Ice pigging is an emerging technique for pipe cleaning in drinking water distribution systems.However,substantial confusion and controversy exist on the potential impacts of ice pigging on bulk water quality.This stud...Ice pigging is an emerging technique for pipe cleaning in drinking water distribution systems.However,substantial confusion and controversy exist on the potential impacts of ice pigging on bulk water quality.This study monitored the microstructural features and composition of sediments and microbial community structures in bulk water in eight multimaterial Chinese networks.Chloride concentration analysis demonstrated that separate cleaning of pipes with different materials in complex networks could mitigate the risk of losing ice pigs and degrading water quality.The microstructural and trace element characterization results showed that ice pigs would scarcely disturb the inner surfaces of long-used pipes.The bacterial richness and diversity of bulk water decreased significantly after ice pigging.Furthermore,correlations were established between pipe service age,temperature,and chloride and total iron concentrations,and the 15 most abundant taxa in bulk water,which could be used to guide practical ice pigging operations.展开更多
We conducted a study on a model drinking water distribution system to evaluate the impact of nutrient in the form of sodium acetate on the growth and survival of coliform and heterotrophic plate count (HPC) bacteria f...We conducted a study on a model drinking water distribution system to evaluate the impact of nutrient in the form of sodium acetate on the growth and survival of coliform and heterotrophic plate count (HPC) bacteria for a maximum of 21 days residence time of water in pipes. Our results show that, besides the nutrient added and the absence of any additional source of contamination and additional supply of nutrient, there was significant growth of the above mentioned bacteria in the pipes and bottles for a couple of days, after which the bacterial population began to decrease. The results indicate that the bacteria used the nutrient to grow and multiply until the nutrient was totally consumed and became depleted in the bulk water phase, after which the bacterial population reached a near stationary level and subsequently declined. This suggests the death of some of the bacteria and their dead cells were used by other bacteria for growth and survival. Using a detection limit of 3.3 CFU/100 mL for the coliforms, the study shows that after sometime, no bacteria were found in the water phase of the pipe, however, the biofilm in the pipes still harbored some of the bacteria. The results have revealed that the bacteria also have the tendency to move from the water phase to the biofilm since the latter provides a more suitable environment for bacteria to thrive on and grow, thus prolonging their survival in the system.展开更多
The leaching behavior of three types of mortars was investigated using a self-design device which could simulate the field conditions of pipe lining. The results by ICP and ESEM measurement show that the developed sla...The leaching behavior of three types of mortars was investigated using a self-design device which could simulate the field conditions of pipe lining. The results by ICP and ESEM measurement show that the developed slag cement mortar is suitable for the lining of cast iron pipe that is used for delivering drinking water.展开更多
The potability of drinking water depends not only on the source and the treatment system, but also on the quality of the waterworks. In fact, the quality of drinking water is considerably degraded by the dilapidated s...The potability of drinking water depends not only on the source and the treatment system, but also on the quality of the waterworks. In fact, the quality of drinking water is considerably degraded by the dilapidated state and lack of maintenance of drinking water networks. In Côte d’Ivoire, the majority of drinking water networks in the various towns are ageing. In Daloa, despite the efforts made by the company in charge of water treatment and distribution to make the water drinkable, the water at consumers’ taps is often colored, has an unpleasant aftertaste and settles after collection. As a result, people are concerned about the potability of tap water, and some are turning to alternative sources of drinking water of unknown quality. In order to determine the factors responsible for the deterioration in water color and taste, as well as the sectors of the network most affected, a diagnosis of the network’s equipment was carried out. Water samples taken from the network were analyzed for color and turbidity. The diagnosis revealed that most of the equipment (suction pads, valves, drains and fire hydrants) is outdated and irregularly maintained. Analyses show that the water is more colored in cast-iron and PVC pipes than in asbestos cement pipes. Coloration values in the network range from 0 to 27 UVC for asbestos cement pipes, from 15 to 56 UCV for ductile iron pipes, and from 11 to 102 UCV for PVC pipes. On the over hand, turbidity values vary from 8.02 to 3.32 NTU for ductile cast iron pipes, 8.51 to 16.98 NTU for asbestos cement pipes and 0.9 to 6.98 NTU for PVC pipes. Old cast-iron pipes release ferric ions on contact with water, degrading their color. Old cast-iron pipes release ferric ions into the water, degrading its color. The high color values observed in the vicinity of drains are thought to be due to irregular maintenance of the network. In fact, after network maintenance, a reduction rate ranging from 2% to 73% is observed for turbidity, while for color, the rate varies from 5% to 72%. In short, the network’s obsolescence and irregular maintenance contribute significantly to the deterioration of water quality.展开更多
