The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of lim...The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of limitations associated with the Na I(Tl) scintillation detector's energy resolution. This paper, based on the physical process of c photons released from decay nuclides, generating an instrument response spectrum, uses the Monte Carlo method to simulate c photons with Na I(Tl) scintillation detector interaction. The Monte Carlo response matrix is established by different single energy γ-rays with detector effects. The Gold and the improved Boosted-Gold iterative algorithms have also been used in this paper to solve the response matrix parameters through decomposing tests,such as simulating a multi-characteristic energy c-ray spectrum and simulating synthesized overlapping peaks cray spectrum. An inversion decomposition of the c instrument response spectrum for measured samples(U series, Th series and U–Th mixed sources, among others)can be achieved under the response matrix. The decomposing spectrum can be better distinguished between the similar energy characteristic peaks, which improve the error levels of activity analysis caused by the overlapping peak with significant effects.展开更多
NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution ...NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.展开更多
The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays a...The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic X-rays.The nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton electrons.Despite the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 keV.The NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma rays.Furthermore,we explored the underlying causes of the observed nonlinearity in these crystals.This study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.展开更多
In this work we calibrated the NaI(Tl) scintillation detectors (5.08 × 5.08 cm2 and 7.62 × 7.62 cm2) and the Full Energy Peak Efficiency (FEPE) for these detectors have been calculated for point sources plac...In this work we calibrated the NaI(Tl) scintillation detectors (5.08 × 5.08 cm2 and 7.62 × 7.62 cm2) and the Full Energy Peak Efficiency (FEPE) for these detectors have been calculated for point sources placed at different positions on the detector axis using the analytical approach of the effective solid angle ratio. This approach is based on the direct mathematical method reported by Selim and Abbas [1,2] and has been used successfully before to calibrate the cylindrical, parallelepiped, and 4π NaI(Tl) detectors by using point, plane and volumetric sources. In addition, the present method is free of some major inconveniences of the conventional methods.展开更多
In this paper full-energy peak (photopeak) efficiency and photopeak attenuation coefficient of 3'' × 3'' NaI(Tl) well-type scintillation detector were calculated using gamma-rayisotropic radiating...In this paper full-energy peak (photopeak) efficiency and photopeak attenuation coefficient of 3'' × 3'' NaI(Tl) well-type scintillation detector were calculated using gamma-rayisotropic radiating point sources (with photon energy: 0.245, 0.344, 0.662, 0.779, 0.964, 1.1732, 1.333 and 1.408 MeV) placed outside the detector well. These energies were obtained from <sup>152</sup>Eu, <sup>137</sup>Cs and <sup>60</sup>Co. The relations between the full energy peak efficiency and photopeak attenuation coefficients, were plotted vs. photon energy at different sources to detector distance, and it found that the full energy peak efficiency decreased by increasing the distance between the source and the detector.展开更多
基金supported by National Natural Science Foundation of China(No.11365001)National Major Scientific Equipment Development Projects(No.041514065)+1 种基金Natural Science Foundation of Jiangxi(No.20161BAB201035)Fundamental Science on Radioactive Geology and Exploration Technology Laboratory,East China Institute of Technology(No.RGET1316)
文摘The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of limitations associated with the Na I(Tl) scintillation detector's energy resolution. This paper, based on the physical process of c photons released from decay nuclides, generating an instrument response spectrum, uses the Monte Carlo method to simulate c photons with Na I(Tl) scintillation detector interaction. The Monte Carlo response matrix is established by different single energy γ-rays with detector effects. The Gold and the improved Boosted-Gold iterative algorithms have also been used in this paper to solve the response matrix parameters through decomposing tests,such as simulating a multi-characteristic energy c-ray spectrum and simulating synthesized overlapping peaks cray spectrum. An inversion decomposition of the c instrument response spectrum for measured samples(U series, Th series and U–Th mixed sources, among others)can be achieved under the response matrix. The decomposing spectrum can be better distinguished between the similar energy characteristic peaks, which improve the error levels of activity analysis caused by the overlapping peak with significant effects.
基金supported by the National Natural Science Foundation of China(Grant No.11365001)National Major Scientific Equipment Development Projects(Grant No.041514065)+2 种基金the Educational Commission of Jiangxi Province of China(Grant No.GJJ13464)Plan of Science and Technology of Jiangxi Province(Grant No.20141BBE50024)the Fundamental Science on Radioactive Geology and Exploration Technology Laboratory,East China Institute of Technology(Grant No.RGET1316)
文摘NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.
基金This work was supported by the National Key Research and Development Program(Nos.2022YFB3503600 and 2021YFA0718500)Strategic Priority Research Program of the Chinese Academy of Sciences(Nos.XDA15360102)National Natural Science Foundation of China(Nos.12273042 and 12075258).
文摘The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic X-rays.The nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton electrons.Despite the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 keV.The NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma rays.Furthermore,we explored the underlying causes of the observed nonlinearity in these crystals.This study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.
文摘In this work we calibrated the NaI(Tl) scintillation detectors (5.08 × 5.08 cm2 and 7.62 × 7.62 cm2) and the Full Energy Peak Efficiency (FEPE) for these detectors have been calculated for point sources placed at different positions on the detector axis using the analytical approach of the effective solid angle ratio. This approach is based on the direct mathematical method reported by Selim and Abbas [1,2] and has been used successfully before to calibrate the cylindrical, parallelepiped, and 4π NaI(Tl) detectors by using point, plane and volumetric sources. In addition, the present method is free of some major inconveniences of the conventional methods.
文摘In this paper full-energy peak (photopeak) efficiency and photopeak attenuation coefficient of 3'' × 3'' NaI(Tl) well-type scintillation detector were calculated using gamma-rayisotropic radiating point sources (with photon energy: 0.245, 0.344, 0.662, 0.779, 0.964, 1.1732, 1.333 and 1.408 MeV) placed outside the detector well. These energies were obtained from <sup>152</sup>Eu, <sup>137</sup>Cs and <sup>60</sup>Co. The relations between the full energy peak efficiency and photopeak attenuation coefficients, were plotted vs. photon energy at different sources to detector distance, and it found that the full energy peak efficiency decreased by increasing the distance between the source and the detector.
