Expeditions during the summers of 2002 and 2003 implemented continuous monitoring of near-surface (2 m height) atmospheric CO2 and H2O concentrations at the 4500 m elevation on Muztagata. The resultant data sets revea...Expeditions during the summers of 2002 and 2003 implemented continuous monitoring of near-surface (2 m height) atmospheric CO2 and H2O concentrations at the 4500 m elevation on Muztagata. The resultant data sets reveal a slight decrease of CO2 concentrations (of about 5 μmol·mol?1) and changes in the diurnal variations from the end of June to the middle August. The daily maximum CO2 concentrations occur between 02:30―05:30 AM (local time) and the minimum levels occur between 12:00―15:30 PM. The atmospheric CO2 concentrations in the summer of 2002 were around 5 μmol·mol?1 lower than those during the same period of 2003, whereas the diurnal amplitude was higher. In contrast, we found that the daily mean atmospheric H2O content in 2003 was much lower than that in 2002 and there exists a striking negative correlation between CO2 and H2O con-centrations. We therefore suggest that the near-surface atmospheric CO2 concentration is affected not only by photosynthesis and respiration, but also by the air H2O content in the glaciated region around Muztagata.展开更多
Based on summer observations of stable isotope of precipitation at Muztagata, western China, during 2002―2003, this paper presents the relationship between δ 18O in precipitation and air temperature, and discusses t...Based on summer observations of stable isotope of precipitation at Muztagata, western China, during 2002―2003, this paper presents the relationship between δ 18O in precipitation and air temperature, and discusses the effect of moisture transport on δ 18O in precipitation. Results show that air temperature correlates positively with δ 18O in precipitation, and the temperature effect controls the δ 18O of precipitation in this area. The Muztagata region exhibits high δ 18O values in summer precipi-tation, similar to those shown at stations in adjacent regions. According to the results of our model set up to trace the moisture trajectories, the westerlies and local moisture circulation contribute to varia-tions of oxygen isotopes in precipitation. In addition, the impacts of the moisture transport distance, the moisture transport level, and the incursion of the polar air mass also influence the variations of δ 18O in precipitation. The moisture origins and transport mechanisms also contribute to the variation of δ 18O in precipitation at Muztagata.展开更多
Expeditions to Muztagata (in the eastern Pamirs) during the summer seasons of2002 and 2003 collected precipitation samples and measured their oxygen isotopes. The δ^(18)O inprecipitation displays a wide range, varyin...Expeditions to Muztagata (in the eastern Pamirs) during the summer seasons of2002 and 2003 collected precipitation samples and measured their oxygen isotopes. The δ^(18)O inprecipitation displays a wide range, varying from -17.40per thousand to +1.33per thousand inJune—September 2002 and from -22.31per thousand to +4.59per thousand in May—August 2003. Theδ^(18)O in precipitation correlates with the initial temperature of precipitation during theobserving periods. The positive correlation between δ^(18)O and temperature suggests that δ^(18)Ocan be used as an indicator of temperature in this region. The δ^(18)O values in fresh-snow samplescollected from two snow events at different elevations on the Muztagata Glacier show a strong''altitude effect'', with a ratio of nearly -0.40per thousand per 100 m from 5500 m to 7450 m.展开更多
A Muztagata ice core recovered at 7010 m altitude in East Pamirs provides a Pb concentration record from 1955 to 2000. The result reveals in- creasing Pb concentrations from 1955 to 1993, with two Pb concentration pea...A Muztagata ice core recovered at 7010 m altitude in East Pamirs provides a Pb concentration record from 1955 to 2000. The result reveals in- creasing Pb concentrations from 1955 to 1993, with two Pb concentration peaks in 1980 and 1993. After 1993, Pb concentrations in ice core show an obvi- ously declining trend. Analysis shows that the lead in the Muztagata ice core mainly came from anthropo- genic emissions from countries in Central Asia, while the local emission had little contribution.展开更多
The dust transport and sediment characteristics are discussed based onanalysis of mi-croparticle size and size distribution in the Muztagata ice core at 6350 m a.s.I. Thefiner particles with diameter of 1—5 μm are t...The dust transport and sediment characteristics are discussed based onanalysis of mi-croparticle size and size distribution in the Muztagata ice core at 6350 m a.s.I. Thefiner particles with diameter of 1—5 μm are the dominant fraction in number, while middle andcoarse particles mainly contribute to the total volume. The lognormal distribution characteristicscan be seen for some high concentration samples, showing that model size and standard variation aregreater than that in the Greenland ice cores. However, size-volume distribution of some lowconcentration samples is abnormal. Those distributions reflect the dust deposit process in highmountain glaciers at mid-low latitudes and show differences from those in polar ice sheet.展开更多
