[Objective] This study aimed to study on influence of rainfall runoff on non-point pollution and to reduce the pollution through control of the contamination produced from rainfall runoff. [Method] In order to explore...[Objective] This study aimed to study on influence of rainfall runoff on non-point pollution and to reduce the pollution through control of the contamination produced from rainfall runoff. [Method] In order to explore effective methods to decrease non-point pollution, we conducted analysis on hydrological process of rainfall runoff, interaction mechanism between the process and non-point pollutants, the influence on non-point pollution and hydrological model application in the research. [Result] It was proved that rainfall runoff was the main factor of non-point pollution. Control from source strengthened clearing and controlling of non-point pollutants on the ground. Growing plants in slope effectively reduced the scour and erosion of rainfall runoff on soil. The study became simple thanks for the hydrological process. [Conclusion] The research indicated that non-point pollution would be effectively reduced through control of rainfall runoff.展开更多
While non-point pollution from agriculture has become an increasingly serious problem in China, some progress has been made in studying the causal biophysical processes. However, few studies have assessed the economic...While non-point pollution from agriculture has become an increasingly serious problem in China, some progress has been made in studying the causal biophysical processes. However, few studies have assessed the economic consequences of non-point pollution in China or the policy options that could be employed to combat it. In this work a sustainable strategy to control non-point pollution from crop production, which involved taxing excessive inputs of irrigation water and fertilizer, was proposed. The approach taken to assess these measures combined biophysical and economic models,having a trade-off between economic returns and an improved environment. A proven and practical spatially referenced water and nutrient management model was used to determine the quantities of excessive irrigation water and fertilizer for specific soil and land use. Also, a set of indicators were proposed for evaluating the effects of agricultural economic output and agricultural practices on the environment.展开更多
Lake Uluabat, having an international significance and subject to the Ramsar Convention, is fed by the basin of Mustafakemalpasa Stream which runs through fertile lands utilized for livestock breeding and agriculture....Lake Uluabat, having an international significance and subject to the Ramsar Convention, is fed by the basin of Mustafakemalpasa Stream which runs through fertile lands utilized for livestock breeding and agriculture. In this study, total amount of nitrogen (TN) and phosphorus (TP) loads of non-point pollutants (agriculture, livestock breeding, vegetation, surface runoff and small settlements) was calculated. It was found out that most intensive pollution load stemmed from livestock breeding which causes dispersion of 13653.57 tons·year-1 of TN and 3224.45 tons·year-1 of TP into the Lake Uluabat. Additionally, seasonal changes in concentration of TN and TP were observed during the period of 2008-2009 in Lake Uluabat. It was concluded that the rise of agricultural activities in summer months was the reason underlying the increase in pollution during the months in question.展开更多
China is now the world’s largest producer and user of industrial fertilizers and manures. Consequently China plays a substantial role in global N cycle dynamics and in man’s disruption of the nitrogen cycle though t...China is now the world’s largest producer and user of industrial fertilizers and manures. Consequently China plays a substantial role in global N cycle dynamics and in man’s disruption of the nitrogen cycle though there are still significant uncertainties about the size and importance of emission and leaching rates. A major cause of China’s global role is the overuse of nitrogen fertilizers, which is most serious with intensive vegetable production where application rates can be up to 50% greater than crop needs, but is also a problem with wheat, rice and maize. China’s overuse of nitrogen fertiliser over the past 10-20 years has resulted in non-point source (NPS) pollution from crop production becoming a major cause of water pollution, and the situation is projected to get worse. In contrast, water pollution from point sources such as intensive livestock production and urban or industrial development is being brought more under control. The consequences for air pollution are equally serious. Emissions of nitrous oxide from fertilizers and manures may be so large that China could be responsible for 25-30% of global emissions of this damaging greenhouse gas and of the global warming resulting from it. The main national and local issues relate particularly to low fertilizer use efficiency and the losses of ammonia and NOx that lead to acid precipitation, and leaching and run-off losses that result in high nitrate levels in groundwater and eutrophication of rivers and lakes. The reasons why farmers overuse nitrogen fertilizer are complex and not fully understood. They involve agro-climate differences between provinces and counties, farming systems and farm income structures. Although there is a wide range of institutional and technological improvements that can greatly reduce this overuse rapid progress in reducing NPS is unlikely.展开更多
Non-point source (NPS) pollution is the main threat to regional water quality, and the estimation of NPS pollution load has become an important task for NPS pollution control in China. Combined with geographical inf...Non-point source (NPS) pollution is the main threat to regional water quality, and the estimation of NPS pollution load has become an important task for NPS pollution control in China. Combined with geographical information system (GIS), the long. term hydrologic impact assessment (L-THIA) model was used to evaluate the temporal.spatial changes of chemical oxygen demand (COD), total nitrogen (TN) and total phosphorus (TP) in Nansi Lake basin from 2000 to 2010. The results show: 1 ) the estimated COD, TN and TP loads in 2010 are 260017.5, 111607. 7 and 6372.0 t with the relative errors of 2.1%, 2. 0 % and - 8.8 % respectively, and more than 90% concentrated in the raining period from June to September; 2) cultivated land and construction land take up more than 80% of the whole Nansi Lake basin, and the proportions of the three kinds of NPS pollution loads coming from cultivated land and construction land are more than 98%; 3 ) during 2000- 2010, the COD, TN and TP loads increase by 8801. 6, 180.3 and 71.9 t respectively, and become the main impact factors on the water quality of Nansi Lake.展开更多
