Topological Dirac semimetals are a parent state from which other exotic topological phases of matter, such as Weyl semimetals and topological insulators, can emerge. In this study, we investigate a Dirac semimetal pos...Topological Dirac semimetals are a parent state from which other exotic topological phases of matter, such as Weyl semimetals and topological insulators, can emerge. In this study, we investigate a Dirac semimetal possessing sixfold rotational symmetry and hosting higher-order topological hinge Fermi arc states, which is irradiated by circularly polarized light. Our findings reveal that circularly polarized light splits each Dirac node into a pair of Weyl nodes due to the breaking of time-reversal symmetry, resulting in the realization of the Weyl semimetal phase. This Weyl semimetal phase exhibits rich boundary states, including two-dimensional surface Fermi arc states and hinge Fermi arc states confined to six hinges.Furthermore, by adjusting the incident direction of the circularly polarized light, we can control the degree of tilt of the resulting Weyl cones, enabling the realization of different types of Weyl semimetals.展开更多
Spin–momentum locking is a key feature of the topological surface state, which plays an important role in spintronics.The electrical detection of current-induced spin polarization protected by the spin–momentum lock...Spin–momentum locking is a key feature of the topological surface state, which plays an important role in spintronics.The electrical detection of current-induced spin polarization protected by the spin–momentum locking in nonmagnetic systems provides a new platform for developing spintronics, while previous studies were mostly based on magnetic materials.In this study, the spin transport measurement of Dirac semimetal Cd_(3)As_(2) was studied by three-terminal geometry, and a hysteresis loop signal with high resistance and low resistance state was observed. The hysteresis was reversed by reversing the current direction, which illustrates the spin–momentum locking feature of Cd_(3)As_(2). Furthermore, we realized the on–off states of the spin signals through electric modulation of the Fermi arc via the three-terminal configuration, which enables the great potential of Cd_(3)As_(2) in spin field-effect transistors.展开更多
Optical bistability(OB)is capable of rapidly and reversibly transforming a parameter of an optical signal from one state to another,and homologous nonlinear optical bistable devices are core components of high-speed a...Optical bistability(OB)is capable of rapidly and reversibly transforming a parameter of an optical signal from one state to another,and homologous nonlinear optical bistable devices are core components of high-speed all-optical communication and all-optical networks.In this paper,we theoretically investigated the controllable OB from a Fabry-Pérot(FP)cavity with a nonlinear three-dimensional Dirac semimetal(3D DSM)in the terahertz band.The OB stems from the third-order nonlinear bulk conductivity of the 3D DSM and the resonance mode has a positive effect on the generation of OB.This FP cavity structure is able to tune the OB because the transmittance and the reflectance can be modulated by the Fermi energy of the 3D DSM.We believe that this FP cavity configuration could provide a reference concept for realizing tunable bistable devices.展开更多
Intercalated transition metal dichalcogenides(TMDCs)attract much attention due to their rich properties and potential applications.In this article,we grew successfully high-quality V_(1/3)TaS_(2) crystals by a vapor t...Intercalated transition metal dichalcogenides(TMDCs)attract much attention due to their rich properties and potential applications.In this article,we grew successfully high-quality V_(1/3)TaS_(2) crystals by a vapor transport method.We measured the magnetization,longitudinal resistivityρxx(T,H),Hall resistivityρxy(T,H),as well as performed calculations of the electronic band structure.It was found that V_(1/3)TaS_(2) is an A-type antiferromagnet with the Neel temperature T_(N)=6.20 K,and exhibits a negative magnetoresistance(MR)near T_(N).Both band structure calculations and Hall resistivity measurements demonstrated it is a magnetic semimetal.展开更多
We theoretically investigate the reflected spatial Imbert–Fedorov(IF)shift of transverse-electric(TE)-polarized beam illuminating on a bulk Weyl semimetal(WSM).The spatial IF shift is enhanced significantly at two di...We theoretically investigate the reflected spatial Imbert–Fedorov(IF)shift of transverse-electric(TE)-polarized beam illuminating on a bulk Weyl semimetal(WSM).The spatial IF shift is enhanced significantly at two different frequencies close to the epsilon-near-zero(ENZ)frequency,where large values of reflection coefficients|r_(pp)|/|r_(ss)|are obtained due to the ENZ response induced different rapid increasing trends of|r_(pp)|and|r_(ss)|.Particularly,the tunable ENZ effect with tilt degree of Weyl cones and Fermi energy enables the enhanced spatial IF shift at different frequencies.The enhanced spatial IF shift also shows the adjustability of WSM thickness,incident angle and Weyl node separation.Our findings provide easy and available methods to enlarge and adjust the reflected IF shift of TE-polarized light with a WSM.展开更多
One could tune a topological double-Weyl semimetal or a topological triple-Weyl semimetal to become a topologically trivial insulator by opening a band gap.This kind of quantum phase transition is characterized by the...One could tune a topological double-Weyl semimetal or a topological triple-Weyl semimetal to become a topologically trivial insulator by opening a band gap.This kind of quantum phase transition is characterized by the change of certain topological invariant.A new gapless semimetallic state emerges at each topological quantum critical point.Here we perform a renormalization group analysis to investigate the stability of such critical points against perturbations induced by random scalar potential and random vector potential.We find that the quantum critical point between double-Weyl semimetal and band insulator is unstable and can be easily turned into a compressible diffusive metal by any type of weak disorder.The quantum critical point between triple-Weyl semimetal and band insulator flows to a stable strong-coupling fixed point if the system contains a random vector potential merely along the z-axis,but becomes a compressible diffusive metal when other types of disorders exist.展开更多
