Herein, a stable and efficient CoS_(2)-ReS_(2) electrocatalyst is successfully constructed by using the different molar ratios of CoS_(2) on ReS_(2). The size and morphology of the catalysts are significantly changed ...Herein, a stable and efficient CoS_(2)-ReS_(2) electrocatalyst is successfully constructed by using the different molar ratios of CoS_(2) on ReS_(2). The size and morphology of the catalysts are significantly changed after the CoS_(2) is grown on ReS_(2), providing regulation of the catalytic activity of ReS_(2). Particularly, the optimized CoS_(2)-ReS_(2) shows superior electrocatalytic properties with a low voltage of 1.48 V at 20 mA cm^(-2) for overall water splitting in 1.0 M KOH, which is smaller than the noble metal-based catalysts(1.77 V at 20 mA cm^(-2)). The XPS, XAS, and theoretical data confirm that the interfacial regulation of ReS_(2) by CoS_(2) can provide rich edge catalytic sites, which greatly optimizes the catalytic kinetics and drop the energy barrier for oxygen/hydrogen evolution reactions. Our results demonstrated that interfacial engineering is an efficient route for fabricating high-performance water splitting electrocatalysts.展开更多
Photodetectors based on two-dimensional materials have attracted much attention because of their unique structure and outstanding performance.The response speed of single ReS_(2)photodetector is slow exceptionally,the...Photodetectors based on two-dimensional materials have attracted much attention because of their unique structure and outstanding performance.The response speed of single ReS_(2)photodetector is slow exceptionally,the heterostructure could improves the response speed of ReS_(2)-based photodetector,but the photodetectors responsivity is reduced greatly,which restricts the development of ReS_(2).In this paper,a vertically structured ReS_(2)/SnS_(2)van der Waals heterostructure photodetectors is prepared,using ReS_(2)as the transport layer and SnS_(2)as the light absorbing layer to regulate the channel current.The device has an ultra-high photoconductive gain of 10^(10),which exhibits an ultra-high responsivity of4706 A/W under 365-nm illumination and response speed in seconds,and has an ultra-high external quantum efficiency of1.602×10^(6)%and a high detectivity of 5.29×10^(12)jones.The study for ReS_(2)-based photodetector displays great potential for developing future optoelectronic devices.展开更多
The magnitude and spatial variability of CO_(2)surface emissions and processes involving CO_(2)released to the atmosphere from the soils are relevant issues in the context of climate change.This work evaluated CO_(2)f...The magnitude and spatial variability of CO_(2)surface emissions and processes involving CO_(2)released to the atmosphere from the soils are relevant issues in the context of climate change.This work evaluated CO_(2)fluxes and^(13)C/^(12)C ratio of vegetation,organic matter,and soil gases from no disturbed soils of Chaco Pampean Plain(Argentina)with different soil properties and environmental conditions(PL and PA units).Soil organic decomposition from individual layers was accompanied byδ^(13)C of total organic carbon(δ^(13)C-TOC)values more enriched to depth.δ^(13)C-TOC values in the upper soil profile~ca.0–15 cm were like the plant community of this area(~−33 to−29‰)whileδ^(13)CTOC varied stronger bellow horizon A,till~−24‰.Bothδ^(13)C-TOC and soilδ^(13)C-CO_(2)were similar(~−24 to 26‰)at deeper horizons(~50–60 cm).Toward the superficial layers,δ^(13)C-TOC andδ^(13)C-CO_(2)showed more differences(till~4‰),due influence of the diffusion process.Horizon A layer(~0–20 cm)from both PL and PA units contained the most enrichedδ^(13)C-CO_(2)values(~−15–17‰)because atmospheric CO_(2)permeated the soil air.A simple two-component mixing model between sources(atmosphericδ^(13)C-CO_(2)and soil CO_(2))confirmed that process.Isotopically,CO_(2)fluxes reflected the biodegradation of C3 plants(source),diffusive transport,and CO_(2)exchange(atmosphere/soil).Soil moisture content appeared as a determining factor in the diffusion process and the magnitude of CO_(2)surface emissions(12–60 g·m^(−2)·d^(−1)).That condition was confirmed by CO_(2)diffusion coefficients estimated by air-filled porosity parameters and soil radon gradient model.展开更多
This study determines if there is a correlation between rising carbon dioxide levels and global warming. Historical data were reviewed from three different time periods spanning 500 million years. It showed that the c...This study determines if there is a correlation between rising carbon dioxide levels and global warming. Historical data were reviewed from three different time periods spanning 500 million years. It showed that the curves and trends were too dissimilar to establish a connection. Observations from CO<sub>2</sub>/temp ratios showed that the CO<sub>2</sub> and the temperature moved in opposite directions 42% of the time. Many ratios displayed zero or near zero values, reflecting a lack of response. As much as 87% of the ratios revealed negative or near zero values, which strongly negate a correlation. The