The growth of society and population has led to a range of water pollution issues.Among these,non-point source pollution assessment and treatment pose a particular challenge due to its formation mechanism.This has bec...The growth of society and population has led to a range of water pollution issues.Among these,non-point source pollution assessment and treatment pose a particular challenge due to its formation mechanism.This has become a focal point and challenge in water pollution treatment research.The study area for this research was the Huanghou basin in Guizhou Province,southwest China.The land use type of the basin was analyzed using remote sensing technology,and water quality data was collected by distributing points throughout the basin,based on source-sink landscape theory.The distribution map of the basin’s source-sink landscape and the results of water quality data accurately and efficiently identified the areas with high risk of non-point source pollution in the western and southwestern residential and agricultural areas of the upper basin.Hence,a strategy of“increasing sinks and decreasing sources”was proposed.The strategy was implemented at both macro and micro levels to address non-point source pollution in the basin using ecological remediation techniques.The work to control karst rocky desertification should continue at a macro level.The rocky desertification area in the basin should gradually transform into grassland and forested land,while increasing the overall area of the sink landscape.Ecological restoration techniques,such as slope planting,riparian zone vegetation restoration,increasing plant abundance,and restoring aquatic plants,can effectively control non-point source pollution at the micro level.Compared to traditional control methods,this remediation strategy focuses on source and process control.It is more effective and does not require large-scale water pollution control projects,which can save a lot of environmental control funds and management costs.Therefore,it has greater research significance and application value.展开更多
An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption l...An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption lidar(DIAL) and coherent-doppler lidar(CDL) techniques using a dual tunable TEA CO_(2)laser in the 9—11 μm band and a 1.55 μm fiber laser.By combining the principles of differential absorption detection and pulsed coherent detection,the system enables agile and remote sensing of atmospheric pollution.Extensive static tests validate the system’s real-time detection capabilities,including the measurement of concentration-path-length product(CL),front distance,and path wind speed of air pollution plumes over long distances exceeding 4 km.Flight experiments is conducted with the helicopter.Scanning of the pollutant concentration and the wind field is carried out in an approximately 1 km slant range over scanning angle ranges from 45°to 65°,with a radial resolution of 30 m and10 s.The test results demonstrate the system’s ability to spatially map atmospheric pollution plumes and predict their motion and dispersion patterns,thereby ensuring the protection of public safety.展开更多
Decarbonization and decontamination of the iron and steel industry(ISI),which contributes up to 15%to anthropogenic CO_(2) emissions(or carbon emissions)and significant proportions of air and water pollutant emissions...Decarbonization and decontamination of the iron and steel industry(ISI),which contributes up to 15%to anthropogenic CO_(2) emissions(or carbon emissions)and significant proportions of air and water pollutant emissions in China,are challenged by the huge demand for steel.Carbon and pollutants often share common emission sources,indicating that emission reduction could be achieved synergistically.Here,we explored the inherent potential of measures to adjust feedstock composition and technological structure and to control the size of the ISI to achieve carbon emission reduction(CER)and pollution emission reduction(PER).We investigated five typical pollutants in this study,namely,petroleum hydrocarbon pollutants and chemical oxygen demand in wastewater,particulate matter,SO_(2),and NO_(x) in off gases,and examined synergies between CER and PER by employing cross elasticity for the period between 2022 and 2035.The results suggest that a reduction of 8.7%-11.7%in carbon emissions and 20%-31%in pollution emissions(except for particulate matter emissions)could be achieved by 2025 under a high steel scrap ratio(SSR)scenario.Here,the SSR and electric arc furnace(EAF)ratio serve critical roles in enhancing synergies between CER and PER(which vary with the type of pollutant).However,subject to a limited volume of steel scrap,a focused increase in the EAF ratio with neglection of the available supply of steel scrap to EAF facilities would lead to an increase carbon and pollution emissions.Although CER can be achieved through SSR and EAF ratio optimization,only when the crude steel production growth rate remains below 2.2%can these optimization measures maintain the emissions in 2030 at a similar level to that in 2021.Therefore,the synergistic effects between PER and CER should be considered when formulating a development route for the ISI in the future.展开更多
Ensuring food safety while reducing agricultural non-point source pollution is quite challenging,especially in developing and underdeveloped countries.Effective systematic strategies and comprehensive technologies nee...Ensuring food safety while reducing agricultural non-point source pollution is quite challenging,especially in developing and underdeveloped countries.Effective systematic strategies and comprehensive technologies need to be developed for agricultural non-point source pollution control at the watershed scale to improve surface water quality.In this review,a proposal is made for a full time-space governance strategy that prioritizes source management followed by endpoint water pollution control.The 4R chain technology system is specifically reviewed,including source reduction,process retention,nutrient reuse and water restoration.The 4R chain technology system with the full time-space governance strategy was applied at the scale of an administrative village and proved to be a feasible solution for reducing agricultural non-point source pollution in China.In the future,a monitoring system needs to be established to trace N and P transport.Additionally,new smart fertilizer and intelligent equipment need to be developed,and relevant governance standards and supportive policies need to be set to enhance the efficacy of agricultural non-point source pollution control.展开更多
Fine particulate matter(PM_(2.5))and ground-level ozone(O_(3))are the primary air pollutants that degrade air quality in urban and regional areas of China.Since the implementation of the“Air Pollution Preven-tion and...Fine particulate matter(PM_(2.5))and ground-level ozone(O_(3))are the primary air pollutants that degrade air quality in urban and regional areas of China.Since the implementation of the“Air Pollution Preven-tion and Control Action Plan”in 2013,ambient concentrations of PM_(2.5)have significantly decreased across China.However,O_(3)levels exhibited an upward trend until 2019 and have since remained elevated,despite the COVID-19 pandemic.Currently,no city in China has achieved the World Health Organization’s guidelines for PM_(2.5)(24-hour mean of 15μg m^(−3)and annual mean of 5μg m^(−3))and O_(3)(8-hour mean of 100μg m^(−3)).Therefore,more rigorous measures are necessary to alleviate PM_(2.5)and O_(3)pollution in China.展开更多