Ta As,the first experimentally discovered Weyl semimetal material,has attracted a lot of attention due to its high carrier mobility,high anisotropy,nonmagnetic properties and strong interaction with light.These make i...Ta As,the first experimentally discovered Weyl semimetal material,has attracted a lot of attention due to its high carrier mobility,high anisotropy,nonmagnetic properties and strong interaction with light.These make it an ideal candidate for the study of Weyl fermions and applications in quantum computation,thermoelectric devices,and photodetection.For further basic physics studies and potential applications,large-size and high-quality Ta As films are urgently needed.However,it is difficult to grow As-stoichiometry Ta As films due to the volatilization of As during the growth.To solve this problem,we attempted to grow Ta As films on different substrates using targets with different As stoichiometric ratios via pulsed laser deposition(PLD).In this work,we found that partial As ions of the Ga As substrate are likely to diffuse into the Ta As films during growth,which was preliminarily confirmed by structural characterization,surface topography and composition analysis.As a result,the As content in the Ta As film was improved and the Ta As phase was achieved.Our work presents an effective method for the fabrication of Ta As films using PLD,enabling possible use of the Weyl semimetal film for functional devices.展开更多
Topological insulators and semimetals have exotic surface and bulk states with massless Dirac or Weyl fermions,demonstrating microscopic transport phenomenon based on relativistic theory.Chiral anomaly induced negativ...Topological insulators and semimetals have exotic surface and bulk states with massless Dirac or Weyl fermions,demonstrating microscopic transport phenomenon based on relativistic theory.Chiral anomaly induced negative magnetoresistance(negative MR)under parallel magnetic field and current has been used as a probable evidence ofWeyl fermions in recent years.Here we report a novel negative MR result with mutually perpendicular in-plane magnetic field and current in Cd_(3)As_(2)nanowires.The negative MR has a considerable value of-16%around 1.5 K and could persist to room temperature of 300 K with value of-1%.The gate tuning and angle dependence of the negative MR demonstrate the mechanism of the observed negative MR is different from the chiral anomaly.Percolating current paths induced by charge puddles and disorder might be involved to produce such considerable negative MR.Our results indicate the negative MR effect in topological semimetals involves synergistic effects of many mechanisms besides chiral anomaly.展开更多
Chiral anomaly is a distinct quantum anomaly associated with chiral fermions in Dirac or Weyl semimetals.The use of negative magnetoresistance(negative MR)as a signature for this anomaly remains contentious,as trivial...Chiral anomaly is a distinct quantum anomaly associated with chiral fermions in Dirac or Weyl semimetals.The use of negative magnetoresistance(negative MR)as a signature for this anomaly remains contentious,as trivial mechanisms such as current jetting and weak localization can also induce negative MR.In this study,we report a novel nonlinear behavior of the chiral anomaly in the longitudinal direction,which we observed by applying parallel current and magnetic field to the Dirac semimetal Cd_(3)A_(s_(2)).This nonlinear characteristic peaks at an intermediate magnetic field of approximately5 T,displaying a resistance-increasing property concomitant with strengthening of the current source.Through angledependence experiments,we were able to rule out trivial factors,such as thermal effects,geometric artifacts,and anisotropy.Furthermore,additional electric quantum oscillations were observed when the direct current(DC)was applied as high as300μA.Such an unusual phenomenon is ascribed to the formation of quantized levels due to Bloch oscillation in the high DC regime,suggesting that an oscillatory density distribution may arise as the electric field increases.The non-Ohmic electric quantum oscillations open a new avenue for exploring chiral anomaly and other nontrivial topological properties,which is also one of the salient features of nonequilibrium steady states in condensed matter physics.展开更多
The reflected group delay from a multilayer structure comprising a one-dimensional photonic crystal coated with a bulk Dirac semimetal(BDS)separated by a spacer layer is investigated theoretically.It is shown that the...The reflected group delay from a multilayer structure comprising a one-dimensional photonic crystal coated with a bulk Dirac semimetal(BDS)separated by a spacer layer is investigated theoretically.It is shown that the group delay of the reflected beam in this structure can be significantly negatively enhanced and switched from negative to positive.The enhanced group delay originates from the steep phase change caused by the excitation of the optical Tamm state at the interface between the BDS and spacer layer.Moreover,positive and negative group delays can be actively tuned through the Fermi energy and the relaxation time of the BDS.We believe that this enhanced and tunable delay scheme has important research significance for the fabrication of optical delay devices.展开更多