Based on the oxygen isotope ratio and microparticle record in ice cores recovered at Mt. Muztagata, Eastern Pamirs, the seasonal variations of atmospheric dust have been reconstructed for the past four decades. High d...Based on the oxygen isotope ratio and microparticle record in ice cores recovered at Mt. Muztagata, Eastern Pamirs, the seasonal variations of atmospheric dust have been reconstructed for the past four decades. High dust concentrations and coarser particle grains have the similar trend with oxygen iso- tope value. Our statistical results indicate that 50%―60% high dust concentration samples occur dur- ing the season with high oxygen isotope values (summer), while low dust storm frequency during spring and winter. Back-trajectory analysis shows that the air mass hitting Muztagata predominately came from West Asia (such as Iran-Afghanistan Plateau) and Central Asia, which are the main dust source area for Muztagata. Dust storms in those source areas most frequently occur during summer (from May to August), while frequent dust storm events in northern China mainly occur during spring (March to May). Regions in the path of Asian dust transport, such as in Japan, the North Pacific, and Greenland, also show high dust concentrations during spring (from March to May). Our results indicate that dust storms have different seasonality in different regions within Asia.展开更多
The total activity variation with depth from a 41.6 m Muztagata ice core drilled at 7010 m, recorded not only the 1963 radioactive layer due to the thermonuclear test, but also clearly the radioactive peak released by...The total activity variation with depth from a 41.6 m Muztagata ice core drilled at 7010 m, recorded not only the 1963 radioactive layer due to the thermonuclear test, but also clearly the radioactive peak released by the Chernobyl accident in 1986. This finding indicates that the Chernobyl nuclear accident was clearly recorded in alpine glaciers in the Pamirs of west China, and the layer can be potentially used for ice core dating in other high alpine glaciers in the surrounding regions.展开更多
As a major alkaline gas in the atmosphere, ammonia (NH3) plays an important role in atmospheric chemistry. However, there is little knowledge about NH3 variations in the Central Asia. Here we ana- lyzed the ammonium (...As a major alkaline gas in the atmosphere, ammonia (NH3) plays an important role in atmospheric chemistry. However, there is little knowledge about NH3 variations in the Central Asia. Here we ana- lyzed the ammonium (NH+4) history recorded in an ice core from the East Pamir in Central Asia, which was drilled on the Mt. Muztagata at the elevation of 7010 m a.s.l. in 2003. The core was carefully dated and NH4+ concentration history during 1907―2002 was reconstructed. The result shows that NH4+ con- centration remained approximately constant until the 1930s after a sudden decrease at the very begin- ning of the 20th century, followed by a minimum in 1940 before increasing steadily to the peak at the end of 1990s. It is found that the annual mean NH4+ concentration was strongly associated with the Northern Hemisphere temperature, suggesting the impact of temperature on NH3 emissions in the Central Asia. Moreover, an increase of NH+4 concentration after 1940 also reflects the enhancement of NH3 emissions from anthropogenic sources such as fertilizer applications and livestock wastes in the 20th century.展开更多
Formate and acetate concentrations are meas- ured in a 22.56 m-depth ice core recovered in Mt. Muztagata Glacier, northwest Tibetan Plateau. The mean concentrations for formate and acetate in this ice core are 186.6...Formate and acetate concentrations are meas- ured in a 22.56 m-depth ice core recovered in Mt. Muztagata Glacier, northwest Tibetan Plateau. The mean concentrations for formate and acetate in this ice core are 186.6±160.1 and 136.4±133.9 ng/g, respectively. Study shows that there is a positive correlation between formate and nitrate, suggesting both continental origins. However, no significant relationship has been found between formate and acetate, though they both have obvious periodical variations. Because Mt. Muz- tagata lies in the mid-latitude and is correlative to the nearby human activities, formate and acetate concentrations are higher than those in Greenland and Antarctica. During re- cent decades, the increase of formate concentration in the Muztagata ice core and formaldehyde production shows a close correlation. We preliminarily presume that the high formate concentration in the Muztagata ice core is concerned with the thriving of house decoration in which excess for- maldehyde was used.展开更多
基金supported by the Chinese Academy of Sciences(Grant No.KZCX1-SW-01-10 and KZCX3-SW-339)the National Basic Research Program of China(Grant No.2005CB422004)the National Natural Science Foundation of China(Grant Nos.40471022 and 40121101).