Groundwater is an important source of drinking water.Groundwater pollution severely endangers drinking water safety and sustainable social development.In the case of groundwater pollution,the top priority is to identi...Groundwater is an important source of drinking water.Groundwater pollution severely endangers drinking water safety and sustainable social development.In the case of groundwater pollution,the top priority is to identify pollution sources,and accurate information on pollution sources is the premise of efficient remediation.Then,an appropriate pollution remediation scheme should be developed according to information on pollution sources,site conditions,and economic costs.The methods for identifying pollution sources mainly include geophysical exploration,geochemistry,isotopic tracing,and numerical modeling.Among these identification methods,only the numerical modeling can recognize various information on pollution sources,while other methods can only identify a certain aspect of pollution sources.The remediation technologies of groundwater can be divided into in-situ and ex-situ remediation technologies according to the remediation location.The in-situ remediation technologies enjoy low costs and a wide remediation range,but their remediation performance is prone to be affected by environmental conditions and cause secondary pollution.The ex-situ remediation technologies boast high remediation efficiency,high processing capacity,and high treatment concentration but suffer high costs.Different methods for pollution source identification and remediation technologies are applicable to different conditions.To achieve the expected identification and remediation results,it is feasible to combine several methods and technologies according to the actual hydrogeological conditions of contaminated sites and the nature of pollutants.Additionally,detailed knowledge about the hydrogeological conditions and stratigraphic structure of the contaminated site is the basis of all work regardless of the adopted identification methods or remediation technologies.展开更多
Mercury is a threatening pollutant in food,herein,we developed a Tb^(3+)-nucleic acid probe-based label-free assay for mix-and-read,rapid detection of mercury pollution.The assay utilized the feature of light-up fluor...Mercury is a threatening pollutant in food,herein,we developed a Tb^(3+)-nucleic acid probe-based label-free assay for mix-and-read,rapid detection of mercury pollution.The assay utilized the feature of light-up fluorescence of terbium ions(Tb^(3+))via binding with single-strand DNA.Mercury ion,Hg^(2+)induced thymine(T)-rich DNA strand to form a double-strand structure(T-Hg^(2+)-T),thus leading to fluorescence reduction.Based on the principle,Hg^(2+)can be quantified based on the fluorescence of Tb^(3+),the limit of detection was 0.0689μmol/L and the linear range was 0.1-6.0μmol/L.Due to the specificity of T-Hg^(2+)-T artificial base pair,the assay could distinguish Hg^(2+)from other metal ions.The recovery rate was ranged in 98.71%-101.34%for detecting mercury pollution in three food samples.The assay is low-cost,separation-free and mix-to-read,thus was a competitive tool for detection of mercury pollution to ensure food safety.展开更多
This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the w...This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the wet period and the other in the dry season. The measurements were taken using a monitor called an “Air Quality Monitor”. For data processing, the multiple comparison methods of Dun (1961) and the Wilcoxon test were used. To maintain legitimacy, all spatial data were included in the official cartographic repository of Benin: WGS 1984, Transverse Mercator Universe Projection (UTM), Zone 31 North. The Moran statistic was used to measure the levels of spatial autocorrelation of the variables studied and to test the significance. In order to locate the spatial subsets, the local spatial association indices of Anselin Local Moran and Getis-Ord, Gi* were used. In terms of results, on the 13 monitoring sites and the 8 parameters chosen to determine air quality, we do not note any significant inter-seasonal difference. Of the eight parameters, only three parameters present spatial autocorrelation leading to predictions of ambient air quality over the entire study area based on the distance separating the points, namely, PM<sub>2.5</sub>, PM<sub>10</sub> and ambient air quality index (AQI). The localities affected by atmospheric pollution in South Benin are located in the south-western part of Benin, headed by Cotonou, which is heavily polluted by CO<sub>2</sub>, TCOV, PM<sub>10</sub> and PM<sub>2.5</sub>.展开更多
To meet the growing emission of water contaminants,the development of new materials that enhance the efficiency of the water treatment system is urgent.Ordered mesoporous materials provide opportunities in environment...To meet the growing emission of water contaminants,the development of new materials that enhance the efficiency of the water treatment system is urgent.Ordered mesoporous materials provide opportunities in environmental processing applications due to their exceptionally high surface areas,large pore sizes,and enough pore volumes.These properties might enhance the performance of materials concerning adsorption/catalysis capability,durability,and stability.In this review,we enumerate the ordered mesoporous materials as adsorbents/catalysts and their modifications in water pollution treatment from the past decade,including heavy metals(Hg^(2+),Pb^(2+),Cd^(2+),Cr^(6+),etc.),toxic anions(nitrate,phosphate,fluoride,etc.),and organic contaminants(organic dyes,antibiotics,etc.).These contributions demonstrate a deep understanding of the synergistic effect between the incorporated framework and homogeneous active centers.Besides,the challenges and perspectives of the future developments of ordered mesoporous materials in wastewater treatment are proposed.This work provides a theoretical basis and complete summary for the application of ordered mesoporous materials in the removal of contaminants from aqueous solutions.展开更多
Microplastics pollution has become one of the focuses of global environmental science research.Microplastics include micro plastic particles and nano-plastic particles,which come from the decomposition of plastic prod...Microplastics pollution has become one of the focuses of global environmental science research.Microplastics include micro plastic particles and nano-plastic particles,which come from the decomposition of plastic products,the release of microfibers and the industrial process of plastic particles.The distribution of microplastics in water,soil and atmosphere is summarized,and the widespread existence of microplastics in different environmental media is emphasized.This paper also summarizes the potential impact of microplastics on ecosystems and organisms,and pays attention to the transmission and accumulation of microplastics in the food chain,as well as its potential threat to human health.Finally,the paper discusses the methods and technologies of microplastics treatment and monitoring at present,and puts forward the direction of further research on microplastics pollution in order to formulate more effective management and mitigation strategies.展开更多
The petroleum industry is a significant source of anthropogenic volatile organic compounds(VOCs),but up to now,its exact impact on urban VOCs and ozone(O_(3))remains unclear.This study conducted year-long VOC ob-serva...The petroleum industry is a significant source of anthropogenic volatile organic compounds(VOCs),but up to now,its exact impact on urban VOCs and ozone(O_(3))remains unclear.This study conducted year-long VOC ob-servations in Dongying,China,a petroleum industrial region.The VOCs from the petroleum industry(oil and gas volatilization and petrochemical production)were identified by employing the positive matrix factorization model,and their contribution to O_(3) formation was quantitatively evaluated using an observation-based chemical box model.The observed annual average concentration of VOCs was 68.6±63.5 ppbv,with a maximum daily av-erage of 335.3 ppbv.The petroleum industry accounted for 66.5%of total VOCs,contributing 54.9%from oil and gas evaporation and 11.6%from petrochemical production.Model results indicated that VOCs from the petroleum industry contributed to 31%of net O_(3) production,with 21.3%and 34.2%contributions to HO_(2)+NO and RO_(2)+NO pathways,respectively.The larger impact on the RO_(2) pathway is primarily due to the fact that OH+VOCs ac-count for 86.9%of the primary source of RO_(2).This study highlights the critical role of controlling VOCs from the petroleum industry in urban O_(3) pollution,especially those from previously overlooked low-reactivity alkanes.展开更多
