Atomic structure data and effective collision strengths from literature for 1s2 2s2 2p6 3s2 3p63d10 and 34 fine-structure levels contained in the configurations 1s2 2s2 2p6 3s2 3p63d9 4l (l = s, p, d) for the nickel-l...Atomic structure data and effective collision strengths from literature for 1s2 2s2 2p6 3s2 3p63d10 and 34 fine-structure levels contained in the configurations 1s2 2s2 2p6 3s2 3p63d9 4l (l = s, p, d) for the nickel-like Au ion are used in the determination of the reduced population for these levels over a wide range of electron densities and at various electron plasma temperatures. The gain coefficient for those transitions with positive population inversion factor are determined and plotted against the electron density.展开更多
气氛环境下原位研究催化剂的烧结行为,能够为理解催化剂在预处理以及反应条件下的烧结机理和高稳定催化剂的设计提供重要的实验依据。本文以Au/CeO_(2)模型纳米催化剂为研究对象,利用环境透射电子显微镜原位观察其在O_(2)与CO气氛下的...气氛环境下原位研究催化剂的烧结行为,能够为理解催化剂在预处理以及反应条件下的烧结机理和高稳定催化剂的设计提供重要的实验依据。本文以Au/CeO_(2)模型纳米催化剂为研究对象,利用环境透射电子显微镜原位观察其在O_(2)与CO气氛下的高温动态烧结过程。实验发现,负载在CeO_(2)上的Au纳米颗粒在O_(2)与CO气氛环境中表现出不同的烧结行为,其在O_(2)气氛下具有较高的烧结速度,同时存在颗粒迁移与聚集长大(particle migration and coalescence,PMC)和奥斯特瓦尔德熟化(Ostwald ripening,OR)两种烧结过程;在CO气氛下烧结速度较慢,烧结过程以OR为主。对比不同气氛环境下烧结后催化剂的表面结构可知,CO增加了CeO_(2)表面台阶的数量以及表面氧空位浓度,增强了载体对Au颗粒的锚定作用,从而提升Au/CeO_(2)催化剂的稳定性。展开更多
For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer （several nm ...For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer （several nm depth） of silver is plated on the surface of some other materials. Furthermore, the Ni-like Ag 13.9 nm x-ray laser produced by three new kinds of two-layer target with CH, Al and Ge as foundation, was theoretically studied.展开更多
We calculate the electron impact excitation of Ni-like gold by using the Dirac R-matrix theory, and the cor- responding collision strengths and effective collision strengths are obtained. In the calculations of the le...We calculate the electron impact excitation of Ni-like gold by using the Dirac R-matrix theory, and the cor- responding collision strengths and effective collision strengths are obtained. In the calculations of the level energy, （1sZ2sZ2p6）3sZ3p63d10, 3s23p63d94/, 3s23p53d104/, and 3s3p63d104/（l = 0, 1,2,3） configurations are included and 107 fine-structure levels are generated. In the calculations of the collision strengths, only the first 59 levels are included. Com- parisons are made with the distorted wave （DW） results of Zeng et al. for both collision strengths and effective collision strengths. For the collision strengths, the two sets of calculations are in excellent agreement for most of the transitions. However, because of the inclusion of the resonances, our effective collision strengths are generally several times larger than those of Zeng et al.. The accuracy of our calculations is assessed.展开更多
文摘Atomic structure data and effective collision strengths from literature for 1s2 2s2 2p6 3s2 3p63d10 and 34 fine-structure levels contained in the configurations 1s2 2s2 2p6 3s2 3p63d9 4l (l = s, p, d) for the nickel-like Au ion are used in the determination of the reduced population for these levels over a wide range of electron densities and at various electron plasma temperatures. The gain coefficient for those transitions with positive population inversion factor are determined and plotted against the electron density.
文摘气氛环境下原位研究催化剂的烧结行为,能够为理解催化剂在预处理以及反应条件下的烧结机理和高稳定催化剂的设计提供重要的实验依据。本文以Au/CeO_(2)模型纳米催化剂为研究对象,利用环境透射电子显微镜原位观察其在O_(2)与CO气氛下的高温动态烧结过程。实验发现,负载在CeO_(2)上的Au纳米颗粒在O_(2)与CO气氛环境中表现出不同的烧结行为,其在O_(2)气氛下具有较高的烧结速度,同时存在颗粒迁移与聚集长大(particle migration and coalescence,PMC)和奥斯特瓦尔德熟化(Ostwald ripening,OR)两种烧结过程;在CO气氛下烧结速度较慢,烧结过程以OR为主。对比不同气氛环境下烧结后催化剂的表面结构可知,CO增加了CeO_(2)表面台阶的数量以及表面氧空位浓度,增强了载体对Au颗粒的锚定作用,从而提升Au/CeO_(2)催化剂的稳定性。
文摘For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer （several nm depth） of silver is plated on the surface of some other materials. Furthermore, the Ni-like Ag 13.9 nm x-ray laser produced by three new kinds of two-layer target with CH, Al and Ge as foundation, was theoretically studied.
基金supported by the National Natural Science Foundation of China(Grant Nos.11174213 and 11304266)
文摘We calculate the electron impact excitation of Ni-like gold by using the Dirac R-matrix theory, and the cor- responding collision strengths and effective collision strengths are obtained. In the calculations of the level energy, （1sZ2sZ2p6）3sZ3p63d10, 3s23p63d94/, 3s23p53d104/, and 3s3p63d104/（l = 0, 1,2,3） configurations are included and 107 fine-structure levels are generated. In the calculations of the collision strengths, only the first 59 levels are included. Com- parisons are made with the distorted wave （DW） results of Zeng et al. for both collision strengths and effective collision strengths. For the collision strengths, the two sets of calculations are in excellent agreement for most of the transitions. However, because of the inclusion of the resonances, our effective collision strengths are generally several times larger than those of Zeng et al.. The accuracy of our calculations is assessed.
