We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules.We derive a long-duration control scheme that allows for highly efficient population...We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules.We derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth pulse.To overcome fluctuations in control field parameters,we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral amplitude.It is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields,leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired states.The method demonstrates resilience to fluctuations in control field parameters,making it a promising approach for reliable and efficient population transfer in practical applications.展开更多
Non-Hermitian dissipation dynamics,capable of turning the conventionally detrimental decoherence effects to useful resources for state engineering,is highly attractive to quantum information processing.In this work,an...Non-Hermitian dissipation dynamics,capable of turning the conventionally detrimental decoherence effects to useful resources for state engineering,is highly attractive to quantum information processing.In this work,an effective scheme is developed for implementing fast population transfer with a superconducting qutrit via the non-Hermitian shortcut to adiabaticity(STA).We first deal with aΛ-configuration interaction between the qutrit and microwave drivings,in which the dephasing-assisted qubit state inversion requiring an overlarge dephasing rate is constructed non-adiabatically.After introducing a feasible ancillary driving that directly acts upon the qubit states,the target state transfer can be well realized but with an accessible qubit dephasing rate.Moreover,a high fidelity could be numerically obtained in the considered system.The strategy could provide a new route towards the non-Hermitian shortcut operations on superconducting quantum circuits.展开更多
The utilization of qudits in quantum systems has led to significant advantages in quantum computation and information processing.Therefore,qudits have gained increased attention in recent research for their precise an...The utilization of qudits in quantum systems has led to significant advantages in quantum computation and information processing.Therefore,qudits have gained increased attention in recent research for their precise and efficient operations.In this work,we demonstrate the complete population transfer between the next-adjacent energy levels of a transmon qudit using the Pythagorean coupling method and energy level mapping.We achieve a|0>to|2>transfer with a process fidelity of 97.76%in the subspace spanned by|0>to|2>.Moreover,the transfer operation is achieved within a remarkably fast timescale,as short as 20 ns.This study may present a promising avenue for enhancing the operation flexibility and efficiency of qudits in future implementations.展开更多
This paper has calculated that Rydberg atoms can be transferred to states of lower principal quantum number by exposing them to a frequency chirped microwave pulse. The atoms experience the consequence: 70p-69s-68p-6...This paper has calculated that Rydberg atoms can be transferred to states of lower principal quantum number by exposing them to a frequency chirped microwave pulse. The atoms experience the consequence: 70p-69s-68p-67s-66p by a constant amplitude field in the adopted model. This study shows that the complete population transfer is related to the chirp rate and the carrier frequency.展开更多
Using the time-dependent multilevel approach, we have calculated the coherent population transfer between the quantum states of potassium atom by a single frequency-chirped laser pulse. The result shows that a pair of...Using the time-dependent multilevel approach, we have calculated the coherent population transfer between the quantum states of potassium atom by a single frequency-chirped laser pulse. The result shows that a pair of sequential 'broadband' frequency-chirped laser pulses can efficiently transfer population from the initial state of the ladder system to the target state. It is also found that the population can be efficiently transferred to a target state and trapped there by using an 'intuitive' or a 'counterintuitive' frequency sweep laser pulse in the case of 'narrowband' frequency-chirped laser pulse. Our research shows that the complete population transfer is related to the pulse duration, chirp rate, and amplitude of the laser pulse.展开更多
Fine control of the dynamics of a quantum system is the key element to perform quantum information processing and coherent manipulations for atomic and molecular systems. We propose a control protocol using a tangentp...Fine control of the dynamics of a quantum system is the key element to perform quantum information processing and coherent manipulations for atomic and molecular systems. We propose a control protocol using a tangentpulse driven model and demonstrate that it indicates a desirable design, i.e., of being both fast and accurate for population transfer. As opposed to other existing strategies, a remarkable character of the present scheme is that high velocity of the nonadiabatic evolution itself not only will not lead to unwanted transitions but also can suppress the error caused by the truncation of the driving pulse.展开更多
