This paper reports that a one-colour fs pump probe measurement has been carried out for studying photoionization/photodissociation of cyclohexanone （C6H10O） in intense laser field. Two of the fragments from eyclohex...This paper reports that a one-colour fs pump probe measurement has been carried out for studying photoionization/photodissociation of cyclohexanone （C6H10O） in intense laser field. Two of the fragments from eyclohexanone, C2H＋ and C3H3＋, are studied under 800 nm laser pump-probe and the results obtained show similar time evolutions. It proposes a feasible model for analysing the experimental observations of the one-colour fs pump-probe measurement. The results demonstrate that as an intermediate product, the excited molecular parent ions play a very important role in photionization/photodissociation processes in intense laser field.展开更多
We present new diagnostics for use in optical laser pump-X-ray Free Electron Laser(XFEL)probe experiments to monitor dimensions,intensity profile and focusability of the XFEL beam and to control initial quality and ho...We present new diagnostics for use in optical laser pump-X-ray Free Electron Laser(XFEL)probe experiments to monitor dimensions,intensity profile and focusability of the XFEL beam and to control initial quality and homogeneity of targets to be driven by optical laser pulse.By developing X-ray imaging,based on the use of an LiF crystal detector,we were able to measure the distribution of energy inside a hard X-ray beam with unprecedented high spatial resolution(~1 mm)and across a field of view larger than some millimetres.This diagnostic can be used in situ,provides a very high dynamic range,has an extremely limited cost,and is relatively easy to be implemented in pump-probe experiments.The proposed methods were successfully applied in pump-probe experiments at the SPring-8 Angstrom Compact free electron LAser(SACLA)XFEL facility and its potential was demonstrated for current and future High Energy Density Science experiments.展开更多
A terminal ballistic analysis of the effects of 7.62 mm × 51 AP P80 rounds on inclined high-strength armor steel plates is the focus of the presented study.The findings of an instrumented ballistic testing combin...A terminal ballistic analysis of the effects of 7.62 mm × 51 AP P80 rounds on inclined high-strength armor steel plates is the focus of the presented study.The findings of an instrumented ballistic testing combined with 3D advanced numerical simulations performed using the IMPETUS Afea? software yielded the conclusions.The experimental verification proved that slight differences in the pitch-andyaw angles of a projectile upon an impact caused different damage types to the projectile’s core.The residual velocities predicted numerically were close to the experimental values and the calculated core deviations were in satisfactory agreement with the experimental results.An extended matrix of the core deviation angles with combinations of pitch-and-yaw upon impact angles was subsequently built on the basis of the numerical study.The presented experimental and numerical investigation examined thoroughly the influence of the initial pitch and yaw angles on the after-perforation projectile’s performance.展开更多
Femtosecond laser-induced periodic surface structures(LIPSS)have been extensively studied over the past few decades.In particular,the period and groove width of high-spatial-frequency LIPSS(HSFL)is much smaller than t...Femtosecond laser-induced periodic surface structures(LIPSS)have been extensively studied over the past few decades.In particular,the period and groove width of high-spatial-frequency LIPSS(HSFL)is much smaller than the diffraction limit,making it a useful method for efficient nanomanufacturing.However,compared with the low-spatial-frequency LIPSS(LSFL),the structure size of the HSFL is smaller,and it is more easily submerged.Therefore,the formation mechanism of HSFL is complex and has always been a research hotspot in this field.In this study,regular LSFL with a period of 760 nm was fabricated in advance on a silicon surface with two-beam interference using an 800 nm,50 fs femtosecond laser.The ultrafast dynamics of HSFL formation on the silicon surface of prefabricated LSFL under single femtosecond laser pulse irradiation were observed and analyzed for the first time using collinear pump-probe imaging method.In general,the evolution of the surface structure undergoes five sequential stages:the LSFL begins to split,becomes uniform HSFL,degenerates into an irregular LSFL,undergoes secondary splitting into a weakly uniform HSFL,and evolves into an irregular LSFL or is submerged.The results indicate that the local enhancement of the submerged nanocavity,or the nanoplasma,in the prefabricated LSFL ridge led to the splitting of the LSFL,and the thermodynamic effect drove the homogenization of the splitting LSFL,which evolved into HSFL.展开更多