Nodal-line semimetals have become a research hot-spot due to their novel properties and great potential application in spin electronics. It is more challenging to find 2D nodal-line semimetals that can resist the spin...Nodal-line semimetals have become a research hot-spot due to their novel properties and great potential application in spin electronics. It is more challenging to find 2D nodal-line semimetals that can resist the spin–orbit coupling(SOC)effect. Here, we predict that 2D tetragonal Zn B is a nodal-line semimetal with great transport properties. There are two crossing bands centered on the S point at the Fermi surface without SOC, which are mainly composed of the pxy orbitals of Zn and B atoms and the pz orbitals of the B atom. Therefore, the system presents a nodal line centered on the S point in its Brillouin zone(BZ). And the nodal line is protected by the horizontal mirror symmetry M_(z). We further examine the robustness of a nodal line under biaxial strain by applying up to-4% in-plane compressive strain and 5% tensile strain on the Zn B monolayer, respectively. The transmission along the a direction is significantly stronger than that along the b direction in the conductive channel. The current in the a direction is as high as 26.63 μA at 0.8 V, and that in the b direction reaches 8.68 μA at 0.8 V. It is interesting that the transport characteristics of Zn B show the negative differential resistance(NDR) effect after 0.8 V along the a(b) direction. The results provide an ideal platform for research of fundamental physics of 2D nodal-line fermions and nanoscale spintronics, as well as the design of new quantum devices.展开更多
Recently, the Dirac and Weyl semimetals have attracted extensive attention in condensed matter physics due to both the fundamental interest and the potential application of a new generation of electronic devices. Here...Recently, the Dirac and Weyl semimetals have attracted extensive attention in condensed matter physics due to both the fundamental interest and the potential application of a new generation of electronic devices. Here we review the exotic electrical transport phenomena in Dirac andWeyl semimetals. Section 1 is a brief introduction to the topological semimetals(TSMs). In Section 2 and Section 3, the intriguing transport phenomena in Dirac semimetals(DSMs) andWeyl semimetals(WSMs) are reviewed, respectively. The most widely studied Cd_3A_(s2) and the TaAs family are selected as representatives to show the typical properties of DSMs and WSMs, respectively. Beyond these systems, the advances in other TSM materials,such as ZrTe_5 and the MoTe_2 family, are also introduced. In Section 4, we provide perspectives on the study of TSMs especially on the magnetotransport investigations.展开更多
We study the Kondo screening of a spin-1/2 magnetic impurity in the hybrid nodal line semimetals(NLSMs) and the type-Ⅱ NLSMs by using the variational method. We mainly study the binding energy and the spin–spin corr...We study the Kondo screening of a spin-1/2 magnetic impurity in the hybrid nodal line semimetals(NLSMs) and the type-Ⅱ NLSMs by using the variational method. We mainly study the binding energy and the spin–spin correlation between magnetic impurity and conduction electrons. We find that in both the hybrid and type-Ⅱ cases, the density of states(DOS) is always finite, so the impurity and the conduction electrons always form bound states, and the bound state is more easily formed when the DOS is large. Meanwhile, due to the unique dispersion relation and the spin–orbit couplings in the NLSMs, the spatial spin–spin correlation components show very interesting features. Most saliently, various components of the spatial spin–spin correlation function decay with 1/r^(2) in the hybrid NLSMs, while they follow 1/r^(3) decay in the type-Ⅱ NLSMs. This property is mainly caused by the special band structures in the NLSMs, and it can work as a fingerprint to distinguish the two types of NLSMs.展开更多
Helicity-dependent ultrafast spin current generated by circularly polarized photons in topological materials holds the crux to many technological improvements,such as quantum communications,on-chip communication proce...Helicity-dependent ultrafast spin current generated by circularly polarized photons in topological materials holds the crux to many technological improvements,such as quantum communications,on-chip communication processing and storage.Here,we present the manipulation of helicity-dependent terahertz emission generated in a nodal line semimetal candidate Mg3Bi2 by using photon polarization states.The terahertz emission is mainly ascribed to the helicity-dependent photocurrent that is originated from circular photogalvanic effects,and the helicity-independent photocurrent that is attributed to linear photogalvanic effect.Our work will inspire more explorations into novel nodal line semimetals and open up new opportunities for developing ultrafast optoelectronics in the topological system.展开更多
YbMnBi2 is a recently discovered time-reversal-symmetry breaking type-Ⅱ Weyl semimetal.However, as a representation of the new category of topological matters, the scanning tunneling microcopy(STM) results on such im...YbMnBi2 is a recently discovered time-reversal-symmetry breaking type-Ⅱ Weyl semimetal.However, as a representation of the new category of topological matters, the scanning tunneling microcopy(STM) results on such important material are still absent.Here, we report the STM investigations on the morphology of vacuum cleaved single crystalline YbMnBi2 samples.A hill and valley type of topography is observed on the YbMnBi2 surface, which is consistent with the non-layer nature of its crystal structure.Analysis of STM images yields the information of the index of the vicinal surface.Our results here lay a playground of future atomic scale research on YbMnBi2.展开更多
Recently, the non-centrosymmetric WC-type materials(i.e., MoP, ZrTe, TaN, etc) have attracted extensive interest due to the discovery of their topological properties.By means of the first-principles calculations, here...Recently, the non-centrosymmetric WC-type materials(i.e., MoP, ZrTe, TaN, etc) have attracted extensive interest due to the discovery of their topological properties.By means of the first-principles calculations, here we have investigated the structural, thermodynamic, elastic, and electronic properties of the WC-type MX compounds(TiS, TiSe, TiTe, ZrS, ZrSe,ZrTe, HfS, HfSe, and HfTe).Among these nine compounds, five of them(TiS, ZrS, ZrSe0.9, ZrTe, and Hf0.92 Se) have been experimentally synthesized to crystallize in the WC-type structure and other four members have never been reported.Our calculations demonstrated that they are all structurally, thermodynamically, and dynamically stable, indicating that all of them should be possibly synthesized.We have also derived their elastic constants of single crystalline and their bulk and shear moduli in terms of the R.Hill approximations.Furthermore, in similarity to ZrTe, all these compounds have been theoretically derived to be topological semimetals.Whereas TiS is unique because of the coexistence of the Dirac nodal lines(DNLs) and sixfold degenerate nodal points(sixfold DNPs), the other eight members are revealed to exhibit coexisted Weyl nodes(WPs) and triply degenerate nodal points(TDNPs).Their electronic and topological properties have been further discussed.展开更多