On the basis of the relationship between the Hamiltonian of spin 1/2 quantum system under control and the energy level structure and transitions, a radio frequency pulse sequence is designed using intuitive and half c...On the basis of the relationship between the Hamiltonian of spin 1/2 quantum system under control and the energy level structure and transitions, a radio frequency pulse sequence is designed using intuitive and half counter-intuitive sequences of pulse to transfer the population of the 3-qubit system coherently. The effectiveness of the designed control sequence is verified through the system simulation experiment of the evolution of state. In principle, the design method of the control pulse sequence proposed can be generalized to use in the quantum systems of higher dimension.展开更多
This work explores the effect of spontaneous emission on coherence generation and population transfer in a three- level ladder atomic system driven by two pulses in counterintuitive order. With adiabatic evolution and...This work explores the effect of spontaneous emission on coherence generation and population transfer in a three- level ladder atomic system driven by two pulses in counterintuitive order. With adiabatic evolution and the weak- dephasing approximation, we find that a large coherence and population transfer can be achieved even with spontaneous decay rate. The maximum coherence and population transfer decrease with the increase of spontaneous decay rate from the highest state to intermediate state. But this effect can be compensated by shortening the pulse width and enlarging the delay time. Results show that the coherence generation and population transfer never depend on the spontaneous decay rate from the intermediate state to ground state. The validity of the analytic solution is examined by numerical calculation.展开更多
The population transfer in a ladder-type atomic system driven by linearly polarized sech-shape femtosecond laser pulses is investigated by numerically solving Schr6dinger equation without including the rotating wave a...The population transfer in a ladder-type atomic system driven by linearly polarized sech-shape femtosecond laser pulses is investigated by numerically solving Schr6dinger equation without including the rotating wave approximation (RWA). It is shown that population transfer is mainly determined by the Rabi frequency (strength) of the driving laser field and the chirp rate, and that the ratio of the dipole moments and the pulse width also have a prominent effect on the population transfer. By choosing appropriate values of the above parameters, complete population transfer can be realized.展开更多
The effect of delay time on photoelectron spectra and state populations of a four-level ladder K2 molecule is investigated by a pump1–pump2–probe pulse via the time-dependent wave packet approach. The periodical mot...The effect of delay time on photoelectron spectra and state populations of a four-level ladder K2 molecule is investigated by a pump1–pump2–probe pulse via the time-dependent wave packet approach. The periodical motion of the wave packet leads to the periodical change of the photoelectron spectra. The Autler–Townes triple splitting appears at zero delay time, double splitting appears at nonzero delay time between pump1 and pump2 pulses, and no splitting appears at nonzero delay time between pump2 and probe pulses. The periodical change of the state populations with the delay time may be due to the coupling effect between the two pulses. It is found that the selectivity of the state populations may be attained by regulating the delay time. The results can provide an important basis for realizing the optical control of molecules experimentally.展开更多
By using the time-dependent multilevel approach, we have calculated the coherent population transfer among the quantum states of potassium atom by a single frequency-chirped laser pulse. The results show that the popu...By using the time-dependent multilevel approach, we have calculated the coherent population transfer among the quantum states of potassium atom by a single frequency-chirped laser pulse. The results show that the population can be efficiently transferred to a target state and be trapped there by using an 'intuitive' or a 'counter-intuitive' frequency sweep laser pulse in the case of 'narrowband' frequency-chirped laser pulse. It is also found that a pair of sequential 'broadband' frequency-chirped laser pulses can efficiently transfer population from one ground state of the A atom to the other one.展开更多
Stimulated-Raman-adiabatic-passage (STIRAP) process provides an effective technique to transfer electron population from an initial state (e.g. ground state) to excited final state for both atoms and molecules. In thi...Stimulated-Raman-adiabatic-passage (STIRAP) process provides an effective technique to transfer electron population from an initial state (e.g. ground state) to excited final state for both atoms and molecules. In this paper, we present the results of the study on electron population transfer in three level system. We have analyzed the effects of various conditions on the transfer process, such as the time delay of the two laser beams, two-photon off-resonance, one-photon off-resonance and the change of relative laser intensity. The numerical result is compared with experiment, and the reasons for the effects are also given.展开更多
The population transfer of sodium in a single analytical laser pulse was studied in three models:two-level sodium,three-level sodium and many-level sodium.The effect of a third state on a two-level system was studied ...The population transfer of sodium in a single analytical laser pulse was studied in three models:two-level sodium,three-level sodium and many-level sodium.The effect of a third state on a two-level system was studied by investigating a ladder three-level system.Two effects were found in the vicinity of the resonance frequency.展开更多