Shadowgraphic imaging was employed to investigate the mid-IR laser induced heat transfer through a double layer thin film. The effect of thin metal coat on the polymer film enhanced the transfer of heat and shock wave...Shadowgraphic imaging was employed to investigate the mid-IR laser induced heat transfer through a double layer thin film. The effect of thin metal coat on the polymer film enhanced the transfer of heat and shock waves due to rapid thermal expansion and the explosive evaporation of the thin fluid layer. Sixty two percent of deposited heat expended for water enthalpy and 38% for other factors. A power of 8.8 kW was launched at the surface of aluminium. The thermal coupling of 45% further reduced the input energy to the film and the non-adiabatic heat diffusion (i.e., ) was transmitted instantaneously within the metal with very small loss. The temperature at the surface of the film was determined ≈301 K, well below the aluminium melting point. The Biot number showed that the metal as single layer and the whole film as double layer satisfies the thermally thin film (i.e., ). Considering the Newtons’s law of cooling, the overall film heat transfer coefficient was found 3 k W·m-2·K-1 equivalent of 3.3 × 10-3 W·m2·K-1 thermal resistance. The analysis of images indicated a reducing percentage of heat transfer as a function of delay time based on the comparison of volume ratios. A calculated power of ≈3 kW was transmitted from the rear side of the film sufficient to thermalize the surrounding water layer and form vapor bubble.展开更多
Femtosecond laser technology has attracted significant attention from the viewpoints of fundamental and application;especially femtosecond laser processing materials present the unique mechanism of laser-material inte...Femtosecond laser technology has attracted significant attention from the viewpoints of fundamental and application;especially femtosecond laser processing materials present the unique mechanism of laser-material interaction.Under the extreme nonequilibrium conditions imposed by femtosecond laser irradiation,many fundamental questions concerning the physical origin of the material removal process remain unanswered.In this review,cutting-edge ultrafast dynamic observation techniques for investigating the fundamental questions,including timeresolved pump-probe shadowgraphy,ultrafast continuous optical imaging,and four-dimensional ultrafast scanning electron microscopy,are comprehensively surveyed.Each technique is described in depth,beginning with its basic principle,followed by a description of its representative applications in laser-material interaction and its strengths and limitations.The consideration of temporal and spatial resolutions and panoramic measurement at different scales are two major challenges.Hence,the prospects for technical advancement in this field are discussed finally.展开更多
Understanding shielding cross-effects is a prerequisite for maximal power-specific nanosecond laser ablation in liquids(LAL).However,discrimination between cavitation bubble(CB),nanoparticle(NP),and shielding,e.g.,by ...Understanding shielding cross-effects is a prerequisite for maximal power-specific nanosecond laser ablation in liquids(LAL).However,discrimination between cavitation bubble(CB),nanoparticle(NP),and shielding,e.g.,by the plasma or a transient vapor layer,is challenging.Therefore,CB imaging by shadowgraphy is performed to better understand the plasma and laser beam-NP interaction during LAL.By comparing the fluence-dependent CB volume for ablations performed with 1 ns pulses with reports from the literature,we find larger energy-specific CB volumes for 7 ns-ablation.The increased CB for laser ablation with higher ns pulse durations could be a first explanation of the efficiency decrease reported for these laser systems having higher pulse durations.Consequently,1 ns-LAL shows superior ablation efficiency.Moreover,a CB cascade occurs when the focal plane is shifted into the liquid.This effect is enhanced when NPs are present in the fluid.Even minute amounts of NPs trapped in a stationary layer decrease the laser energy significantly,even under liquid flow.However,this local concentration in the sticking film has so far not been considered.It presents an essential obstacle in high-yield LAL,shielding already the second laser pulse that arrives and presenting a source of satellite bubbles.Hence,measures to lower the NP concentration on the target must be investigated in the future.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No 10534010)
文摘This paper reports that a one-colour fs pump probe measurement has been carried out for studying photoionization/photodissociation of cyclohexanone （C6H10O） in intense laser field. Two of the fragments from eyclohexanone, C2H＋ and C3H3＋, are studied under 800 nm laser pump-probe and the results obtained show similar time evolutions. It proposes a feasible model for analysing the experimental observations of the one-colour fs pump-probe measurement. The results demonstrate that as an intermediate product, the excited molecular parent ions play a very important role in photionization/photodissociation processes in intense laser field.
