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Realizing mode conversion and optical diode effect by coupling photonic crystal waveguides with cavity 被引量:2
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作者 叶寒 张金倩楠 +2 位作者 俞重远 王东林 陈智辉 《Chinese Physics B》 SCIE EI CAS CSCD 2015年第9期284-288,共5页
We propose a novel two-dimensional photonic crystal structure consisting of two line defect waveguides and a cavity to realize mode conversion based on the coupling effect. The W1/cavity/W2 structure breaks the spatia... We propose a novel two-dimensional photonic crystal structure consisting of two line defect waveguides and a cavity to realize mode conversion based on the coupling effect. The W1/cavity/W2 structure breaks the spatial symmetry and successfully converts the even(odd) mode to the odd(even) mode in the W2 waveguide during the forward(backward)transmission. When considering the incidence of only the even mode, the optical diode effect emerges and achieves approximate 35 d B unidirectionality at the resonant frequency. Moreover, owing to the narrow bandpass feature and the flexibility of the tuning cavity, utilization of the proposed structure as a wavelength filter is demonstrated in a device with a Y-branch splitter. Here, we provide a heuristic design for a mode converter, optical diode, and wavelength filter derived from the coupling effect between a cavity and adjacent waveguides, and expect that the proposed structure can be applied as a building block in future all-optical integrated circuits. 展开更多
关键词 mode conversion optical diode photonic crystal
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Bias-Free Solar-to-Hydrogen Conversion in a BiVO_(4)/PM6:Y6 Compact Tandem with Optically Balanced Light Absorption
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作者 Catarina G.Ferreira Constanza Sansierra +3 位作者 Francisco Bernal-Texca Mingyu Zhang Carles Ros Jordi Martorell 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第4期231-238,共8页
The high voltage required to overcome the thermodynamic threshold and the complicated kinetics of the water splitting reaction limit the efficiency of single semiconductor-based photoelectrochemistry.A semiconductor/s... The high voltage required to overcome the thermodynamic threshold and the complicated kinetics of the water splitting reaction limit the efficiency of single semiconductor-based photoelectrochemistry.A semiconductor/solar cell tandem structure has been theoretically demonstrated as a viable path to achieve an efficient direct transformation of sunlight into chemical energy.However,compact designs exhibiting the indispensable optimally balanced light absorption have not been demonstrated.In the current work,we design and implement a compact tandem providing the complementary absorption of a highly transparent BiVO_(4)photoanode and a PM6:Y6 solar cell.Such bandgap combination approaches the optimal to reach the solar-to-hydrogen(STH)conversion upper limit for tandem photoelectrochemical cells(PECs).We demonstrate that,by using a photonic multilayer structure to adequately balance sunlight absorption among both tandem materials,a 25%increase in the bias-free STH conversion can be achieved,setting a clear path to take compact tandem PECs to the theoretical limit performance. 展开更多
关键词 bismuth vanadate compact tandem organic solar cells photonic multilayers solar-to-hydrogen conversion
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Quantum frequency down-conversion of single photons at 1552 nm from single InAs quantum dot 被引量:2
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作者 Ben Ma Si-Hang Wei +3 位作者 Ze-Sheng Chen Xiang-Jun Shang Hai-Qiao Ni Zhi-Chuan Niu 《Chinese Physics B》 SCIE EI CAS CSCD 2018年第9期595-599,共5页
Near-infrared single photon sources in telecommunication bands, especially at 1550 nm, are required for long-distance quantum communication. Here a down-conversion quantum interface is implemented, where the single ph... Near-infrared single photon sources in telecommunication bands, especially at 1550 nm, are required for long-distance quantum communication. Here a down-conversion quantum interface is implemented, where the single photons emitted from single In As quantum dot at 864 nm is down converted to 1552 nm by using a fiber-coupled periodically poled lithium niobate(PPLN) waveguide and a 1.95 μmm pump laser, and the frequency conversion efficiency is ~40%. The singlephoton purity of quantum dot emission is preserved during the down-conversion process, i.e., g^((2))(0), only 0.22 at 1552 nm.This present technique advances the Ⅲ-Ⅴ semiconductor quantum dots as a promising platform for long-distance quantum communication. 展开更多
