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Monitoring Surface Water Change in Northeast China in 1999–2020:Evidence from Satellite Observation and Refined Classification
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作者 LIU Kai ZHANG Dapeng +3 位作者 CHEN Tan CUI Peipei FAN Chenyu SONG Chunqiao 《Chinese Geographical Science》 SCIE CSCD 2024年第1期106-117,共12页
As a typical region with high water demand for agricultural production,understanding the spatiotemporal surface water changes in Northeast China is critical for water resources management and sustainable development.H... As a typical region with high water demand for agricultural production,understanding the spatiotemporal surface water changes in Northeast China is critical for water resources management and sustainable development.However,the long-term variation characteristics of surface water of different water body types in Northeast China remain rarely explored.This study investigated how surface water bodies of different types(e.g.,lake,reservoir,river,coastal aquaculture,marsh wetland,ephemeral water) changed during1999–2020 in Northeast China based on various remote sensing-based datasets.The results showed that surface water in Northeast China grew dramatically in the past two decades,with an equivalent area increasing from 24 394 km^(2) in 1999 to 34 595 km^(2) in 2020.The surge of ephemeral water is the primary driver of surface water expansion,which could ascribe to shifted precipitation pattern.Marsh wetlands,rivers,and reservoirs experienced a similar trend,with an approximate 20% increase at the interdecadal scale.By contrast,coastal aquacultures and natural lakes remain relatively stable.This study is expected to provide a more comprehensive investigation of the surface water variability in Northeast China and has important practical significance for the scientific management of different types of surface water. 展开更多
关键词 surface water spatiotemporal variation water body classification remote sensing Northeast China
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Impacts of Comorbidity and Mental Shock on Organic Micropollutants in Surface Water During and After the First Wave of COVID-19 Pandemic in Wuhan (2019–2021), China
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作者 Jian Zhao Jin Kang +10 位作者 Xiaofeng Cao Rui Bian Gang Liu Shengchao Hu Xinghua Wu Chong Li Dianchang Wang Weixiao Qi Cunrui Huang Huijuan Liu Jiuhui Qu 《Engineering》 SCIE EI CAS CSCD 2024年第6期40-48,共9页
The first pandemic wave of coronavirus disease 2019(COVID-19)induced a considerable increase in several antivirals and antibiotics in surface water.The common symptoms of COVID-19 are viral and bacterial infections,wh... The first pandemic wave of coronavirus disease 2019(COVID-19)induced a considerable increase in several antivirals and antibiotics in surface water.The common symptoms of COVID-19 are viral and bacterial infections,while comorbidities(e.g.,hypertension and diabetes)and mental shock(e.g.,insomnia and anxiety)are nonnegligible.Nevertheless,little is known about the long-term impacts of comorbidities and mental shock on organic micropollutants(OMPs)in surface waters.Herein,we monitored 114 OMPs in surface water and wastewater treatment plants(WWTPs)in Wuhan,China,between 2019 and 2021.The pandemic-induced OMP pollution in surface water was confirmed by significant increases in 26 OMP concentrations.Significant increases in four antihypertensives and one diabetic drug suggest that the treatment of comorbidities may induce OMP pollution.Notably,cotinine(a metabolite of nicotine)increased 155 times to 187 ngL1,which might be associated with increased smoking.Additionally,the increases in zolpidem and sulpiride might be the result of worsened insomnia and depression.Hence,it is reasonable to note that mental-health protecting drugs/behavior also contributed to OMP pollution.Among the observed OMPs,telmisartan,lopinavir,and ritonavir were associated with significantly higher ecological risks because of their limited WWTP-removal rate and high ecotoxicity.This study provides new insights into the effects of comorbidities and mental shock on OMPs in surface water during a pandemic and highlights the need to monitor the fate of related pharmaceuticals in the aquatic environment and to improve their removal efficiencies in WWTPs。 展开更多
关键词 Coronavirus disease 2019 COMORBIDITIES Mental shock MICROPOLLUTANT surface water
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A CFD Model to Evaluate Near-Surface Oil Spill from a Broken Loading Pipe in Shallow Coastal Waters
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作者 Portia Felix Lee Leon +2 位作者 Derek Gay Stefano Salon Hazi Azamathulla 《Fluid Dynamics & Materials Processing》 EI 2024年第1期59-77,共19页
