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Filtration performance and modeling of granular bed for dust removal from coal pyrolytic vapors
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作者 Shuaiqiang Yang Lin Du +3 位作者 Guangchao Ding Runguo Liu Wenli Song Songgeng Li 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第1期35-42,共8页
Dust removal from pyrolytic vapors at high temperatures is an obstacle to the industrialization of the coal pyrolysis process.In this work,a granular bed with expanded perlites as filtration media was designed and int... Dust removal from pyrolytic vapors at high temperatures is an obstacle to the industrialization of the coal pyrolysis process.In this work,a granular bed with expanded perlites as filtration media was designed and integrated into a 10 t·d^(–1)coal pyrolysis facility.The testing results showed that around 97.56%dust collection efficiency was achieved.As a result,dust content in tar was significantly lowered.The pressure drop of the granular bed maintained in the range of 356 Pa to 489 Pa.The dust size in the effluent after filtration exhibited a bimodal distribution,which was attributed to the heterogeneity of the dust components.The effects of filtration bed on pyrolytic product yields were also discussed.A modified filtration model based on the macroscopic phenomenological theory was proposed to describe the performance of the granular bed.The computation results were well agreed with the experimental data. 展开更多
关键词 Granular bed filtration Dust removal PYROLYSIS FILTRATION FIXED-BED
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Efficient removal of U(VI) from wastewater by a sponge-like 3D porous architecture with hybrid electrospun nanofibers
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作者 Lin Hu Lin Chen +4 位作者 Xian-kun Wu Rui Luo Rong-guan Lv Zheng-hao Fei Feng Yang 《Water Science and Engineering》 EI CAS CSCD 2024年第2期150-156,共7页
Removal of uranium(VI)from nuclear wastewater is urgent due to the global nuclear energy exploitation.This study synthesized novel sponge-like 3D porous materials for enhanced uranium adsorption by combining electrosp... Removal of uranium(VI)from nuclear wastewater is urgent due to the global nuclear energy exploitation.This study synthesized novel sponge-like 3D porous materials for enhanced uranium adsorption by combining electrospinning and fibrous freeze-shaping techniques.The materials possessed an organic-inorganic hybrid architecture based on the electrospun fibers of polyacrylonitrile(PAN)and SiO_(2).As a sup-porting material,the surface of fibrous SiO_(2) could be further functionalized by cyano groups via(3-cyanopropyl)triethoxysilane.All the cyano groups were turned into amidoxime(AO)groups to obtain a amidoxime-functionalized sponge(PAO/SiO_(2)-AO)through the subsequent ami-doximation process.The proposed sponge exhibited enhanced uranium adsorption performance with a high removal capacity of 367.12 mg/g,a large adsorption coefficient of 4.0×10^(4)mL/g,and a high removal efficiency of 97.59%.The UO_(2)^(2+)adsorption kinetics perfectly conformed to the pseudo-second-order reaction.The sorbent also exhibited an excellent selectivity for UO_(2)^(2+) with other interfering metal ions.2023 Hohai University.Production and hosting by Elsevier B.V. 展开更多
关键词 Uranium removal SPONGE Amidoximation Organic-inorganic hybrid structure ELECTROSPINNING
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Damage evolution and removal behaviors of GaN crystals involved in double-grits grinding
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作者 Chen Li Yuxiu Hu +4 位作者 Zongze Wei Chongjun Wu Yunfeng Peng Feihu Zhang Yanquan Geng 《International Journal of Extreme Manufacturing》 SCIE EI CAS CSCD 2024年第2期469-484,共16页
Elucidating the complex interactions between the work material and abrasives during grinding of gallium nitride(GaN)single crystals is an active and challenging research area.In this study,molecular dynamics simulatio... Elucidating the complex interactions between the work material and abrasives during grinding of gallium nitride(GaN)single crystals is an active and challenging research area.In this study,molecular dynamics simulations were performed on double-grits interacted grinding of GaN crystals;and the grinding force,coefficient of friction,stress distribution,plastic damage behaviors,and abrasive damage were systematically investigated.The results demonstrated that the interacted distance in both radial and transverse directions achieved better grinding quality than that in only one direction.The grinding force,grinding induced stress,subsurface damage depth,and abrasive wear increase as the transverse interacted distance increases.However,there was no clear correlation between the interaction distance and the number of atoms in the phase transition and dislocation length.Appropriate interacted distances between abrasives can decrease grinding force,coefficient of friction,grinding induced stress,subsurface damage depth,and abrasive wear during the grinding process.The results of grinding tests combined with cross-sectional transmission electron micrographs validated the simulated damage results,i.e.amorphous atoms,high-pressure phase transition,dislocations,stacking faults,and lattice distortions.The results of this study will deepen our understanding of damage accumulation and material removal resulting from coupling between abrasives during grinding and can be used to develop a feasible approach to the wheel design of ordered abrasives. 展开更多
