The comparative study of technogenic ^(90)Sr behavior features in Crimea lakes’ ecosystems with different levels of salinity was carried out in 2016-2021.Two sources of ^(90)Sr input were identified for all the studi...The comparative study of technogenic ^(90)Sr behavior features in Crimea lakes’ ecosystems with different levels of salinity was carried out in 2016-2021.Two sources of ^(90)Sr input were identified for all the studied lakes:the primary source concerned with atmospheric fallout immediately after the Chernobyl NPP accident and the secondary long-term input of this radionuclide by waterway.The half-life of the ^(90)Sr concentration in the water of the hypers aline Lake Sasyk-Sivash was estimated to vary from 0.8 to 1.1 years after the closure of the North Crimean Canal(NCC).Biogeochemical processes in the lake under the absence of the secondary source of the radionuclide input were shown to decrease in the ^(90)Sr residence time in the water column by 131 times.For brackish water bodies,a significant factor influencing the radionuclide concentration in ecosystems of lakes was the pH of their water,while for hypers aline lakes the level of water salinity was the main factor determining ^(90)Sr behavior.The concentration of ^(90)Sr in bottom sediments of studied lakes depended mainly on this radionuclide concentration in a water environment.Calculated ^(90)Sr distribution factors(Kd) for studied lakes’ bottom sediments varied in a range of n·10^(0)÷n·10^(2) for hypersaline lakes and of n·10^(1)÷n·10^(2) for lakes with brackish waters.Due to the closure of the NCC,the ^(90)Sr redistribution took place in lake ecosystems only under the geochemical processes within the water bodies themselves.The results obtained in this work are of particular importance as a starting point or a basis for further radioecological studies of the Crimean inland waters after the reopening of the NCC and the Dnieper waters re-entering the territory of Crimea in 2022after the 8 years of their absence.展开更多
对美国3M公司的锶特效固相萃取片(EmporeTMStrontium Rad Disk)分离水溶液中锶离子的性能进行了系统研究,包括酸度、流速、样品体积对吸附百分比的影响,吸附容量的测定,137 Cs和99 Tc在萃取片上的吸附情况等,并对萃取片上90Sr的解吸及片...对美国3M公司的锶特效固相萃取片(EmporeTMStrontium Rad Disk)分离水溶液中锶离子的性能进行了系统研究,包括酸度、流速、样品体积对吸附百分比的影响,吸附容量的测定,137 Cs和99 Tc在萃取片上的吸附情况等,并对萃取片上90Sr的解吸及片上90Sr的放射性测量进行了研究。在此基础上,给出了萃取片法分析环境水中90Sr的推荐程序。样品体积为1L,液闪测量时间为1h时,分析程序的最小可探测活度浓度为0.033Bq/L。最后应用一些实际环境水样对该程序进行了检验。展开更多
基金Scientific research on salt and brackish water lakes was supported by the Russian Science Foundation,with grant No.18-16-00001Development of biological and geochemical foundations for the development of aquaculture in hypersaline lakes and lagoons of Crimea,2021-2022Comparative studies on the Black Sea were carried out within the framework of the State Assignment for the IBSS,Molismological and biogeochemical foundations of the homeostasis of marine ecosystems,with State registration number of the state assignment 121031500515-8。
文摘The comparative study of technogenic ^(90)Sr behavior features in Crimea lakes’ ecosystems with different levels of salinity was carried out in 2016-2021.Two sources of ^(90)Sr input were identified for all the studied lakes:the primary source concerned with atmospheric fallout immediately after the Chernobyl NPP accident and the secondary long-term input of this radionuclide by waterway.The half-life of the ^(90)Sr concentration in the water of the hypers aline Lake Sasyk-Sivash was estimated to vary from 0.8 to 1.1 years after the closure of the North Crimean Canal(NCC).Biogeochemical processes in the lake under the absence of the secondary source of the radionuclide input were shown to decrease in the ^(90)Sr residence time in the water column by 131 times.For brackish water bodies,a significant factor influencing the radionuclide concentration in ecosystems of lakes was the pH of their water,while for hypers aline lakes the level of water salinity was the main factor determining ^(90)Sr behavior.The concentration of ^(90)Sr in bottom sediments of studied lakes depended mainly on this radionuclide concentration in a water environment.Calculated ^(90)Sr distribution factors(Kd) for studied lakes’ bottom sediments varied in a range of n·10^(0)÷n·10^(2) for hypersaline lakes and of n·10^(1)÷n·10^(2) for lakes with brackish waters.Due to the closure of the NCC,the ^(90)Sr redistribution took place in lake ecosystems only under the geochemical processes within the water bodies themselves.The results obtained in this work are of particular importance as a starting point or a basis for further radioecological studies of the Crimean inland waters after the reopening of the NCC and the Dnieper waters re-entering the territory of Crimea in 2022after the 8 years of their absence.
文摘对美国3M公司的锶特效固相萃取片(EmporeTMStrontium Rad Disk)分离水溶液中锶离子的性能进行了系统研究,包括酸度、流速、样品体积对吸附百分比的影响,吸附容量的测定,137 Cs和99 Tc在萃取片上的吸附情况等,并对萃取片上90Sr的解吸及片上90Sr的放射性测量进行了研究。在此基础上,给出了萃取片法分析环境水中90Sr的推荐程序。样品体积为1L,液闪测量时间为1h时,分析程序的最小可探测活度浓度为0.033Bq/L。最后应用一些实际环境水样对该程序进行了检验。