Oil spills continue to generate various issues and concerns regarding their effect and behavior in the marine environment,owing to the related potential for detrimental environmental,economic and social implications.I... Oil spills continue to generate various issues and concerns regarding their effect and behavior in the marine environment,owing to the related potential for detrimental environmental,economic and social implications.It is essential to have a solid understanding of the ways in which oil interacts with the water and the coastal ecosystems that are located nearby.This study proposes a simplified model for predicting the plume-like transport behavior of heavy Bunker C fuel oil discharging downward from an acutely-angled broken pipeline located on the water surface.The results show that the spill overall profile is articulated in three major flow areas.The first,is the source field,i.e.,a region near the origin of the initial jet,followed by the intermediate or transport field,namely,the region where the jet oil flow transitions into an underwater oil plume flow and starts to move horizontally,and finally,the far-field,where the oil re-surface and spreads onto the shore at a significant distance from the spill site.The behavior of the oil in the intermediate field is investigated using a simplified injection-type oil spill model capable of mimicking the undersea trapping and lateral migration of an oil plume originating from a negatively buoyant jet spill.A rectangular domain with proper boundary conditions is used to implement the model.The Projection approach is used to discretize a modified version of the Navier-Stokes equations in two dimensions.A benchmark fluid flow issue is used to verify the model and the results indicate a reasonable relationship between specific gravity and depth as well as agreement with the aerial data and a vertical temperature profile plot. 展开更多
关键词 CFD model Navier-Stokes equations projection method water surface oil spill shallow coastal waters
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Isotope Tracking of Surface Water Groundwater Interaction in the Beninese Part of the Iullemeden Aquifer System
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作者 Houégnon Géraud Vinel Gbewezoun Samuel Yao Ganyaglo +4 位作者 Abdoukarim Alassane Samuel Boakye Dampare Gaya Salifou Orou Pete Alou Moussa Boukari Daouda Mama 《Journal of Water Resource and Protection》 CAS 2024年第7期489-501,共13页
The Kandi basin is located in northeast Benin (West Africa). This study is focused on the estimation of water fluxes exchanged between the river Niger (and its tributaries) and the transboundary Iullemeden Aquifer Sys... The Kandi basin is located in northeast Benin (West Africa). This study is focused on the estimation of water fluxes exchanged between the river Niger (and its tributaries) and the transboundary Iullemeden Aquifer System. In that framework, an innovative approach based on the application of the Bayesian Mixing Model (MixSIAR) analysis on water isotopes (oxygen-18, deuterium and tritium) was performed. Moreover, to assess the relevance of the model outputs, Pearson’s correlation and Principal Component Analysis (PCA) have been done. A complex relationship between surface water and groundwater has been found. Sixty percent (60%) of groundwater samples are made of more than 70% river water and rainwater;while 31.25% of surface water samples are made of about 84% groundwater. To safeguard sustainable water resources for the well-being of the local communities, surface water and groundwater must be managed as a unique component in the Kandi basin. 展开更多
关键词 BENIN West Africa Kandi basin Iullemeden Aquifer System surface water Groundwater Interaction
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Impact of climate change and human activities on the spatiotemporal dynamics of surface water area in Gansu Province, China
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作者 LU Haitian ZHAO Ruifeng +3 位作者 ZHAO Liu LIU Jiaxin LYU Binyang YANG Xinyue 《Journal of Arid Land》 SCIE CSCD 2024年第6期798-815,共18页
Understanding the dynamics of surface water area and their drivers is crucial for human survival and ecosystem stability in inland arid and semi-arid areas.This study took Gansu Province,China,a typical area with comp... Understanding the dynamics of surface water area and their drivers is crucial for human survival and ecosystem stability in inland arid and semi-arid areas.This study took Gansu Province,China,a typical area with complex terrain and variable climate,as the research subject.Based on Google Earth Engine,we used Landsat data and the Open-surface Water Detection Method with Enhanced Impurity Control method to monitor the spatiotemporal dynamics of surface water area in Gansu Province from 1985 to 2022,and quantitatively analyzed the main causes of regional differences in surface water area.The findings revealed that surface water area in Gansu Province expanded by 406.88 km2 from 1985 to 2022.Seasonal surface water area exhibited significant fluctuations,while permanent surface water area showed a steady increase.Notably,terrestrial water storage exhibited a trend of first decreasing and then increasing,correlated with the dynamics of surface water area.Climate change and human activities jointly affected surface hydrological processes,with the impact of climate change being slightly higher than that of human activities.Spatially,climate change affected the'source'of surface water to a greater extent,while human activities tended to affect the'destination'of surface water.Challenges of surface water resources faced by inland arid and semi-arid areas like Gansu Province are multifaceted.Therefore,we summarized the surface hydrology patterns typical in inland arid and semi-arid areas and tailored surface water'supply-demand'balance strategies.The study not only sheds light on the dynamics of surface water area in Gansu Province,but also offers valuable insights for ecological protection and surface water resource management in inland arid and semi-arid areas facing water scarcity. 展开更多