关键词 GRINDING double-grits molecular dynamics damage material removal gallium nitride
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Hydrodynamic Cavitation Enhanced SR-Aops Degradation of Organic Pollutants in Water:A Review
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作者 Xiufeng Zhu Jingying Wang 《Fluid Dynamics & Materials Processing》 EI 2024年第4期671-692,共22页
SR-AOP(sulfate radical advanced oxidation process)is a novel water treatment method able to eliminate refractory organic pollutants.Hydrodynamic cavitation(HC)is a novel green technology,that can effectively produce s... SR-AOP(sulfate radical advanced oxidation process)is a novel water treatment method able to eliminate refractory organic pollutants.Hydrodynamic cavitation(HC)is a novel green technology,that can effectively produce strong oxidizing sulfate radicals.This paper presents a comprehensive review of the research advancements in these fields and a critical discussion of the principal factors influencing HC-enhanced SR-AOP and the mechanisms of synergistic degradation.Furthermore,some insights into the industrial application of HC/PS are also provided.Current research shows that this technology is feasible at the laboratory stage,but its application on larger scales requires further understanding and exploration.In this review,some attention is also paid to the design of the hydrodynamic cavitation reactor and the related operating parameters. 展开更多
关键词 Hydrodynamic cavitation organic pollutant PERSULFATE DEGRADATION influence factor
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Influences of the Fresh Air Volume on the Removal of Cough-Released Droplets in a Passenger Car of a High-Speed Train Using CFD
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作者 Jun Xu Kai Bi +7 位作者 Yibin Lu TiantianWang Hang Zhang Zeyuan Zheng Fushan Shi Yaxin Zheng Xiaoying Li Jingping Yang 《Computer Modeling in Engineering & Sciences》 SCIE EI 2024年第3期2727-2748,共22页
The spread and removal of pollution sources,namely,cough-released droplets in three different areas(front,middle,and rear areas)of a fully-loaded passenger car in a high-speed train under different fresh air flow volu... The spread and removal of pollution sources,namely,cough-released droplets in three different areas(front,middle,and rear areas)of a fully-loaded passenger car in a high-speed train under different fresh air flow volume were studied using computational fluid dynamics(CFD)method.In addition,the structure of indoor flow fields was also analysed.The results show that the large eddies are more stable and flow faster in the air supply under Mode 2(fresh air volume:2200m3/h)compared to Mode 1(fresh air volume:1100m3/h).By analysing the spreading process of droplets sprayed at different locations in the passenger car and with different particle sizes,the removal trends for droplets are found to be similar under the two air supply modes.However,when increasing the fresh air flow volume,the droplets in the middle and front areas of the passenger car are removed faster.When the droplets had dispersed for 60s,Mode 2 exhibited a removal rate approximately 1%–3%higher than Mode 1 for small and medium-sized droplets with diameters of 10 and 50μm.While those in the rear area,the situation is reversed,with Mode 1 slightly surpassing Mode 2 by 1%–3%.For large droplets with a diameter of 100μm,both modes achieved a removal rate of over 96%in all three regions at the 60 s.The results can provide guidance for air supply modes of passenger cars of high-speed trains,thus suppressing the spread of virus-carrying droplets and reducing the risk of viral infection among passengers. 展开更多
关键词 Cough-released pollutants CFD ventilation inside trains supply air volume
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Effects of thinning and understory removal on water use efficiency of Pinus massoniana:evidence from photosynthetic capacity and stable carbon isotope analyses
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作者 Ting Wang Qing Xu +4 位作者 Beibei Zhang Deqiang Gao Ying Zhang Jing Jiang Haijun Zuo 《Journal of Forestry Research》 SCIE EI CAS CSCD 2024年第2期42-53,共12页
Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate change.However,the effects of thinning and understory removal on WUE and... Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate change.However,the effects of thinning and understory removal on WUE and its key controlling processes are not well understood,which limits our comprehension of the physiological mechanisms of various management practices.In this study,four forest management measures(no thinning:NT;understory removal:UR;light thinning:LT;and heavy thinning:HT)were carried out in Pinus massoniana plantations in a subtropical region of China.Photosynthetic capacity and needle stable carbon isotope composition(δ^(13)C)were measured to assess instantaneous water use efficiency(WUE_(inst))and long-term water use efficiency(WUE_(i)).Multiple regression models and structural equation modelling(SEM)identified the effects of soil properties and physiological performances on WUE_(inst)and WUE_(i).The results show that WUE_(inst)values among the four treatments were insignificant.However,compared with the NT stand(35.8μmol·mol^(-1)),WUE_(i)values significantly increased to 41.7μmol·mol^(-1)in the UR,50.1μmol·mol^(-1)in the LT and 46.6μmol·mol^(-1)in HT treatments,largely explained by photosynthetic capacity and soil water content.Understory removal did not change physiological performance(needle water potential and photosynthetic capacity).Thinning increased the net photosynthetic rate(A_n)but not stomatal conductance(g_s)or predawn needle water potential(ψ_(pd)),implying that the improvement in water use efficiency for thinned stands was largely driven by radiation interception than by soil water availability.In general,thinning may be an appropriate management measure to promote P.massoniana WUE to cope with seasonal droughts under future extreme climates. 展开更多
关键词 Stable carbon isotope Water use efficiency THINNING Understory removal Photosynthetic capacity Needle water potential
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Burden of routine orthopedic implant removal a single center retrospective study
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作者 Ammar K AlOmran Nader Alosaimi +6 位作者 Ahmed A Alshaikhi Omar M Bakhurji Khalid J Alzahrani Basil Ziyad Salloot Tamim Omar Alabduladhem Ahmed I AlMulhim Arwa Alumran 《World Journal of Orthopedics》 2024年第2期139-146,共8页
BACKGROUND Open reduction and internal fixation represent prevalent orthopedic procedures,sparking ongoing discourse over whether to retain or remove asymptomatic implants.Achieving consensus on this matter is paramou... BACKGROUND Open reduction and internal fixation represent prevalent orthopedic procedures,sparking ongoing discourse over whether to retain or remove asymptomatic implants.Achieving consensus on this matter is paramount for orthopedic surgeons.This study aims to quantify the impact of routine implant removal on patients and healthcare facilities.A retrospective analysis of implant removal cases from 2016 to 2022 at King Fahad Hospital of the University(KFHU)was conducted and subjected to statistical scrutiny.Among these cases,44%necessitated hospitalization exceeding one day,while 56%required only a single day.Adults exhibited a 55%need for extended hospital stays,contrasting with 22.8%among the pediatric cohort.The complication rate was 6%,with all patients experiencing at least one complication.Notably,34.1%required sick leave and 4.8%exceeded 14 d.General anesthesia was predominant(88%).Routine implant removal introduces unwarranted complications,particularly in adults,potentially prolonging hospitalization.This procedure strains hospital resources,tying up the operating room that could otherwise accommodate critical surgeries.Clearly defined institutional guidelines are imperative to regulate this practice.AIM To measure the burden of routine implant removal on the patients and hospital.METHODS This is a retrospective analysis study of 167 routine implant removal cases treated at KFHU,a tertiary hospital in Saudi Arabia.Data were collected in the orthopedic department at KFHU from February 2016 to August 2022,which includes routine asymptomatic implant removal cases across all age categories.Nonroutine indications such as infection,pain,implant failure,malunion,nonunion,restricted range of motion,and prominent hardware were excluded.Patients who had external fixators removed or joints replaced were also excluded.RESULTS Between February 2016 and August 2022,360 implants were retrieved;however,only 167 of those who met the inclusion criteria were included in this study.The remaining implants were rejected due to exclusion criteria.Among the cases,44%required more than one day in the hospital,whereas 56%required only one day.55%of adults required more than one day of hospitalization,while 22.8%of pediatric patients required more than one day of inpatient care.The complication rate was 6%,with each patient experiencing at least one complication.Sick leave was required in 34.1%of cases,with 4.8%requiring more than 14 d.The most common type of anesthesia used in the surgeries was general anesthesia(88%),and the mean(SD)surgery duration was 77.1(54.7)min.CONCLUSION Routine implant removal causes unnecessary complications,prolongs hospital stays,depletes resources and monopolizing operating rooms that could serve more critical procedures. 展开更多
关键词 Implant removal Healed fracture Orthopedic implant COMPLICATIONS Healthcare system
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Efficient and selective removal of Pb(Ⅱ) from landfill leachate using L-serine-modified polyethylene/polypropylene nonwoven fabric synthesized via radiation grafting technique
