A convolutional neural network is employed to retrieve the time-domain envelop and phase of few-cycle femtosecond pulses from transient-grating frequency-resolved optical gating(TG-FROG) traces.We use theoretically ge...A convolutional neural network is employed to retrieve the time-domain envelop and phase of few-cycle femtosecond pulses from transient-grating frequency-resolved optical gating(TG-FROG) traces.We use theoretically generated TGFROG traces to complete supervised trainings of the convolutional neural networks,then use similarly generated traces not included in the training dataset to test how well the networks are trained.Accurate retrieval of such traces by the neural network is realized.In our case,we find that networks with exponential linear unit(ELU) activation function perform better than those with leaky rectified linear unit(LRELU) and scaled exponential linear unit(SELU).Finally,the issues that need to be addressed for the retrieval of experimental data by this method are discussed.展开更多
The carrier-density-dependent spin relaxation dynamics for modulation-doped GaAs/Al0.3 Gao,TAs quantum wells is studied using the time-resolved magneto-Kerr rotation measurements. The electron spin relaxation time and...The carrier-density-dependent spin relaxation dynamics for modulation-doped GaAs/Al0.3 Gao,TAs quantum wells is studied using the time-resolved magneto-Kerr rotation measurements. The electron spin relaxation time and its in-plane anisotropy are studied as a function of the optically injected electron density, Moreover, the relative strength of the Rashba and the Dresselhaus spin-rbit coupling fields, and thus the observed spin relaxation time anisotropy, is further tuned by the additional excitation of a 532nm continuous wave laser, demonstrating an effective spin relaxation manipulation via an optical gating method.展开更多
Both polarization gating (PG) and double optical gating (DOG) are productive methods to generate single attosecond (as) pulses. In this paper, considering the ground-state depletion effect, we investigate the wa...Both polarization gating (PG) and double optical gating (DOG) are productive methods to generate single attosecond (as) pulses. In this paper, considering the ground-state depletion effect, we investigate the wavelength-dependence of the DOG method in order to optimize the generation of single attosecond pulses for the future application. By calculating the ionization probabilities of the leading edge of the pulse at different driving laser wavelengths, we obtain the upper limit of duration for the driving laser pulse for the DOG setup. We find that the upper limit duration increases with the increase of laser wavelength. We further describe the technical method of choosing and calculating the thickness values of optical components for the DOG setup.展开更多
This study proposes a novel scheme of a cross- correlation frequency-resolved optical gating (X-FROG) measurement for an optical based on the sum frequency arbitrary waveform (OAW) generation (SFG) effect of a p...This study proposes a novel scheme of a cross- correlation frequency-resolved optical gating (X-FROG) measurement for an optical based on the sum frequency arbitrary waveform (OAW) generation (SFG) effect of a periodically poled lithium niobate (PPLN) waveguide. Based on the SFG effect and combined with the principal component generalized projects algorithm on a matrix, the theory model of the scheme is established. Using Matlab, the proposed OAW measurement X-FROG scheme using the PPLN waveguide is simulated and studied. Simulation results show that a rectangular pulse is a suitable gate pulse because of its low errors. Moreover, the increased complexity of OAW and phase mismatch decrease measurement accuracy.展开更多
Optical microscopy has become an indispensable tool for visualizing sub-cellular structures andbiological processes.However,scattering in biological tissues is a major obstacle that preventshigh-resolution images from...Optical microscopy has become an indispensable tool for visualizing sub-cellular structures andbiological processes.However,scattering in biological tissues is a major obstacle that preventshigh-resolution images from being obtained from deep regions of tissue.We review commontechniques,such as multiphoton microscopy(MPM)and optical coherence microscopy(OCM),for diffraction limited imaging beyond an imaging depth of 0.5 mm.Novel implementations havebeen emerging in recent years giving higher imaging speed,deeper penetration,and better imagequality.Focal modulation microscopy(FMM)is a novel method that combines confocal spatialfltering with focal modulation to reject out-of-focus background.FMM has demonstrated animaging depth comparable to those of MPM and OCM,near-real-time image acquisition,and thecapability for multiple contrast mechanisms.展开更多
A femtosecond optical Kerr gate time-gated ballistic imaging method is demonstrated to image a transparent object in a turbid medium. The shape features of the object are obtained by time-resolved selection of the bal...A femtosecond optical Kerr gate time-gated ballistic imaging method is demonstrated to image a transparent object in a turbid medium. The shape features of the object are obtained by time-resolved selection of the ballistic photons with different optical path lengths, the thickness distribution of the object is mapped, and the maximum is less than 3.6%. This time-resolved ballistic imaging has potential applications in studying properties of the liquid core in the near field of the fuel spray.展开更多