The B-spline expansion technique and the time-dependent multilevel approach (TDMA) are used to study the interaction between a microwave field and sodium atoms. The Rydberg sodium atom energy levels of p states in z...The B-spline expansion technique and the time-dependent multilevel approach (TDMA) are used to study the interaction between a microwave field and sodium atoms. The Rydberg sodium atom energy levels of p states in zero field are calculated, and the results are in good agreement with the other theoretical ones. The time evolutions during the population transfers of the five states from n = 75 to n = 79 in different microwave fields are obtained. The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters.展开更多
The time-dependent multilevel approach(TDMA) and B-spline expansion technique are used to study the coherent population transfer between the quantum states of a potassium atom by a single frequency-chirped microwave...The time-dependent multilevel approach(TDMA) and B-spline expansion technique are used to study the coherent population transfer between the quantum states of a potassium atom by a single frequency-chirped microwave pulse.The Rydberg potassium atom energy levels of n=6-15,l=0-5 states in zero field are calculated and the results are in good agreement with other theoretical values.The time evolutions of the population transfer of the six states from n=70 to n=75 in different microwave fields are obtained.The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters.展开更多
The Autler-Townes (AT) splitting in femtosecond photoelectron spectrum of three-level Li2 molecules is theoretically investigated using time-dependent quantum wave packet method. With proper femtosecond laser pulses...The Autler-Townes (AT) splitting in femtosecond photoelectron spectrum of three-level Li2 molecules is theoretically investigated using time-dependent quantum wave packet method. With proper femtosecond laser pulses, three peaks of the AT splitting can be observed in the photoelectron spectrum. The AT splitting stems from rapid Rabi oscillation caused by intense ultrashort laser pluses. The effects of laser parameters on the molecular ionization dynamics are also discussed.展开更多
Using time-dependent multilevel approach (TDML), this paper studies the dynamics of coherent control of Rydberg lithium atoms and demonstrates that Rydberg lithium atoms can be transferred to states of higher princi...Using time-dependent multilevel approach (TDML), this paper studies the dynamics of coherent control of Rydberg lithium atoms and demonstrates that Rydberg lithium atoms can be transferred to states of higher principal quantum number by exposing them to specially designed frequency-chirped laser pulses. The population transfer from n=70 to n=75 states of lithium atoms with efficiency more than 90% is achieved by means of the sequential adiabatic rapid passages. The results agree well with the experimental ones and show that the coherent control of the population transfer from the lower n to the higher n states can be accomplished by the optimization of the chirping parameters and the intensity of laser field.展开更多
The method of quantum wave packet dynamics is used to study the multiphoton ionization of NO molecules via a two-photon Raman coupling and a laser-induced continuum structure (LICS) state in two-colour strong femtos...The method of quantum wave packet dynamics is used to study the multiphoton ionization of NO molecules via a two-photon Raman coupling and a laser-induced continuum structure (LICS) state in two-colour strong femtosecond pulsed laser fields. Time-and energy-resolved photoelectron energy spectra are calculated for describing three photoionization channels. The population transfers through the LICS and the Raman coupling passages are discussed.展开更多
The effect of pulse temporal profiles on the Autler-Townes (AT) splitting in photoelectron spectra is theoretically studied by employing the time-dependent wave packet method for a rotational Na2 molecule. The AT sp...The effect of pulse temporal profiles on the Autler-Townes (AT) splitting in photoelectron spectra is theoretically studied by employing the time-dependent wave packet method for a rotational Na2 molecule. The AT splitting which results from the sufficient Rabi oscillations is affected by the pulse profile and molecular alignment. The AT splitting may be observed only by utilizing proper pulse profiles with a certain intensity.展开更多
The technique of stimulated Raman adiabatic passage (STIRAP) is used to transfer potassium atoms from the 22p state to the 21p Rydberg state through the intermediate state 22s. The results show that complete populat...The technique of stimulated Raman adiabatic passage (STIRAP) is used to transfer potassium atoms from the 22p state to the 21p Rydberg state through the intermediate state 22s. The results show that complete population transfer is related to pulse duration and overlap, and occurs when the pulse duration and overlap have adequate values. At the same time, population trapping is also formed. Complete population transfer can also occurs when the two-photon resonance condition (△s = △p) is met.展开更多
基金This work was supported by the National Natural Science Foundations of China(Grant Nos.12275033,61973317,and 12274470)the Natural Science Foundation of Hunan Province for Distinguished Young Scholars(Grant No.2022JJ10070)+1 种基金the Natural Science Foundation of Hunan Province(Grant No.2022JJ30582)the Scientific Research Fund of Hunan Provincial Education Department(Grant No.20A025).
