In this study,we isolated and cultured phytoplankton along the coast of China and measured the cellular carbon,nitrogen,and sulfur contents under four temperatures.The results showed that the contents of the cellular ...In this study,we isolated and cultured phytoplankton along the coast of China and measured the cellular carbon,nitrogen,and sulfur contents under four temperatures.The results showed that the contents of the cellular elements varied widely among different phytoplankton.We found that temperature is one of the important factors affecting the carbon,nitrogen,and sulfur contents in phytoplankton cells;however,the degree of influence of temperature is different for different kinds of phytoplankton.By measuring the nitrogen content in cells,we found that the C:N ratio indirectly measured in the experiment fluctuated in the range of 3.50-8.97,and the average C:N ratio was 5.52.In this experiment,we accurately measured the cell elemental contents at different temperatures and transformed the cell count results into carbon,nitrogen,and sulfur contents to express the biomass.This method ensures that the contribution of species that are small in number but with a large cell volume in biomass is considered.Moreover,this method comprehensively considers the interspecific differences of species and the uneven distribution of elements in phytoplankton cells,which is of significance in the estimation of marine carbon and nitrogen budget.The distribution of nitrogen content in marine phytoplankton can well indicate the marine eutrophication caused by human activities.Climate change can affect the community structure and element composition of marine phytoplankton,meanwhile marine carbon and nitrogen element can regulate the climate to a certain extent.展开更多
A series of nitrogen-doped SrMoO_(4) with different Sr/N mole ratio (R=0,0.05,0.10,0.15,0.20,0.40,and 0.60) were synthesized using urea as the N source via the vapor-thermal method.The photocatalytic degradation abili...A series of nitrogen-doped SrMoO_(4) with different Sr/N mole ratio (R=0,0.05,0.10,0.15,0.20,0.40,and 0.60) were synthesized using urea as the N source via the vapor-thermal method.The photocatalytic degradation ability of all samples was evaluated using methylene blue (MB) as a target contaminant.The band gaps of N-doped samples are all higher than that of pristine ones,which is only 3.12 eV.BET specific surface area S_(BET) and pore volume are increased due to the N doping.And the greater increase of S_(BET),the faster the photodegradation speed of methylene blue on SrMoO_(4).More specifically,the degradation efficiency of MB is improved up to 87%in 100 min.展开更多
为深入探讨氮沉降影响草原植物金属养分吸收及其与土壤养分的耦合关系,以内蒙古典型草原4种主要物种为研究对象,设置0、5、10、15 g N/(m^(2)·yr)4个氮添加处理,分析不同施氮量对草原物种及群落水平植物叶片盐基、微量元素含量和...为深入探讨氮沉降影响草原植物金属养分吸收及其与土壤养分的耦合关系,以内蒙古典型草原4种主要物种为研究对象,设置0、5、10、15 g N/(m^(2)·yr)4个氮添加处理,分析不同施氮量对草原物种及群落水平植物叶片盐基、微量元素含量和储量的影响。结果表明:(1)杂类草比禾本科植物具有更高的养分浓度;(2)不同金属养分对氮沉降的响应具有高度的物种特异性;植物群落叶片盐基元素含量对氮添加无显著响应且与土壤盐基离子相关性较低;随氮添加量的增加,叶片中Mn、Cu含量增加,但Fe含量降低,草原植物微量元素失衡严重主要受土壤微量养分有效性和元素拮抗作用的影响;(3)植物金属元素地上储量的饱和阈值出现在10 g N/(m^(2)·yr);优势物种地上生物量对氮添加的非线性响应是驱动植物元素地上储量变化的主要机制。展开更多
In order to evaluate interstitial strengthening effect on the properties of high entropy alloy(HEA),a nitrogen-doped Cr Mn Fe VTi6 HEA was fabricated by mechanical alloying(MA)and spark plasma sintering(SPS).XRD,SEM,T...In order to evaluate interstitial strengthening effect on the properties of high entropy alloy(HEA),a nitrogen-doped Cr Mn Fe VTi6 HEA was fabricated by mechanical alloying(MA)and spark plasma sintering(SPS).XRD,SEM,TEM and FIB were used to characterize the phase composition and microstructure of this material.The sintered bulk HEA exhibits a microstructure comprising TiNx,BCC,Laves and B2 phases.The HEA exhibits high yield strength(>2729 MPa)and hardness in lower temperature range of<380℃.Quantitative calculations of the contributions from each strengthening mechanism in the BCC phase indicate that the interstitial strengthening by nitrogen is the dominant mechanism.Nitrogen additions in the BCC phase can produce a yield strength increase of-634 MPa/at.%,which is much higher than the strengthening effects of carbon or boron additions in other alloys.This demonstrates that adding nitrogen is a viable approach for enhancing the strength of HEAs.展开更多
