Radon(Rn)is a naturally occurring radioactive inert gas in nature,and^(222)Rn has been routinely used as a powerful tracer in various aquatic environmental research on timescales of hours to days,such as submarine gro...Radon(Rn)is a naturally occurring radioactive inert gas in nature,and^(222)Rn has been routinely used as a powerful tracer in various aquatic environmental research on timescales of hours to days,such as submarine groundwater discharge.Here we developed a new approach to measure^(222)Rn in discrete water samples with a wide range of^(222)Rn concentrations using a Pulsed Ionization Chamber(PIC)Radon Detector.The sensitivity of the new PIC system is evaluated at 6.06 counts per minute for 1 Bq/L when a 500 mL water sample volume is used.A robust logarithmic correlation between sample volumes,ranging from 250 mL to 5000 mL,and system sensitivity obtained in this study strongly suggests that this approach is suitable for measuring radon concentration levels in various natural waters.Compared to the currently available methods for measuring radon in grab samples,the PIC system is cheaper,easier to operate and does not require extra accessories(e.g.,drying tubes etc.)to maintain stable measurements throughout the counting procedure.展开更多
We solve the Riemann problems for isentropic compressible Euler equations of polytropic gases in the class of Radon measures,and the solutions admit the concentration of mass.It is found that under the requirement of ...We solve the Riemann problems for isentropic compressible Euler equations of polytropic gases in the class of Radon measures,and the solutions admit the concentration of mass.It is found that under the requirement of satisfying the over-compressing entropy condition:(i)there is a unique delta shock solution,corresponding to the case that has two strong classical Lax shocks;(ii)for the initial data that the classical Riemann solution contains a shock wave and a rarefaction wave,or two shocks with one being weak,there are infinitely many solutions,each consists of a delta shock and a rarefaction wave;(iii)there are no delta shocks for the case that the classical entropy weak solutions consist only of rarefaction waves.These solutions are self-similar.Furthermore,for the generalized Riemann problem with mass concentrated initially at the discontinuous point of initial data,there always exists a unique delta shock for at least a short time.It could be prolonged to a global solution.Not all the solutions are self-similar due to the initial velocity of the concentrated point-mass(particle).Whether the delta shock solutions constructed satisfy the over-compressing entropy condition is clarified.This is the first result on the construction of singular measure solutions to the compressible Euler system of polytropic gases,that is strictly hyperbolic,and whose characteristics are both genuinely nonlinear.We also discuss possible physical interpretations and applications of these new solutions.展开更多
Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been dev...Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been developed to some extent but still lack underwater in-situ measurements.Here we present an in-situ detection equipment for radon-in-water(pulsed ionization chamber(PIC)-radon)to measure dissolved radon in ocean and groundwater settings.The equipment has been successfully deployed in the Jiaozhou Bay in July 2022 and has achieved 14 d of unattended underwater in-situ observation.Then it was successfully placed in a groundwater monitoring well in the Laizhou Bay in November 2022 and monitored radon activities for over 30 d.The results showed that this instrument had a good indication of submarine groundwater discharge.The PIC-radon detector takes advantage of smaller size,lower power consumption,and is barely influenced by humidity,making it particularly suitable for long-term in-situ measurement,especially in harsh environments with limited human care or deployment spaces.展开更多
Soil radon measurement of high stability and sensitivity is widely applied,and in some applications,such as in uranium prospecting,^(222)Rn should be distinguished from ^(220)Rn.To meet this requirement,a practical me...Soil radon measurement of high stability and sensitivity is widely applied,and in some applications,such as in uranium prospecting,^(222)Rn should be distinguished from ^(220)Rn.To meet this requirement,a practical method based on soil radon diffusion and accumulation theory to measure soil radon by Alpha Particle Spectroscopy(α-PS)is discussed in this paper.Theα-PS measurement method can effectively overcome the effects of ^(220)Rn and its daughters (^(216)Po,^(212)Bi,^(212)Po).The system can eliminate the impact of soil radon field disturbance and non-uniformity through soil radon static diffusion.Radon daughters(^(218)Po,^(214)Po)are accumulated under the action of an electrostatic force, which not only enhances the measurement sensitivity,but also increases robustness of the measurement.Simultaneous measurement of multiple points can increase the comparability of measurement data and the measurement efficiency. Experimental data shows that the soil radon measurement method was robust.So it has wide applications such as in geological prospecting,in fissure groundwater exploration and in ground subsidence inspection.展开更多
基金The National Natural Science Foundation of China under contract Nos 42130410,41876075 and U1906210the Fundamental Research Funds for the Central Universities under contract No.201962003.