We propose a simple all-optical diode which is comprised of an asymmetric ring cavity containing a two-level atomic ensemble. Attributed to spatial symmetry breaking of the ring cavity, direction-dependent optical bis...We propose a simple all-optical diode which is comprised of an asymmetric ring cavity containing a two-level atomic ensemble. Attributed to spatial symmetry breaking of the ring cavity, direction-dependent optical bistability is obtained in a classical bistable system. Therefore, a giant optical non-reciprocity is generated, which guarantees an all-optical diode with a high contrast up to 22 d B. Furthermore, its application as an all-optical logic AND gate is also discussed.展开更多
This paper describes the generation of shaped femtosecond multiple pulses by using the phase-only Dammann filters in 4f femtosecond shaper and gives the experimental result of femtosecond pulse characterization by the...This paper describes the generation of shaped femtosecond multiple pulses by using the phase-only Dammann filters in 4f femtosecond shaper and gives the experimental result of femtosecond pulse characterization by the frequency- resolved optical gating (FROG) technique. With the theoretical simulation, it concludes that the quality of the generated output array is relevant to the number of pixels and the spacing between the components.展开更多
Photonic crystal based ring resonators are best choice for designing all-optical devices. In this paper, we used a basic structure of photonic crystal ring resonators and designed all optical logic gates which are wor...Photonic crystal based ring resonators are best choice for designing all-optical devices. In this paper, we used a basic structure of photonic crystal ring resonators and designed all optical logic gates which are working using the Kerr effect. The proposed gates consisted of upper and lower wavegnides coupled through a resonator which was designed for dropping of special wavelength. The resonance wavelength was designed for 1550 nm telecom operation wavelength. We used numerical meth- ods such as plane wave expansion and finite difference time domain (FDTD) for performing our simulations and studied the optical properties of the proposed structures. Our results showed that the critical input power for triggering the gate output was lower compared to previously reported gates.展开更多
Atomically-precise clusterzymes have been widely studied for their special physicochemical properties,but it is still a challenge to enhance their peroxidase-like activity.Herein,we demonstrated that by substituting a...Atomically-precise clusterzymes have been widely studied for their special physicochemical properties,but it is still a challenge to enhance their peroxidase-like activity.Herein,we demonstrated that by substituting a single Ag atom into Au25 nanoclusters to form Au_(24)Ag_(1) nanoclusters,the peroxidase-like activity was enhanced greatly.In the presence of H_(2)O_(2),Au_(24)Ag_(1) could produce reactive oxygen species(ROS)to oxidize colorless 3,3'5,5'-tetramethylbenzidine(TMB)to the blue oxidized TMB(oxTMB).It is worth mentioning that pyrophosphate compounds inhibit the activity of Au_(24)Ag_(1).Since alkaline phosphatase(ALP)can dephosphorylate the substrate phosphate compound,that is,remove the phosphate group on the substrate by hydrolysis,the enzymatic activity of the clusterzyme is restored.Based on this,we have developed a sensitive and reliable colorimetric sensing system for the detection of pyrophosphate ion(PPi),adenosine triphosphate(ATP),adenosine diphosphate(ADP)and ALP,respectively.Importantly,the detection limit of the assay system is lower than those of most of the assays that have been reported.In addition,we also built a simple optical logic gate on this basis,further extending the application of metal nanoclusters as peroxidase mimics in bioanalysis.This work could help to shed light on the structure-activity relationship of nanozyme.展开更多
Spatio-temporal imaging of light propagation is very important in photonics because it provides the most direct tool available to study the interaction between light and its host environment.Sub-ps time resolution is ...Spatio-temporal imaging of light propagation is very important in photonics because it provides the most direct tool available to study the interaction between light and its host environment.Sub-ps time resolution is needed to investigate the fine and complex structural features that characterize disordered and heterogeneous structures,which are responsible for a rich array of transport physics that have not yet been fully explored.A newly developed wide-field imaging system enables us to present a spatiotemporal study on light transport in various disordered media,revealing properties that could not be properly assessed using standard techniques.By extending our investigation to an almost transparent membrane,a configuration that has been difficult to characterize until now,we unveil the peculiar physics exhibited by such thin scattering systems with transport features that go beyond mainstream diffusion modeling,despite the occurrence of multiple scattering.展开更多
基金Project supported by the National Key R&D Program of China(Grant No.2017YFB0405202)the National Natural Science Foundation of China(Grant Nos.61690221,91850209,and 11774277)。
文摘A convolutional neural network is employed to retrieve the time-domain envelop and phase of few-cycle femtosecond pulses from transient-grating frequency-resolved optical gating(TG-FROG) traces.We use theoretically generated TGFROG traces to complete supervised trainings of the convolutional neural networks,then use similarly generated traces not included in the training dataset to test how well the networks are trained.Accurate retrieval of such traces by the neural network is realized.In our case,we find that networks with exponential linear unit(ELU) activation function perform better than those with leaky rectified linear unit(LRELU) and scaled exponential linear unit(SELU).Finally,the issues that need to be addressed for the retrieval of experimental data by this method are discussed.
