Solid sorbents adsorption is considered as one of the potential options for CO2 capture process. CO2 adsorption on MCM-68 (Si/AI ratio 22) sorbent material was investigated. MCM-68 was synthesized using N,N,N',N'-...Solid sorbents adsorption is considered as one of the potential options for CO2 capture process. CO2 adsorption on MCM-68 (Si/AI ratio 22) sorbent material was investigated. MCM-68 was synthesized using N,N,N',N'-tetraethylbicyclo [2.2.2] oct-7-ene-2,3:5,6-dipyrrolidinium diiodide (TEBOP^2+(I^+)2) as a structure-directing agent (SDA). CO2 adsorption capacity on MCM-68 sorbent was measured at a broad temperature window i.e. 60 ℃, 300 ℃ and at 400 ℃. The presence of ordered mesoporous structure, high surface area (456 me/g) and high thermal stability (TGA analysis up to 900℃) in MCM-68 are thought to be to be advantageous for the CO2 adsorption in broad temperature window.展开更多
文摘Solid sorbents adsorption is considered as one of the potential options for CO2 capture process. CO2 adsorption on MCM-68 (Si/AI ratio 22) sorbent material was investigated. MCM-68 was synthesized using N,N,N',N'-tetraethylbicyclo [2.2.2] oct-7-ene-2,3:5,6-dipyrrolidinium diiodide (TEBOP^2+(I^+)2) as a structure-directing agent (SDA). CO2 adsorption capacity on MCM-68 sorbent was measured at a broad temperature window i.e. 60 ℃, 300 ℃ and at 400 ℃. The presence of ordered mesoporous structure, high surface area (456 me/g) and high thermal stability (TGA analysis up to 900℃) in MCM-68 are thought to be to be advantageous for the CO2 adsorption in broad temperature window.