关键词 surface water area terrestrial water storage Open-surface water Detection Method with Enhanced Impurity Control method Google Earth Engine climate change human activities inland arid and semi-arid areas
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Unveiling three-dimensional sea surface signatures caused by internal solitary waves:insights from the surface water ocean topography mission
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作者 Xudong ZHANG Xiaofeng LI 《Journal of Oceanology and Limnology》 SCIE CAS CSCD 2024年第3期709-714,共6页
Internal solitary waves(ISW),characterized by large amplitude and long propagation distance,are widespread in global oceans.While remote sensing images have played an essential role in studying ISWs,they mainly exploi... Internal solitary waves(ISW),characterized by large amplitude and long propagation distance,are widespread in global oceans.While remote sensing images have played an essential role in studying ISWs,they mainly exploit two-dimensional image information.However,with the launch of the surface water ocean topography(SWOT)satellite on December 16,2022,a unique opportunity has emerged to capture wide-swath three-dimensional ISW-induced sea surface information.In this study,we examine ISWs in the Andaman Sea using data from the Ka-band Radar Interferometer(KaRIN),a crucial sensor onboard SWOT.KaRIN not only provides backscattering satellite images but also employs synthetic aperture interferometry techniques to retrieve wide-swath two-dimensional sea surface height measurements.Our observations in the Andaman Sea revealed the presence of ISWs characterized by dark-bright strips and surface elevation solitons.The surface soliton has an amplitude of 0.32 m,resulting in an estimation of ISW amplitude of approximately 60 m.In contrast to traditional two-dimensional satellite images or nadir-looking altimetry data,the SWOT mission’s capability to capture threedimensional sea surface information represents a significant advancement.This breakthrough holds substantial promise for ISW studies,particularly in the context of ISW amplitude inversion. 展开更多
关键词 internal solitary wave(ISW) surface water ocean topography(SWOT) ALTIMETER
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Surface Water Quality Profiling Using Physicochemical Parameters in Open Defecation Free and Non-Open Defecation Free Local Government Areas in Benue State, Nigeria
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作者 Moses T. Asoo Celestine U. Aguoru +1 位作者 Innocent O. Ogbonna Hyacinth O.A. Oluma 《Open Journal of Modern Hydrology》 CAS 2024年第3期174-191,共18页
Physicochemical parameters of surface water sources in the study of local government areas (LGAs) were assessed using standard procedures. The mean physicochemical parameters for pH (5.49), NO2 (0.23 mg/L), SO4 (0.77 ... Physicochemical parameters of surface water sources in the study of local government areas (LGAs) were assessed using standard procedures. The mean physicochemical parameters for pH (5.49), NO2 (0.23 mg/L), SO4 (0.77 mg/L), Na (28.72 mg/L), Ca (28.94 mg/L), Mg (17.50 mg/L), Cl (11.65 mg/L), TSS (6.27 mg/L), TDS (104.23 mg/L), BOD (2.83 mg/L) and F (0.87 mg/L) were below WHO standards irrespective of their defecation status. The values for electrical conductivity (EC) (2770.50 µs/cm, turbidity (481.24 NTU), dissolved oxygen (DO) (5.32 mg/L), chemical oxygen demand (COD) (445.50 mg/L), K (125.06 mg/L), PO4 (0.78 mg/L) and Fe (0.57 mg/L) were above the WHO limits for safe water. Higher EC and COD values obtained in the study is evidence of pollution of the water sources by organic matter. 展开更多
关键词 Open Defecation surface water water Quality Standard Physicochemical Parameters
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Agricultural Contamination of the Surface Waters of the Upper Ouémé in Benin: The Case of Heavy Metals and Pesticides
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作者 Armelle Sabine Yélignan Hounkpatin Nonvignon Martial Fassinou +5 位作者 Fadéby Modeste Gouissi Zoulkanerou Orou Piami Dossou Armel Géraldo Houndeton Souradjou Orou Goura Wakili Bolatito Yessoufou Tayéwo Sylvain Biaou 《Journal of Agricultural Chemistry and Environment》 2024年第1期83-99,共17页
Objective: The main objective of this study was to assess the degree of contamination of surface waters by heavy metals and pesticides. Method: To this end, data were collected in December 2022 from four specific samp... Objective: The main objective of this study was to assess the degree of contamination of surface waters by heavy metals and pesticides. Method: To this end, data were collected in December 2022 from four specific sampling stations: Okpara, Térou, Affon and Adjiro. Levels of heavy metals, including cadmium, chromium, copper, iron, mercury, nickel and lead, were measured and subjected to in-depth statistical analysis using graphical summation models. In addition, the concentrations of pesticide active ingredients present in the samples were interpreted and evaluated. The statistical data collected during this study were processed using R software, version 3.5.0. Results: The values obtained at the different stations Okpara, Térou, Affon and Adjiro are respectively Arsenic (2 × 10<sup>-4</sup> mg/L;2.2 × 10<sup>-1</sup> mg/L;1.2 × 10<sup>-4</sup> mg/L;2 × 10<sup>-4</sup> mg/L), Cadmium (4.4 × 