基金The XFEL experiments were performed at the BL3 of SACLA with the approval of the Japan Synchrotron Radiation Research Institute(JASRI)(Proposals Nos.2014A8045,and 2014B8068)This research was partially supported by grants from Grants-in-Aid for Scientific Research(Kakenhi Grant Nos.15H02153 and 17K05729)+1 种基金the Core-to-Core Program on International Alliance for Material Science in Extreme States with High Power Laser of the Japan Society for the Promotion of Science(JSPS),from the X-ray Free Electron Laser Priority Strategy Program of the MEXT,contract 12005014,and within the state assignment of FASO of Russia(theme N01201357846)The part of work was supported by the Agence Nationale de la Recherche in the frame of the ANR project TurboHEDP(ANR-15-CE30-0011).
文摘We present new diagnostics for use in optical laser pump-X-ray Free Electron Laser(XFEL)probe experiments to monitor dimensions,intensity profile and focusability of the XFEL beam and to control initial quality and homogeneity of targets to be driven by optical laser pulse.By developing X-ray imaging,based on the use of an LiF crystal detector,we were able to measure the distribution of energy inside a hard X-ray beam with unprecedented high spatial resolution(~1 mm)and across a field of view larger than some millimetres.This diagnostic can be used in situ,provides a very high dynamic range,has an extremely limited cost,and is relatively easy to be implemented in pump-probe experiments.The proposed methods were successfully applied in pump-probe experiments at the SPring-8 Angstrom Compact free electron LAser(SACLA)XFEL facility and its potential was demonstrated for current and future High Energy Density Science experiments.
文摘A terminal ballistic analysis of the effects of 7.62 mm × 51 AP P80 rounds on inclined high-strength armor steel plates is the focus of the presented study.The findings of an instrumented ballistic testing combined with 3D advanced numerical simulations performed using the IMPETUS Afea? software yielded the conclusions.The experimental verification proved that slight differences in the pitch-andyaw angles of a projectile upon an impact caused different damage types to the projectile’s core.The residual velocities predicted numerically were close to the experimental values and the calculated core deviations were in satisfactory agreement with the experimental results.An extended matrix of the core deviation angles with combinations of pitch-and-yaw upon impact angles was subsequently built on the basis of the numerical study.The presented experimental and numerical investigation examined thoroughly the influence of the initial pitch and yaw angles on the after-perforation projectile’s performance.
基金supports from the National Natural Science Foundation of China(12074123,12174108)the Foundation of‘Manufacturing beyond limits’of Shanghai‘Talent Program'of Henan Academy of Sciences.
文摘Femtosecond laser-induced periodic surface structures(LIPSS)have been extensively studied over the past few decades.In particular,the period and groove width of high-spatial-frequency LIPSS(HSFL)is much smaller than the diffraction limit,making it a useful method for efficient nanomanufacturing.However,compared with the low-spatial-frequency LIPSS(LSFL),the structure size of the HSFL is smaller,and it is more easily submerged.Therefore,the formation mechanism of HSFL is complex and has always been a research hotspot in this field.In this study,regular LSFL with a period of 760 nm was fabricated in advance on a silicon surface with two-beam interference using an 800 nm,50 fs femtosecond laser.The ultrafast dynamics of HSFL formation on the silicon surface of prefabricated LSFL under single femtosecond laser pulse irradiation were observed and analyzed for the first time using collinear pump-probe imaging method.In general,the evolution of the surface structure undergoes five sequential stages:the LSFL begins to split,becomes uniform HSFL,degenerates into an irregular LSFL,undergoes secondary splitting into a weakly uniform HSFL,and evolves into an irregular LSFL or is submerged.The results indicate that the local enhancement of the submerged nanocavity,or the nanoplasma,in the prefabricated LSFL ridge led to the splitting of the LSFL,and the thermodynamic effect drove the homogenization of the splitting LSFL,which evolved into HSFL.