Strontium has four naturally occurring stable isotopes,84Sr,86Sr,87Sr,and 88Sr,with abundances of 0.56,9.87,approximately 7.04,and 82.53 atomic %,respectively.The 87Sr/86Sr isotope ratio is variable due to the additio...Strontium has four naturally occurring stable isotopes,84Sr,86Sr,87Sr,and 88Sr,with abundances of 0.56,9.87,approximately 7.04,and 82.53 atomic %,respectively.The 87Sr/86Sr isotope ratio is variable due to the addition of radiogenic 87Sr produced by the beta decay of 87Rb with a half-life of 4.88 ± 0.05 Ga.Thus,展开更多
The article addresses the results of effective water losses prevention in public water supply systems, focusing on procedures for monitoring hidden leaks as the main part of losses and as the first step to control and...The article addresses the results of effective water losses prevention in public water supply systems, focusing on procedures for monitoring hidden leaks as the main part of losses and as the first step to control and prevent them. The described methodology has been applied based on a cross-border cooperation between twin capital cities Vienna and Bratislava in the Central Europe Region within the project deWaloP （Developing Water Loss Prevention） and adopted in Bratislava Water Company （BVS） in the Slovak Republic. The paper provides a complex of simple and easily available practices for analyses of water distribution measurements bringing essential information as to the necessity to use advanced procedures to actively reduce leakage. These practices involve minimum night flows analyses, hydrodynamic pressures analyses, pinpointing of water leakages by working with valves in the water network, the methodology of setting alarm limits for measured data, as well as use of advanced practices to obtain missing topologic data. As the water infrastructure in former socialistic countries are in bad technical condition and the lack of pertinent operational data is a significant obstacle to the application of a more sophisticated methodology based on GIS and other information systems, the procedures focus on using the most simple way to evaluate and control water losses. Finally, the introduction of described methodology in Bratislava Water Company after many years of unsuccessful effort even with expensive sophisticated leakage equipment brought positive outputs and the graph line of water losses level is finally going down. The use of expensive multi-correlating equipment together with human resources on the basis of implementing the above described leakage monitoring will subsequently become more effective, as it shall pinpoint major leakages, disclosure and removal of that shall significantly contribute to the effective reduction of water losses.展开更多
The qualified finished water from water treatment plants(WTPs) may become discolored and deteriorated during transportation in drinking water distribution systems(DWDSs), which affected tap water quality seriously. Th...The qualified finished water from water treatment plants(WTPs) may become discolored and deteriorated during transportation in drinking water distribution systems(DWDSs), which affected tap water quality seriously. This water stability problem often occurs due to pipe corrosion and the destabilization of corrosion scales. This paper provides a comprehensive review of pipe corrosion in DWDSs, including corrosion process, corrosion scale formation, influencing factors and monitoring technologies utilized in DWDSs. In terms of corrosion process, corrosion occurrence, development mechanisms, currently applied assays, and indices used to determine the corrosion possibility are summarized, as well as the chemical and bacterial influences. In terms of scale formation, explanations for the nature of corrosion and scale formation mechanisms are discussed and its typical multilayered structure is illustrated. Furthermore, the influences of water quality and microbial activity on scale transformation are comprehensively discussed. Corrosion-related bacteria at the genus level and their associated corrosion mechanism are also summarized. This review helps deepen the current understanding of pipe corrosion and scale formation in DWDSs, providing guidance for water supply utilities to ensure effective measures to maintain water quality stability and guarantee drinking water safety.展开更多