10<sup>-5</sup> mg/L;1.1 × 10<sup>-2</sup> mg/L;10<sup>-4</sup> mg/L;4 × 10<sup>-4</sup> mg/L). Then Copper (7 × 10<sup>-4</sup> mg/L;3 × 10<sup>-3</sup> mg/L;7 × 10<sup>-4</sup> mg/L;1 × 10<sup>-4</sup> mg/L), Iron (1.51 mg/L;6.4 × 10<sup>-1</sup> mg/L;2.0012 mg/L;2.9 × 10<sup>-1</sup> mg/L), Lead (0 mg/L;0 mg/L;1.5 × 10<sup>-3</sup> mg/L;1.5 × 10<sup>-3</sup> mg/L). Mercury, nickel and chromium were not detected in surface waters. It is important to note that the values obtained for trace metals (Cadmium, Chromium, Copper, Iron, Mercury, nickel and chromium were not detected in surface waters. It is important to note that the values obtained for trace metals (cadmium, chromium, copper, iron, mercury, nickel and lead) were all below the guideline standards set by the WHO in 2006 for uncontaminated surface waters. This indicates that the surface waters of the Upper Ouémé were below acceptable contamination thresholds in terms of heavy metals. However, the presence of pesticide active ingredients such as cyfluthrin, endosulfan-alpha, endosulfan-beta, profenosfos, tihan, atrazine, gala super and glycel clearly indicates that these surface waters are subject to agricultural contamination. 展开更多
关键词 Agricultural Contamination Heavy Metals PESTICIDES surface water North Benin
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Seasonal constraint of dynamic water temperature on riverine dissolved inorganic nitrogen transport in land surface modeling
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作者 Shuang Liu Kaiheng Hu +1 位作者 Zhenghui Xie Yan Wang 《Atmospheric and Oceanic Science Letters》 CSCD 2024年第4期35-40,共6页
水体温度变化对河流可溶性无机氮(DIN)输送有着强烈控制作用.然而,在全球尺度上河流DIN输送量对水温度变化的响应尚不清楚.因此,本文基于陆面过程模式,耦合河流水温估算和DIN传输方案,设定有,无动态水温情景,对比研究陆面模拟中水温变... 水体温度变化对河流可溶性无机氮(DIN)输送有着强烈控制作用.然而,在全球尺度上河流DIN输送量对水温度变化的响应尚不清楚.因此,本文基于陆面过程模式,耦合河流水温估算和DIN传输方案,设定有,无动态水温情景,对比研究陆面模拟中水温变化对河流DIN通量变化的影响.结果表明:在考虑水温动态变化后,在30°N和30°S之间, DIN通量年振幅减小5%–25%.在中国东部地区,水温动态变化使河流DIN通量在夏季减少1%–3%,在冬季增加1%–5%,对DIN通量具有明显的季节性约束作用,表明动态水温的表达在河流DIN输送模拟中的重要性. 展开更多
关键词 陆面模拟 河流氮输送 水温变化 季节变化 全球尺度
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Different bactericidal abilities of plasma-activated saline with various reactive species prepared by surface plasma-activated air and plasma jet combinations
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作者 贾怡康 李甜会 +5 位作者 张瑞 赵鹏瑜 王子丰 陈旻 郭莉 刘定新 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第1期50-61,共12页
Plasma-activated water(PAW),as an extended form of cold atmospheric-pressure plasma,greatly expands the application of plasma-based technology.The biological effects of PAW are closely related to the aqueous reactive ... Plasma-activated water(PAW),as an extended form of cold atmospheric-pressure plasma,greatly expands the application of plasma-based technology.The biological effects of PAW are closely related to the aqueous reactive species,which can be regulated by the activation process.In this study,surface plasma-activated air(SAA)and a He+O_(2)plasma jet(Jet)were parallelly combined(the SAA+Jet combination)or sequentially combined(the SAA→Jet combination and the Jet→SAA combination)to prepare plasma-activated saline(PAS).The PAS activated by the combinations exhibited stronger bactericidal effects than that activated by the SAA or the Jet alone.The concentrations of H_(2)O_(2)and NO_(2)^(-)were higher in the PAS activated by the Jet→SAA combination,while ONOO^(-)concentrations were close in the three kinds of PAS and^(1)O_(2)concentrations were higher in the PAS activated by the SAA+Jet combination.The analysis of scavengers also demonstrated that H_(2)O_(2),^(1)O_(2),and ONOO^(-)in the PAS activated by the SAA+Jet combination,and^(1)O_(2)in the PAS activated by the Jet→SAA combination played critical roles in bactericidal effects.Further,the effective placement time of the three PAS varied,and the PAS activated by the Jet→SAA combination could also inactivate 2.6-log_(10)of MRSA cells after placement for more than 60 min.The regulation of reactive species in plasma-activated water via different combinations of plasma devices could improve the directional application of plasma-activated water in the biomedical field. 展开更多
关键词 plasma-activated water surface plasma-activated air plasma jet bactericidal effect reactive species
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Impact of Initial Soil Conditions on Soil Hydrothermal and Surface Energy Fluxes in the Permafrost Region of the Tibetan Plateau
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作者 Siqiong LUO Zihang CHEN +3 位作者 Jingyuan WANG Tonghua WU Yao XIAO Yongping QIAO 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第4期717-736,共20页