文摘We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules.We derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth pulse.To overcome fluctuations in control field parameters,we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral amplitude.It is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields,leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired states.The method demonstrates resilience to fluctuations in control field parameters,making it a promising approach for reliable and efficient population transfer in practical applications.
基金the Natural Science Foundation of Henan Province(Grant Nos.212300410388 and 212300410238)the Scientific Research Innovation Team of Xuchang University(Grant No.2022CXTD005)+2 种基金the National Scientific Research Project Cultivation Fund of Xuchang University(Grant No.2022GJPY001)the Key Research Project in Universities of Henan Province(Grant No.23B140010)the“316"Project Plan of Xuchang University.
文摘Non-Hermitian dissipation dynamics,capable of turning the conventionally detrimental decoherence effects to useful resources for state engineering,is highly attractive to quantum information processing.In this work,an effective scheme is developed for implementing fast population transfer with a superconducting qutrit via the non-Hermitian shortcut to adiabaticity(STA).We first deal with aΛ-configuration interaction between the qutrit and microwave drivings,in which the dephasing-assisted qubit state inversion requiring an overlarge dephasing rate is constructed non-adiabatically.After introducing a feasible ancillary driving that directly acts upon the qubit states,the target state transfer can be well realized but with an accessible qubit dephasing rate.Moreover,a high fidelity could be numerically obtained in the considered system.The strategy could provide a new route towards the non-Hermitian shortcut operations on superconducting quantum circuits.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.11890704,12004042,12104055,and 12104056)Natural Science Foundation of Beijing (Grant No.Z190012)Key Area Research and Development Program of Guangdong Province (Grant No.2018B030326001)。
文摘The utilization of qudits in quantum systems has led to significant advantages in quantum computation and information processing.Therefore,qudits have gained increased attention in recent research for their precise and efficient operations.In this work,we demonstrate the complete population transfer between the next-adjacent energy levels of a transmon qudit using the Pythagorean coupling method and energy level mapping.We achieve a|0>to|2>transfer with a process fidelity of 97.76%in the subspace spanned by|0>to|2>.Moreover,the transfer operation is achieved within a remarkably fast timescale,as short as 20 ns.This study may present a promising avenue for enhancing the operation flexibility and efficiency of qudits in future implementations.
基金Project supported by the National Natural Science Foundation of China (Grant No 10774039)
文摘This paper has calculated that Rydberg atoms can be transferred to states of lower principal quantum number by exposing them to a frequency chirped microwave pulse. The atoms experience the consequence: 70p-69s-68p-67s-66p by a constant amplitude field in the adopted model. This study shows that the complete population transfer is related to the chirp rate and the carrier frequency.
文摘Using the time-dependent multilevel approach, we have calculated the coherent population transfer between the quantum states of potassium atom by a single frequency-chirped laser pulse. The result shows that a pair of sequential 'broadband' frequency-chirped laser pulses can efficiently transfer population from the initial state of the ladder system to the target state. It is also found that the population can be efficiently transferred to a target state and trapped there by using an 'intuitive' or a 'counterintuitive' frequency sweep laser pulse in the case of 'narrowband' frequency-chirped laser pulse. Our research shows that the complete population transfer is related to the pulse duration, chirp rate, and amplitude of the laser pulse.
文摘Fine control of the dynamics of a quantum system is the key element to perform quantum information processing and coherent manipulations for atomic and molecular systems. We propose a control protocol using a tangentpulse driven model and demonstrate that it indicates a desirable design, i.e., of being both fast and accurate for population transfer. As opposed to other existing strategies, a remarkable character of the present scheme is that high velocity of the nonadiabatic evolution itself not only will not lead to unwanted transitions but also can suppress the error caused by the truncation of the driving pulse.