infrared spectra showed the Greenhouse Gases had an exceptionally low absorption band between 11.67 μm to 9.1 μm, which is a zone called the infrared atmospheric window. Most of the Greenhouse Gases absorb little infrared inside that zone. And that zone is where the Earth’s surface emits almost all infrared radiation. Even with minimal absorbance, water vapor captures the most infrared radiation. It absorbs 84 times more than CO<sub>2</sub>, 407 thousand times more than methane, 452 thousand times more than ozone and 2.3 million times more than nitrous oxide. The Intergovernmental Panel on Climate Change (IPCC) and the United States EPA excluded water vapor because it was not associated with man-made activities. They reported that water vapor and clouds were simply feedback mechanisms from CO<sub>2</sub>. Clouds reflect radiation from the sun. The Northern Hemisphere is 2.7°F warmer than the Southern Hemisphere because of clouds. The world cloud cover has gone down 4.1% from 1982 to 2018. Calculations show that this could be responsible for 2.4°F of the 2.7°F. The research shows that most of the recent increase in temperature (89.9%) is because of fewer clouds.展开更多
We measured the IR back radiation using a relatively low-cost experimental setup and a test chamber with increasing CO2 concentrations starting with a pure N2 atmosphere against a temperature-controlled black referenc...We measured the IR back radiation using a relatively low-cost experimental setup and a test chamber with increasing CO2 concentrations starting with a pure N2 atmosphere against a temperature-controlled black reference background. The results confirm estimations within this work and previous finding about CO2-induced infrared radiation saturation within realistic atmospheric conditions. We used this setup also to study thermal forcing effects with stronger and rare greenhouse gases against a clear night sky. Our results and their interpretation are another indication for having a more critical approach in climate modelling and against monocausal interpretation of climate indices only caused by anthropogenic greenhouse gas emissions. Basic physics combined with measurements and data taken from the literature allow us to conclude that CO2 induced infrared back-radiation must follow an asymptotic logarithmic-like behavior, which is also widely accepted in the climate-change community. The important question of climate sensitivity by doubling current CO2 concentrations is estimated to be below 1˚C. This value is important when the United Nations consider climate change as an existential threat and many governments intend rigorously to reduce net greenhouse gas emissions, led by an ambitious European Union inspired by IPCC assessments is targeting for more than 55% in 2030 and up to 100% in 2050 [1]. But probably they should also listen to experts [2] [3] who found that all these predictions have considerable flaws in basic models, data and impact scenarios.展开更多
Two-dimensional(2D)materials have gained considerable attention in chemical sensing owing to their naturally high surface-to-volume ratio.However,the poor response time and incomplete recovery re-strict their applicat...Two-dimensional(2D)materials have gained considerable attention in chemical sensing owing to their naturally high surface-to-volume ratio.However,the poor response time and incomplete recovery re-strict their application in practical,high performance gas sensors.In this work,we fabricated air-stable ReS_(2)/GaSe heterostructure-based NO_(2)gas sensors with excellent gas sensing response,recovery,selectiv-ity and a low limit of detection(LOD)toward nitrogen dioxide(NO_(2)).The ReS_(2)/GaSe heterostructure was prepared via mechanical exfoliation and an all-dry transfer method.Before the sensing measurements,temperature-dependant transport measurements were carried out.The Schottky Barrier Height(SBH)of the ReS_(2)/GaSe heterostructure was calculated and the corresponding transport mechanisms were dis-cussed.The fabricated gas sensors showed a significant response enhancement with full reversibility to-ward ppm-level NO_(2)(response of∼17%at 3 ppm,a LOD of∼556 ppb)at an operating temperature of(33°C).In particular,the total response and recovery time of the ReS_(2)/GaSe was revealed to be less than 4 min(∼38 s and∼174 s,respectively)for the 250 ppm concentration,which is one of the best response and recovery time toward ppm-level NO_(2).The excellent sensing performances and recovery characteris-tics of the ReS_(2)/GaSe structure are attributed to its efficient charge separation,unique interlayer coupling and desirable band alignments.This atomically thin,ultrasensitive gas sensor that operates at room tem-perature is a strong technological contender to conventional metal oxide gas sensors,which often require elevated temperatures.展开更多