Accurate initial soil conditions play a crucial role in simulating soil hydrothermal and surface energy fluxes in land surface process modeling.This study emphasized the influence of the initial soil temperature(ST)an... Accurate initial soil conditions play a crucial role in simulating soil hydrothermal and surface energy fluxes in land surface process modeling.This study emphasized the influence of the initial soil temperature(ST)and soil moisture(SM)conditions on a land surface energy and water simulation in the permafrost region in the Tibetan Plateau(TP)using the Community Land Model version 5.0(CLM5.0).The results indicate that the default initial schemes for ST and SM in CLM5.0 were simplistic,and inaccurately represented the soil characteristics of permafrost in the TP which led to underestimating ST during the freezing period while overestimating ST and underestimating SLW during the thawing period at the XDT site.Applying the long-term spin-up method to obtain initial soil conditions has only led to limited improvement in simulating soil hydrothermal and surface energy fluxes.The modified initial soil schemes proposed in this study comprehensively incorporate the characteristics of permafrost,which coexists with soil liquid water(SLW),and soil ice(SI)when the ST is below freezing temperature,effectively enhancing the accuracy of the simulated soil hydrothermal and surface energy fluxes.Consequently,the modified initial soil schemes greatly improved upon the results achieved through the long-term spin-up method.Three modified initial soil schemes experiments resulted in a 64%,88%,and 77%reduction in the average mean bias error(MBE)of ST,and a 13%,21%,and 19%reduction in the average root-mean-square error(RMSE)of SLW compared to the default simulation results.Also,the average MBE of net radiation was reduced by 7%,22%,and 21%. 展开更多
关键词 initial soil conditions soil temperature soil liquid water soil ice surface energy fluxes PERMAFROST
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Study of the ability of SWOT to detect sea surface height changes caused by internal solitary waves
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作者 Hao Zhang Chenqing Fan +1 位作者 Lina Sun Junmin Meng 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2024年第5期54-64,共11页
Surface Water and Ocean Topography(SWOT)is a next-generation radar altimeter that offers high resolution,wide swath,imaging capabilities.It has provided free public data worldwide since December 2023.This paper aims t... Surface Water and Ocean Topography(SWOT)is a next-generation radar altimeter that offers high resolution,wide swath,imaging capabilities.It has provided free public data worldwide since December 2023.This paper aims to preliminarily analyze the detection capabilities of the Ka-band radar interferometer(KaRIn)and Nadir altimeter(NALT),which are carried out by SWOT for internal solitary waves(ISWs),and to gather other remote sensing images to validate SWOT observations.KaRIn effectively detects ISW surface features and generates surface height variation maps reflecting the modulations induced by ISWs.However,its swath width does not completely cover the entire wave packet,and the resolution of L2/L3 level products(about 2 km)cannot be used to identify ISWs with smaller wavelengths.Additionally,significant wave height(SWH)images exhibit blocky structures that are not suitable for ISW studies;sea surface height anomaly(SSHA)images display systematic leftright banding.We optimize this imbalance using detrending methods;however,more precise treatment should commence with L1-level data.Quantitative analysis based on L3-level SSHA data indicates that the average SSHA variation induced by ISWs ranges from 10 cm to 20 cm.NALTs disturbed by ISWs record unusually elevated SWH and SSHA values,rendering the data unsuitable for analysis and necessitating targeted corrections in future retracking algorithms.For the normalized radar cross section,Ku-band and four-parameter maximum likelihood estimation retracking demonstrated greater sensitivity to minor changes in the sea surface,making them more suitable for ISW detection.In conclusion,SWOT demonstrates outstanding capabilities in ISW detection,significantly advancing research on the modulation of the sea surface by ISWs and remote sensing imaging mechanisms. 展开更多
关键词 internal solitary waves surface water and Ocean Topography(SWOT) Ka-band radar interferometer(KaRIn) Nadir altimeter(NALT) sea surface height anomaly(SSHA) normalized radar cross section(NRCS)
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Surface flow constructed wetland with composite plant bed for pretreatment of micro-polluted Yellow River raw water in China
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作者 杨旭 于水利 +3 位作者 严晓菊 赵焱 修春海 张洪洋 《Journal of Harbin Institute of Technology(New Series)》 EI CAS 2008年第3期426-429,共4页
In order to investigate the feasibility of pretreating the micro-polluted Yellow River raw water by constructed wetland, an experiment was conducted using a surface flow constructed wetland with composite plant bed. T... In order to investigate the feasibility of pretreating the micro-polluted Yellow River raw water by constructed wetland, an experiment was conducted using a surface flow constructed wetland with composite plant bed. The contamination removal efficiency and their trends in the wetland treatment system were studied under different hydraulic loading rates(HLR). The contamination removal efficiencies were compared according to the seasonal change under optimum HLR. The result shows that in the same season, under different hydraulic loadings ranging from 2 to 6 m3/(m2·d) at the same period, the best HLR is 4 m3/(m2·d) in the experimental system. The average removal rates of COD, TN, ammoniacal nitrogen(NH4+-N), and TP in the constructed wetland are 38.37%, 45.97%, 39.86% and 41.69%, respectively. According to China Standard for Surface Water Resources (GB3838-2002), mean effluent of COD, TN, NH4+-N and TP can nearly reach Grade Ⅲ, GradeⅤ, GradeⅠand GradeⅠ, respectively. Furthermore, treatment efficiency of the system in summer is obvious higher than that in other seasons. The expenditure of constructing the constructed wetland with the average treating capacity of 176 m3/d and lifetime of 20 years is 17075.00 RMB. The average disposal cost is summed up to 0.17 RMB/m3, which shows that the pretreatment of the micro-polluted Yellow River raw water by constructed wetland is feasible. 展开更多