In artificially controlled pot experiments,perennial ryegrass was mixed with other leguminous plants(white clo-ver and alfalfa)and treated with lead,zinc and cadmium(337 mg·kg^(-1),648 mg·kg^(-1),and 9 mg...In artificially controlled pot experiments,perennial ryegrass was mixed with other leguminous plants(white clo-ver and alfalfa)and treated with lead,zinc and cadmium(337 mg·kg^(-1),648 mg·kg^(-1),and 9 mg·kg^(-1),respectively)to simulate compound pollution conditions.The results showed that the concentrations of heavy metals,trans-port factors,and bioconcentration factors in mixed planting of ryegrass decreased compared with those in mono-culture.Regardless of whether heavy metal pollution was introduced,mixed planting increased the aboveground and underground biomasses of ryegrass.The different mixed planting treatments had no significant impact on the chlorophyll concentration of ryegrass.The mowing time,mixed planting treatment,and heavy metal treatment had impacts on antioxidant and osmotic adjustment substances,and there were some interactions.The mixed planting treatment did not significantly affect glutathione concentration,cysteine concentration,or nonprotein thiol.Mixed planting generally increased the nitrogen and phosphorus concentrations of ryegrass while reducing the stoichiometric ratio of carbon,nitrogen,and phosphorus.These results suggest that the mixed planting of ryegrass with legumes promotes the growth of ryegrass in the presence of high concentrations of heavy metal pollution.However,it does not enhance the ability of ryegrass to remediate heavy metal pollution in the soil.展开更多
This paper investigates the effect and transmission mechanism of air pollution on urbanization based on data from China’s 107 cities during 2005–2018.In order to identify the impact of air pollution on China’s urba...This paper investigates the effect and transmission mechanism of air pollution on urbanization based on data from China’s 107 cities during 2005–2018.In order to identify the impact of air pollution on China’s urbanization,we utilized night light data to represent the level of urbanization and used temperature inversion as an instrumental variable to mitigate endogeneity within the two-stage least squares framework.The results suggest that air pollution significantly slowed China’s urbanization process with economic growth acting as the transmission mechanism.The heterogeneity analyses revealed that air pollution had a greater negative impact on urbanization in northern regions than that in southern regions,and a greater negative impact in resource-oriented cities than that in non-resource-based cities.We also find that air pollution was to the detriment of urbanization in larger cities,which have more than 3 million residents,while it did not have a significant impact on Type II large cities,which have fewer than 3 million residents.展开更多
Using China’s regional input–output table,the paper constructs indicators of manufacturing servitization,matches manufacturing servitization at the regional level with city data,and uses spatial econometrics to empi...Using China’s regional input–output table,the paper constructs indicators of manufacturing servitization,matches manufacturing servitization at the regional level with city data,and uses spatial econometrics to empirically analyze the impact of manufacturing servitization on urban sulfur dioxide(SO_(2))emissions within the classical Environmental Kuznets Curve(EKC)framework.The results show that manufacturing servitization can reduce SO_(2) emissions.Producer servitization and consumptive services can both significantly reduce industrial SO_(2) emissions.Transportation and warehousing servitization,information servitization,leasing,and commercial servitization,technology research and development servitization significantly reduce SO_(2) emissions;technology research and development servitization,in particular,have the largest influence coefficient,while the reduction effect of servitization in the wholesale and retail and finance sectors is not significant.The study also found that servitization reduced the SO_(2) emissions through technological innovation and industrial structure upgrading.展开更多
Due to the transboundary nature of air pollutants,a province's efforts to improve air quality can reduce PM2.5 concentration in the surrounding area.The inter-provincial PM2.5 pollution transport could bring great...Due to the transboundary nature of air pollutants,a province's efforts to improve air quality can reduce PM2.5 concentration in the surrounding area.The inter-provincial PM2.5 pollution transport could bring great challenges to related environmental management work,such as financial fund allocation and subsidy policy formulation.Herein,we examined the transport characteristics of PM2.5 pollution across provinces in 2013 and 2020 via chemical transport modeling and then monetized inter-provincial contributions of PM2.5 improvement based on pollutant emission control costs.We found that approximately 60%of the PM2.5 pollution was from local sources,while the remaining 40%originated from outside provinces.Furthermore,about 1011 billion RMB of provincial air pollutant abatement costs contributed to the PM2.5 concentration decline in other provinces during 2013-2020,accounting for 41.2%of the total abatement costs.Provinces with lower unit improvement costs for PM2.5,such as Jiangsu,Hebei,and Shandong,were major contributors,while Guangdong,Guangxi,and Fujian,bearing higher unit costs,were among the main beneficiaries.Our study identifies provinces that contribute to air quality improvement in other provinces,have high economic efficiency,and provide a quantitative framework for determining inter-provincial compensations.This study also reveals the uneven distribution of pollution abatement costs(PM2.5 improvement/abatement costs)due to transboundary PM2.5 transport,calling for adopting inter-provincial economic compensation policies.Such mechanisms ensure equitable cost-sharing and effective regional air quality management.展开更多
基金Supported by Major Special Fund of National Technology Program of China(2008ZX07421-002,2008ZX07421-004)the National High Technology Research and Development Program of China(2008AA06A412)Project Studied and Developed by Ministry of Housing and Urban-Rural Construction(2009-K7-4)~~
文摘[Objective] This study aimed to study on influence of rainfall runoff on non-point pollution and to reduce the pollution through control of the contamination produced from rainfall runoff. [Method] In order to explore effective methods to decrease non-point pollution, we conducted analysis on hydrological process of rainfall runoff, interaction mechanism between the process and non-point pollutants, the influence on non-point pollution and hydrological model application in the research. [Result] It was proved that rainfall runoff was the main factor of non-point pollution. Control from source strengthened clearing and controlling of non-point pollutants on the ground. Growing plants in slope effectively reduced the scour and erosion of rainfall runoff on soil. The study became simple thanks for the hydrological process. [Conclusion] The research indicated that non-point pollution would be effectively reduced through control of rainfall runoff.