An electrochemical mass spectrometry technique was developed based on a homemade analytical device for sequential analysis of the heavy metals with various speciations in the scales.Four speciations(e.g.,water-soluble...An electrochemical mass spectrometry technique was developed based on a homemade analytical device for sequential analysis of the heavy metals with various speciations in the scales.Four speciations(e.g.,water-soluble speciation,organic speciation,indissoluble speciation and elemental speciation)of heavy metals are sequentially extracted by H_(2)O,CH_(3)OH,EDTA-2Na and electrolysis for online electrospray ionization mass spectrometry(ESI-MS)detection.The method takes significant advantages,such as requiring no tedious offline sample pretreatment,high speed of analysis(20 min),high throughput(multi-metals),good sensitivity(0.5µg/L)and rich chemical information(four speciations).As a result,the rapid comprehensive characterization of four speciations of Pb,Ni,Cu,Zn,Fe,Ba,Mn,Cr and Ca in water pipe scales has been qualitatively achieved.It demonstrated that the present method is a powerful tool for the effective assessment of potential hazards in drinking water,which provides a new analytical idea for evaluating water quality.展开更多
The occurrence of per-and polyfluoroalkyl substances(PFAS)in water cycles poses a challenge to drinking water quality and safety.In order to counteract the large knowledge gap regarding PFAS in German drinking water,8...The occurrence of per-and polyfluoroalkyl substances(PFAS)in water cycles poses a challenge to drinking water quality and safety.In order to counteract the large knowledge gap regarding PFAS in German drinking water,89 drinking water samples from all over Germany were collected with the help of residents and were analyzed for 26 PFAS by high-performance liquid chromatography with tandem mass spectrometry(HPLC-MS/MS).The 20 PFAS recently regulated by sum concentration(PFAS_(∑20)),as well as six other PFAS,were quantified by targeted analysis.In all drinking water samples,PFAS_(∑20 )was below the limit of 0.1μg/L,but the sum concentrations ranged widely from below the limit of quantification up to 80.2 ng/L.The sum concentrations(PFASP4)of perfluorohexanesulfonate(PFHxS),perfluorooctanesulfonate(PFOS),perfluorooctanoate(PFOA),and perfluorononanoate of 20 ng/L were exceeded in two samples.The most frequently detected individual substances were PFOS(in 52%of the samples),perfluorobutanesulfonate(52%),perfluorohexanoate(PFHxA)(44%),perfluoropentanoate(43%)and PFHxS(35%).The highest single concentrations were 23.5 ng/L for PFHxS,15.3 ng/L for PFOS,and 10.1 ng/L for PFHxA.No regionally elevated concentrations were identified,but some highly urbanized areas showed elevated levels.Concentrations of substitution PFAS,including 2,3,3,3-tetrafluoro-2-(heptafluoropropoxy)propanoate and 2,2,3-trifluor-3-[1,1,2,2,3,3-hexafluor-3-(trifluormethoxy)propoxy]-propanoate(anion of ADONA),were very low compared to regulated PFAS.The most frequently detected PFAS were examined for co-occurrences,but no definite correlations could be found.展开更多
基金financially supported by the National Natural Science Foundation of China(52100015)the Zhejiang Provincial Natural Science Foundation of China(LQ22E080018)the China Postdoctoral Science Foundation(2021M692860).
文摘Ice pigging is an emerging technique for pipe cleaning in drinking water distribution systems.However,substantial confusion and controversy exist on the potential impacts of ice pigging on bulk water quality.This study monitored the microstructural features and composition of sediments and microbial community structures in bulk water in eight multimaterial Chinese networks.Chloride concentration analysis demonstrated that separate cleaning of pipes with different materials in complex networks could mitigate the risk of losing ice pigs and degrading water quality.The microstructural and trace element characterization results showed that ice pigs would scarcely disturb the inner surfaces of long-used pipes.The bacterial richness and diversity of bulk water decreased significantly after ice pigging.Furthermore,correlations were established between pipe service age,temperature,and chloride and total iron concentrations,and the 15 most abundant taxa in bulk water,which could be used to guide practical ice pigging operations.
文摘We conducted a study on a model drinking water distribution system to evaluate the impact of nutrient in the form of sodium acetate on the growth and survival of coliform and heterotrophic plate count (HPC) bacteria for a maximum of 21 days residence time of water in pipes. Our results show that, besides the nutrient added and the absence of any additional source of contamination and additional supply of nutrient, there was significant growth of the above mentioned bacteria in the pipes and bottles for a couple of days, after which the bacterial population began to decrease. The results indicate that the bacteria used the nutrient to grow and multiply until the nutrient was totally consumed and became depleted in the bulk water phase, after which the bacterial population reached a near stationary level and subsequently declined. This suggests the death of some of the bacteria and their dead cells were used by other bacteria for growth and survival. Using a detection limit of 3.3 CFU/100 mL for the coliforms, the study shows that after sometime, no bacteria were found in the water phase of the pipe, however, the biofilm in the pipes still harbored some of the bacteria. The results have revealed that the bacteria also have the tendency to move from the water phase to the biofilm since the latter provides a more suitable environment for bacteria to thrive on and grow, thus prolonging their survival in the system.