We report the magnetoresistance(MR), de Haas-van Alphen(dHvA) effect and Hall effect measurements on a single crystal of TiSi, which is predicted to be a nodal line semimetal. With application of a magnetic field,...We report the magnetoresistance(MR), de Haas-van Alphen(dHvA) effect and Hall effect measurements on a single crystal of TiSi, which is predicted to be a nodal line semimetal. With application of a magnetic field, a metal-to-insulator-like transition in ρ(T) and a nonsaturating MR are observed at low temperatures. The dHvA oscillations reveal a small Fermi-surface pocket with a nontrivial Berry phase. The analysis of the nonlinear Hall resistivity shows that TiSi is a multiband system with low carrier densities and high mobilities. All these results unambiguously prove the existence of Dirac fermions in TiSi.展开更多
Thermoelectrics has long been considered as a promising way of power generation for the next decades. So far, extensive efforts have been devoted to the search of ideal thermoelectric materials, which require both hig...Thermoelectrics has long been considered as a promising way of power generation for the next decades. So far, extensive efforts have been devoted to the search of ideal thermoelectric materials, which require both high electrical conductivity and low thermal conductivity. Recently, the emerging Dirac semimetal Cd3As2, a three-dimensional analogue of graphene, has been reported to host ultra-high mobility and good electrical conductivity as metals. Here, we report the observation of unexpected low thermal conductivity in Cd3As2, one order of magnitude lower than the conventional metals or semimetals with a similar electrical conductivity, despite the semimetal band structure and high electron mobility. The power factor also reaches a large value of 1.58 mW.m 1 .K-2 at room temperature and remains non-saturated up to 400 K. Corroborating with the first-principles calculations, we find that the thermoelectric performance can be well-modulated by the carrier concentration in a wide range. This work demonstrates the Dirac semimetal Cd3As2 as a potential candidate of thermoelectric materials.展开更多
Based on Dirac semimetal metamaterials,the tunable plasmon induced transparency(PIT)is investigated elaborately in this work.The designed unit cell consists of a strip and a square bracket,which is periodically aligne...Based on Dirac semimetal metamaterials,the tunable plasmon induced transparency(PIT)is investigated elaborately in this work.The designed unit cell consists of a strip and a square bracket,which is periodically aligned on the dielectric substrate.Our numerical results illustrate that a pronounced transparency window exists due to near field coupling between two bright modes,which can be dynamically tuned with Fermi energy.Namely,the transparency window demonstrates a distinct blue shift with a larger Fermi energy.Moreover,an on-to-off switch of the PIT transparency window is realized with different polarization angles.In addition,the accompanied slow light property is examined with the calculation of phase and group delay.Finally,a small variation of the refractive index of the substrate can induce a clear movement of the PIT transparency window which delivers a guidance in the application of optical sensing.Thus,this work provides us a new strategy to design compact and adjustable PIT devices and has potential applications in highly tunable optical switchers,sensors,and slow light devices.展开更多
Topological semimetals are a new type of matter with one-dimensional Fermi lines or zero-dimensional Weyl or Dirac points in momentum space. Here using first-principles calculations, we find that the non-centrosymmetr...Topological semimetals are a new type of matter with one-dimensional Fermi lines or zero-dimensional Weyl or Dirac points in momentum space. Here using first-principles calculations, we find that the non-centrosymmetric PbTaS2 is a topological nodal line semimetal. In the absence of spin-orbit coupling (SOC), one band inversion happens around a high symmetrical H point, which leads to forming a nodal line. The nodal line is robust and protected against gap opening by mirror reflection symmetry even with the inclusion of strong SOC. In addition, it also hosts exotic drumhead surface states either inside or outside the projected nodal ring depending on surface termination. The robust bulk nodal lines and drumhead-like surface states with SOC in PbTaS2 make it a potential candidate material for exploring the freakish properties of the topological nodal line fermions in condensed matter systems.展开更多
基金Project supported by the National Key R&D Program of China (Grant No. 2022YFA1403700)the National Natural Science Foundation of China (Grant Nos. 12074108 and 12347101)+3 种基金the Chongqing Natural Science Foundation (Grant No. CSTB2022NSCQ-MSX0568)the Fundamental Research Funds for the Central Universities (Grant No. 2023CDJXY048)the Natural Science Foundation of Jiangsu Province(Grant No. BK20230066)the Jiangsu Shuang Chuang Project (Grant No. JSSCTD202209)。
文摘Topological Dirac semimetals are a parent state from which other exotic topological phases of matter, such as Weyl semimetals and topological insulators, can emerge. In this study, we investigate a Dirac semimetal possessing sixfold rotational symmetry and hosting higher-order topological hinge Fermi arc states, which is irradiated by circularly polarized light. Our findings reveal that circularly polarized light splits each Dirac node into a pair of Weyl nodes due to the breaking of time-reversal symmetry, resulting in the realization of the Weyl semimetal phase. This Weyl semimetal phase exhibits rich boundary states, including two-dimensional surface Fermi arc states and hinge Fermi arc states confined to six hinges.Furthermore, by adjusting the incident direction of the circularly polarized light, we can control the degree of tilt of the resulting Weyl cones, enabling the realization of different types of Weyl semimetals.