基金Project supported by the Canadian International Development Agency, Canada and the Chinese Academy of Sciences. China (No.KZCX2-413).
文摘While non-point pollution from agriculture has become an increasingly serious problem in China, some progress has been made in studying the causal biophysical processes. However, few studies have assessed the economic consequences of non-point pollution in China or the policy options that could be employed to combat it. In this work a sustainable strategy to control non-point pollution from crop production, which involved taxing excessive inputs of irrigation water and fertilizer, was proposed. The approach taken to assess these measures combined biophysical and economic models,having a trade-off between economic returns and an improved environment. A proven and practical spatially referenced water and nutrient management model was used to determine the quantities of excessive irrigation water and fertilizer for specific soil and land use. Also, a set of indicators were proposed for evaluating the effects of agricultural economic output and agricultural practices on the environment.
基金funded by the Environment,Atmosphere,Earth and Marine Sciences group(CAYDAG)(Project No:107Y278)of the Scientific and Technical Research Council of Turkey(TUBITAK)Scientific Research Foundation(Project No:M-2007/27)of Uludag University.
文摘Lake Uluabat, having an international significance and subject to the Ramsar Convention, is fed by the basin of Mustafakemalpasa Stream which runs through fertile lands utilized for livestock breeding and agriculture. In this study, total amount of nitrogen (TN) and phosphorus (TP) loads of non-point pollutants (agriculture, livestock breeding, vegetation, surface runoff and small settlements) was calculated. It was found out that most intensive pollution load stemmed from livestock breeding which causes dispersion of 13653.57 tons·year-1 of TN and 3224.45 tons·year-1 of TP into the Lake Uluabat. Additionally, seasonal changes in concentration of TN and TP were observed during the period of 2008-2009 in Lake Uluabat. It was concluded that the rise of agricultural activities in summer months was the reason underlying the increase in pollution during the months in question.
基金Project supported by the Canadian International Development Agency, Canada and the Chinese Academy of Sciences,China (No. KZCX2-413).
文摘China is now the world’s largest producer and user of industrial fertilizers and manures. Consequently China plays a substantial role in global N cycle dynamics and in man’s disruption of the nitrogen cycle though there are still significant uncertainties about the size and importance of emission and leaching rates. A major cause of China’s global role is the overuse of nitrogen fertilizers, which is most serious with intensive vegetable production where application rates can be up to 50% greater than crop needs, but is also a problem with wheat, rice and maize. China’s overuse of nitrogen fertiliser over the past 10-20 years has resulted in non-point source (NPS) pollution from crop production becoming a major cause of water pollution, and the situation is projected to get worse. In contrast, water pollution from point sources such as intensive livestock production and urban or industrial development is being brought more under control. The consequences for air pollution are equally serious. Emissions of nitrous oxide from fertilizers and manures may be so large that China could be responsible for 25-30% of global emissions of this damaging greenhouse gas and of the global warming resulting from it. The main national and local issues relate particularly to low fertilizer use efficiency and the losses of ammonia and NOx that lead to acid precipitation, and leaching and run-off losses that result in high nitrate levels in groundwater and eutrophication of rivers and lakes. The reasons why farmers overuse nitrogen fertilizer are complex and not fully understood. They involve agro-climate differences between provinces and counties, farming systems and farm income structures. Although there is a wide range of institutional and technological improvements that can greatly reduce this overuse rapid progress in reducing NPS is unlikely.
基金National Natural Science Foundation of China(No.41401663)Natural Science Foundation of Shandong Province,China(No.ZR2016EEM18)+1 种基金Science Foundation of Ministry of Education of China(No.12YJC790254)Excellent Young Scholars Research Fund of Shandong Normal University,China
文摘Non-point source (NPS) pollution is the main threat to regional water quality, and the estimation of NPS pollution load has become an important task for NPS pollution control in China. Combined with geographical information system (GIS), the long. term hydrologic impact assessment (L-THIA) model was used to evaluate the temporal.spatial changes of chemical oxygen demand (COD), total nitrogen (TN) and total phosphorus (TP) in Nansi Lake basin from 2000 to 2010. The results show: 1 ) the estimated COD, TN and TP loads in 2010 are 260017.5, 111607. 7 and 6372.0 t with the relative errors of 2.1%, 2. 0 % and - 8.8 % respectively, and more than 90% concentrated in the raining period from June to September; 2) cultivated land and construction land take up more than 80% of the whole Nansi Lake basin, and the proportions of the three kinds of NPS pollution loads coming from cultivated land and construction land are more than 98%; 3 ) during 2000- 2010, the COD, TN and TP loads increase by 8801. 6, 180.3 and 71.9 t respectively, and become the main impact factors on the water quality of Nansi Lake.