关键词 quantum frequency down-conversion quantum dot telecommunication band single photon
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Polarization Conversion of Single Photon via Scattering by a Λ System in a Semi-Infinite Waveguide
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作者 Fu-Qiang Yu Mu-Tian Cheng +3 位作者 Shao-Ming Li Xiao-San Ma Zhi-Feng Zhu Xian-Shan Huang 《Chinese Physics Letters》 SCIE CAS CSCD 2019年第5期27-30,共4页
We theoretically investigate single-photon polarization conversion via scattering by an atom with Λ configuration coupled to a semi-infinite waveguide and discuss the two cases in which the Λ system is non-degenerat... We theoretically investigate single-photon polarization conversion via scattering by an atom with Λ configuration coupled to a semi-infinite waveguide and discuss the two cases in which the Λ system is non-degenerated and degenerated. By applying the hard-wall boundary condition of the semi-infinite waveguide, it is found that singlephoton polarization conversion can be realized with unit probability for both cases under the ideal condition.Together with the polarization conversion, the frequency conversion of a single photon can also be realized with unit probability in the ideal case if the Λ system is not degenerated. 展开更多
关键词 Polarization conversion Single photon VIA SCATTERING
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Influences of Uncaptured Electron on Energy Conversion of Photon Compton Scattering in High Power Laser-plasma
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作者 ZHENGJing-hua HAOXiao-fei HAODong-shan 《Semiconductor Photonics and Technology》 CAS 2004年第4期285-288,共4页
Using the single particle theory and the non-flexibility collision model of electron and photon, the influence of the uncaptured electrons on the energy conversion efficiency of multi-photon nonlinear Compton scatteri... Using the single particle theory and the non-flexibility collision model of electron and photon, the influence of the uncaptured electrons on the energy conversion efficiency of multi-photon nonlinear Compton scattering in the extra stationary laser-plasma is investigated. It shows that in extra stationary laser-plasma,the uncaptured electrons make the Δω of the scattering frequency of the multi-photon Compton fall down with the increases of the incident radiation electron speed,the materials of the incident collision of electron and photon, and the number of the photons which work with the electrons at the same time. Under the modulation of the uncaptured electrons to the laser field, the energy conversion efficiency between electrons and photons will fall down with the increase of the electron incident radiation speed, using the low-power electrons for incident source, the loss can be efficiently reduced. 展开更多
关键词 photon Compton scattering Energy conversion Captured electron LASER-PLASMA
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Two-photon Up-conversion Luminescent Properties of HMASPS and HEASPS in Three Different Polymer Matrices
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作者 Yan REN Xiao Qiang YU +7 位作者 Dong WANG Guang Yong ZHOU Zhi Qiang LIU Yu Fang ZHOU Xian ZHAO Zong Shu SHAO Ji Yang WANG Min Hua JIANG 《Chinese Chemical Letters》 SCIE CAS CSCD 2002年第5期452-455,共4页
Three dye-doped polymer rods in different matrices were synthesized in which weak hydrogen bond, strong hydrogen bond and covalent bond existed between the dye and the polymer chain. And the two-photon up-conversion... Three dye-doped polymer rods in different matrices were synthesized in which weak hydrogen bond, strong hydrogen bond and covalent bond existed between the dye and the polymer chain. And the two-photon up-conversion luminescent properties of HMASPS and HEASPS1 in three different microenvironments were studied. 展开更多
关键词 TWO-photon up-conversion lasing solid-state laser dye.