Ni/ZrO2 catalysts were prepared by the incipient-wetness impregnation method and were investigated in activity and selectivity for the selective catalytic methanation of CO in hydrogen-rich gases with more than 20 vol...Ni/ZrO2 catalysts were prepared by the incipient-wetness impregnation method and were investigated in activity and selectivity for the selective catalytic methanation of CO in hydrogen-rich gases with more than 20 vol% CO2. The result showed that Ni loadings significantly influenced the performance of Ni/ZrO2 catalyst. The 1.6 wt% Ni loading catalyst exhibited the highest catalytic activity among all the catalysts in the selective methanation of CO in hydrogen-rich gas. The outlet concentration of CO was less than 20 ppm with the hydrogen consumption below 7%, at a gas-hourly-space velocity as high as 10000 h-1 and a temperature range of 260 °C to 280 °C. The X-ray diffraction (XRD) and temperature programmed reduction (TPR) measurements showed that NiO was dispersed thoroughly on the surface of ZrO2 support if Ni loading was under 1.6 wt%. When Ni loading was increased to 3 wt% or above, the free bulk NiO species began to assemble, which was not favorable to increase the selectivity of the catalyst.展开更多
In order to reduce the number of accidents due to explosions of flammable gases in the goaf of coalmines,the conditions for explosion of flammable gases and their explosion limits,affected to a considerable extent by ...In order to reduce the number of accidents due to explosions of flammable gases in the goaf of coalmines,the conditions for explosion of flammable gases and their explosion limits,affected to a considerable extent by CO2,are explored.With the use of our experimental equipment suitable for the study of explosion of polybasic explosive gas mixtures,we investigated the effect of CH4/H2=10/1 and CH4/C2H4=10/1 gases mixed with CO2 on their explosion limits.The results indicate that after adding CO2,the explosion limit of the CH4/H2(or C2H4) =10/1 gas mixtures decreased markedly with increasing amounts of CO2.When the amount of CO2 exceeded 25%,the CH4/C2H4=10/1 flammable gas mixture did not lead to explosions.Similar results were obtained when the amount of CO2 exceeded 23% in the CH4/H2=10/1 flammable gas mixture.We also compared the explosion limits and the explosion suppression effect of N2 or CO2 on the explosion limits of the CH4+CO and CH4+C2H4 dual explosive gas mixtures.Along with the increases in the amounts of CO2 or N2,the area of the explosion limits of gas mixtures decreased.Under the same conditions,the explosion suppression effect of CO2 was greater than that of N2.CO2 has clearly the better suppression effect on the explosion of flammable gases in goafs.展开更多
Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gas...Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gases in China and its policy implications. The results show that at present, China is a country with the greatest emission of non-CO2 greenhouse gases in the world, and the emission will account for about 20% of the world's total emission in 2020. The proportion of emission of non-CO2 greenhouse gases from the agricultural sector reaches 73%. In the next 10 years, the emission of non-CO2 gases from cattle and sheep, industry and service industry will experience the highest growth rate; the growth rate of emission from service industry will be higher than that of emission from industry, and the emission from service industry will exceed that from industry after 2010. China can implement emission reduction policy of non-CO2 greenhouse gases to ease the international pressure of CO2 emission reduction. Although the high carbon tax collected can reduce considerable non-CO2 emission, there is little difference in policy efficiency between high carbon tax and low carbon tax. So, in the implementation of emission reduction carbon tax policy of non-CO2 gases, it is necessary to control the carbon tax at a low level.展开更多
基金supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT)(NRF-2022R1A2C2093415) and (NRF-2018R1A2B6006721)Institute for Basic Science of Korea (IBS-R011-D1)the Korea Medical Device Development Fund grant funded by the Korean government (the Ministry of Science and ICT, the Ministry of Trade, Industry and Energy, the Ministry of Health & Welfare, the Ministry of Food and Drug Safety) (Project Number: KMDF_PR_20200901_0004)。
文摘Herein, a stable and efficient CoS_(2)-ReS_(2) electrocatalyst is successfully constructed by using the different molar ratios of CoS_(2) on ReS_(2). The size and morphology of the catalysts are significantly changed after the CoS_(2) is grown on ReS_(2), providing regulation of the catalytic activity of ReS_(2). Particularly, the optimized CoS_(2)-ReS_(2) shows superior electrocatalytic properties with a low voltage of 1.48 V at 20 mA cm^(-2) for overall water splitting in 1.0 M KOH, which is smaller than the noble metal-based catalysts(1.77 V at 20 mA cm^(-2)). The XPS, XAS, and theoretical data confirm that the interfacial regulation of ReS_(2) by CoS_(2) can provide rich edge catalytic sites, which greatly optimizes the catalytic kinetics and drop the energy barrier for oxygen/hydrogen evolution reactions. Our results demonstrated that interfacial engineering is an efficient route for fabricating high-performance water splitting electrocatalysts.