基金Project supported by the National Key Research and Development Program of China (Grant Nos.2020YFA0309300 and 2022YFA1403700)the National Natural Science Foundation of China (Grant Nos.12004158,12074162,and 91964201)+2 种基金the Key-Area Research and Development Program of Guangdong Province (Grant No.2018B030327001)Guangdong Provincial Key Laboratory (Grant No.2019B121203002)Guangdong Basic and Applied Basic Research Foundation (Grant No.2022B1515130005)。
文摘Spin–momentum locking is a key feature of the topological surface state, which plays an important role in spintronics.The electrical detection of current-induced spin polarization protected by the spin–momentum locking in nonmagnetic systems provides a new platform for developing spintronics, while previous studies were mostly based on magnetic materials.In this study, the spin transport measurement of Dirac semimetal Cd_(3)As_(2) was studied by three-terminal geometry, and a hysteresis loop signal with high resistance and low resistance state was observed. The hysteresis was reversed by reversing the current direction, which illustrates the spin–momentum locking feature of Cd_(3)As_(2). Furthermore, we realized the on–off states of the spin signals through electric modulation of the Fermi arc via the three-terminal configuration, which enables the great potential of Cd_(3)As_(2) in spin field-effect transistors.
基金Project supported by the Wenzhou Major Science and Technology Innovation Project:Research and Industrialization of Key Technologies for Intelligent Dynamic Ultrahigh Pressure Microfluidizer(Grant No.ZG2023012)Wenzhou Major Science and Technology Innovation PR Project(Grant No.ZG2022011)+3 种基金the National Natural Science Foundation of China(Grant No.62305254)the Scientific Research Fund of the Natural Science Foundation of Hunan Province(Grant No.2022JJ30394)the Changsha Natural Science Foundation(Grant Nos.kq2202236 and kq2202246)the Science and Technology Project of Jiangxi Provincial Education Department(Grant No.GJJ190911).
文摘Optical bistability(OB)is capable of rapidly and reversibly transforming a parameter of an optical signal from one state to another,and homologous nonlinear optical bistable devices are core components of high-speed all-optical communication and all-optical networks.In this paper,we theoretically investigated the controllable OB from a Fabry-Pérot(FP)cavity with a nonlinear three-dimensional Dirac semimetal(3D DSM)in the terahertz band.The OB stems from the third-order nonlinear bulk conductivity of the 3D DSM and the resonance mode has a positive effect on the generation of OB.This FP cavity structure is able to tune the OB because the transmittance and the reflectance can be modulated by the Fermi energy of the 3D DSM.We believe that this FP cavity configuration could provide a reference concept for realizing tunable bistable devices.
基金Project supported by the National Key Research and Development Program of China(Grant No.2022YFA1403202)the National Natural Science Foundation of China(Grant Nos.NSFC-12074335,11974095,5177115,11974095,and 12188101)the Natural Science Foundation of Shaanxi Province of China(Grant No.2022JM-028).
文摘Intercalated transition metal dichalcogenides(TMDCs)attract much attention due to their rich properties and potential applications.In this article,we grew successfully high-quality V_(1/3)TaS_(2) crystals by a vapor transport method.We measured the magnetization,longitudinal resistivityρxx(T,H),Hall resistivityρxy(T,H),as well as performed calculations of the electronic band structure.It was found that V_(1/3)TaS_(2) is an A-type antiferromagnet with the Neel temperature T_(N)=6.20 K,and exhibits a negative magnetoresistance(MR)near T_(N).Both band structure calculations and Hall resistivity measurements demonstrated it is a magnetic semimetal.
基金the National Natural Science Foundation of China(Grant Nos.61875133 and 11874269).
文摘We theoretically investigate the reflected spatial Imbert–Fedorov(IF)shift of transverse-electric(TE)-polarized beam illuminating on a bulk Weyl semimetal(WSM).The spatial IF shift is enhanced significantly at two different frequencies close to the epsilon-near-zero(ENZ)frequency,where large values of reflection coefficients|r_(pp)|/|r_(ss)|are obtained due to the ENZ response induced different rapid increasing trends of|r_(pp)|and|r_(ss)|.Particularly,the tunable ENZ effect with tilt degree of Weyl cones and Fermi energy enables the enhanced spatial IF shift at different frequencies.The enhanced spatial IF shift also shows the adjustability of WSM thickness,incident angle and Weyl node separation.Our findings provide easy and available methods to enlarge and adjust the reflected IF shift of TE-polarized light with a WSM.
基金the Natural Science Foundation of Anhui Province,China(Grant No.2208085MA11)the National Natural Science Foundation of China(Grants Nos.11974356,12274414,and U1832209)。
文摘One could tune a topological double-Weyl semimetal or a topological triple-Weyl semimetal to become a topologically trivial insulator by opening a band gap.This kind of quantum phase transition is characterized by the change of certain topological invariant.A new gapless semimetallic state emerges at each topological quantum critical point.Here we perform a renormalization group analysis to investigate the stability of such critical points against perturbations induced by random scalar potential and random vector potential.We find that the quantum critical point between double-Weyl semimetal and band insulator is unstable and can be easily turned into a compressible diffusive metal by any type of weak disorder.The quantum critical point between triple-Weyl semimetal and band insulator flows to a stable strong-coupling fixed point if the system contains a random vector potential merely along the z-axis,but becomes a compressible diffusive metal when other types of disorders exist.