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Nonreciprocal Single Photon Frequency Conversion via Chiral Coupling between a V-Type System and a Pair of Waveguides
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作者 Ce Shi Mu-Tian Cheng +4 位作者 Xiao-San Ma Dong Wang Xianshan Huang Bing Wang Jia-Yan Zhang 《Chinese Physics Letters》 SCIE CAS CSCD 2018年第5期34-38,共5页
The single photon frequency conversion is investigated theoretically in the system composed of a V-type system chiral coupling to a pair of waveguides. The single photon scattering amplitudes are obtained using the re... The single photon frequency conversion is investigated theoretically in the system composed of a V-type system chiral coupling to a pair of waveguides. The single photon scattering amplitudes are obtained using the real-space Hamiltonian. The calculated results show that the probability of single photon frequency down-or up-conversion can reach a unit by choosing appropriate parameters in the non-dissipative system with perfect chiral coupling.We present a nonreciprocal single photon beam splitter whose frequency of the output photon is different from that of the input photon. The influences of dissipations and non-perfect chiral coupling on the single frequency conversion are also shown. Our results may be useful in designing quantum devices at the single-photon level. 展开更多
关键词 Nonreciprocal Single photon Frequency conversion via Chiral Coupling between a V-Type System and a Pair of Waveguides
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Six-bit all-optical quantization using photonic crystal fiber with soliton self-frequency shift and pre-chirp spectral compression techniques 被引量:1
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作者 康哲 苑金辉 +4 位作者 李莎 解松霖 颜玢玢 桑新柱 余重秀 《Chinese Physics B》 SCIE EI CAS CSCD 2013年第11期345-349,共5页
In this paper, we propose an optical quantization scheme for all-optical analog-to-digital conversion that facilitates photonics integration. A segment of 10-m photonic crystal fiber with a high nonlinear coefficient ... In this paper, we propose an optical quantization scheme for all-optical analog-to-digital conversion that facilitates photonics integration. A segment of 10-m photonic crystal fiber with a high nonlinear coefficient of 62.8 W-1/kin is utilized to realize large scale soliton self-frequency shift relevant to the power of the sampled optical signal. Furthermore, a 100-m dispersion-increasing fiber is used as the spectral compression module for further resolution enhancement. Simulation results show that 317-nm maximum wavelength shift is realized with 1550-nm initial wavelength and 6-bit quantization resolution is obtained with a subsequent spectral compression process. 展开更多
关键词 all-optical analog-to-digital conversion photonic crystal fiber soliton self-frequency shift spectralcompression
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Optimizational 6-bit all-optical quantization with soliton self-frequency shift and pre-chirp spectral compression techniques based on photonic crystal fiber 被引量:1
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作者 李莎 王建萍 +1 位作者 康哲 余重秀 《Chinese Physics B》 SCIE EI CAS CSCD 2015年第8期381-385,共5页
In this paper, we optimize a proposed all-optical quantization scheme based on soliton self-frequency shift(SSFS)and pre-chirp spectral compression techniques. A 10m-long high-nonlinear photonic crystal fiber(PCF) is ... In this paper, we optimize a proposed all-optical quantization scheme based on soliton self-frequency shift(SSFS)and pre-chirp spectral compression techniques. A 10m-long high-nonlinear photonic crystal fiber(PCF) is used as an SSFS medium relevant to the power of the sampled optical pulses. Furthermore, a 10m-long dispersion flattened hybrid cladding hexagonal-octagonal PCF(6/8-PCF) is utilized as a spectral compression medium to further enhance the resolution. Simulation results show that 6-bit quantization resolution is still obtained when a 100m-long dispersion-increasing fiber(DIF)is replaced by a 6/8-PCF in spectral compression module. 展开更多
关键词 all-optical analog-to-digital conversion soliton self-frequency shift spectral compression photonic crystal fiber
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Up-conversion luminescence tuning in Er^3+ -doped ceramic glass by femtosecond laser pulse at different laser powers 被引量:1
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作者 Wen-Jing Cheng Guo Liang +4 位作者 Ping Wu Shi-Hua Zhao Tian-Qing Jia Zhen-Rong Sun Sift-An Zhang 《Chinese Physics B》 SCIE EI CAS CSCD 2018年第12期224-230,共7页