关键词 湿地 表面流 预处理 黄河 水质污染 未净化水
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Dynamically-evolved surface heterojunction in iridium nanocrystals boosting acidic oxygen evolution and overall water splitting 被引量:1
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作者 Chenyu Yang Xiuxiu Zhang +6 位作者 Qizheng An Meihuan Liu Wanlin Zhou Yuanli Li Fengchun Hu Qinghua Liu Hui Su 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2023年第3期374-380,I0011,共8页
Simultaneously realizing improved activity and stability of acidic oxygen evolution reaction(OER) electrocatalysts is highly promising for developing cost-effective sustainable energy in the splitting of water techniq... Simultaneously realizing improved activity and stability of acidic oxygen evolution reaction(OER) electrocatalysts is highly promising for developing cost-effective sustainable energy in the splitting of water technique.Herein,we report iridium nanocrystals embedded into 3D conductive clothes(Ir-NCT/CC) as a low iridium electrocatalyst realizing ultrahigh acidic OER activity and robust stability.The well-designed Ir-NCT/CC requires a low overpotential of 202 mV to reach the current density of 10 mA cm^(-2)with a high mass activity of 1754 A g^(-1).Importantly,in acidic overall water splitting,Ir-NCT/CC merely delivers a cell voltage of 1.469 V at a typical current density of 10 mA cm^(-2)and also maintains robust durability under continuous operation.We identify that a low working voltage drives the formation of a highly stable amorphous IrOxactive phase over the surface of Ir nanocrystals(surface heterojunction IrOx/Ir-NCT) during operating conditions,which contributes to an effective and durable OER process. 展开更多
关键词 ELECTROCATALYST surface heterojunction In-situ synchrotron radiation techniques Reaction kinetics Acidic overall water splitting
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Current Situation and Countermeasures of Antibiotic Pollu-tion in the Surface Water of the Yangtze River Basin in a Province of Central China 被引量:1
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作者 Zhao WANG Bin ZHAO +3 位作者 Chao ZHU Xiaofei TANG Bangben YAO Min ZHANG 《Meteorological and Environmental Research》 CAS 2023年第1期63-67,共5页
Antibiotics are widely used in the process of human medical treatment,livestock and poultry breeding,and aquaculture.With the excretion of urine and feces,they enter the water environment of human life and become an i... Antibiotics are widely used in the process of human medical treatment,livestock and poultry breeding,and aquaculture.With the excretion of urine and feces,they enter the water environment of human life and become an important source of water environment pollution.Antibiotic residues in the environment have high ecological and health risks.Through the pilot monitoring of antibiotics in the main stream of the Yangtze River,Chaohu Lake and the drinking water source of Hefei City,the current situation and impact of antibiotic pollution were analyzed.The results show that 32 kinds of antibiotics and their derivatives of the six major categories involved were detected to varying degrees,and the concentrations at some points reached 1.26μg/L.Finally,the prevention and control of antibiotic pollution in the surface water of the Yangtze River basin in a province of central China were summarized,and relevant suggestions were given. 展开更多
关键词 ANTIBIOTICS surface water Pollution status COUNTERMEASURES
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Estimation of surface water content at the Tianwen-1 Zhurong landing site 被引量:1
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作者 Xiang Zhou Yang Liu +2 位作者 Xing Wu ZhenXing Zhao YongLiao Zou 《Earth and Planetary Physics》 EI CSCD 2023年第3期347-355,共9页
China’s first Mars rover,Zhurong,successfully landed in the south of Utopia Planitia.The surface water content at the landing area can provide constraints on mineral formation conditions and help us better understand... China’s first Mars rover,Zhurong,successfully landed in the south of Utopia Planitia.The surface water content at the landing area can provide constraints on mineral formation conditions and help us better understand the evolution of the Martian aqueous and geological environment.In this work,the surface kinetic temperature of the Zhurong landing area was derived by analyzing data from the Mars Express Observatoire pour la Minéralogie,l’Eau,les Glaces et l’Activité(OMEGA)spectrometer.Using the Discrete Ordinate Radiative Transfer(DISORT)model,we performed atmospheric correction and thermal correction for the OMEGA data to obtain the surface effective single-particle absorption thickness(ESPAT)parameter to evaluate the surface water content.The surface water content distribution at the landing area was relatively uniform at a lateral scale of~10 km.At the Zhurong landing site,the surface water content in the topmost layer(a few hundred micrometers)of the regolith was 5−8 weight percent water(wt%H_(2)O),assuming surface particle sizes of<45μm,or 1.6−2.5 wt%H_(2)O,assuming surface particle sizes in the range of 125−250μm.The Mars Surface Composition Detector(MarSCoDe)onboard Zhurong also observed significant H_(2)O/OH signals in the landing area.Our results provide an important regional context for the hydration state of the area and can be further verified by the H content derived from the Laser-Induced Breakdown Spectrometer(LIBS)data of MarSCoDe. 展开更多