基金Supported by the National Natural Science Foundation Program of China under Grant Nos 11274302,11474276 and 61290303
文摘The carrier-density-dependent spin relaxation dynamics for modulation-doped GaAs/Al0.3 Gao,TAs quantum wells is studied using the time-resolved magneto-Kerr rotation measurements. The electron spin relaxation time and its in-plane anisotropy are studied as a function of the optically injected electron density, Moreover, the relative strength of the Rashba and the Dresselhaus spin-rbit coupling fields, and thus the observed spin relaxation time anisotropy, is further tuned by the additional excitation of a 532nm continuous wave laser, demonstrating an effective spin relaxation manipulation via an optical gating method.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11125416,and 11121091)the National Basic Research Program of China(Grant No.2013CB922403)
文摘Both polarization gating (PG) and double optical gating (DOG) are productive methods to generate single attosecond (as) pulses. In this paper, considering the ground-state depletion effect, we investigate the wavelength-dependence of the DOG method in order to optimize the generation of single attosecond pulses for the future application. By calculating the ionization probabilities of the leading edge of the pulse at different driving laser wavelengths, we obtain the upper limit of duration for the driving laser pulse for the DOG setup. We find that the upper limit duration increases with the increase of laser wavelength. We further describe the technical method of choosing and calculating the thickness values of optical components for the DOG setup.
文摘This study proposes a novel scheme of a cross- correlation frequency-resolved optical gating (X-FROG) measurement for an optical based on the sum frequency arbitrary waveform (OAW) generation (SFG) effect of a periodically poled lithium niobate (PPLN) waveguide. Based on the SFG effect and combined with the principal component generalized projects algorithm on a matrix, the theory model of the scheme is established. Using Matlab, the proposed OAW measurement X-FROG scheme using the PPLN waveguide is simulated and studied. Simulation results show that a rectangular pulse is a suitable gate pulse because of its low errors. Moreover, the increased complexity of OAW and phase mismatch decrease measurement accuracy.
文摘Optical microscopy has become an indispensable tool for visualizing sub-cellular structures andbiological processes.However,scattering in biological tissues is a major obstacle that preventshigh-resolution images from being obtained from deep regions of tissue.We review commontechniques,such as multiphoton microscopy(MPM)and optical coherence microscopy(OCM),for diffraction limited imaging beyond an imaging depth of 0.5 mm.Novel implementations havebeen emerging in recent years giving higher imaging speed,deeper penetration,and better imagequality.Focal modulation microscopy(FMM)is a novel method that combines confocal spatialfltering with focal modulation to reject out-of-focus background.FMM has demonstrated animaging depth comparable to those of MPM and OCM,near-real-time image acquisition,and thecapability for multiple contrast mechanisms.
基金Supported by the National Natural Science Foundation of China under Grant Nos 61427816 and 61690221the Collaborative Innovation Center of Suzhou Nano Science and Technology
文摘A femtosecond optical Kerr gate time-gated ballistic imaging method is demonstrated to image a transparent object in a turbid medium. The shape features of the object are obtained by time-resolved selection of the ballistic photons with different optical path lengths, the thickness distribution of the object is mapped, and the maximum is less than 3.6%. This time-resolved ballistic imaging has potential applications in studying properties of the liquid core in the near field of the fuel spray.