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作者 Xin-Xin Feng Cheng Li +6 位作者 Xuan-Zhi Mao Wan-Ning Ren Yang Gao Yu-Long He Zhe Xing Rong Li Guo-Zhong Wu 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第4期144-155,共12页
In this study,to efficiently remove Pb(Ⅱ) from aqueous environments,a novel L-serine-modified polyethylene/polypropylene nonwoven fabric sorbent(NWF-serine)was fabricated through the radiation grafting of glycidyl me... In this study,to efficiently remove Pb(Ⅱ) from aqueous environments,a novel L-serine-modified polyethylene/polypropylene nonwoven fabric sorbent(NWF-serine)was fabricated through the radiation grafting of glycidyl methacrylate and subsequent L-serine modification.The effect of the absorbed dose was investigated in the range of 5–50 kGy.NWF-serine was characterized by Fourier transform infrared spectroscopy,thermogravimetric analysis,and scanning electron microscopy.Batch adsorption tests were conducted to investigate the influences of pH,adsorption time,temperature,initial concentration,and sorbent dosage on the Pb(Ⅱ) adsorption performance of NWF-serine.The results indicated that Pb(Ⅱ) adsorption onto NWF-serine was an endothermic process,following the pseudo-second-order kinetic model and Langmuir isotherm model.The saturated adsorption capacity was 198.1 mg/g.NWF-serine exhibited Pb(Ⅱ) removal rates of 99.8% for aqueous solutions with initial concentrations of 100 mg/L and 82.1% for landfill leachate containing competitive metal ions such as Cd,Cu,Ni,Mn,and Zn.Furthermore,NWF-serine maintained 86% of its Pb(Ⅱ) uptake after five use cycles.The coordination of the carboxyl and amino groups with Pb(Ⅱ) was confirmed using X-ray photoelectron spectroscopy and extended X-ray absorption fine structure analysis. 展开更多
关键词 Landfill leachate Radiation grafting Polyethylene/polypropylene nonwoven fabric Pb(Ⅱ)removal
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Removal Effect of Precipitation on Atmospheric Particulate Matter (PM_(2.5) ) in Bengbu City
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作者 Lei TIAN Lei SHAN Jingyang CHEN 《Meteorological and Environmental Research》 2024年第1期12-15,26,共5页
Based on the monitoring data of PM_(2.5) concentration in Bengbu Environmental Monitoring Station and precipitation observation data of Bengbu National Meteorological Observation Station from 2016 to 2019, the influen... Based on the monitoring data of PM_(2.5) concentration in Bengbu Environmental Monitoring Station and precipitation observation data of Bengbu National Meteorological Observation Station from 2016 to 2019, the influence of precipitation on PM_(2.5) mass concentration in Bengbu City was analyzed. The results show that precipitation had a washing and removal effect on PM_(2.5) in the air, and the removal effect was related to precipitation level, precipitation intensity, precipitation duration and PM_(2.5) concentration. The removal effect of precipitation on PM_(2.5) increased with the increase of precipitation level, and the seasonal difference was obvious. Precipitation intensity was positively correlated with the removal effect of PM_(2.5) , but the average removal rate began to decline when precipitation intensity exceeded 10 mm. With the increase of precipitation intensity, the proportion of positive removal showed an overall upward trend, but there was a low-value area as precipitation intensity was 3-10 mm. Precipitation duration was also positively correlated with the removal effect of PM_(2.5) , and there was a low-value area when precipitation duration was 10-15 h. When PM_(2.5) concentration was low before the precipitation process began, the removal effect was not good, and the average removal rate was negative. As PM_(2.5) concentration was high before the precipitation process started, the removal effect was obvious. 展开更多
关键词 PRECIPITATION PM_(2.5) removal efficiency Bengbu
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Long-term outcomes after endoscopic removal of malignant colorectal polyps:Results from a 10-year cohort
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作者 Anna Fábián Renáta Bor +13 位作者 Béla Vasas Mónika Szűcs Tibor Tóth Zsófia Bősze Kata Judit Szántó Péter Bacsur Anita Bálint Bernadett Farkas Klaudia Farkas Ágnes Milassin Mariann Rutka Tamás Resál Tamás Molnár Zoltán Szepes 《World Journal of Gastrointestinal Endoscopy》 2024年第4期193-205,共13页
BACKGROUND Choosing an optimal post-polypectomy management strategy of malignant colorectal polyps is challenging,and evidence regarding a surveillance-only strategy is limited.AIM To evaluate long-term outcomes after... BACKGROUND Choosing an optimal post-polypectomy management strategy of malignant colorectal polyps is challenging,and evidence regarding a surveillance-only strategy is limited.AIM To evaluate long-term outcomes after endoscopic removal of malignant colorectal polyps.METHODS A single-center retrospective cohort study was conducted to evaluate outcomes after endoscopic removal of malignant colorectal polyps between 2010 and 2020.Residual disease rate and nodal metastases after secondary surgery and local and distant recurrence rate for those with at least 1 year of follow-up were