基金Project supported by the National Key Research and Development Program of China(Grant No.2021YFA0718700)the National Natural Science Foundation of China(Grant No.12174347)+1 种基金the Synergetic Extreme Condition User Facility(SECUF)the Center for Materials Genome。
文摘Ta As,the first experimentally discovered Weyl semimetal material,has attracted a lot of attention due to its high carrier mobility,high anisotropy,nonmagnetic properties and strong interaction with light.These make it an ideal candidate for the study of Weyl fermions and applications in quantum computation,thermoelectric devices,and photodetection.For further basic physics studies and potential applications,large-size and high-quality Ta As films are urgently needed.However,it is difficult to grow As-stoichiometry Ta As films due to the volatilization of As during the growth.To solve this problem,we attempted to grow Ta As films on different substrates using targets with different As stoichiometric ratios via pulsed laser deposition(PLD).In this work,we found that partial As ions of the Ga As substrate are likely to diffuse into the Ta As films during growth,which was preliminarily confirmed by structural characterization,surface topography and composition analysis.As a result,the As content in the Ta As film was improved and the Ta As phase was achieved.Our work presents an effective method for the fabrication of Ta As films using PLD,enabling possible use of the Weyl semimetal film for functional devices.
基金This work was supported by the National Natural Science Foundation of China(Grant Nos.12004158,12074162,and 91964201)the National Key Research and Development Program of China(Grant Nos.2022YFA1403700 and 2020YFA0309300)+2 种基金the Key-Area Research and Development Program of Guangdong Province,China(Grant No.2018B030327001)Guangdong Provincial Key Laboratory(Grant No.2019B121203002)Guangdong Basic and Applied Basic Research Foundation(Grant No.2022B1515130005).
文摘Topological insulators and semimetals have exotic surface and bulk states with massless Dirac or Weyl fermions,demonstrating microscopic transport phenomenon based on relativistic theory.Chiral anomaly induced negative magnetoresistance(negative MR)under parallel magnetic field and current has been used as a probable evidence ofWeyl fermions in recent years.Here we report a novel negative MR result with mutually perpendicular in-plane magnetic field and current in Cd_(3)As_(2)nanowires.The negative MR has a considerable value of-16%around 1.5 K and could persist to room temperature of 300 K with value of-1%.The gate tuning and angle dependence of the negative MR demonstrate the mechanism of the observed negative MR is different from the chiral anomaly.Percolating current paths induced by charge puddles and disorder might be involved to produce such considerable negative MR.Our results indicate the negative MR effect in topological semimetals involves synergistic effects of many mechanisms besides chiral anomaly.
基金supported by the National Natural Science Foundation of China(Grant Nos.12074162,12004158,and 91964201)the National Key Research and Development Program of China(Grant Nos.2022YFA1403700 and 2020YFA0309300)+2 种基金the Key-Area Research and Development Program of Guangdong Province(Grant No.2018B030327001)Guangdong Provincial Key Laboratory(Grant No.2019B121203002)Guangdong Basic and Applied Basic Research Foundation(Grant No.2022B1515130005)。
文摘Chiral anomaly is a distinct quantum anomaly associated with chiral fermions in Dirac or Weyl semimetals.The use of negative magnetoresistance(negative MR)as a signature for this anomaly remains contentious,as trivial mechanisms such as current jetting and weak localization can also induce negative MR.In this study,we report a novel nonlinear behavior of the chiral anomaly in the longitudinal direction,which we observed by applying parallel current and magnetic field to the Dirac semimetal Cd_(3)A_(s_(2)).This nonlinear characteristic peaks at an intermediate magnetic field of approximately5 T,displaying a resistance-increasing property concomitant with strengthening of the current source.Through angledependence experiments,we were able to rule out trivial factors,such as thermal effects,geometric artifacts,and anisotropy.Furthermore,additional electric quantum oscillations were observed when the direct current(DC)was applied as high as300μA.Such an unusual phenomenon is ascribed to the formation of quantized levels due to Bloch oscillation in the high DC regime,suggesting that an oscillatory density distribution may arise as the electric field increases.The non-Ohmic electric quantum oscillations open a new avenue for exploring chiral anomaly and other nontrivial topological properties,which is also one of the salient features of nonequilibrium steady states in condensed matter physics.
基金Project supported by the Scientific research project of Zhejiang Provincial Department of Education(Grant No.Y202250547)the Scientific Research Project ofWenzhou University of Technology(Grant No.ky202205)the Hunan Provincial Natural Science Foundation of China(Grant No.2022JJ30394).
文摘The reflected group delay from a multilayer structure comprising a one-dimensional photonic crystal coated with a bulk Dirac semimetal(BDS)separated by a spacer layer is investigated theoretically.It is shown that the group delay of the reflected beam in this structure can be significantly negatively enhanced and switched from negative to positive.The enhanced group delay originates from the steep phase change caused by the excitation of the optical Tamm state at the interface between the BDS and spacer layer.Moreover,positive and negative group delays can be actively tuned through the Fermi energy and the relaxation time of the BDS.We believe that this enhanced and tunable delay scheme has important research significance for the fabrication of optical delay devices.