文摘Radon(Rn)is a naturally occurring radioactive inert gas in nature,and^(222)Rn has been routinely used as a powerful tracer in various aquatic environmental research on timescales of hours to days,such as submarine groundwater discharge.Here we developed a new approach to measure^(222)Rn in discrete water samples with a wide range of^(222)Rn concentrations using a Pulsed Ionization Chamber(PIC)Radon Detector.The sensitivity of the new PIC system is evaluated at 6.06 counts per minute for 1 Bq/L when a 500 mL water sample volume is used.A robust logarithmic correlation between sample volumes,ranging from 250 mL to 5000 mL,and system sensitivity obtained in this study strongly suggests that this approach is suitable for measuring radon concentration levels in various natural waters.Compared to the currently available methods for measuring radon in grab samples,the PIC system is cheaper,easier to operate and does not require extra accessories(e.g.,drying tubes etc.)to maintain stable measurements throughout the counting procedure.
基金supported by the National Natural Science Foundation of China under Grants No.11871218,No.12071298the Science and Technology Commission of Shanghai Municipality under Grant No.18dz2271000.
文摘We solve the Riemann problems for isentropic compressible Euler equations of polytropic gases in the class of Radon measures,and the solutions admit the concentration of mass.It is found that under the requirement of satisfying the over-compressing entropy condition:(i)there is a unique delta shock solution,corresponding to the case that has two strong classical Lax shocks;(ii)for the initial data that the classical Riemann solution contains a shock wave and a rarefaction wave,or two shocks with one being weak,there are infinitely many solutions,each consists of a delta shock and a rarefaction wave;(iii)there are no delta shocks for the case that the classical entropy weak solutions consist only of rarefaction waves.These solutions are self-similar.Furthermore,for the generalized Riemann problem with mass concentrated initially at the discontinuous point of initial data,there always exists a unique delta shock for at least a short time.It could be prolonged to a global solution.Not all the solutions are self-similar due to the initial velocity of the concentrated point-mass(particle).Whether the delta shock solutions constructed satisfy the over-compressing entropy condition is clarified.This is the first result on the construction of singular measure solutions to the compressible Euler system of polytropic gases,that is strictly hyperbolic,and whose characteristics are both genuinely nonlinear.We also discuss possible physical interpretations and applications of these new solutions.
基金The National Natural Science Foundation of China under contract Nos U22A20580 and 42130410the Fundamental Research Funds for the Central Universities under contract No.202341002the Pilot Project for the Integration of Science,Education,and Industry under contract No.2022PY069.
文摘Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been developed to some extent but still lack underwater in-situ measurements.Here we present an in-situ detection equipment for radon-in-water(pulsed ionization chamber(PIC)-radon)to measure dissolved radon in ocean and groundwater settings.The equipment has been successfully deployed in the Jiaozhou Bay in July 2022 and has achieved 14 d of unattended underwater in-situ observation.Then it was successfully placed in a groundwater monitoring well in the Laizhou Bay in November 2022 and monitored radon activities for over 30 d.The results showed that this instrument had a good indication of submarine groundwater discharge.The PIC-radon detector takes advantage of smaller size,lower power consumption,and is barely influenced by humidity,making it particularly suitable for long-term in-situ measurement,especially in harsh environments with limited human care or deployment spaces.
文摘Soil radon measurement of high stability and sensitivity is widely applied,and in some applications,such as in uranium prospecting,^(222)Rn should be distinguished from ^(220)Rn.To meet this requirement,a practical method based on soil radon diffusion and accumulation theory to measure soil radon by Alpha Particle Spectroscopy(α-PS)is discussed in this paper.Theα-PS measurement method can effectively overcome the effects of ^(220)Rn and its daughters (^(216)Po,^(212)Bi,^(212)Po).The system can eliminate the impact of soil radon field disturbance and non-uniformity through soil radon static diffusion.Radon daughters(^(218)Po,^(214)Po)are accumulated under the action of an electrostatic force, which not only enhances the measurement sensitivity,but also increases robustness of the measurement.Simultaneous measurement of multiple points can increase the comparability of measurement data and the measurement efficiency. Experimental data shows that the soil radon measurement method was robust.So it has wide applications such as in geological prospecting,in fissure groundwater exploration and in ground subsidence inspection.