invest-igated.Event rates for categorical variables and means for continuous variables with 95%confidence intervals were calculated,and Fisher’s exact test and Mann-Whitney test were performed.Potential risk factors of adverse outcomes were RESULTS In total,135 lesions(mean size:22.1 mm;location:42%rectal)from 129 patients(mean age:67.7 years;56%male)were enrolled.The proportion of pedunculated and non-pedunculated lesions was similar,with en bloc resection in 82%and 47%of lesions,respectively.Tumor differentiation,distance from resection margins,depth of submucosal invasion,lymphovascular invasion,and budding were reported at 89.6%,45.2%,58.5%,31.9%,and 25.2%,respectively.Residual tumor was found in 10 patients,and nodal metastasis was found in 4 of 41 patients who underwent secondary surgical resection.Univariate analysis identified piecemeal resection as a risk factor for residual malignancy(odds ratio:1.74;P=0.042).At least 1 year of follow-up was available for 117 lesions from 111 patients(mean follow-up period:5.59 years).Overall,54%,30%,30%,11%,and 16%of patients presented at the 1-year,3-year,5-year,7-year,and 9-10-year surveillance examinations.Adverse outcomes occurred in 9.0%(local recurrence and dissemination in 4 patients and 9 patients,respectively),with no difference between patients undergoing secondary surgery and surveillance only.CONCLUSION Reporting of histological features and adherence to surveillance colonoscopy needs improvement.Long-term adverse outcome rates might be higher than previously reported,irrespective of whether secondary surgery was performed. 展开更多
关键词 Malignant colorectal polyps T1 tumor Endoscopic removal OUTCOMES LONG-TERM SURVEILLANCE
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Screening of Polyphosphate Accumulating Organisms and Their Phosphorus Removal Performance
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作者 Miaoxuan HONG Qitong LIANG +1 位作者 Yating HUANG Shasha LIU 《Asian Agricultural Research》 2024年第1期22-24,共3页
[Objectives]To study the phosphorus removal performance of phosphate accumulating organisms(PAOs).[Methods]Activated sludge from domestic sewage treatment plant was used as the strain source,and phosphate accumulating... [Objectives]To study the phosphorus removal performance of phosphate accumulating organisms(PAOs).[Methods]Activated sludge from domestic sewage treatment plant was used as the strain source,and phosphate accumulating organisms were screened by plate streaking method and dilution coating plate method.Six kinds of excellent phosphate accumulating organisms were obtained by metachromatic granule staining experiment,total phosphorus experiment and simulated sewage phosphorus removal experiment to assist the observation of bac-terial morphology and experiment of phosphorus removal capacity.In addition,the influencing factors of phosphorus removal capacity(nitrogen source,trace metal ions)were analyzed.[Results]In the case of simulated sewage,the phosphorus removal rate of strain b was the highest,reaching 66.25%,while the phosphorus removal rate of strain e and f was about 10%lower than that of the phosphorus uptake experiment.[Conclusions]This study is expected to provide a theoretical reference for the gradual optimization of the screening method of phosphorus re-moval bacteria in domestic sewage treatment. 展开更多
关键词 Phosphate accumulating organisms(PAOs) Separation and screening Biological phosphorus removal
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Design and Numerical Simulation of Dust Removal System for Sutomotive Iongitudinal Beam Plasma Cutting
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作者 Wenqiang GAO Xudong MA Heyu TIAN 《Mechanical Engineering Science》 2024年第1期30-34,共5页
To improve the poor efficiency of the dust removal system in the plasma cutting station of automotive longitudinal beams,and reduce the cutting surface quality degradation due to dust,a bottom-side suction dust remova... To improve the poor efficiency of the dust removal system in the plasma cutting station of automotive longitudinal beams,and reduce the cutting surface quality degradation due to dust,a bottom-side suction dust removal system is designed,and the dust removal effect is optimized through the setting of the following dampers and diversion plates.The result of numerical simulation indicates that the particle collection rate can reach 99.44%,and the field test also proves the effectiveness of the dust removal system,which is of guiding significance for the transformation of other similar dust removal systems. 展开更多
关键词 plasma cutting dust removal equipment SIMULATION
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Comprehensive Analysis of Indoor Formaldehyde Removal Techniques:Exploring Physical,Chemical,and Biological Methods
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作者 Yizhe Li 《Journal of Architectural Research and Development》 2024年第1期8-13,共6页