基金Project supported by the Natural Science Foundation of Shandong Province, China (Grant No. ZR2019MA041)Taishan Scholar Project of Shandong Province, China (Grant No. ts20190939)the National Natural Science Foundation of China (Grant No. 62071200)。
文摘Nodal-line semimetals have become a research hot-spot due to their novel properties and great potential application in spin electronics. It is more challenging to find 2D nodal-line semimetals that can resist the spin–orbit coupling(SOC)effect. Here, we predict that 2D tetragonal Zn B is a nodal-line semimetal with great transport properties. There are two crossing bands centered on the S point at the Fermi surface without SOC, which are mainly composed of the pxy orbitals of Zn and B atoms and the pz orbitals of the B atom. Therefore, the system presents a nodal line centered on the S point in its Brillouin zone(BZ). And the nodal line is protected by the horizontal mirror symmetry M_(z). We further examine the robustness of a nodal line under biaxial strain by applying up to-4% in-plane compressive strain and 5% tensile strain on the Zn B monolayer, respectively. The transmission along the a direction is significantly stronger than that along the b direction in the conductive channel. The current in the a direction is as high as 26.63 μA at 0.8 V, and that in the b direction reaches 8.68 μA at 0.8 V. It is interesting that the transport characteristics of Zn B show the negative differential resistance(NDR) effect after 0.8 V along the a(b) direction. The results provide an ideal platform for research of fundamental physics of 2D nodal-line fermions and nanoscale spintronics, as well as the design of new quantum devices.
基金Project supported by the National Basic Research Program of China(Grant Nos.2018YFA0305604,2017YFA0303300,and 2013CB934600)the Research Fund for the Doctoral Program of Higher Education(RFDP)of China(Grant No.20130001110003)+2 种基金the Open Project Program of the Pulsed High Magnetic Field Facility(Grant No.PHMFF2015002) at the Huazhong University of Science and Technologythe Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics,Tsinghua University(Grant No.KF201703)the Key Research Program of the Chinese Academy of Sciences(Grant No.XDPB08-2)
文摘Recently, the Dirac and Weyl semimetals have attracted extensive attention in condensed matter physics due to both the fundamental interest and the potential application of a new generation of electronic devices. Here we review the exotic electrical transport phenomena in Dirac andWeyl semimetals. Section 1 is a brief introduction to the topological semimetals(TSMs). In Section 2 and Section 3, the intriguing transport phenomena in Dirac semimetals(DSMs) andWeyl semimetals(WSMs) are reviewed, respectively. The most widely studied Cd_3A_(s2) and the TaAs family are selected as representatives to show the typical properties of DSMs and WSMs, respectively. Beyond these systems, the advances in other TSM materials,such as ZrTe_5 and the MoTe_2 family, are also introduced. In Section 4, we provide perspectives on the study of TSMs especially on the magnetotransport investigations.
基金supported by the Zhejiang Provincial Natural Science Foundation of China (Grant No. LY19A040003)。
文摘We study the Kondo screening of a spin-1/2 magnetic impurity in the hybrid nodal line semimetals(NLSMs) and the type-Ⅱ NLSMs by using the variational method. We mainly study the binding energy and the spin–spin correlation between magnetic impurity and conduction electrons. We find that in both the hybrid and type-Ⅱ cases, the density of states(DOS) is always finite, so the impurity and the conduction electrons always form bound states, and the bound state is more easily formed when the DOS is large. Meanwhile, due to the unique dispersion relation and the spin–orbit couplings in the NLSMs, the spatial spin–spin correlation components show very interesting features. Most saliently, various components of the spatial spin–spin correlation function decay with 1/r^(2) in the hybrid NLSMs, while they follow 1/r^(3) decay in the type-Ⅱ NLSMs. This property is mainly caused by the special band structures in the NLSMs, and it can work as a fingerprint to distinguish the two types of NLSMs.
基金We thank Prof.J.B.Qi for helpful discussions and are grateful for financial support from the National Natural Science Foundation of China(Grant Nos.11804387,11802339,11805276,11902358,61805282,and 61801498)the Scientific Researches Foundation of National University of Defense Technology(Grant Nos.ZK18-03-22,ZK18-01-03 and ZK18-03-36).
文摘Helicity-dependent ultrafast spin current generated by circularly polarized photons in topological materials holds the crux to many technological improvements,such as quantum communications,on-chip communication processing and storage.Here,we present the manipulation of helicity-dependent terahertz emission generated in a nodal line semimetal candidate Mg3Bi2 by using photon polarization states.The terahertz emission is mainly ascribed to the helicity-dependent photocurrent that is originated from circular photogalvanic effects,and the helicity-independent photocurrent that is attributed to linear photogalvanic effect.Our work will inspire more explorations into novel nodal line semimetals and open up new opportunities for developing ultrafast optoelectronics in the topological system.
基金Project supported by the “Shuguang Program” from Shanghai Education Development Foundation and Shanghai Municipal Education Commission,Ministry of Science and Technology of China(Grant Nos.2016YFA0301003 and 2016YFA0300403)the National Natural Science Foundation of China(Grant Nos.11521404,11634009,11874256,11574202,11874258,11790313,11674226,U1632102,11674222,and 11861161003)the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB28000000)
文摘YbMnBi2 is a recently discovered time-reversal-symmetry breaking type-Ⅱ Weyl semimetal.However, as a representation of the new category of topological matters, the scanning tunneling microcopy(STM) results on such important material are still absent.Here, we report the STM investigations on the morphology of vacuum cleaved single crystalline YbMnBi2 samples.A hill and valley type of topography is observed on the YbMnBi2 surface, which is consistent with the non-layer nature of its crystal structure.Analysis of STM images yields the information of the index of the vicinal surface.Our results here lay a playground of future atomic scale research on YbMnBi2.
