Biomaterials,often imparted time-dependent mechanical properties,which are promising in fields rang-ing from sensors to robotics.Here,a facile method was proposed to fabricate post-tunable mechanical properties compos...Biomaterials,often imparted time-dependent mechanical properties,which are promising in fields rang-ing from sensors to robotics.Here,a facile method was proposed to fabricate post-tunable mechanical properties composites based on hydrogels and ceramic nanofiller.The wide tunable range of Young’s modulus(27.3 kPa to 3.5 GPa)and ultimate stress(173 kPa to 102 MPa)can be achieved by combining solvent absorption and evaporation process with platelets reinforcement effect.Additionally,a large fracture toughness(∼32,000 J m^(-2))is obtained as a result of the nacre-liked“brick and mortar”structure introduced by shear force during fabrication.The superior flexibility and designability of this material were demonstrated via actuators,portable structure,and metamaterials.Above all,this study provides a new thought to fabricate tough materials with post-tunable mechanical properties.展开更多
基金financial support provided by the Guangdong Provincial Department of Science and Technology (KeyArea Research and Development Program of Guangdong Province) under the grant 2020B090923002Shenzhen-Hong Kong Science and Technology Innovation Cooperation Zone Shenzhen Park Project (HZQB-KCZYB-2020030)+2 种基金National Key R&D Program of China (Project No. 2017YFA0204403)the Hong Kong Innovation and Technology Commission via the Hong Kong Branch of National Precious Metals Material Engineering Research Centerthe JLFS-RGC-joint Laboratory Funding Scheme (Reference No. JLFS/E103/18)
文摘Biomaterials,often imparted time-dependent mechanical properties,which are promising in fields rang-ing from sensors to robotics.Here,a facile method was proposed to fabricate post-tunable mechanical properties composites based on hydrogels and ceramic nanofiller.The wide tunable range of Young’s modulus(27.3 kPa to 3.5 GPa)and ultimate stress(173 kPa to 102 MPa)can be achieved by combining solvent absorption and evaporation process with platelets reinforcement effect.Additionally,a large fracture toughness(∼32,000 J m^(-2))is obtained as a result of the nacre-liked“brick and mortar”structure introduced by shear force during fabrication.The superior flexibility and designability of this material were demonstrated via actuators,portable structure,and metamaterials.Above all,this study provides a new thought to fabricate tough materials with post-tunable mechanical properties.