This research focuses on the evaluation of diverse approaches for removing formaldehyde from indoor environments,which is a significant concern for indoor air quality.The study systematically examines physical,chemica... This research focuses on the evaluation of diverse approaches for removing formaldehyde from indoor environments,which is a significant concern for indoor air quality.The study systematically examines physical,chemical,and biological methods to ascertain their effectiveness in formaldehyde mitigation.Physical methods,including air circulation and adsorption,particularly with activated carbon and molecular sieves,are assessed for their efficiency in various concentration scenarios.Chemical methods,such as photocatalytic oxidation using titanium dioxide and plasma technology,are analyzed for their ability to decompose formaldehyde into non-toxic substances.Additionally,biological methods involving plant purification and microbial transformation are explored for their eco-friendly and sustainable removal capabilities.The paper concludes that while each method has its merits,a combined approach may offer the most effective solution for reducing indoor formaldehyde levels.The study underscores the need for further research to integrate these methods in a practical,cost-effective,and environmentally sustainable manner,highlighting their potential to improve indoor air quality significantly. 展开更多
关键词 Indoor air quality Formaldehyde removal Photocatalytic oxidation Activated carbon Biological purification
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The Ultrafiltration Process Enhances Antibiotic Removal in the Full-Scale Advanced Treatment of Drinking Water 被引量:1
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作者 Lingfei Li Yuanxiang Mao +6 位作者 Huiyu Dong Yan Wang Lei Xu Shaogang Liu Qian Xu Zhimin Qiang Fangying Ji 《Engineering》 SCIE EI CAS CSCD 2023年第9期16-20,共5页
1.Introduction A considerable proportion(30%–90%)of consumed antibiotics are excreted from organisms after intake,and wastewater treatment facilities lack sufficient capacity to remove antibiotics in water[1].Thus,th... 1.Introduction A considerable proportion(30%–90%)of consumed antibiotics are excreted from organisms after intake,and wastewater treatment facilities lack sufficient capacity to remove antibiotics in water[1].Thus,the issue of antibiotics contamination in drinking water is raising increasing attention.Adverse consequences of antibiotics in drinking water include potential human health risks(e.g.,they may be carcinogenic or provoke allergic reactions)and risks to the aquatic ecology due to the promotion of bacterialresistant genes[2,3]. 展开更多
关键词 WASTEWATER consequences REMOVE
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Synthesis of porous carbon nanomaterials and their application in tetracycline removal from aqueous solutions 被引量:1
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作者 Sufei Wang Mengjie Hao +3 位作者 Danyang Xiao Tianmiao Zhang Hua Li Zhongshan Chen 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2023年第7期200-209,共10页
The low-cost and efficient elimination of tetracycline from wastewater and to decrease the concentration in soils,sediments,rivers,underground water,or lakes are crucial to human health.Herein,threedimensional porous ... The low-cost and efficient elimination of tetracycline from wastewater and to decrease the concentration in soils,sediments,rivers,underground water,or lakes are crucial to human health.Herein,threedimensional porous carbon nanomaterials were synthesized using glucose and NH_(4)Cl by sugarblowing process at 900℃ and then oxidized under air atmosphere for surface functional group modification.The prepared 3D porous carbon nanomaterials were applied for the removal of tetracycline from aqueous solutions.The sorption isotherms were well simulated by the Langmuir model,with the calculated sorption capacity of 2378 mg·g^(-1) for C-450 at pH=6.5,which was the highest value of today's reported materials.The porous carbon nanomaterials showed high stability at acidic conditions and selectivity in high salt concentrations.The good recycle ability and high removal efficiency of tetracycline from natural groundwater indicated the potential application of the porous carbon nanomaterials in natural environmental antibiotic pollution cleanup.The outstanding sorption properties were attributed to the structures,surface areas and functional groups,strong interactions such as H-bonding,π-π interaction,electrostatic attraction,etc.This paper highlighted the synthesis of porous carbon nanomaterials with high specific surfaces,high sorption capacities,stability,and reusability in organic chemicals'pollution treatment. 展开更多
关键词 Porous carbon nanomaterials TETRACYCLINE SORPTION Pollution management
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Investigation of paint removal by atmospheric pressure plasma jet 被引量:1
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作者 王志君 陈忠文 +1 位作者 康皓 叶宗标 《Plasma Science and Technology》 SCIE EI CAS CSCD 2023年第8期130-140,共11页