基金Project supported by the National Natural Science Foundation of China(Grant No.51671193)
文摘Recently, the non-centrosymmetric WC-type materials(i.e., MoP, ZrTe, TaN, etc) have attracted extensive interest due to the discovery of their topological properties.By means of the first-principles calculations, here we have investigated the structural, thermodynamic, elastic, and electronic properties of the WC-type MX compounds(TiS, TiSe, TiTe, ZrS, ZrSe,ZrTe, HfS, HfSe, and HfTe).Among these nine compounds, five of them(TiS, ZrS, ZrSe0.9, ZrTe, and Hf0.92 Se) have been experimentally synthesized to crystallize in the WC-type structure and other four members have never been reported.Our calculations demonstrated that they are all structurally, thermodynamically, and dynamically stable, indicating that all of them should be possibly synthesized.We have also derived their elastic constants of single crystalline and their bulk and shear moduli in terms of the R.Hill approximations.Furthermore, in similarity to ZrTe, all these compounds have been theoretically derived to be topological semimetals.Whereas TiS is unique because of the coexistence of the Dirac nodal lines(DNLs) and sixfold degenerate nodal points(sixfold DNPs), the other eight members are revealed to exhibit coexisted Weyl nodes(WPs) and triply degenerate nodal points(TDNPs).Their electronic and topological properties have been further discussed.
基金Supported by the National Key Research Program of China under Grant Nos 2016YFA0401000 and 2016YFA0300604the National Basic Research Program of China under Grant No 2015CB921303+1 种基金the Strategic Priority Research Program(B)of Chinese Academy of Sciences under Grant No XDB07020100the National Natural Science Foundation of China under Grant No11874417
文摘We report the magnetoresistance(MR), de Haas-van Alphen(dHvA) effect and Hall effect measurements on a single crystal of TiSi, which is predicted to be a nodal line semimetal. With application of a magnetic field, a metal-to-insulator-like transition in ρ(T) and a nonsaturating MR are observed at low temperatures. The dHvA oscillations reveal a small Fermi-surface pocket with a nontrivial Berry phase. The analysis of the nonlinear Hall resistivity shows that TiSi is a multiband system with low carrier densities and high mobilities. All these results unambiguously prove the existence of Dirac fermions in TiSi.
基金supported by the National Young 1000 Talent Plan Chinathe Pujiang Talent Plan in Shanghai,China+2 种基金the National Natural Science Foundation of China(Grant Nos.61322407 and 11474058)the Fund for Fostering Talents in Basic Science of the National Natural Science Foundation of China(Grant No.J1103204)the National Basic Research Program of China(Grant No.2011CB921803)
文摘Thermoelectrics has long been considered as a promising way of power generation for the next decades. So far, extensive efforts have been devoted to the search of ideal thermoelectric materials, which require both high electrical conductivity and low thermal conductivity. Recently, the emerging Dirac semimetal Cd3As2, a three-dimensional analogue of graphene, has been reported to host ultra-high mobility and good electrical conductivity as metals. Here, we report the observation of unexpected low thermal conductivity in Cd3As2, one order of magnitude lower than the conventional metals or semimetals with a similar electrical conductivity, despite the semimetal band structure and high electron mobility. The power factor also reaches a large value of 1.58 mW.m 1 .K-2 at room temperature and remains non-saturated up to 400 K. Corroborating with the first-principles calculations, we find that the thermoelectric performance can be well-modulated by the carrier concentration in a wide range. This work demonstrates the Dirac semimetal Cd3As2 as a potential candidate of thermoelectric materials.
基金Project supported by the Natural Science Foundation of Henan Provincial Educational Committee,China(Grant No.21A140026).
文摘Based on Dirac semimetal metamaterials,the tunable plasmon induced transparency(PIT)is investigated elaborately in this work.The designed unit cell consists of a strip and a square bracket,which is periodically aligned on the dielectric substrate.Our numerical results illustrate that a pronounced transparency window exists due to near field coupling between two bright modes,which can be dynamically tuned with Fermi energy.Namely,the transparency window demonstrates a distinct blue shift with a larger Fermi energy.Moreover,an on-to-off switch of the PIT transparency window is realized with different polarization angles.In addition,the accompanied slow light property is examined with the calculation of phase and group delay.Finally,a small variation of the refractive index of the substrate can induce a clear movement of the PIT transparency window which delivers a guidance in the application of optical sensing.Thus,this work provides us a new strategy to design compact and adjustable PIT devices and has potential applications in highly tunable optical switchers,sensors,and slow light devices.
基金Supported by the National Natural Science Foundation of China under Grant No 11504366the National Basic Research Program of China under Grant Nos 2015CB921503 and 2016YFE0110000
文摘Topological semimetals are a new type of matter with one-dimensional Fermi lines or zero-dimensional Weyl or Dirac points in momentum space. Here using first-principles calculations, we find that the non-centrosymmetric PbTaS2 is a topological nodal line semimetal. In the absence of spin-orbit coupling (SOC), one band inversion happens around a high symmetrical H point, which leads to forming a nodal line. The nodal line is robust and protected against gap opening by mirror reflection symmetry even with the inclusion of strong SOC. In addition, it also hosts exotic drumhead surface states either inside or outside the projected nodal ring depending on surface termination. The robust bulk nodal lines and drumhead-like surface states with SOC in PbTaS2 make it a potential candidate material for exploring the freakish properties of the topological nodal line fermions in condensed matter systems.