基金the National Natural Science Foundation of China(Grant Nos.61574011,60908012,61575008,61775007,61731019,61874145,62074011,and 62134008)the Beijing Natural Science Foundation(Grant Nos.4182015,4172011,and 4202010)Beijing Nova Program(Grant No.Z201100006820096)。
文摘Photodetectors based on two-dimensional materials have attracted much attention because of their unique structure and outstanding performance.The response speed of single ReS_(2)photodetector is slow exceptionally,the heterostructure could improves the response speed of ReS_(2)-based photodetector,but the photodetectors responsivity is reduced greatly,which restricts the development of ReS_(2).In this paper,a vertically structured ReS_(2)/SnS_(2)van der Waals heterostructure photodetectors is prepared,using ReS_(2)as the transport layer and SnS_(2)as the light absorbing layer to regulate the channel current.The device has an ultra-high photoconductive gain of 10^(10),which exhibits an ultra-high responsivity of4706 A/W under 365-nm illumination and response speed in seconds,and has an ultra-high external quantum efficiency of1.602×10^(6)%and a high detectivity of 5.29×10^(12)jones.The study for ReS_(2)-based photodetector displays great potential for developing future optoelectronic devices.
基金Financial support was provided through the Instituto de Geociencias Básicas,Aplicadas y Ambientales de Buenos Aires(IGEBA)and the Instituto de Geocronología y Geología Isotópica(INGEIS),both dependent of the Consejo Nacional de Investigaciones Científi cas y Técnicas(National Council for Scientific and Technological Research),and the Universidad de Buenos Aires(Buenos Aires University)of Argentinasupported by the Agencia Nacional de Promoción Científi ca y Tecnológica(National Agency for Scientific and Technological Promotion)projects PICT2010-0035 and PICT2010-2749。
文摘The magnitude and spatial variability of CO_(2)surface emissions and processes involving CO_(2)released to the atmosphere from the soils are relevant issues in the context of climate change.This work evaluated CO_(2)fluxes and^(13)C/^(12)C ratio of vegetation,organic matter,and soil gases from no disturbed soils of Chaco Pampean Plain(Argentina)with different soil properties and environmental conditions(PL and PA units).Soil organic decomposition from individual layers was accompanied byδ^(13)C of total organic carbon(δ^(13)C-TOC)values more enriched to depth.δ^(13)C-TOC values in the upper soil profile~ca.0–15 cm were like the plant community of this area(~−33 to−29‰)whileδ^(13)CTOC varied stronger bellow horizon A,till~−24‰.Bothδ^(13)C-TOC and soilδ^(13)C-CO_(2)were similar(~−24 to 26‰)at deeper horizons(~50–60 cm).Toward the superficial layers,δ^(13)C-TOC andδ^(13)C-CO_(2)showed more differences(till~4‰),due influence of the diffusion process.Horizon A layer(~0–20 cm)from both PL and PA units contained the most enrichedδ^(13)C-CO_(2)values(~−15–17‰)because atmospheric CO_(2)permeated the soil air.A simple two-component mixing model between sources(atmosphericδ^(13)C-CO_(2)and soil CO_(2))confirmed that process.Isotopically,CO_(2)fluxes reflected the biodegradation of C3 plants(source),diffusive transport,and CO_(2)exchange(atmosphere/soil).Soil moisture content appeared as a determining factor in the diffusion process and the magnitude of CO_(2)surface emissions(12–60 g·m^(−2)·d^(−1)).That condition was confirmed by CO_(2)diffusion coefficients estimated by air-filled porosity parameters and soil radon gradient model.