Acrylic polyurethane paint on the surface of 2A12 Al alloy was cleaned utilizing an atmospheric pressure plasma jet in this work.The dynamic evolution of the paint removal process during plasma treatment with time was... Acrylic polyurethane paint on the surface of 2A12 Al alloy was cleaned utilizing an atmospheric pressure plasma jet in this work.The dynamic evolution of the paint removal process during plasma treatment with time was explored through analysis of morphology and chemical states.The results showed that although the thickness of paint could be reduced effectively with an increase in cleaning time,the removal rate of paint gradually decreased with time.During the initial cleaning process range,its original smooth morphology of paint turned rugged quickly and was almost unchanged with further plasma treatment.Element and chemical state analysis showed that the content of C in the paint layer decreased obviously after plasma treatment.In contrast,the O content increased remarkably.The cleaning mechanism could be mainly attributed to the reaction between active O-containing species in air plasma and organic components in the paint.After removal of superficial organic matter,residue inorganic metal oxide substances aggregated on the base.The exposed metal oxides on the one hand elevated the superficial O content,but on the other hand hindered further plasma penetration,resulting in a gradual decrease in cleaning rate with cleaning time.Therefore,physical wiping was proposed to be incorporated with the plasma method and effective removal of paint was realized. 展开更多
关键词 atmospheric pressure plasma jet paint removal dynamic evolution
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Material Removal Characteristics of Single-Crystal 4H-SiC Based on Varied-Load Nanoscratch Tests 被引量:1
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作者 Kun Tang Wangping Ou +4 位作者 Cong Mao Jie Liang Moke Zhang Mingjun Zhang Yongle Hu 《Chinese Journal of Mechanical Engineering》 SCIE EI CAS CSCD 2023年第4期125-138,共14页
Single-crystal silicon carbide(SiC)has been widely applied in the military and civil fields because of its excellent physical and chemical properties.However,as is typical in hard-to-machine materials,the good mechani... Single-crystal silicon carbide(SiC)has been widely applied in the military and civil fields because of its excellent physical and chemical properties.However,as is typical in hard-to-machine materials,the good mechanical properties result in surface defects and subsurface damage during precision or ultraprecision machining.In this study,single-and double-varied-load nanoscratch tests were systematically performed on single-crystal 4H-SiC using a nanoindenter system with a Berkovich indenter.The material removal characteristics and cracks under different planes,indenter directions,normal loading rates,and scratch intervals were analyzed using SEM,FIB,and a 3D profilometer,and the mechanisms of material removal and crack propagation were studied.The results showed that the Si-plane of the single-crystal 4H-SiC and edge forward indenter direction are most suitable for material removal and machining.The normal loading rate had little effect on the scratch depth,but a lower loading rate increased the ductile region and critical depth of transition.Additionally,the crack interaction and fluctuation of the depth-distance curves of the second scratch weakened with an increase in the scratch interval,the status of scratches and chips changed,and the comprehensive effects of the propagation and interaction of the three cracks resulted in material fractures and chip accumulation.The calculated and experimental values of the median crack depth also showed good consistency and relativity.Therefore,this study provides an important reference for the high-efficiency and precision machining of single-crystal SiC to ensure high accuracy and a long service life. 展开更多
关键词 Single crystal silicon carbides Varied-load nanoscratch Material removal Crack propagation
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Introducing oxygen vacancies in TiO_(2) lattice through trivalent iron to enhance the photocatalytic removal of indoor NO 被引量:2
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作者 Peng Sun Sumei Han +7 位作者 Jinhua Liu Jingjing Zhang Shuo Yang Faguo Wang Wenxiu Liu Shu Yin Zhanwu Ning Wenbin Cao 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2023年第10期2025-2035,共11页
The synthesis of oxygen vacancies(OVs)-modified TiO_(2)under mild conditions is attractive.In this work,OVs were easily introduced in TiO_(2)lattice during the hydrothermal doping process of trivalent iron ions.Theore... The synthesis of oxygen vacancies(OVs)-modified TiO_(2)under mild conditions is attractive.In this work,OVs were easily introduced in TiO_(2)lattice during the hydrothermal doping process of trivalent iron ions.Theoretical calculations based on a novel charge-compensation structure model were employed with experimental methods to reveal the intrinsic photocatalytic mechanism of Fe-doped TiO_(2)(Fe-TiO_(2)).The OVs formation energy in Fe-TiO_(2)(1.12 eV)was only 23.6%of that in TiO_(2)(4.74 eV),explaining why Fe^(3+)doping could introduce OVs in the TiO_(2)lattice.The calculation results also indicated that impurity states introduced by Fe^(3+)and OVs enhanced the light absorption activity of TiO_(2).Additionally,charge carrier transport was investigated through the carrier lifetime and relative mass.The carrier lifetime of Fe-TiO_(2)(4.00,4.10,and 3.34 ns for 1at%,2at%,and 3at%doping contents,respectively)was longer than that of undoped TiO_(2)(3.22 ns),indicating that Fe^(3+) and OVs could promote charge carrier separation,which can be attributed to the larger relative effective mass of electrons and holes.Herein,Fe-TiO_(2)has higher photocatalytic indoor NO removal activity compared with other photocatalysts because it has strong light absorption activity and high carrier separation efficiency. 展开更多
