The internal flow of a droplet in the nonlinear extensional flow field will exhibit more than two internal circulations with the variation of nonlinear intensity(E).In this paper,the effect of positions and sizes of i...The internal flow of a droplet in the nonlinear extensional flow field will exhibit more than two internal circulations with the variation of nonlinear intensity(E).In this paper,the effect of positions and sizes of internal circulations on internal mass transfer rate of a single spherical droplet in a nonlinear extensional flow field is studied and compared with that in a linear extensional flow field.The simulation results show that when E≥0,there are two symmetrical internal circulations in the droplet,which is the same with that in a linear extensional flow.The limit value of mass transfer rate Sh is 15,which is equal to that in a linear extensional flow,no matter how large E is.When E≤-3/7,the number of internal flow circulation of a droplet increase to four and the transfer rate Sh increases.When E=-1,the maximum internal transfer rate Sh equals 30 which is twice of that in a linear extensional flow.The generation of new flow circulations in droplets and the circulation positions will enhance mass transfer when E≤-3/7,which provides a new idea for enhancing the internal mass transfer rate of droplets.展开更多
This work systematically simulates the external mass transfer from/to a spherical drop and solid particle suspended in a nonlinear uniaxial extensional creeping flow.The mass transfer problem is governed by three dime...This work systematically simulates the external mass transfer from/to a spherical drop and solid particle suspended in a nonlinear uniaxial extensional creeping flow.The mass transfer problem is governed by three dimensionless parameters:the viscosity ratio(λ),the Peclet number(Pe),and the nonlinear intensity of the flow(E).The existing mass transfer theory,valid for very large Peclet numbers only,is expanded,by numerical simulations,to include a much larger range of Peclet numbers(1≤Pe≤105).The simulation results show that the dimensionless mass transfer rate,expressed as the Sherwood number(5 h),agrees well with the theoretical results at the convection-dominated regime(Pe>103).Only when E>5/4,the simulated Sh for a solid sphere in the nonlinear uniaxial extensional flow is larger than theoretical results because the theory neglects the effect of the vortex formed outside the particle on the rate of mass transfer.Empirical correlations are proposed to predict the influence of the dimensionless governing parameters(λ,Pe,E)on the Sherwood number(Sh).The maximum deviations of all empirical correlations are less than 15%when compared to the numerical simulated results.展开更多
Distributed Lagrange Multiplier/Fictitious Domain (DLM/FD) method was employed to simulate the channel flow with polymer suspension. The polymer molecules were modeled as Finitely Extensible Nonlinear Elastic (FENE...Distributed Lagrange Multiplier/Fictitious Domain (DLM/FD) method was employed to simulate the channel flow with polymer suspension. The polymer molecules were modeled as Finitely Extensible Nonlinear Elastic (FENE) chains and FENE chain cluster. The coiled stretched transition of FENE chains was examined and the change in configuration of FENE chains was presented. The average velocity profile of the fully developed channel flow with 64 FENE chains was given and fitted well with the power-law curve. The change of chain cluster configuration was also simulated. These simulations show that DLM/FD method is capable of simulating the motion of not only FENE chain, but also FENE chain cluster.展开更多
基金supported by the National Key Research and Development Program of China(2021YFC2902502)the National Natural Science Foundation of China(22078320,22035007)+4 种基金the NSFC-EU project(31961133018)the Shandong Provincial Key Research and Development Program(2022CXGC020106)the Shandong Key Research and Development Program(International Cooperation Office)(2019GHZ018)the Shandong Province Postdoctoral Innovative Talents Support Plan(SDBX2020018)the External Cooperation Program of BIC,Chinese Academy of Sciences(122111KYSB20190032)。
文摘The internal flow of a droplet in the nonlinear extensional flow field will exhibit more than two internal circulations with the variation of nonlinear intensity(E).In this paper,the effect of positions and sizes of internal circulations on internal mass transfer rate of a single spherical droplet in a nonlinear extensional flow field is studied and compared with that in a linear extensional flow field.The simulation results show that when E≥0,there are two symmetrical internal circulations in the droplet,which is the same with that in a linear extensional flow.The limit value of mass transfer rate Sh is 15,which is equal to that in a linear extensional flow,no matter how large E is.When E≤-3/7,the number of internal flow circulation of a droplet increase to four and the transfer rate Sh increases.When E=-1,the maximum internal transfer rate Sh equals 30 which is twice of that in a linear extensional flow.The generation of new flow circulations in droplets and the circulation positions will enhance mass transfer when E≤-3/7,which provides a new idea for enhancing the internal mass transfer rate of droplets.
基金support and helpful insight.This work was supported by the National Key Research and Development Program(2021YFC2902502)the National Natu-ral Science Foundation of China(21938009,91934301,22078320)+5 种基金the Major Scientific and Technological Innovation Projects in Shan-dong Province(2019JZZY010302)the Shandong Key Research and Development Program(International Cooperation Office)(2019GHZ018)the Shandong Province Postdoctoral Innovative Talents Support Plan(SDBX2020018)the External Cooperation Program of BIC,Chinese Academy of Sciences(122111KYSB20190032)Chemistry and Chemical Engineering Guangdong Laboratory(1922006)GHfund B(202107021062).
文摘This work systematically simulates the external mass transfer from/to a spherical drop and solid particle suspended in a nonlinear uniaxial extensional creeping flow.The mass transfer problem is governed by three dimensionless parameters:the viscosity ratio(λ),the Peclet number(Pe),and the nonlinear intensity of the flow(E).The existing mass transfer theory,valid for very large Peclet numbers only,is expanded,by numerical simulations,to include a much larger range of Peclet numbers(1≤Pe≤105).The simulation results show that the dimensionless mass transfer rate,expressed as the Sherwood number(5 h),agrees well with the theoretical results at the convection-dominated regime(Pe>103).Only when E>5/4,the simulated Sh for a solid sphere in the nonlinear uniaxial extensional flow is larger than theoretical results because the theory neglects the effect of the vortex formed outside the particle on the rate of mass transfer.Empirical correlations are proposed to predict the influence of the dimensionless governing parameters(λ,Pe,E)on the Sherwood number(Sh).The maximum deviations of all empirical correlations are less than 15%when compared to the numerical simulated results.
文摘Distributed Lagrange Multiplier/Fictitious Domain (DLM/FD) method was employed to simulate the channel flow with polymer suspension. The polymer molecules were modeled as Finitely Extensible Nonlinear Elastic (FENE) chains and FENE chain cluster. The coiled stretched transition of FENE chains was examined and the change in configuration of FENE chains was presented. The average velocity profile of the fully developed channel flow with 64 FENE chains was given and fitted well with the power-law curve. The change of chain cluster configuration was also simulated. These simulations show that DLM/FD method is capable of simulating the motion of not only FENE chain, but also FENE chain cluster.