文摘Expeditions during the summers of 2002 and 2003 implemented continuous monitoring of near-surface (2 m height) atmospheric CO2 and H2O concentrations at the 4500 m elevation on Muztagata. The resultant data sets reveal a slight decrease of CO2 concentrations (of about 5 μmol·mol?1) and changes in the diurnal variations from the end of June to the middle August. The daily maximum CO2 concentrations occur between 02:30―05:30 AM (local time) and the minimum levels occur between 12:00―15:30 PM. The atmospheric CO2 concentrations in the summer of 2002 were around 5 μmol·mol?1 lower than those during the same period of 2003, whereas the diurnal amplitude was higher. In contrast, we found that the daily mean atmospheric H2O content in 2003 was much lower than that in 2002 and there exists a striking negative correlation between CO2 and H2O con-centrations. We therefore suggest that the near-surface atmospheric CO2 concentration is affected not only by photosynthesis and respiration, but also by the air H2O content in the glaciated region around Muztagata.
基金supported by the National Natural Science Foundation of China(Grant No.40121101,40571039)the Chinese Academy of Sciences(Grant No.KZCX3-SW-339)+1 种基金the Ministry of Science and Technology of the People's Republic of China(Grant No.2005CB422004)the National Natural Science Foundation of China(Grant No.40271025).
文摘Based on summer observations of stable isotope of precipitation at Muztagata, western China, during 2002―2003, this paper presents the relationship between δ 18O in precipitation and air temperature, and discusses the effect of moisture transport on δ 18O in precipitation. Results show that air temperature correlates positively with δ 18O in precipitation, and the temperature effect controls the δ 18O of precipitation in this area. The Muztagata region exhibits high δ 18O values in summer precipi-tation, similar to those shown at stations in adjacent regions. According to the results of our model set up to trace the moisture trajectories, the westerlies and local moisture circulation contribute to varia-tions of oxygen isotopes in precipitation. In addition, the impacts of the moisture transport distance, the moisture transport level, and the incursion of the polar air mass also influence the variations of δ 18O in precipitation. The moisture origins and transport mechanisms also contribute to the variation of δ 18O in precipitation at Muztagata.
基金supported by the National Natural Science Foundation of China(Grant Nos.40121101 and 40571039)the Chinese Academy of Sciences(Grant No.KZCX3-SW-339)the Ministry of Science and Technology of the People's Republic of China(Grant No.2005CB422004).
文摘Expeditions to Muztagata (in the eastern Pamirs) during the summer seasons of2002 and 2003 collected precipitation samples and measured their oxygen isotopes. The δ^(18)O inprecipitation displays a wide range, varying from -17.40per thousand to +1.33per thousand inJune—September 2002 and from -22.31per thousand to +4.59per thousand in May—August 2003. Theδ^(18)O in precipitation correlates with the initial temperature of precipitation during theobserving periods. The positive correlation between δ^(18)O and temperature suggests that δ^(18)Ocan be used as an indicator of temperature in this region. The δ^(18)O values in fresh-snow samplescollected from two snow events at different elevations on the Muztagata Glacier show a strong''altitude effect'', with a ratio of nearly -0.40per thousand per 100 m from 5500 m to 7450 m.
基金This work was supported by the National Natural Science Foundation of China (Grant Nos. 40121101, 90102005)the Chinese Academy of Sciences (Grant No. KZCX3-SW-339)National Basic Research Program of China (Grant No. 2005CB422004).
文摘A Muztagata ice core recovered at 7010 m altitude in East Pamirs provides a Pb concentration record from 1955 to 2000. The result reveals in- creasing Pb concentrations from 1955 to 1993, with two Pb concentration peaks in 1980 and 1993. After 1993, Pb concentrations in ice core show an obvi- ously declining trend. Analysis shows that the lead in the Muztagata ice core mainly came from anthropo- genic emissions from countries in Central Asia, while the local emission had little contribution.
基金This work was supported by the National Basic Research Program of China(Grant Nos.2001CB711001 and 2005CB422004)the Collective Innovation of the the National Natural Science Foundation of China(Grant No.40121101)+1 种基金the Program of the NNSFC(Grant No.40301009)the Chinese Academy of Sciences(Grant No.KZCX3-SW-339).
