The study of temporal and spatial distribution of ozone is very important for understanding the atmospheric chemistry and thereby its impact on environment, weather and climate. The intra-seasonal variability plays a ...The study of temporal and spatial distribution of ozone is very important for understanding the atmospheric chemistry and thereby its impact on environment, weather and climate. The intra-seasonal variability plays a major role in the inter-annual variability of weather parameters such as rainfall, temperature, pressure and atmospheric trace gas constituents such as atmospheric ozone. The strength of monsoon circulation and deep convection greatly modifies the atmospheric compositions and meteorological parameters such as rainfall amount, distributions of atmospheric trace gas concentrations and other weather parameters over the summer monsoon region. The daily total column ozone (TCO) measured over maritime station (Lakshadweep Island— 10°10'N & 73°30'E) and coastal station (Cochin—9°55'N and 76°16'E) using Microtop II Ozonometer were considered for the comparative study of seasonal and intra-seasonal variability for the year 2015. The annual average of total column ozone over Lakshadweep Islands and Cochin was 290 DU and 280 DU respectively for the year 2015. The greater concentrations in daily TCO measurements over Lakshadweep Islands for all seasons compared to Cochin lead to the speculations that, the surface ozone concentration is more because of pollution from the diesel burning emissions, since the whole Island’s population completely depends on diesel generator for the power supply. During winter season maritime station shows a decrease of ~30 DU in TCO over Lak-shadweep Island compared to coastal station Cochin (~18 DU) from the annual mean in the month of December. During pre-monsoon season TCO concentration is high over both locations. There is gradual increase of TCO concentration over Cochin from pre-monsoon to monsoon season and peak in the month of September, but decreasing TCO concentrations measured over Lakshadweep during July to August. In the analysis it was found that Intra-Seasonal Variability (ISV) in total column ozone over Lakshadweep Islands and Cochin during summer monsoon season was modulated by the monsoon dynamics and convection, thereby changes in the photochemistry of ozone production and distributions over the monsoon region. Two significant intra-seasonal oscillations (ISOs) such as Madden Julian Oscillation (MJO) and Quasi-Biweekly Oscillations (QBW) were identified in the TCO during monsoon season. The MJO shows higher periodicity (~54 days) over Lakshadweep Islands compared to the coastal station, Cochin (~48 days). Intra-seasonal variability of TCO over the maritime and coastal stations varies with geographic locations, marine boundary layer characteristics and also with seasons. The intra-seasonal variability or ISOs controls the interannual variability of TCO over a region. Hence deeper knowledge of ISOs in trace gases such as ozone helps us to understand more about the regional climate and air quality.展开更多
The interaction between the low-frequency atmospheric oscillation(Madden-Julian Oscillation,MJO) and the diabatic heating over the Qinghai-Xizang Plateau(QXP) from March to June is analyzed.The results show that there...The interaction between the low-frequency atmospheric oscillation(Madden-Julian Oscillation,MJO) and the diabatic heating over the Qinghai-Xizang Plateau(QXP) from March to June is analyzed.The results show that there are respectively two and one wave trains around the QXP during the onset of the South China Sea monsoon in strong and weak monsoon years.The locations and strength of the wave train propagation differ between the strong and weak monsoon years.Because diabatic heating of the QXP prevents the low-frequency oscillation,the wave train of interaction between the diabatic heating and the zonal wind MJO propagates along the west and east of the QXP in the strong monsoon years.The distribution of the wave train interaction between the diabatic heating and the zonal wind MJO traverses the QXP and coincides with the location of the southern and northern upper-level jet streams,showing that they are remarkably correlated.An interesting and notable phenomenon is that the interaction between diabatic heating and the zonal wind MJO over the QXP suddenly disappears during the monsoon onset in weak monsoon years.展开更多
文摘The study of temporal and spatial distribution of ozone is very important for understanding the atmospheric chemistry and thereby its impact on environment, weather and climate. The intra-seasonal variability plays a major role in the inter-annual variability of weather parameters such as rainfall, temperature, pressure and atmospheric trace gas constituents such as atmospheric ozone. The strength of monsoon circulation and deep convection greatly modifies the atmospheric compositions and meteorological parameters such as rainfall amount, distributions of atmospheric trace gas concentrations and other weather parameters over the summer monsoon region. The daily total column ozone (TCO) measured over maritime station (Lakshadweep Island— 10°10'N & 73°30'E) and coastal station (Cochin—9°55'N and 76°16'E) using Microtop II Ozonometer were considered for the comparative study of seasonal and intra-seasonal variability for the year 2015. The annual average of total column ozone over Lakshadweep Islands and Cochin was 290 DU and 280 DU respectively for the year 2015. The greater concentrations in daily TCO measurements over Lakshadweep Islands for all seasons compared to Cochin lead to the speculations that, the surface ozone concentration is more because of pollution from the diesel burning emissions, since the whole Island’s population completely depends on diesel generator for the power supply. During winter season maritime station shows a decrease of ~30 DU in TCO over Lak-shadweep Island compared to coastal station Cochin (~18 DU) from the annual mean in the month of December. During pre-monsoon season TCO concentration is high over both locations. There is gradual increase of TCO concentration over Cochin from pre-monsoon to monsoon season and peak in the month of September, but decreasing TCO concentrations measured over Lakshadweep during July to August. In the analysis it was found that Intra-Seasonal Variability (ISV) in total column ozone over Lakshadweep Islands and Cochin during summer monsoon season was modulated by the monsoon dynamics and convection, thereby changes in the photochemistry of ozone production and distributions over the monsoon region. Two significant intra-seasonal oscillations (ISOs) such as Madden Julian Oscillation (MJO) and Quasi-Biweekly Oscillations (QBW) were identified in the TCO during monsoon season. The MJO shows higher periodicity (~54 days) over Lakshadweep Islands compared to the coastal station, Cochin (~48 days). Intra-seasonal variability of TCO over the maritime and coastal stations varies with geographic locations, marine boundary layer characteristics and also with seasons. The intra-seasonal variability or ISOs controls the interannual variability of TCO over a region. Hence deeper knowledge of ISOs in trace gases such as ozone helps us to understand more about the regional climate and air quality.
基金supported by National Basic Research Program of China (Grant No. 2007CB411506)National Natural Science Foundation of China (Grant No. 40875050)
文摘The interaction between the low-frequency atmospheric oscillation(Madden-Julian Oscillation,MJO) and the diabatic heating over the Qinghai-Xizang Plateau(QXP) from March to June is analyzed.The results show that there are respectively two and one wave trains around the QXP during the onset of the South China Sea monsoon in strong and weak monsoon years.The locations and strength of the wave train propagation differ between the strong and weak monsoon years.Because diabatic heating of the QXP prevents the low-frequency oscillation,the wave train of interaction between the diabatic heating and the zonal wind MJO propagates along the west and east of the QXP in the strong monsoon years.The distribution of the wave train interaction between the diabatic heating and the zonal wind MJO traverses the QXP and coincides with the location of the southern and northern upper-level jet streams,showing that they are remarkably correlated.An interesting and notable phenomenon is that the interaction between diabatic heating and the zonal wind MJO over the QXP suddenly disappears during the monsoon onset in weak monsoon years.