文摘The leaching behavior of three types of mortars was investigated using a self-design device which could simulate the field conditions of pipe lining. The results by ICP and ESEM measurement show that the developed slag cement mortar is suitable for the lining of cast iron pipe that is used for delivering drinking water.
文摘The potability of drinking water depends not only on the source and the treatment system, but also on the quality of the waterworks. In fact, the quality of drinking water is considerably degraded by the dilapidated state and lack of maintenance of drinking water networks. In Côte d’Ivoire, the majority of drinking water networks in the various towns are ageing. In Daloa, despite the efforts made by the company in charge of water treatment and distribution to make the water drinkable, the water at consumers’ taps is often colored, has an unpleasant aftertaste and settles after collection. As a result, people are concerned about the potability of tap water, and some are turning to alternative sources of drinking water of unknown quality. In order to determine the factors responsible for the deterioration in water color and taste, as well as the sectors of the network most affected, a diagnosis of the network’s equipment was carried out. Water samples taken from the network were analyzed for color and turbidity. The diagnosis revealed that most of the equipment (suction pads, valves, drains and fire hydrants) is outdated and irregularly maintained. Analyses show that the water is more colored in cast-iron and PVC pipes than in asbestos cement pipes. Coloration values in the network range from 0 to 27 UVC for asbestos cement pipes, from 15 to 56 UCV for ductile iron pipes, and from 11 to 102 UCV for PVC pipes. On the over hand, turbidity values vary from 8.02 to 3.32 NTU for ductile cast iron pipes, 8.51 to 16.98 NTU for asbestos cement pipes and 0.9 to 6.98 NTU for PVC pipes. Old cast-iron pipes release ferric ions on contact with water, degrading their color. Old cast-iron pipes release ferric ions into the water, degrading its color. The high color values observed in the vicinity of drains are thought to be due to irregular maintenance of the network. In fact, after network maintenance, a reduction rate ranging from 2% to 73% is observed for turbidity, while for color, the rate varies from 5% to 72%. In short, the network’s obsolescence and irregular maintenance contribute significantly to the deterioration of water quality.
文摘Strontium has four naturally occurring stable isotopes,84Sr,86Sr,87Sr,and 88Sr,with abundances of 0.56,9.87,approximately 7.04,and 82.53 atomic %,respectively.The 87Sr/86Sr isotope ratio is variable due to the addition of radiogenic 87Sr produced by the beta decay of 87Rb with a half-life of 4.88 ± 0.05 Ga.Thus,
文摘The article addresses the results of effective water losses prevention in public water supply systems, focusing on procedures for monitoring hidden leaks as the main part of losses and as the first step to control and prevent them. The described methodology has been applied based on a cross-border cooperation between twin capital cities Vienna and Bratislava in the Central Europe Region within the project deWaloP （Developing Water Loss Prevention） and adopted in Bratislava Water Company （BVS） in the Slovak Republic. The paper provides a complex of simple and easily available practices for analyses of water distribution measurements bringing essential information as to the necessity to use advanced procedures to actively reduce leakage. These practices involve minimum night flows analyses, hydrodynamic pressures analyses, pinpointing of water leakages by working with valves in the water network, the methodology of setting alarm limits for measured data, as well as use of advanced practices to obtain missing topologic data. As the water infrastructure in former socialistic countries are in bad technical condition and the lack of pertinent operational data is a significant obstacle to the application of a more sophisticated methodology based on GIS and other information systems, the procedures focus on using the most simple way to evaluate and control water losses. Finally, the introduction of described methodology in Bratislava Water Company after many years of unsuccessful effort even with expensive sophisticated leakage equipment brought positive outputs and the graph line of water losses level is finally going down. The use of expensive multi-correlating equipment together with human resources on the basis of implementing the above described leakage monitoring will subsequently become more effective, as it shall pinpoint major leakages, disclosure and removal of that shall significantly contribute to the effective reduction of water losses.