基金supported by the National Natural Science Foundation of China (60774098)the National Key Basic Research Program (2006922004)
文摘On the basis of the relationship between the Hamiltonian of spin 1/2 quantum system under control and the energy level structure and transitions, a radio frequency pulse sequence is designed using intuitive and half counter-intuitive sequences of pulse to transfer the population of the 3-qubit system coherently. The effectiveness of the designed control sequence is verified through the system simulation experiment of the evolution of state. In principle, the design method of the control pulse sequence proposed can be generalized to use in the quantum systems of higher dimension.
基金Project supported by the National Natural Science Foundation of China (Grant No. 10774059)the National Basic Research Program of China (Grant No. 2006CB921101)the Natural Science Foundation of Heilongjiang Province,China (Grant No. F200928)
文摘This work explores the effect of spontaneous emission on coherence generation and population transfer in a three- level ladder atomic system driven by two pulses in counterintuitive order. With adiabatic evolution and the weak- dephasing approximation, we find that a large coherence and population transfer can be achieved even with spontaneous decay rate. The maximum coherence and population transfer decrease with the increase of spontaneous decay rate from the highest state to intermediate state. But this effect can be compensated by shortening the pulse width and enlarging the delay time. Results show that the coherence generation and population transfer never depend on the spontaneous decay rate from the intermediate state to ground state. The validity of the analytic solution is examined by numerical calculation.
基金supported by National Basic Research Program of China (Grant No 2006CB806003)the Natural Science Foundation of Shandong Province,China (Grant No Y2006A21)+1 种基金the National Natural Science Foundation of China (Grant No 10675076)State Key Laboratory of High Field Laser Physics,Shanghai Institute of Optics and Fine Mechanics,Chinese Academy of Sciences,China
文摘The population transfer in a ladder-type atomic system driven by linearly polarized sech-shape femtosecond laser pulses is investigated by numerically solving Schr6dinger equation without including the rotating wave approximation (RWA). It is shown that population transfer is mainly determined by the Rabi frequency (strength) of the driving laser field and the chirp rate, and that the ratio of the dipole moments and the pulse width also have a prominent effect on the population transfer. By choosing appropriate values of the above parameters, complete population transfer can be realized.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11704178 and 11764041)the Scientific Research Fund of Hunan Provincial Education Department,China(Grant No.15B204)
文摘The effect of delay time on photoelectron spectra and state populations of a four-level ladder K2 molecule is investigated by a pump1–pump2–probe pulse via the time-dependent wave packet approach. The periodical motion of the wave packet leads to the periodical change of the photoelectron spectra. The Autler–Townes triple splitting appears at zero delay time, double splitting appears at nonzero delay time between pump1 and pump2 pulses, and no splitting appears at nonzero delay time between pump2 and probe pulses. The periodical change of the state populations with the delay time may be due to the coupling effect between the two pulses. It is found that the selectivity of the state populations may be attained by regulating the delay time. The results can provide an important basis for realizing the optical control of molecules experimentally.
基金Project supported by the Natural Science Foundation of Henan Province, China (Grant No 0411011900).
文摘By using the time-dependent multilevel approach, we have calculated the coherent population transfer among the quantum states of potassium atom by a single frequency-chirped laser pulse. The results show that the population can be efficiently transferred to a target state and be trapped there by using an 'intuitive' or a 'counter-intuitive' frequency sweep laser pulse in the case of 'narrowband' frequency-chirped laser pulse. It is also found that a pair of sequential 'broadband' frequency-chirped laser pulses can efficiently transfer population from one ground state of the A atom to the other one.
文摘Stimulated-Raman-adiabatic-passage (STIRAP) process provides an effective technique to transfer electron population from an initial state (e.g. ground state) to excited final state for both atoms and molecules. In this paper, we present the results of the study on electron population transfer in three level system. We have analyzed the effects of various conditions on the transfer process, such as the time delay of the two laser beams, two-photon off-resonance, one-photon off-resonance and the change of relative laser intensity. The numerical result is compared with experiment, and the reasons for the effects are also given.