文摘The growth of society and population has led to a range of water pollution issues.Among these,non-point source pollution assessment and treatment pose a particular challenge due to its formation mechanism.This has become a focal point and challenge in water pollution treatment research.The study area for this research was the Huanghou basin in Guizhou Province,southwest China.The land use type of the basin was analyzed using remote sensing technology,and water quality data was collected by distributing points throughout the basin,based on source-sink landscape theory.The distribution map of the basin’s source-sink landscape and the results of water quality data accurately and efficiently identified the areas with high risk of non-point source pollution in the western and southwestern residential and agricultural areas of the upper basin.Hence,a strategy of“increasing sinks and decreasing sources”was proposed.The strategy was implemented at both macro and micro levels to address non-point source pollution in the basin using ecological remediation techniques.The work to control karst rocky desertification should continue at a macro level.The rocky desertification area in the basin should gradually transform into grassland and forested land,while increasing the overall area of the sink landscape.Ecological restoration techniques,such as slope planting,riparian zone vegetation restoration,increasing plant abundance,and restoring aquatic plants,can effectively control non-point source pollution at the micro level.Compared to traditional control methods,this remediation strategy focuses on source and process control.It is more effective and does not require large-scale water pollution control projects,which can save a lot of environmental control funds and management costs.Therefore,it has greater research significance and application value.
文摘An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption lidar(DIAL) and coherent-doppler lidar(CDL) techniques using a dual tunable TEA CO_(2)laser in the 9—11 μm band and a 1.55 μm fiber laser.By combining the principles of differential absorption detection and pulsed coherent detection,the system enables agile and remote sensing of atmospheric pollution.Extensive static tests validate the system’s real-time detection capabilities,including the measurement of concentration-path-length product(CL),front distance,and path wind speed of air pollution plumes over long distances exceeding 4 km.Flight experiments is conducted with the helicopter.Scanning of the pollutant concentration and the wind field is carried out in an approximately 1 km slant range over scanning angle ranges from 45°to 65°,with a radial resolution of 30 m and10 s.The test results demonstrate the system’s ability to spatially map atmospheric pollution plumes and predict their motion and dispersion patterns,thereby ensuring the protection of public safety.
基金supported by the National Key Research and Development Program of China(2019YFC1904800)the National Natural Science Foundation of China(72274105).
文摘Decarbonization and decontamination of the iron and steel industry(ISI),which contributes up to 15%to anthropogenic CO_(2) emissions(or carbon emissions)and significant proportions of air and water pollutant emissions in China,are challenged by the huge demand for steel.Carbon and pollutants often share common emission sources,indicating that emission reduction could be achieved synergistically.Here,we explored the inherent potential of measures to adjust feedstock composition and technological structure and to control the size of the ISI to achieve carbon emission reduction(CER)and pollution emission reduction(PER).We investigated five typical pollutants in this study,namely,petroleum hydrocarbon pollutants and chemical oxygen demand in wastewater,particulate matter,SO_(2),and NO_(x) in off gases,and examined synergies between CER and PER by employing cross elasticity for the period between 2022 and 2035.The results suggest that a reduction of 8.7%-11.7%in carbon emissions and 20%-31%in pollution emissions(except for particulate matter emissions)could be achieved by 2025 under a high steel scrap ratio(SSR)scenario.Here,the SSR and electric arc furnace(EAF)ratio serve critical roles in enhancing synergies between CER and PER(which vary with the type of pollutant).However,subject to a limited volume of steel scrap,a focused increase in the EAF ratio with neglection of the available supply of steel scrap to EAF facilities would lead to an increase carbon and pollution emissions.Although CER can be achieved through SSR and EAF ratio optimization,only when the crude steel production growth rate remains below 2.2%can these optimization measures maintain the emissions in 2030 at a similar level to that in 2021.Therefore,the synergistic effects between PER and CER should be considered when formulating a development route for the ISI in the future.
基金supported by grants from the National Key Research and Development Program of China(2021YFD1700803)Jiangsu Agriculture Science and Technology Innovation Fund,China(CX(19)1007).
文摘Ensuring food safety while reducing agricultural non-point source pollution is quite challenging,especially in developing and underdeveloped countries.Effective systematic strategies and comprehensive technologies need to be developed for agricultural non-point source pollution control at the watershed scale to improve surface water quality.In this review,a proposal is made for a full time-space governance strategy that prioritizes source management followed by endpoint water pollution control.The 4R chain technology system is specifically reviewed,including source reduction,process retention,nutrient reuse and water restoration.The 4R chain technology system with the full time-space governance strategy was applied at the scale of an administrative village and proved to be a feasible solution for reducing agricultural non-point source pollution in China.In the future,a monitoring system needs to be established to trace N and P transport.Additionally,new smart fertilizer and intelligent equipment need to be developed,and relevant governance standards and supportive policies need to be set to enhance the efficacy of agricultural non-point source pollution control.
文摘Fine particulate matter(PM_(2.5))and ground-level ozone(O_(3))are the primary air pollutants that degrade air quality in urban and regional areas of China.Since the implementation of the“Air Pollution Preven-tion and Control Action Plan”in 2013,ambient concentrations of PM_(2.5)have significantly decreased across China.However,O_(3)levels exhibited an upward trend until 2019 and have since remained elevated,despite the COVID-19 pandemic.Currently,no city in China has achieved the World Health Organization’s guidelines for PM_(2.5)(24-hour mean of 15μg m^(−3)and annual mean of 5μg m^(−3))and O_(3)(8-hour mean of 100μg m^(−3)).Therefore,more rigorous measures are necessary to alleviate PM_(2.5)and O_(3)pollution in China.
基金funded by the National Natural Science Foundation of China(41907175)the Open Fund of Key Laboratory(WSRCR-2023-01)the project of the China Geological Survey(DD20230459).