基金supported by the National Natural Science Foundation of China(Grant Nos.11274242,11474221,and 11574229)the Joint Fund of the National Natural Science Foundation of China and the China Academy of Engineering Physics(Grant No.U1330203)the National Key Basic Research Special Foundation of China(Grant Nos.2011CB922203 and 2013CB632701)
文摘We propose a simple all-optical diode which is comprised of an asymmetric ring cavity containing a two-level atomic ensemble. Attributed to spatial symmetry breaking of the ring cavity, direction-dependent optical bistability is obtained in a classical bistable system. Therefore, a giant optical non-reciprocity is generated, which guarantees an all-optical diode with a high contrast up to 22 d B. Furthermore, its application as an all-optical logic AND gate is also discussed.
文摘This paper describes the generation of shaped femtosecond multiple pulses by using the phase-only Dammann filters in 4f femtosecond shaper and gives the experimental result of femtosecond pulse characterization by the frequency- resolved optical gating (FROG) technique. With the theoretical simulation, it concludes that the quality of the generated output array is relevant to the number of pixels and the spacing between the components.
文摘Photonic crystal based ring resonators are best choice for designing all-optical devices. In this paper, we used a basic structure of photonic crystal ring resonators and designed all optical logic gates which are working using the Kerr effect. The proposed gates consisted of upper and lower wavegnides coupled through a resonator which was designed for dropping of special wavelength. The resonance wavelength was designed for 1550 nm telecom operation wavelength. We used numerical meth- ods such as plane wave expansion and finite difference time domain (FDTD) for performing our simulations and studied the optical properties of the proposed structures. Our results showed that the critical input power for triggering the gate output was lower compared to previously reported gates.
基金supported by the National Natural Science Foundation of China(Nos.22172063 and 32202145)the Fund of Young Taishan Scholar Program,China(No.tsqn201812080)+1 种基金the Natural Science Foundation of Shandong Province,China(No.ZR2019YQ10)the Independent Cultivation Program of Innovation Team of Ji’nan City,China(No.2021GXRC052).
文摘Atomically-precise clusterzymes have been widely studied for their special physicochemical properties,but it is still a challenge to enhance their peroxidase-like activity.Herein,we demonstrated that by substituting a single Ag atom into Au25 nanoclusters to form Au_(24)Ag_(1) nanoclusters,the peroxidase-like activity was enhanced greatly.In the presence of H_(2)O_(2),Au_(24)Ag_(1) could produce reactive oxygen species(ROS)to oxidize colorless 3,3'5,5'-tetramethylbenzidine(TMB)to the blue oxidized TMB(oxTMB).It is worth mentioning that pyrophosphate compounds inhibit the activity of Au_(24)Ag_(1).Since alkaline phosphatase(ALP)can dephosphorylate the substrate phosphate compound,that is,remove the phosphate group on the substrate by hydrolysis,the enzymatic activity of the clusterzyme is restored.Based on this,we have developed a sensitive and reliable colorimetric sensing system for the detection of pyrophosphate ion(PPi),adenosine triphosphate(ATP),adenosine diphosphate(ADP)and ALP,respectively.Importantly,the detection limit of the assay system is lower than those of most of the assays that have been reported.In addition,we also built a simple optical logic gate on this basis,further extending the application of metal nanoclusters as peroxidase mimics in bioanalysis.This work could help to shed light on the structure-activity relationship of nanozyme.
基金supported by the European Network of Excellence Nanophotonics for Energy Efficiency and the ERC through the Advanced Grant PhotBots(Proj.Ref.291349).
文摘Spatio-temporal imaging of light propagation is very important in photonics because it provides the most direct tool available to study the interaction between light and its host environment.Sub-ps time resolution is needed to investigate the fine and complex structural features that characterize disordered and heterogeneous structures,which are responsible for a rich array of transport physics that have not yet been fully explored.A newly developed wide-field imaging system enables us to present a spatiotemporal study on light transport in various disordered media,revealing properties that could not be properly assessed using standard techniques.By extending our investigation to an almost transparent membrane,a configuration that has been difficult to characterize until now,we unveil the peculiar physics exhibited by such thin scattering systems with transport features that go beyond mainstream diffusion modeling,despite the occurrence of multiple scattering.