基金The author is grateful to the scientific research foundation from Binzhou University。
文摘The population transfer of sodium in a single analytical laser pulse was studied in three models:two-level sodium,three-level sodium and many-level sodium.The effect of a third state on a two-level system was studied by investigating a ladder three-level system.Two effects were found in the vicinity of the resonance frequency.
基金Project supported by the National Natural Science Foundation of China (Grant No. 10774039)the Natural Science Foundation of Education Bureau of Henan Province, China (Grant Nos. 2010C140002 and 2010A140006)the Research Planning Project of Basic and Advanced Technology of Henan Province, China (Grant No. 112300410025)
文摘The B-spline expansion technique and the time-dependent multilevel approach (TDMA) are used to study the interaction between a microwave field and sodium atoms. The Rydberg sodium atom energy levels of p states in zero field are calculated, and the results are in good agreement with the other theoretical ones. The time evolutions during the population transfers of the five states from n = 75 to n = 79 in different microwave fields are obtained. The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters.
基金Project supported by the National Natural Science Foundation of China (Grant No. 10774039)the Natural Science Foundation of Education Bureau of Henan Province,China (Grant Nos. 2010C140002 and 2010A140006)the Research Planning Project of Basic and Advanced Technology of Henan Province,China (Grant No. 112300410025)
文摘The time-dependent multilevel approach(TDMA) and B-spline expansion technique are used to study the coherent population transfer between the quantum states of a potassium atom by a single frequency-chirped microwave pulse.The Rydberg potassium atom energy levels of n=6-15,l=0-5 states in zero field are calculated and the results are in good agreement with other theoretical values.The time evolutions of the population transfer of the six states from n=70 to n=75 in different microwave fields are obtained.The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10374012 and 10674022.
文摘The Autler-Townes (AT) splitting in femtosecond photoelectron spectrum of three-level Li2 molecules is theoretically investigated using time-dependent quantum wave packet method. With proper femtosecond laser pulses, three peaks of the AT splitting can be observed in the photoelectron spectrum. The AT splitting stems from rapid Rabi oscillation caused by intense ultrashort laser pluses. The effects of laser parameters on the molecular ionization dynamics are also discussed.
基金Project supported by the National Natural Science Foundation of China(Grant No.10774039)the Basic Research Program of Education Bureau of Henan Province of China(Grant No.072300410130)
文摘Using time-dependent multilevel approach (TDML), this paper studies the dynamics of coherent control of Rydberg lithium atoms and demonstrates that Rydberg lithium atoms can be transferred to states of higher principal quantum number by exposing them to specially designed frequency-chirped laser pulses. The population transfer from n=70 to n=75 states of lithium atoms with efficiency more than 90% is achieved by means of the sequential adiabatic rapid passages. The results agree well with the experimental ones and show that the coherent control of the population transfer from the lower n to the higher n states can be accomplished by the optimization of the chirping parameters and the intensity of laser field.
基金Supported by the National Natural Science Foundation of China under Grant No 10374012.
文摘The method of quantum wave packet dynamics is used to study the multiphoton ionization of NO molecules via a two-photon Raman coupling and a laser-induced continuum structure (LICS) state in two-colour strong femtosecond pulsed laser fields. Time-and energy-resolved photoelectron energy spectra are calculated for describing three photoionization channels. The population transfers through the LICS and the Raman coupling passages are discussed.
基金Supported by the National Natural Science Foundation of China under Grant No 10374012.
文摘The effect of pulse temporal profiles on the Autler-Townes (AT) splitting in photoelectron spectra is theoretically studied by employing the time-dependent wave packet method for a rotational Na2 molecule. The AT splitting which results from the sufficient Rabi oscillations is affected by the pulse profile and molecular alignment. The AT splitting may be observed only by utilizing proper pulse profiles with a certain intensity.
基金Project sapported by the National Natural Science Foundation of China (Grant No 10574096).
文摘The technique of stimulated Raman adiabatic passage (STIRAP) is used to transfer potassium atoms from the 22p state to the 21p Rydberg state through the intermediate state 22s. The results show that complete population transfer is related to pulse duration and overlap, and occurs when the pulse duration and overlap have adequate values. At the same time, population trapping is also formed. Complete population transfer can also occurs when the two-photon resonance condition (△s = △p) is met.