文摘The dust transport and sediment characteristics are discussed based onanalysis of mi-croparticle size and size distribution in the Muztagata ice core at 6350 m a.s.I. Thefiner particles with diameter of 1—5 μm are the dominant fraction in number, while middle andcoarse particles mainly contribute to the total volume. The lognormal distribution characteristicscan be seen for some high concentration samples, showing that model size and standard variation aregreater than that in the Greenland ice cores. However, size-volume distribution of some lowconcentration samples is abnormal. Those distributions reflect the dust deposit process in highmountain glaciers at mid-low latitudes and show differences from those in polar ice sheet.
基金the National Basic Research Program (Grant No. 2005CB422004) the National Natural Science Foundation of China (Grant Nos. 40571038, 40121101 and 40301009)
文摘Based on the oxygen isotope ratio and microparticle record in ice cores recovered at Mt. Muztagata, Eastern Pamirs, the seasonal variations of atmospheric dust have been reconstructed for the past four decades. High dust concentrations and coarser particle grains have the similar trend with oxygen iso- tope value. Our statistical results indicate that 50%―60% high dust concentration samples occur dur- ing the season with high oxygen isotope values (summer), while low dust storm frequency during spring and winter. Back-trajectory analysis shows that the air mass hitting Muztagata predominately came from West Asia (such as Iran-Afghanistan Plateau) and Central Asia, which are the main dust source area for Muztagata. Dust storms in those source areas most frequently occur during summer (from May to August), while frequent dust storm events in northern China mainly occur during spring (March to May). Regions in the path of Asian dust transport, such as in Japan, the North Pacific, and Greenland, also show high dust concentrations during spring (from March to May). Our results indicate that dust storms have different seasonality in different regions within Asia.
基金Supported by the National Basic Research Program of China (Grant No. 2005CB422002)the Innovation Program of Chinese Academy of Sciences (Grant No. KZCX3-SW-339)+1 种基金the National Natural Science Foundation of China (Grant Nos. 40121101 and 40571039)the Ministry of Science and Technology of China (Grant No. 2001CCB00300)
文摘The total activity variation with depth from a 41.6 m Muztagata ice core drilled at 7010 m, recorded not only the 1963 radioactive layer due to the thermonuclear test, but also clearly the radioactive peak released by the Chernobyl accident in 1986. This finding indicates that the Chernobyl nuclear accident was clearly recorded in alpine glaciers in the Pamirs of west China, and the layer can be potentially used for ice core dating in other high alpine glaciers in the surrounding regions.
基金the National Basic Research Program of China (Grant No. 2005CB422004) the National Natural Science Foundation of China (Grant Nos. 40121101, 40571039 and 40471022)
文摘As a major alkaline gas in the atmosphere, ammonia (NH3) plays an important role in atmospheric chemistry. However, there is little knowledge about NH3 variations in the Central Asia. Here we ana- lyzed the ammonium (NH+4) history recorded in an ice core from the East Pamir in Central Asia, which was drilled on the Mt. Muztagata at the elevation of 7010 m a.s.l. in 2003. The core was carefully dated and NH4+ concentration history during 1907―2002 was reconstructed. The result shows that NH4+ con- centration remained approximately constant until the 1930s after a sudden decrease at the very begin- ning of the 20th century, followed by a minimum in 1940 before increasing steadily to the peak at the end of 1990s. It is found that the annual mean NH4+ concentration was strongly associated with the Northern Hemisphere temperature, suggesting the impact of temperature on NH3 emissions in the Central Asia. Moreover, an increase of NH+4 concentration after 1940 also reflects the enhancement of NH3 emissions from anthropogenic sources such as fertilizer applications and livestock wastes in the 20th century.
文摘Formate and acetate concentrations are meas- ured in a 22.56 m-depth ice core recovered in Mt. Muztagata Glacier, northwest Tibetan Plateau. The mean concentrations for formate and acetate in this ice core are 186.6±160.1 and 136.4±133.9 ng/g, respectively. Study shows that there is a positive correlation between formate and nitrate, suggesting both continental origins. However, no significant relationship has been found between formate and acetate, though they both have obvious periodical variations. Because Mt. Muz- tagata lies in the mid-latitude and is correlative to the nearby human activities, formate and acetate concentrations are higher than those in Greenland and Antarctica. During re- cent decades, the increase of formate concentration in the Muztagata ice core and formaldehyde production shows a close correlation. We preliminarily presume that the high formate concentration in the Muztagata ice core is concerned with the thriving of house decoration in which excess for- maldehyde was used.