing protocol for acoustic communications. Proposed method by use of depth clustering is able to reduce consumed energy and end-to-end delay in dense underwater sensor networks (DUSNs) and this issue is proved by simulation. 展开更多
关键词 Network Information (NI) Depth-Based Routing (DBR) Dense Underwater Sensor Networks (DUSNs) Energy Efficient and low Delay-DBR (EELD-DBR)
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High voltage generator circuit with low power and high efficiency applied in EEPROM 被引量:1
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作者 刘彦 张世林 赵毅强 《Journal of Semiconductors》 EI CAS CSCD 2012年第6期79-83,共5页
This paper presents a low power and high efficiency high voltage generator circuit embedded in electrically erasable programmable read-only memory(EEPROM).The low power is minimized by a capacitance divider circuit ... This paper presents a low power and high efficiency high voltage generator circuit embedded in electrically erasable programmable read-only memory(EEPROM).The low power is minimized by a capacitance divider circuit and a regulator circuit using the controlling clock switch technique.The high efficiency is dependent on the zero threshold voltage(V_(th)) MOSFET and the charge transfer switch(CTS) charge pump.The proposed high voltage generator circuit has been implemented in a 0.35μm EEPROM CMOS process.Measured results show that the proposed high voltage generator circuit has a low power consumption of about 150.48μW and a higher pumping efficiency(83.3%) than previously reported circuits.This high voltage generator circuit can also be widely used in low-power flash devices due to its high efficiency and low power dissipation. 展开更多
关键词 CTS charge pump high efficiency high voltage generator circuit low power EEPROM oscillation zero V_(th)
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More Discussion on High Efficiency & Low Cost Clean Steel Production Platform
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作者 YIN Rui-yu (Central Iron and Steel Research Institute, Beijing, 100081) 《Journal of Iron and Steel Research International》 SCIE EI CAS CSCD 2011年第S2期1-8,共8页
The construction of high efficiency, low cost clean steel platform is one of the common key technologies concerning efficiency, quality and cost. It is basic and universal and not only applicable in the R&D and pr... The construction of high efficiency, low cost clean steel platform is one of the common key technologies concerning efficiency, quality and cost. It is basic and universal and not only applicable in the R&D and production of "high-end" products, but also in the production of bulk ordinary steel products. The platform of high efficiency, low cost clean steel is the important direction of modern steel technology progress and has great significance on the competitiveness of each steel plant. The research of high efficiency, low cost platform not only involves the production and management of the steel plant, but also the academic research field (process engineering and dynamic operation) and theories and methods innovation of engineering design (theory and method of dynamic-precision design). The integrated theory and method of high efficiency and low cost clean steel platform is the binding point of metallurgical process engineering and material engineering. Different types of high efficiency, low cost clean steel platform should combine with the corresponding rolling process and iron making process so that high efficiency, low cost clean steel manufacturing system would come into being. 展开更多
关键词 more discussion high efficiency & low cost clean steel platform integration technology
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Dynamic Power Dissipation Control Method for Real-Time Processors Based on Hardware Multithreading
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作者 罗新强 齐悦 +1 位作者 王磊 王沁 《China Communications》 SCIE CSCD 2013年第5期156-166,共11页
In order to eliminate the energy waste caused by the traditional static hardware multithreaded processor used in real-time embedded system working in the low workload situation, the energy efficiency of the hardware m... In order to eliminate the energy waste caused by the traditional static hardware multithreaded processor used in real-time embedded system working in the low workload situation, the energy efficiency of the hardware multithread is discussed and a novel dynamic multithreaded architecture is proposed. The proposed architecture saves the energy wasted by removing idle threads without manipulation on the original architecture, fulfills a seamless switching mechanism which protects active threads and avoids pipeline stall during power mode switching. The report of an implemented dynamic multithreaded processor with 45 nm process from synthesis tool indicates that the area of dynamic multithreaded architecture is only 2.27% higher than the static one in achieving dynamic power dissipation, and consumes 1.3% more power in the same peak performance. 展开更多
关键词 dynamic power dissipation control real-time processor hardware multithread low power design energy efficiency
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Novel thioxanthone host material with thermally activated delayed fluorescence for reduced efficiency roll-off of phosphorescent OLEDs 被引量:1
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作者 Hui Wang Xiaopeng Lv +3 位作者 Lingqiang Meng Xiaofang Wei Ying Wang Pengfei Wang 《Chinese Chemical Letters》 SCIE CAS CSCD 2018年第3期471-474,共4页
2,7-Di(9,9-dimethyl-9H-fluoren-l-yl)-9H-thioxanthen-9-one (DMBFTX) with thermally activated delayed fluorescence (TADF) was well designed and synthesized. The phosphorescent organic lightemitting device (PHOLED... 2,7-Di(9,9-dimethyl-9H-fluoren-l-yl)-9H-thioxanthen-9-one (DMBFTX) with thermally activated delayed fluorescence (TADF) was well designed and synthesized. The phosphorescent organic lightemitting device (PHOLED) based on this novel TADF host material displays a stable red phosphorescence region, a peak external quantum efficiency (EQE) value of 12.9% and a low EQE roll-off of 38.8%at a luminance of 10000 cd/m2, which is benefited from the reverse intersystem crossing (RISC) of TADF host and less populated triplet exitons. Notably, the red device based on the TADF host DMBFrX exhibits superior electroluminescence performance and reduced efficiency roll-offcompared with the one hosted by commercially available host 1,3-bis(9-carbazolyl)benzene (mCP), illustrating the high potential of employing the TADF host material with small energy gap to reduce efficiency roll-off in PHOLED. 展开更多
关键词 low efficiency roll-off Thermally activated delayed fluorescence Small energy gap Reverse intersystem crossing Phosphorescent OLEDs
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Scaling trends in energy recovery logic:an analytical approach
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作者 Jitendra Kanungo S.Dasgupta 《Journal of Semiconductors》 EI CAS CSCD 2013年第8期79-83,共5页
This paper presents an analytical model to study the scaling trends in energy recovery logic.The energy performance of conventional CMOS and energy recovery logic are compared with scaling the design and technology pa... This paper presents an analytical model to study the scaling trends in energy recovery logic.The energy performance of conventional CMOS and energy recovery logic are compared with scaling the design and technology parameters such as supply voltage,device threshold voltage and gate oxide thickness.The proposed analytical model is validated with simulation results at 90 nm and 65 nm CMOS technology nodes and predicts the scaling behavior accurately that help us to design an energy-efficient CMOS digital circuit design at the nanoscale.This research work shows the adiabatic switching as an ultra-low-power circuit technique for sub-100 nm digital CMOS circuit applications. 展开更多
关键词 adiabatic logic energy efficient energy recovery logic low power digital CMOS logic
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