The up-conversion luminescence tuning of rare-earth ions is an important research topic for understanding luminescence mechanisms and promoting related applications. In this paper, we experimentally study the up-conve... The up-conversion luminescence tuning of rare-earth ions is an important research topic for understanding luminescence mechanisms and promoting related applications. In this paper, we experimentally study the up-conversion luminescence tuning of Er3+-doped ceramic glass excited by the unshaped, V-shaped and cosine-shaped femtosecond laser field with different laser powers. The results show that green and red up-conversion luminescence can be effectively tuned by varying the power or spectral phase of the femtosecond laser field. We further analyze the up-conversion luminescence tuning mechanism by considering different excitation processes, including single-photon absorption(SPA), two-photon absorption(TPA), excited state absorption(ESA), and energy transfer up-conversion(ETU). The relative weight of TPA in the whole excitation process can increase with the increase of the laser power, thereby enhancing the intensity ratio between green and red luminescence(I547/I656). However, the second ETU(ETU2) process can generate red luminescence and reduce the green and red luminescence intensity ratio I547/I656, while the third ESA(ESA3) process can produce green luminescence and enhance its control efficiency. Moreover, the up-conversion luminescence tuning mechanism is further validated by observing the up-conversion luminescence intensity, depending on the laser power and the down-conversion luminescence spectrum under the excitation of 400-nm femtosecond laser pulse. These studies can present a clear physical picture that enables us to understand the up-conversion luminescence tuning mechanism in rare-earth ions, and can also provide an opportunity to tune up-conversion luminescence to promote its related applications. 展开更多
关键词 rare-earth ions up-conversion luminescence pulse shaping two-photon absorption
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Optical Analog-to-digital Conversion Scheme Based on Tunable Fabry-Perot Resonator
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作者 LI Zheng 《Semiconductor Photonics and Technology》 CAS 2007年第4期298-304,共7页
Proposed is an interference type of optical analog-to-digital conversion(ADC). The refractive index of Fabry-Perot cavity changes with different voltages. The Fabry-Perot resonator converts electronic intensity into l... Proposed is an interference type of optical analog-to-digital conversion(ADC). The refractive index of Fabry-Perot cavity changes with different voltages. The Fabry-Perot resonator converts electronic intensity into light wavelength through selecting lights of different wavelengthes. The parameters of the scheme are acquired with the transmission matrix of optical element and the time of steady-state light field. The maximum sampling speedes of 4-bit, 6-bit, 7-bit, 8-bit and 9-bit(ADC) are 1.695×1010 count/s, 4.33×109 count/s, 2.38×109 count/s, 1.24×109 count/s and 5.9×108 count/s, respectively. 展开更多
关键词 optical A/D conversion photonic sampling wavelength-division multiplexing Pockels effect
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The Up-conversion Laser Properties of a Non-polar Organic Dye and the Influence of Solvents and Pumping Wavelengths
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作者 Xiao Qiang YU Xian ZHANG Gui Bao XU Hua Ping ZHAO Wei HE Zong Shu SHAO Xian Gang XU Min Hua JIANG 《Chinese Chemical Letters》 SCIE CAS CSCD 2006年第1期81-84,共4页
A non-polar organic dye, E, E-1, 4-bis[4'-(N,N-dibutylamino)styryl]-2,5-dimethoxybenzene (DBASDMB), has been synthesized and characterized, and its structure has been determined. Pumped with a 200fs pulse this dy... A non-polar organic dye, E, E-1, 4-bis[4'-(N,N-dibutylamino)styryl]-2,5-dimethoxybenzene (DBASDMB), has been synthesized and characterized, and its structure has been determined. Pumped with a 200fs pulse this dye showed the up-conversion laser properties. The influences of various organic solvents and different pumping wavelength on the laser properties have been demonstrated. 展开更多
关键词 Up-conversion laser two-photon absorption non-polar organic dye.
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Simple and practical method of characterizing the parametric down-conversion source
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作者 王东 伍娟 +5 位作者 赵良圆 安雪碧 银振强 陈巍 韩正甫 王琴 《Chinese Physics B》 SCIE EI CAS CSCD 2017年第11期83-88,共6页
Parametric down-conversion(PDC) sources play an important role in quantum information processing, therefore characterizing their properties is necessary. Here we present a statistical model to assess the properties ... Parametric down-conversion(PDC) sources play an important role in quantum information processing, therefore characterizing their properties is necessary. Here we present a statistical model to assess the properties of the PDC source with certain distribution, such as the brightness and photon channel transmissions, we only need to measure the singles and coincidences counts in a few seconds. Furthermore, we validate the model by applying it to a PDC source generating highly non-degenerate photon pairs. The results of the experiment indicate that our method is more simple, efficient, and less time consuming. 展开更多
关键词 parametric down-conversion brightness photon channel transmission
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Direct laser-written aperiodic photonic volume elements for complex light shaping with high efficiency:inverse design and fabrication
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作者 Nicolas Barré Ravi Shivaraman +4 位作者 Simon Moser Patrick Salter Michael Schmidt Martin J.Booth Alexander Jesacher 《Advanced Photonics Nexus》 2023年第3期53-61,共9页