基金supported by the Shandong Provincial Key Research and Development Program- Major Scientific and Technological Innovation Project (No. 2020CXGC011406)the R&D project of Suzhou Water Resource and Management (No. 2020011)the National Water Major Project (Nos. 2018ZX07111-006 , 2012ZX07404-002 , 2012ZX07403-001)。
文摘The qualified finished water from water treatment plants(WTPs) may become discolored and deteriorated during transportation in drinking water distribution systems(DWDSs), which affected tap water quality seriously. This water stability problem often occurs due to pipe corrosion and the destabilization of corrosion scales. This paper provides a comprehensive review of pipe corrosion in DWDSs, including corrosion process, corrosion scale formation, influencing factors and monitoring technologies utilized in DWDSs. In terms of corrosion process, corrosion occurrence, development mechanisms, currently applied assays, and indices used to determine the corrosion possibility are summarized, as well as the chemical and bacterial influences. In terms of scale formation, explanations for the nature of corrosion and scale formation mechanisms are discussed and its typical multilayered structure is illustrated. Furthermore, the influences of water quality and microbial activity on scale transformation are comprehensively discussed. Corrosion-related bacteria at the genus level and their associated corrosion mechanism are also summarized. This review helps deepen the current understanding of pipe corrosion and scale formation in DWDSs, providing guidance for water supply utilities to ensure effective measures to maintain water quality stability and guarantee drinking water safety.
基金This work was supported by the National Natural Science Foundation of China(Nos.21727812,21705016)the Doctoral Start-up Fund of East China University of Technology,China(No.DHBK2017115)the Open Fund of Jiangxi Provincial Key Laboratory of Mass Spectrometry Science and Instrumentation,China(No.JXMS202117).
文摘An electrochemical mass spectrometry technique was developed based on a homemade analytical device for sequential analysis of the heavy metals with various speciations in the scales.Four speciations(e.g.,water-soluble speciation,organic speciation,indissoluble speciation and elemental speciation)of heavy metals are sequentially extracted by H_(2)O,CH_(3)OH,EDTA-2Na and electrolysis for online electrospray ionization mass spectrometry(ESI-MS)detection.The method takes significant advantages,such as requiring no tedious offline sample pretreatment,high speed of analysis(20 min),high throughput(multi-metals),good sensitivity(0.5µg/L)and rich chemical information(four speciations).As a result,the rapid comprehensive characterization of four speciations of Pb,Ni,Cu,Zn,Fe,Ba,Mn,Cr and Ca in water pipe scales has been qualitatively achieved.It demonstrated that the present method is a powerful tool for the effective assessment of potential hazards in drinking water,which provides a new analytical idea for evaluating water quality.
文摘The occurrence of per-and polyfluoroalkyl substances(PFAS)in water cycles poses a challenge to drinking water quality and safety.In order to counteract the large knowledge gap regarding PFAS in German drinking water,89 drinking water samples from all over Germany were collected with the help of residents and were analyzed for 26 PFAS by high-performance liquid chromatography with tandem mass spectrometry(HPLC-MS/MS).The 20 PFAS recently regulated by sum concentration(PFAS_(∑20)),as well as six other PFAS,were quantified by targeted analysis.In all drinking water samples,PFAS_(∑20 )was below the limit of 0.1μg/L,but the sum concentrations ranged widely from below the limit of quantification up to 80.2 ng/L.The sum concentrations(PFASP4)of perfluorohexanesulfonate(PFHxS),perfluorooctanesulfonate(PFOS),perfluorooctanoate(PFOA),and perfluorononanoate of 20 ng/L were exceeded in two samples.The most frequently detected individual substances were PFOS(in 52%of the samples),perfluorobutanesulfonate(52%),perfluorohexanoate(PFHxA)(44%),perfluoropentanoate(43%)and PFHxS(35%).The highest single concentrations were 23.5 ng/L for PFHxS,15.3 ng/L for PFOS,and 10.1 ng/L for PFHxA.No regionally elevated concentrations were identified,but some highly urbanized areas showed elevated levels.Concentrations of substitution PFAS,including 2,3,3,3-tetrafluoro-2-(heptafluoropropoxy)propanoate and 2,2,3-trifluor-3-[1,1,2,2,3,3-hexafluor-3-(trifluormethoxy)propoxy]-propanoate(anion of ADONA),were very low compared to regulated PFAS.The most frequently detected PFAS were examined for co-occurrences,but no definite correlations could be found.