文摘This study determines if there is a correlation between rising carbon dioxide levels and global warming. Historical data were reviewed from three different time periods spanning 500 million years. It showed that the curves and trends were too dissimilar to establish a connection. Observations from CO<sub>2</sub>/temp ratios showed that the CO<sub>2</sub> and the temperature moved in opposite directions 42% of the time. Many ratios displayed zero or near zero values, reflecting a lack of response. As much as 87% of the ratios revealed negative or near zero values, which strongly negate a correlation. The infrared spectra showed the Greenhouse Gases had an exceptionally low absorption band between 11.67 μm to 9.1 μm, which is a zone called the infrared atmospheric window. Most of the Greenhouse Gases absorb little infrared inside that zone. And that zone is where the Earth’s surface emits almost all infrared radiation. Even with minimal absorbance, water vapor captures the most infrared radiation. It absorbs 84 times more than CO<sub>2</sub>, 407 thousand times more than methane, 452 thousand times more than ozone and 2.3 million times more than nitrous oxide. The Intergovernmental Panel on Climate Change (IPCC) and the United States EPA excluded water vapor because it was not associated with man-made activities. They reported that water vapor and clouds were simply feedback mechanisms from CO<sub>2</sub>. Clouds reflect radiation from the sun. The Northern Hemisphere is 2.7°F warmer than the Southern Hemisphere because of clouds. The world cloud cover has gone down 4.1% from 1982 to 2018. Calculations show that this could be responsible for 2.4°F of the 2.7°F. The research shows that most of the recent increase in temperature (89.9%) is because of fewer clouds.
文摘We measured the IR back radiation using a relatively low-cost experimental setup and a test chamber with increasing CO2 concentrations starting with a pure N2 atmosphere against a temperature-controlled black reference background. The results confirm estimations within this work and previous finding about CO2-induced infrared radiation saturation within realistic atmospheric conditions. We used this setup also to study thermal forcing effects with stronger and rare greenhouse gases against a clear night sky. Our results and their interpretation are another indication for having a more critical approach in climate modelling and against monocausal interpretation of climate indices only caused by anthropogenic greenhouse gas emissions. Basic physics combined with measurements and data taken from the literature allow us to conclude that CO2 induced infrared back-radiation must follow an asymptotic logarithmic-like behavior, which is also widely accepted in the climate-change community. The important question of climate sensitivity by doubling current CO2 concentrations is estimated to be below 1˚C. This value is important when the United Nations consider climate change as an existential threat and many governments intend rigorously to reduce net greenhouse gas emissions, led by an ambitious European Union inspired by IPCC assessments is targeting for more than 55% in 2030 and up to 100% in 2050 [1]. But probably they should also listen to experts [2] [3] who found that all these predictions have considerable flaws in basic models, data and impact scenarios.
基金Supported by RFBR Project(No.10-02-01452-a)Presidium SB RAS under the Project Ⅶ.63.3.1 of Ⅶ.63.3 Prog.Integrated Projec of 2012-2014 and Join Proj. between Presidium SB RAS and Presidium NAS,Belarus No.10 of 2010
基金supported by the Federal Target Program“The scientific and Scientific-pedagogical Personnel of Innovative Russia”(No.02.740.11.04444)Russian President Grant(SS4297.2010.2)
基金supported by the Basic Science Research Program through the National Research Foundation of Korea(NRF)(No.2018R1A6A1A03025708)supported by the Nano-Material Technology Development Program through the National Research Foundation of Korea(NRF),funded by the Ministry of Science,ICT and Future Planning(No.2009-0082580).