Light plays a central role in many applications.The key to unlocking its versatility lies in shaping it into the most appropriate form for the task at hand.Specifically tailored refractive index modifications,directly... Light plays a central role in many applications.The key to unlocking its versatility lies in shaping it into the most appropriate form for the task at hand.Specifically tailored refractive index modifications,directly manufactured inside glass using a short pulsed laser,enable an almost arbitrary control of the light flow.However,the stringent requirements for quantitative knowledge of these modifications,as well as for fabrication precision,have so far prevented the fabrication of light-efficient aperiodic photonic volume elements(APVEs).Here,we present a powerful approach to the design and manufacturing of light-efficient APVEs.We optimize application-specific three-dimensional arrangements of hundreds of thousands of microscopic voxels and manufacture them using femtosecond direct laser writing inside millimeter-sized glass volumes.We experimentally achieve unprecedented diffraction efficiencies up to 80%,which is enabled by precise voxel characterization and adaptive optics during fabrication.We demonstrate APVEs with various functionalities,including a spatial mode converter and combined intensity shaping and wavelength multiplexing.Our elements can be freely designed and are efficient,compact,and robust.Our approach is not limited to borosilicate glass but is potentially extendable to other substrates,including birefringent and nonlinear materials,giving a preview of even broader functionalities,including polarization modulation and dynamic elements. 展开更多
关键词 integrated photonics HOLOGRAPHY mode conversion inverse design
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Experiment study of wavelength conversion in a dispersion-flattened photonic crystal fiber 被引量:4
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作者 王秋国 杨伯君 +2 位作者 张岚 张虎 何理 《Chinese Optics Letters》 SCIE EI CAS CSCD 2007年第9期538-539,共2页
Wavelength conversion based on four-wave mixing (FWM) has been demonstrated using a 40-m dispersion flattened highly nonlinear photonic crystal fiber (HNL-PCF). A conversion efficiency of -26 dB for a pump power o... Wavelength conversion based on four-wave mixing (FWM) has been demonstrated using a 40-m dispersion flattened highly nonlinear photonic crystal fiber (HNL-PCF). A conversion efficiency of -26 dB for a pump power of 19.5 dBm and a conversion bandwidth of 28 nm have been obtained, which are limited by the continuous wave (CW) laser wavelength range and tunability of optical band pass filters (OBPFs). 展开更多
关键词 Bandpass filters BANDWIDTH conversion efficiency Four wave mixing Optical frequency conversion photonic crystals
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Apodized silicon photonic grating couplers for mode-order conversion 被引量:3
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作者 IOSIF DEMIRTZIOGLOU COSIMO LACAVA +4 位作者 ABDUL SHAKOOR ALI KHOKHAR YONGMIN JUNG DAVID J.THOMSON PERIKLIS PETROPOULOS 《Photonics Research》 SCIE EI CSCD 2019年第9期1036-1041,共6页
An out-of-plane silicon grating coupler capable of mode-order conversion at the chip–fiber interface is designed and fabricated. Optimization of the structure is performed through finite-difference time-domain simula... An out-of-plane silicon grating coupler capable of mode-order conversion at the chip–fiber interface is designed and fabricated. Optimization of the structure is performed through finite-difference time-domain simulations,and the final device is characterized through far-field profile and transmission measurements. A coupling loss of 3.1 dB to a commercial two-mode fiber is measured for a single TE0→ LP11 mode conversion grating, which includes a conversion penalty of 1.3 dB. Far-field patterns of the excited LP11 mode profile are also reported. 展开更多
关键词 Apodized SILICON photonic GRATING COUPLERS for mode-order conversion
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Inverse-designed photonic fibers and metasurfaces for nonlinear frequency conversion[Invited] 被引量:10
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作者 CHAWIN SITAWARIN WEILIANG JIN +1 位作者 ZIN LIN ALEJANDRO W.RODRIGUEZ 《Photonics Research》 SCIE EI 2018年第5期I0107-I0114,共8页
Typically, photonic waveguides designed for nonlinear frequency conversion rely on intuitive and established principles, including index guiding and bandgap engineering, and are based on simple shapes with high degree... Typically, photonic waveguides designed for nonlinear frequency conversion rely on intuitive and established principles, including index guiding and bandgap engineering, and are based on simple shapes with high degrees of symmetry. We show that recently developed inverse-design techniques can be applied to discover new kinds of microstructured fibers and metasurfaces designed to achieve large nonlinear frequency-conversion efficiencies. As a proof of principle, we demonstrate complex, wavelength-scale chalcogenide glass fibers and gallium phosphide three-dimensional metasurfaces exhibiting some of the largest nonlinear conversion efficiencies predicted thus far,e.g., lowering the power requirement for third-harmonic generation by 104 and enhancing second-harmonic generation conversion efficiency by 107. Such enhancements arise because, in addition to enabling a great degree of tunability in the choice of design wavelengths, these optimization tools ensure both frequency-and phase-matching in addition to large nonlinear overlap factors. 展开更多