关键词 oxygen vacancies density functional theory calculations iron-doped titanium dioxide carrier separation photocatalytic removal of indoor nitric oxide
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Removal of Nitrogen, Phosphorus, and Organic Pollutants From Water Using Seeding Type Immobilized Microorganisms 被引量:6
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作者 LIN WANG LI-JING HUANG LUO-JIA YUN FEI TANG JING-HUI ZHAO YAN-QUN LIU XIN ZENG QI-FANG LUO 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2008年第2期150-156,共7页
Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal... Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal of nitrogen, phosphorus, and organic pollutants with the seeding type immobilized microorganisms. Correlations between the quantity of heterotrophic bacteria and the total nitrogen (TN), total phosphorus (TP), and total organic carbon (TOC) in the two lakes were studied. The dominant bacteria were detected, inoculated to the sludge and acclimated by increasing nitrogen, phosphorus and decreasing carbon source in an intermittent, time-controlled and fixed-quantity way. The bacteria were then used to prepare the seeding type immobilized microorganisms, selecting diatomite as the adsorbent cartier. The ability and influence factors of removing nitrogen, phosphorus, and organic pollutant from water samples by the seeding type immobilized microorganisms were studied. Results The coefficients of the heterotrophic bacterial quantity correlated with TOC, TP, and TN were 0.9143, 0.8229, 0.7954 in Lake P and 0.9168, 0.7187, 0.6022 in Lake M. Ten strains of dominant heterotrophic bacteria belonging to Pseudomonas, Coccus, Aeromonas, Bacillus, and Enterobateriaceae, separately, were isolated. The appropriate conditions for the seeding type immobilized microorgansims in purifying the water sample were exposure time=24 h, pH=7.0-8.0, and quantity of the immobilized microorganisms=0.75-1g/50 mL. The removal rates of TOC, TP, and TN under the above conditions were 80.2%, 81.6%, and 86.8%, respectively. Conclusion The amount of heterotrophic bacteria in the two lakes was correlated with TOC, TP, and TN. These bacteria could be acclimatized and prepared for the immobilized microorganisms which could effectively remove nitrogen, phosphorus, and mixed organic pollutants in the water sample. 展开更多
关键词 Heterotrophic bacteria ACCLIMATION Immobilized microorganisms NITROGEN PHOSPHORUS Mixed organic pollutants
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Carbonaceous Nanofibers-titanium Dioxide Nanocomposites: Synthesis and Use as a Platform for Removal of Dye Pollutants 被引量:3
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作者 郭洪影 JIANG Shan +7 位作者 WANG Chaoyuan LI Shenwan FENG Jianjian 孙红梅 ZHU Hongda GUO Huiling LIU Mingxing SUN Honghao 《Journal of Wuhan University of Technology(Materials Science)》 SCIE EI CAS 2019年第2期303-307,共5页
A mild chemistry route was developed to prepare carbonaceous nanofibers-titanium dioxide(CNF-TiO_2) nanocomposites for removal of dye pollutants. In the process of the template-directed hydrothermal carbonization(HTC)... A mild chemistry route was developed to prepare carbonaceous nanofibers-titanium dioxide(CNF-TiO_2) nanocomposites for removal of dye pollutants. In the process of the template-directed hydrothermal carbonization(HTC), ultrathin Te nanowires were adopted as templates and glucose as the carbon source, and TiO_2 was decorated on CNF via the hydrolysis of tetrabutyltitanate in the presence of CNF in ethanol. The as-prepared materials were characterized by scanning electron microscopy(SEM), transmission electron microscopy(TEM), energy-dispersive X-ray(EDX) and X-ray diffraction(XRD). SEM and TEM observations displayed that TiO_2 nanoparticles were anchored on the CNF. EDX and XRD data confirmed that the assynthesized samples were CNF-TiO_2, and TiO_2 belonged to anatase titania. Taking advantage of combined benefits of carbonaceous nanofibers and titanium dioxide, these CNF-TiO_2 nanocomposites exhibited higher removal efficiency in a short time and showed good reusability. It was showed that over 97% of Rhodamine B could be removed in 15 min without generating the solid and liquid wastes. The removal efficiency of dyes was still over 80% after reuse in five cycles. All the results demonstrate that the as-prepared CNF-TiO_2 composites are effective materials for fast and effective removal of dye pollutants and thus can provide a new platform for dye decontamination. 展开更多
关键词 carbon materials NANOCOMPOSITES DYE pollutants
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