文摘Two-dimensional(2D)materials have gained considerable attention in chemical sensing owing to their naturally high surface-to-volume ratio.However,the poor response time and incomplete recovery re-strict their application in practical,high performance gas sensors.In this work,we fabricated air-stable ReS_(2)/GaSe heterostructure-based NO_(2)gas sensors with excellent gas sensing response,recovery,selectiv-ity and a low limit of detection(LOD)toward nitrogen dioxide(NO_(2)).The ReS_(2)/GaSe heterostructure was prepared via mechanical exfoliation and an all-dry transfer method.Before the sensing measurements,temperature-dependant transport measurements were carried out.The Schottky Barrier Height(SBH)of the ReS_(2)/GaSe heterostructure was calculated and the corresponding transport mechanisms were dis-cussed.The fabricated gas sensors showed a significant response enhancement with full reversibility to-ward ppm-level NO_(2)(response of∼17%at 3 ppm,a LOD of∼556 ppb)at an operating temperature of(33°C).In particular,the total response and recovery time of the ReS_(2)/GaSe was revealed to be less than 4 min(∼38 s and∼174 s,respectively)for the 250 ppm concentration,which is one of the best response and recovery time toward ppm-level NO_(2).The excellent sensing performances and recovery characteris-tics of the ReS_(2)/GaSe structure are attributed to its efficient charge separation,unique interlayer coupling and desirable band alignments.This atomically thin,ultrasensitive gas sensor that operates at room tem-perature is a strong technological contender to conventional metal oxide gas sensors,which often require elevated temperatures.
基金the National Natural Science Foundation of China (20576023)the Guangdong Province Natural Science Foundation (06025660)
文摘Ni/ZrO2 catalysts were prepared by the incipient-wetness impregnation method and were investigated in activity and selectivity for the selective catalytic methanation of CO in hydrogen-rich gases with more than 20 vol% CO2. The result showed that Ni loadings significantly influenced the performance of Ni/ZrO2 catalyst. The 1.6 wt% Ni loading catalyst exhibited the highest catalytic activity among all the catalysts in the selective methanation of CO in hydrogen-rich gas. The outlet concentration of CO was less than 20 ppm with the hydrogen consumption below 7%, at a gas-hourly-space velocity as high as 10000 h-1 and a temperature range of 260 °C to 280 °C. The X-ray diffraction (XRD) and temperature programmed reduction (TPR) measurements showed that NiO was dispersed thoroughly on the surface of ZrO2 support if Ni loading was under 1.6 wt%. When Ni loading was increased to 3 wt% or above, the free bulk NiO species began to assemble, which was not favorable to increase the selectivity of the catalyst.
基金provided by the National Natural Science Foundation of China (No.50874088)the Project of Creative Team by the Ministry of Education of China (No.IRT0856)+1 种基金the Excellent Talent Project of the New Century supported by the Ministry of Education of China (No.NECT050874)the Natural Science Foundation of the Education Department of Shaanxi Province (No.08JK351)
文摘In order to reduce the number of accidents due to explosions of flammable gases in the goaf of coalmines,the conditions for explosion of flammable gases and their explosion limits,affected to a considerable extent by CO2,are explored.With the use of our experimental equipment suitable for the study of explosion of polybasic explosive gas mixtures,we investigated the effect of CH4/H2=10/1 and CH4/C2H4=10/1 gases mixed with CO2 on their explosion limits.The results indicate that after adding CO2,the explosion limit of the CH4/H2(or C2H4) =10/1 gas mixtures decreased markedly with increasing amounts of CO2.When the amount of CO2 exceeded 25%,the CH4/C2H4=10/1 flammable gas mixture did not lead to explosions.Similar results were obtained when the amount of CO2 exceeded 23% in the CH4/H2=10/1 flammable gas mixture.We also compared the explosion limits and the explosion suppression effect of N2 or CO2 on the explosion limits of the CH4+CO and CH4+C2H4 dual explosive gas mixtures.Along with the increases in the amounts of CO2 or N2,the area of the explosion limits of gas mixtures decreased.Under the same conditions,the explosion suppression effect of CO2 was greater than that of N2.CO2 has clearly the better suppression effect on the explosion of flammable gases in goafs.
文摘Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gases in China and its policy implications. The results show that at present, China is a country with the greatest emission of non-CO2 greenhouse gases in the world, and the emission will account for about 20% of the world's total emission in 2020. The proportion of emission of non-CO2 greenhouse gases from the agricultural sector reaches 73%. In the next 10 years, the emission of non-CO2 gases from cattle and sheep, industry and service industry will experience the highest growth rate; the growth rate of emission from service industry will be higher than that of emission from industry, and the emission from service industry will exceed that from industry after 2010. China can implement emission reduction policy of non-CO2 greenhouse gases to ease the international pressure of CO2 emission reduction. Although the high carbon tax collected can reduce considerable non-CO2 emission, there is little difference in policy efficiency between high carbon tax and low carbon tax. So, in the implementation of emission reduction carbon tax policy of non-CO2 gases, it is necessary to control the carbon tax at a low level.