关键词 MARS Zhurong surface water content Observatoire pour la Minéralogie l’Eau les Glaces et l’Activité(OMEGA) Discrete Ordinate Radiative Transfer(DISORT)
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Impact of backwater on water surface profile in curved channels
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作者 Rui-hua Nie Qi-hang Zhou +3 位作者 Wen-jie Li Xing-nian Liu Gang Xie Lu Wang 《Water Science and Engineering》 EI CAS CSCD 2023年第3期295-301,共7页
Owing to extensive construction of dams, the impact of backwater on flow may lead to navigation or flood control issues in curved channels. To date, the impact of backwater on the water surface profile in curved chann... Owing to extensive construction of dams, the impact of backwater on flow may lead to navigation or flood control issues in curved channels. To date, the impact of backwater on the water surface profile in curved channels remains unknown and requires investigation. In this study, experiments were conducted in a glass-walled recirculating flume with a length of 19.4 m, a width of 0.6 m, and a depth of 0.8 m, and the impact of backwater on the water surface profile in a 90° channel bend was investigated. The experimental results showed that the backwater degree had a significant impact on the transverse and longitudinal flow depth distributions in the bend. The transverse slope of the flow (Jr) increased linearly with an increase in the Froude number of the approach flow upstream of the bend. Jr increased with the longitudinal location parameter ξ when −0.2 < ξ < 0.5, and decreased with ξ when 0.5 < ξ < 1.2. Furthermore, the results showed that Jr asymptotically decreased to zero with an increase in the degree of backwater. An equation was formulated to estimate the transverse slope of the flow in a 90° bend in backwater zones. 展开更多
关键词 BACKwater Curved channel Experimental model Transverse slope water surface profile
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Spatio-temporal variation of trace elements distributed over surface water of Upper Ganga River Basin in Western Himalayan Region
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作者 Deepika DIMRI Ambika KUMAR +1 位作者 DeepakKumar MISHRA Archana SHARMA 《Journal of Mountain Science》 SCIE CSCD 2023年第1期145-162,共18页
The rivers draining from the Himalayan range distribute enormous amount of fresh water to the people living in downstream regions.Trace metals flowed with river water can lead to serious impact on ecological system an... The rivers draining from the Himalayan range distribute enormous amount of fresh water to the people living in downstream regions.Trace metals flowed with river water can lead to serious impact on ecological system and human health.Nevertheless,the documentation on trace elements of Himalayan rivers is inadequately documented.The current study deals with the spatial and temporal variability of the major and trace elements of Ganga river water in epirhithron,metarhithron and hyporhithron zone belonging to Himalayan segment.Water samples from nineteen monitoring locations were collected in pre-monsoon(May-June),monsoon(AugustSeptember)and post-monsoon(December)seasons and subjected to be assessed for 20 elements(Ag,Al,Ba,Cd,Ca,Cr,Cu,Fe,Ga,K,Mn,Mg,Na,Ni,Pb,Sr,Th,U,Zn,and Zr)using ICP-OES(Inductively Coupled Plasma-Optical Emission Spectrometer).Different water pollution indexes such as HPI(Heavy Metal Pollution Index),MI(Metal Index)and PI(Pollution Index)were used to describe current water quality status at each monitoring station under particular classified ecological zone.The studied stations in hyporhithron zone had the value of Metal Index(MI>1),indicating threshold of warning.Further,the highest values of HPI in hyporhithron zone correspond to poor water quality status.Sites with poor water quality were also found to be contaminated as per the Pollution Index(PI),exhibiting high concentrations for element(Fe).However,the epirhithron and metarhithron zone in Himalayan segment showed excellent water quality mainly contributed from natural sources.Cluster Analysis(CA)and Principal Component Analysis(PCA)were applied to identify the main influential sources for Ganga river water pollution.The Kriging interpolation method was also applied to prepare spatial distribution map of computed indexes(HPI,MI,and PI).With the help of index of local Moran’s I(LMI),identified spatial clusters and spatial outliers revealed the elevated concentration of most elements in hyporhithron zone.The dataset presented in this study would be convenient for government officials in developing more effective management policies and necessary steps to check and monitor the Ganga river water quality.It was also suggested that further investigations in terms of trace elemental sources and their role in self-purification properties of Ganga water can be addressed in future. 展开更多
关键词 Trace elements Spatial variation Temporal variation surface water Ganga River Basin ICP-OES