文摘Shadowgraphic imaging was employed to investigate the mid-IR laser induced heat transfer through a double layer thin film. The effect of thin metal coat on the polymer film enhanced the transfer of heat and shock waves due to rapid thermal expansion and the explosive evaporation of the thin fluid layer. Sixty two percent of deposited heat expended for water enthalpy and 38% for other factors. A power of 8.8 kW was launched at the surface of aluminium. The thermal coupling of 45% further reduced the input energy to the film and the non-adiabatic heat diffusion (i.e., ) was transmitted instantaneously within the metal with very small loss. The temperature at the surface of the film was determined ≈301 K, well below the aluminium melting point. The Biot number showed that the metal as single layer and the whole film as double layer satisfies the thermally thin film (i.e., ). Considering the Newtons’s law of cooling, the overall film heat transfer coefficient was found 3 k W·m-2·K-1 equivalent of 3.3 × 10-3 W·m2·K-1 thermal resistance. The analysis of images indicated a reducing percentage of heat transfer as a function of delay time based on the comparison of volume ratios. A calculated power of ≈3 kW was transmitted from the rear side of the film sufficient to thermalize the surrounding water layer and form vapor bubble.
基金supported by the National Natural Science Foundation of China under Grant Nos.51975054,61605140 and 11704028the National Key R&D Program of China(2017YFB1104300)。
文摘Femtosecond laser technology has attracted significant attention from the viewpoints of fundamental and application;especially femtosecond laser processing materials present the unique mechanism of laser-material interaction.Under the extreme nonequilibrium conditions imposed by femtosecond laser irradiation,many fundamental questions concerning the physical origin of the material removal process remain unanswered.In this review,cutting-edge ultrafast dynamic observation techniques for investigating the fundamental questions,including timeresolved pump-probe shadowgraphy,ultrafast continuous optical imaging,and four-dimensional ultrafast scanning electron microscopy,are comprehensively surveyed.Each technique is described in depth,beginning with its basic principle,followed by a description of its representative applications in laser-material interaction and its strengths and limitations.The consideration of temporal and spatial resolutions and panoramic measurement at different scales are two major challenges.Hence,the prospects for technical advancement in this field are discussed finally.
基金We thank the Deutsche Forschungsgemeinschaft(DFG)for funding within the grants GO 2566/7-1 and GO 2566/8-1.
文摘Understanding shielding cross-effects is a prerequisite for maximal power-specific nanosecond laser ablation in liquids(LAL).However,discrimination between cavitation bubble(CB),nanoparticle(NP),and shielding,e.g.,by the plasma or a transient vapor layer,is challenging.Therefore,CB imaging by shadowgraphy is performed to better understand the plasma and laser beam-NP interaction during LAL.By comparing the fluence-dependent CB volume for ablations performed with 1 ns pulses with reports from the literature,we find larger energy-specific CB volumes for 7 ns-ablation.The increased CB for laser ablation with higher ns pulse durations could be a first explanation of the efficiency decrease reported for these laser systems having higher pulse durations.Consequently,1 ns-LAL shows superior ablation efficiency.Moreover,a CB cascade occurs when the focal plane is shifted into the liquid.This effect is enhanced when NPs are present in the fluid.Even minute amounts of NPs trapped in a stationary layer decrease the laser energy significantly,even under liquid flow.However,this local concentration in the sticking film has so far not been considered.It presents an essential obstacle in high-yield LAL,shielding already the second laser pulse that arrives and presenting a source of satellite bubbles.Hence,measures to lower the NP concentration on the target must be investigated in the future.