文摘Groundwater is an important source of drinking water.Groundwater pollution severely endangers drinking water safety and sustainable social development.In the case of groundwater pollution,the top priority is to identify pollution sources,and accurate information on pollution sources is the premise of efficient remediation.Then,an appropriate pollution remediation scheme should be developed according to information on pollution sources,site conditions,and economic costs.The methods for identifying pollution sources mainly include geophysical exploration,geochemistry,isotopic tracing,and numerical modeling.Among these identification methods,only the numerical modeling can recognize various information on pollution sources,while other methods can only identify a certain aspect of pollution sources.The remediation technologies of groundwater can be divided into in-situ and ex-situ remediation technologies according to the remediation location.The in-situ remediation technologies enjoy low costs and a wide remediation range,but their remediation performance is prone to be affected by environmental conditions and cause secondary pollution.The ex-situ remediation technologies boast high remediation efficiency,high processing capacity,and high treatment concentration but suffer high costs.Different methods for pollution source identification and remediation technologies are applicable to different conditions.To achieve the expected identification and remediation results,it is feasible to combine several methods and technologies according to the actual hydrogeological conditions of contaminated sites and the nature of pollutants.Additionally,detailed knowledge about the hydrogeological conditions and stratigraphic structure of the contaminated site is the basis of all work regardless of the adopted identification methods or remediation technologies.
基金financially supported by National Natural Science Foundation of China(22074100)the Young Elite Scientist Sponsorship Program by CAST(YESS20200036)+3 种基金the Researchers Supporting Project Number RSP-2021/138King Saud University,Riyadh,Saudi ArabiaTechnological Innovation R&D Project of Chengdu City(2019-YF05-31702266-SN)Sichuan University-Panzhihua City joint Project(2020CDPZH-5)。
文摘Mercury is a threatening pollutant in food,herein,we developed a Tb^(3+)-nucleic acid probe-based label-free assay for mix-and-read,rapid detection of mercury pollution.The assay utilized the feature of light-up fluorescence of terbium ions(Tb^(3+))via binding with single-strand DNA.Mercury ion,Hg^(2+)induced thymine(T)-rich DNA strand to form a double-strand structure(T-Hg^(2+)-T),thus leading to fluorescence reduction.Based on the principle,Hg^(2+)can be quantified based on the fluorescence of Tb^(3+),the limit of detection was 0.0689μmol/L and the linear range was 0.1-6.0μmol/L.Due to the specificity of T-Hg^(2+)-T artificial base pair,the assay could distinguish Hg^(2+)from other metal ions.The recovery rate was ranged in 98.71%-101.34%for detecting mercury pollution in three food samples.The assay is low-cost,separation-free and mix-to-read,thus was a competitive tool for detection of mercury pollution to ensure food safety.
文摘This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the wet period and the other in the dry season. The measurements were taken using a monitor called an “Air Quality Monitor”. For data processing, the multiple comparison methods of Dun (1961) and the Wilcoxon test were used. To maintain legitimacy, all spatial data were included in the official cartographic repository of Benin: WGS 1984, Transverse Mercator Universe Projection (UTM), Zone 31 North. The Moran statistic was used to measure the levels of spatial autocorrelation of the variables studied and to test the significance. In order to locate the spatial subsets, the local spatial association indices of Anselin Local Moran and Getis-Ord, Gi* were used. In terms of results, on the 13 monitoring sites and the 8 parameters chosen to determine air quality, we do not note any significant inter-seasonal difference. Of the eight parameters, only three parameters present spatial autocorrelation leading to predictions of ambient air quality over the entire study area based on the distance separating the points, namely, PM<sub>2.5</sub>, PM<sub>10</sub> and ambient air quality index (AQI). The localities affected by atmospheric pollution in South Benin are located in the south-western part of Benin, headed by Cotonou, which is heavily polluted by CO<sub>2</sub>, TCOV, PM<sub>10</sub> and PM<sub>2.5</sub>.
基金supported by the National Natural Science Foundation of China(52370041)National Natural Science Foundation of China(21976134 and 21707104)State Key Laboratory of Pollution treatment and Resource Reuse Foundation(NO.PCRRK21001).
文摘To meet the growing emission of water contaminants,the development of new materials that enhance the efficiency of the water treatment system is urgent.Ordered mesoporous materials provide opportunities in environmental processing applications due to their exceptionally high surface areas,large pore sizes,and enough pore volumes.These properties might enhance the performance of materials concerning adsorption/catalysis capability,durability,and stability.In this review,we enumerate the ordered mesoporous materials as adsorbents/catalysts and their modifications in water pollution treatment from the past decade,including heavy metals(Hg^(2+),Pb^(2+),Cd^(2+),Cr^(6+),etc.),toxic anions(nitrate,phosphate,fluoride,etc.),and organic contaminants(organic dyes,antibiotics,etc.).These contributions demonstrate a deep understanding of the synergistic effect between the incorporated framework and homogeneous active centers.Besides,the challenges and perspectives of the future developments of ordered mesoporous materials in wastewater treatment are proposed.This work provides a theoretical basis and complete summary for the application of ordered mesoporous materials in the removal of contaminants from aqueous solutions.
文摘Microplastics pollution has become one of the focuses of global environmental science research.Microplastics include micro plastic particles and nano-plastic particles,which come from the decomposition of plastic products,the release of microfibers and the industrial process of plastic particles.The distribution of microplastics in water,soil and atmosphere is summarized,and the widespread existence of microplastics in different environmental media is emphasized.This paper also summarizes the potential impact of microplastics on ecosystems and organisms,and pays attention to the transmission and accumulation of microplastics in the food chain,as well as its potential threat to human health.Finally,the paper discusses the methods and technologies of microplastics treatment and monitoring at present,and puts forward the direction of further research on microplastics pollution in order to formulate more effective management and mitigation strategies.