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Linking bacterial and archaeal community dynamics to related hydrological,geochemical and environmental characteristics between surface water and groundwater in a karstic estuary
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作者 Xiaogang Chen Qi Ye +5 位作者 Jinzhou Du Neven Cukrov Nuša Cukrov Yan Zhang Ling Li Jing Zhang 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2023年第8期158-170,共13页
Subterranean estuaries(STEs)are characterized by the mixing of terrestrial fresh groundwater and seawater in coastal aquifers.Although microorganisms are important components of coastal groundwater ecosystems and play... Subterranean estuaries(STEs)are characterized by the mixing of terrestrial fresh groundwater and seawater in coastal aquifers.Although microorganisms are important components of coastal groundwater ecosystems and play critical roles in biogeochemical transformations in STEs,limited information is available about how their community dynamics interact with hydrological,geochemical and environmental characteristics in STEs.Here,we studied bacterial and archaeal diversities and distributions with 16S rRNA-based Illumina MiSeq sequencing technology between surface water and groundwater in a karstic STE.Principal-coordinate analysis found that the bacterial and archaeal communities in the areas where algal blooms occurred were significantly separated from those in other stations without algal bloom occurrence.Canonical correspondence analysis showed that nutrients and salinity can explain the patterns of bacterial and archaeal community dynamics.The results suggest that hydrological,geochemical and environmental characteristics between surface water and groundwater likely control the bacterial and archaeal diversities and distributions in STEs.Furthermore,we found that some key species can utilize terrestrial pollutants such as nitrate and ammonia in STEs,indicating that these species(e.g.,Nitrosopumilus maritimus,Limnohabitans parvus and Simplicispira limi)may be excellent candidates for in situ degradation/remediation of coastal groundwater contaminations concerned with the nitrate and ammonia.Overall,this study reveals the coupling relationship between the microbial communities and hydrochemical environments in STEs,and provides a perspective of in situ degradation/remediation for coastal groundwater quality management. 展开更多
关键词 submarine groundwater discharge surface water and groundwater interaction algal bloom microbial ecology nutrient biogeochemistry ammonia-oxidizing archaea nitrate-utilizing bacteria Krka River Estuary
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Level of Bacteriological and Physicochemical Pollution of Surface Waters in Rural Area: The Case of Mbankomo Municipality (Center Region, Cameroon)
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作者 Vanelle Lontchi Segnou Blandine Pulchérie Tamatcho Kweyang +6 位作者 Ernest Koji Siméon Tchakonte Murielle Patricia Mabou Tokam Olive Vivien Noah Ewoti Fils Mamert Onana Ornella Eunice Wandji Kweya Antoine Tamsa Arfao 《Journal of Geoscience and Environment Protection》 2023年第3期173-188,共16页
A study aimed at evaluating the physicochemical and bacteriological quality of surface water was therefore carried out in a few watercourses in the municipality of Mbankomo, located in the Center Region (Cameroon). Th... A study aimed at evaluating the physicochemical and bacteriological quality of surface water was therefore carried out in a few watercourses in the municipality of Mbankomo, located in the Center Region (Cameroon). The physico-chemical parameters were measured according to the standard method. The organic pollution index (OPI) was determined from the contents of nitrates, phosphates, and ammoniacal nitrogen to characterize the level of organic pollution of the water. The microorganisms sought were total flora, indicators of faecal contamination like total coliforms, faecal coliforms, feacal streptococci and Escherichia coli, as well as the species Clostridium perfringens. The organic pollution index indicates a high-level organic pollution level during the small rainy season and high to moderate during the small dry season. High concentrations of the total and fecal coliforms, streptococci fecal, Escherichia coli and Clostridium perfringens respectively of 1712 × 10<sup>5</sup> CFU/100mL;82 × 10<sup>5</sup> CFU/100mL;10 × 10<sup>5</sup> CFU/100mL;27 × 10<sup>5</sup> and 40 × 10<sup>3</sup> CFU/100mL, all higher than WHO standards, indicate that the waterways of Mbankomo are subject to feacal pollution and harbor pathogenic microflora. The cell densities of main bacteria were significantly correlated with main abiotic parameters, such as Escherichia coli, which was significantly correlated with the pH of the water (r = 0.35;p < 0.05). The variation of organic pollution index category means correspond to a high level of organic pollution during the small rainy season and a high to moderate level during the small dry season. The deterioration of the quality of these waters is favored by their proximity to sources of pollution (toilets, plantation), the runoff of the waters contaminated, the use of detergents and wrong maintenance. These waters without any treatment are not recommendable for human consumption according to standards of the World Health Organization. 展开更多
关键词 Bacteriological Quality Physicochemical Parameters surface waters Organic Pollution Index
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