The tunneling behavior of the Néel vector out of metastable easy directions or between degenerate easy directions is studied for a small single\|domain antiferromagnetic particle at low temperature. The quantum t...The tunneling behavior of the Néel vector out of metastable easy directions or between degenerate easy directions is studied for a small single\|domain antiferromagnetic particle at low temperature. The quantum tunneling rates for these processes are evaluated for two examples of macroscopic quantum tunneling and one example of macroscopic quantum coherence. The calculations are performed by using the two sublattice model and the instanton method in the spin coherent state path integral. Quantum interference or the spin parity effect is also discussed for each case.展开更多
Magnetite is an important magnetic remanence carrier in natural samples and therefore is of great interest in paleo-, rock-, and environmental magnetism. The magnetic properties of magnetite depend on many factors, e....Magnetite is an important magnetic remanence carrier in natural samples and therefore is of great interest in paleo-, rock-, and environmental magnetism. The magnetic properties of magnetite depend on many factors, e.g., concentration and grain size distribution (GSD). In this study, we theoretically investigated the temperature-dependent susceptibility (TDS) of magnetite nanoparticles with a lognormal GSD. Results show that the TDS is affected highly by the GSD mainly in three aspects. Firstly, the unblocking process becomes smoother with the increase of distribution width, characterizing as a wider Hopkinson peak on the TDS curve. Secondly, the blocking temperature increases with the increase of the median diameter or/and the distribution width. Thirdly, the maximum susceptibility decreases with the increase of distribution width, and has a logarithmic function relation with the standard deviation of the distribution. As a case study, this model was further applied to the thermal products of the Chinese loess/paleosol samples to determine the granulometry of newly-formed magnetite upon heating based on TDS curves. The results demonstrate the fidelity and feasibility of this method to determine the GSD of nano-sized magnetic particles.展开更多
文摘The tunneling behavior of the Néel vector out of metastable easy directions or between degenerate easy directions is studied for a small single\|domain antiferromagnetic particle at low temperature. The quantum tunneling rates for these processes are evaluated for two examples of macroscopic quantum tunneling and one example of macroscopic quantum coherence. The calculations are performed by using the two sublattice model and the instanton method in the spin coherent state path integral. Quantum interference or the spin parity effect is also discussed for each case.
基金supported by National Natural Science Foundation of China (Grants Nos. 40974036 and 40821091)the CAS/SAFEA International Partnership Program for Creative Research Teams
文摘Magnetite is an important magnetic remanence carrier in natural samples and therefore is of great interest in paleo-, rock-, and environmental magnetism. The magnetic properties of magnetite depend on many factors, e.g., concentration and grain size distribution (GSD). In this study, we theoretically investigated the temperature-dependent susceptibility (TDS) of magnetite nanoparticles with a lognormal GSD. Results show that the TDS is affected highly by the GSD mainly in three aspects. Firstly, the unblocking process becomes smoother with the increase of distribution width, characterizing as a wider Hopkinson peak on the TDS curve. Secondly, the blocking temperature increases with the increase of the median diameter or/and the distribution width. Thirdly, the maximum susceptibility decreases with the increase of distribution width, and has a logarithmic function relation with the standard deviation of the distribution. As a case study, this model was further applied to the thermal products of the Chinese loess/paleosol samples to determine the granulometry of newly-formed magnetite upon heating based on TDS curves. The results demonstrate the fidelity and feasibility of this method to determine the GSD of nano-sized magnetic particles.