基金funded by the National Natural Science Foundation of China[grant number 42075094]the China Postdoctoral Science Foundation[grant number 2021M691921]+1 种基金the Ministry of Ecology and Environment of the People’s Republic of China[grant number DQGG202121]the Dongying Ecological and Environmental Bureau[grant number 2021DFKY-0779]。
文摘The petroleum industry is a significant source of anthropogenic volatile organic compounds(VOCs),but up to now,its exact impact on urban VOCs and ozone(O_(3))remains unclear.This study conducted year-long VOC ob-servations in Dongying,China,a petroleum industrial region.The VOCs from the petroleum industry(oil and gas volatilization and petrochemical production)were identified by employing the positive matrix factorization model,and their contribution to O_(3) formation was quantitatively evaluated using an observation-based chemical box model.The observed annual average concentration of VOCs was 68.6±63.5 ppbv,with a maximum daily av-erage of 335.3 ppbv.The petroleum industry accounted for 66.5%of total VOCs,contributing 54.9%from oil and gas evaporation and 11.6%from petrochemical production.Model results indicated that VOCs from the petroleum industry contributed to 31%of net O_(3) production,with 21.3%and 34.2%contributions to HO_(2)+NO and RO_(2)+NO pathways,respectively.The larger impact on the RO_(2) pathway is primarily due to the fact that OH+VOCs ac-count for 86.9%of the primary source of RO_(2).This study highlights the critical role of controlling VOCs from the petroleum industry in urban O_(3) pollution,especially those from previously overlooked low-reactivity alkanes.
基金funded through projects of the National Key Research and Development Program of China(2023YFD1301401)Cheng Wei received the grant.Ministry of Science and Technology of the People’s Republic of China(https://www.most.gov.cn/index.html,accessed on 19/03/2024)+1 种基金And the Guizhou Provincial Science and Technology Projects(QKHPTRC-CXTD[2022]1011)Chao Chen received the grant.Guizhou Provincial Department of Science and Technology(https://kjt.guizhou.gov.cn/,accessed on 19/03/2024).
文摘In artificially controlled pot experiments,perennial ryegrass was mixed with other leguminous plants(white clo-ver and alfalfa)and treated with lead,zinc and cadmium(337 mg·kg^(-1),648 mg·kg^(-1),and 9 mg·kg^(-1),respectively)to simulate compound pollution conditions.The results showed that the concentrations of heavy metals,trans-port factors,and bioconcentration factors in mixed planting of ryegrass decreased compared with those in mono-culture.Regardless of whether heavy metal pollution was introduced,mixed planting increased the aboveground and underground biomasses of ryegrass.The different mixed planting treatments had no significant impact on the chlorophyll concentration of ryegrass.The mowing time,mixed planting treatment,and heavy metal treatment had impacts on antioxidant and osmotic adjustment substances,and there were some interactions.The mixed planting treatment did not significantly affect glutathione concentration,cysteine concentration,or nonprotein thiol.Mixed planting generally increased the nitrogen and phosphorus concentrations of ryegrass while reducing the stoichiometric ratio of carbon,nitrogen,and phosphorus.These results suggest that the mixed planting of ryegrass with legumes promotes the growth of ryegrass in the presence of high concentrations of heavy metal pollution.However,it does not enhance the ability of ryegrass to remediate heavy metal pollution in the soil.
基金supported by Preliminary Funding Project of Hubei Provincial Department of Education[Grant No.22ZD100].
文摘This paper investigates the effect and transmission mechanism of air pollution on urbanization based on data from China’s 107 cities during 2005–2018.In order to identify the impact of air pollution on China’s urbanization,we utilized night light data to represent the level of urbanization and used temperature inversion as an instrumental variable to mitigate endogeneity within the two-stage least squares framework.The results suggest that air pollution significantly slowed China’s urbanization process with economic growth acting as the transmission mechanism.The heterogeneity analyses revealed that air pollution had a greater negative impact on urbanization in northern regions than that in southern regions,and a greater negative impact in resource-oriented cities than that in non-resource-based cities.We also find that air pollution was to the detriment of urbanization in larger cities,which have more than 3 million residents,while it did not have a significant impact on Type II large cities,which have fewer than 3 million residents.
基金funded by the National Social Science Foundation of China[Grant No.23CGJ011 and Grant No.22BGJ029]National Natural Science Foundation of China[Grant No.72263015]Science and Technology Youth Project of the Jiangxi Provincial Department of Education[Grant No.GJJ200530].
文摘Using China’s regional input–output table,the paper constructs indicators of manufacturing servitization,matches manufacturing servitization at the regional level with city data,and uses spatial econometrics to empirically analyze the impact of manufacturing servitization on urban sulfur dioxide(SO_(2))emissions within the classical Environmental Kuznets Curve(EKC)framework.The results show that manufacturing servitization can reduce SO_(2) emissions.Producer servitization and consumptive services can both significantly reduce industrial SO_(2) emissions.Transportation and warehousing servitization,information servitization,leasing,and commercial servitization,technology research and development servitization significantly reduce SO_(2) emissions;technology research and development servitization,in particular,have the largest influence coefficient,while the reduction effect of servitization in the wholesale and retail and finance sectors is not significant.The study also found that servitization reduced the SO_(2) emissions through technological innovation and industrial structure upgrading.
基金National Natural Science Foundation of China under Grant No.72171157 and 72140005.
文摘Due to the transboundary nature of air pollutants,a province's efforts to improve air quality can reduce PM2.5 concentration in the surrounding area.The inter-provincial PM2.5 pollution transport could bring great challenges to related environmental management work,such as financial fund allocation and subsidy policy formulation.Herein,we examined the transport characteristics of PM2.5 pollution across provinces in 2013 and 2020 via chemical transport modeling and then monetized inter-provincial contributions of PM2.5 improvement based on pollutant emission control costs.We found that approximately 60%of the PM2.5 pollution was from local sources,while the remaining 40%originated from outside provinces.Furthermore,about 1011 billion RMB of provincial air pollutant abatement costs contributed to the PM2.5 concentration decline in other provinces during 2013-2020,accounting for 41.2%of the total abatement costs.Provinces with lower unit improvement costs for PM2.5,such as Jiangsu,Hebei,and Shandong,were major contributors,while Guangdong,Guangxi,and Fujian,bearing higher unit costs,were among the main beneficiaries.Our study identifies provinces that contribute to air quality improvement in other provinces,have high economic efficiency,and provide a quantitative framework for determining inter-provincial compensations.This study also reveals the uneven distribution of pollution abatement costs(PM2.5 improvement/abatement costs)due to transboundary PM2.5 transport,calling for adopting inter-provincial economic compensation policies.Such mechanisms ensure equitable cost-sharing and effective regional air quality management.