关键词 Inverse-designed photonic fibers and metasurfaces nonlinear frequency conversion
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Time-stretch analog-to-digital conversion with a photonic crystal fiber 被引量:2
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作者 滕云 余重秀 +3 位作者 苑金辉 陈静轩 金沧 许谦 《Optoelectronics Letters》 EI 2011年第2期143-146,共4页
All-optical analog-to-digital conversion (ADC) has been extensively researched to break through the inherently limited operating speed of electronic devices. In this paper, we use the photonic crystal fiber (PCF) for ... All-optical analog-to-digital conversion (ADC) has been extensively researched to break through the inherently limited operating speed of electronic devices. In this paper, we use the photonic crystal fiber (PCF) for time-stretch (TS) analog-to-digital (A/D) conversion system through generating low noise, linear chirp distribution and flat super-continuum (SC). Based on the radio frequency (RF) analog signal modulated to the linearly chirped super-continuum, the large-dispersion photonic crystal fiber is used for time-domain stretching. 展开更多
关键词 Analog to digital conversion Crystal whiskers Digital devices Electric converters Nonlinear optics photonic crystals Time varying systems
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An optical scheme for conditional generation of W state and photon-added coherent state 被引量:2
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作者 李燕 景辉 詹明生 《Chinese Physics B》 SCIE EI CAS CSCD 2007年第7期1883-1888,共6页
We propose a simple scheme to generate an arbitrary photon-added coherent state of a travelling optical field by combining an array of degenerate parametric amplifiers and corresponding single-photon detectors. Partic... We propose a simple scheme to generate an arbitrary photon-added coherent state of a travelling optical field by combining an array of degenerate parametric amplifiers and corresponding single-photon detectors. Particularly, when the single-photon-added coherent state is observed by developing the novel technique of Zavatta et al (2004 Science 306 660), we can simultar/eously obtain the generalized N-qubit W state. 展开更多
关键词 photon-added coherent state W state parametric down-conversion
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Highly Selective Photocatalytic Conversion of Glucose on Holo-Symmetrically Spherical Three-Dimensionally Ordered Macroporous Heterojunction Photonic Crystal 被引量:1
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作者 Ting-Wei Wang Zhi-Wen Yin +8 位作者 Yin-Hao Guo Fang-Yuan Bai Jun Chen Wenda Dong Jing Liu Zhi-Yi Hu Lihua Chen Yu Li Bao-Lian Su 《CCS Chemistry》 CSCD 2023年第8期1773-1788,共16页
Photocatalytic conversion of biomass is considered an effective,clean,and environmentally friendly route to obtain high-valued chemicals and hydrogen.However,the limited conversion efficiency and poor selectivity are ... Photocatalytic conversion of biomass is considered an effective,clean,and environmentally friendly route to obtain high-valued chemicals and hydrogen.However,the limited conversion efficiency and poor selectivity are still the main bottlenecks for photocatalytic biomass conversion.Herein,we report the highly selective photocatalytic conversion of glucose solution on holosymmetrically spherical three-dimensionally ordered macroporous TiO_(2)-CdSe heterojunction photonic crystal structure(s-TCS).The obtained s-TCS photocatalysts show excellent stability and strong light harvesting,uniform mass diffusion and exchange,and efficient photogenerated electrons/holes separation and utilization.The optimized s-TCS-4 photocatalyst displays the highest photocatalytic performance for glucose oxidation and hydrogen production.The glucose conversion,lactic acid selectivity,and yield on s-TCS-4 are about 95.9%,94.3%,and 96.4%,respectively.The photocatalytic production of lactic acid for s-TCS-4(18.5 g/L)is 2.3 times higher than the pure spherical TiO_(2) photonic crystal without CdSe(s-TiO_(2),8.1 g/L),and the hydrogen production rate of s-TCS-4 is 9.4 times that of s-TiO_(2).For the first time,we reveal that the photocatalytic conversion of glucose to lactic acid is a third-order and four-electron-involved reaction.This work could shed some new light on the efficient photocatalysis conversion of biomass to highly value-added products with high selectivity and yield,and simultaneously sustainable hydrogen evolution. 展开更多
关键词 TiO_(2)-CdSe heterojunction spherical photonic crystal high-selective photocatalytic glucose conversion lactic acid photocatalytic H2 production four-electron involved reaction third-order reaction
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