基金supported by the National Natural Science Foundation of China-Shandong Joint Foundation(No.U1806211)。
文摘In this study,we isolated and cultured phytoplankton along the coast of China and measured the cellular carbon,nitrogen,and sulfur contents under four temperatures.The results showed that the contents of the cellular elements varied widely among different phytoplankton.We found that temperature is one of the important factors affecting the carbon,nitrogen,and sulfur contents in phytoplankton cells;however,the degree of influence of temperature is different for different kinds of phytoplankton.By measuring the nitrogen content in cells,we found that the C:N ratio indirectly measured in the experiment fluctuated in the range of 3.50-8.97,and the average C:N ratio was 5.52.In this experiment,we accurately measured the cell elemental contents at different temperatures and transformed the cell count results into carbon,nitrogen,and sulfur contents to express the biomass.This method ensures that the contribution of species that are small in number but with a large cell volume in biomass is considered.Moreover,this method comprehensively considers the interspecific differences of species and the uneven distribution of elements in phytoplankton cells,which is of significance in the estimation of marine carbon and nitrogen budget.The distribution of nitrogen content in marine phytoplankton can well indicate the marine eutrophication caused by human activities.Climate change can affect the community structure and element composition of marine phytoplankton,meanwhile marine carbon and nitrogen element can regulate the climate to a certain extent.
基金Funded by National Key Research and Development Program of China (No.2021YFA1600203)。
文摘A series of nitrogen-doped SrMoO_(4) with different Sr/N mole ratio (R=0,0.05,0.10,0.15,0.20,0.40,and 0.60) were synthesized using urea as the N source via the vapor-thermal method.The photocatalytic degradation ability of all samples was evaluated using methylene blue (MB) as a target contaminant.The band gaps of N-doped samples are all higher than that of pristine ones,which is only 3.12 eV.BET specific surface area S_(BET) and pore volume are increased due to the N doping.And the greater increase of S_(BET),the faster the photodegradation speed of methylene blue on SrMoO_(4).More specifically,the degradation efficiency of MB is improved up to 87%in 100 min.
文摘为深入探讨氮沉降影响草原植物金属养分吸收及其与土壤养分的耦合关系,以内蒙古典型草原4种主要物种为研究对象,设置0、5、10、15 g N/(m^(2)·yr)4个氮添加处理,分析不同施氮量对草原物种及群落水平植物叶片盐基、微量元素含量和储量的影响。结果表明:(1)杂类草比禾本科植物具有更高的养分浓度;(2)不同金属养分对氮沉降的响应具有高度的物种特异性;植物群落叶片盐基元素含量对氮添加无显著响应且与土壤盐基离子相关性较低;随氮添加量的增加,叶片中Mn、Cu含量增加,但Fe含量降低,草原植物微量元素失衡严重主要受土壤微量养分有效性和元素拮抗作用的影响;(3)植物金属元素地上储量的饱和阈值出现在10 g N/(m^(2)·yr);优势物种地上生物量对氮添加的非线性响应是驱动植物元素地上储量变化的主要机制。
文摘In order to evaluate interstitial strengthening effect on the properties of high entropy alloy(HEA),a nitrogen-doped Cr Mn Fe VTi6 HEA was fabricated by mechanical alloying(MA)and spark plasma sintering(SPS).XRD,SEM,TEM and FIB were used to characterize the phase composition and microstructure of this material.The sintered bulk HEA exhibits a microstructure comprising TiNx,BCC,Laves and B2 phases.The HEA exhibits high yield strength(>2729 MPa)and hardness in lower temperature range of<380℃.Quantitative calculations of the contributions from each strengthening mechanism in the BCC phase indicate that the interstitial strengthening by nitrogen is the dominant mechanism.Nitrogen additions in the BCC phase can produce a yield strength increase of-634 MPa/at.%,which is much higher than the strengthening effects of carbon or boron additions in other alloys.This demonstrates that adding nitrogen is a viable approach for enhancing the strength of HEAs.
