Traditional Korean Hanji paper and cotton fabric were introduced as flexible substrates in the fabrication of graphene-coated heaters.Silver nanowires and PEDOT:PSS were added to increase the electrical conductivity o...Traditional Korean Hanji paper and cotton fabric were introduced as flexible substrates in the fabrication of graphene-coated heaters.Silver nanowires and PEDOT:PSS were added to increase the electrical conductivity of the heaters,thereby enhancing their heating performance.The optimal concentrations of silver nanowires and PEDOT:PSS with respect to that of graphene were identified.These active materials were deposited on flexible Hanji/cotton and non-flexible alumina substrates using supersonic spraying.The proposed Hanji-and cotton-based heaters were light,wearable,stretchable,skin-friendly,and biodegradable.The unyielding alumina-based heater exhibited the highest heating temperature of 275°C at 13 V.Wearable heater bendability and stretchability were tested considering multiple bending and stretching cycles.Moreover,water boiling and fabric drying were successfully performed using the alumina-based heater.The supersonic spraying deposition technique was used to produce writable and patternable heaters.展开更多
The interface between graphene and organic layers is a key factor responsible for the performance of graphene-based organic solar cells(OSCs). In this paper, we focus on coating PEDOT:PSS onto the surface of graphene....The interface between graphene and organic layers is a key factor responsible for the performance of graphene-based organic solar cells(OSCs). In this paper, we focus on coating PEDOT:PSS onto the surface of graphene. We demonstrate two approaches, applying UV/Ozone treatment on graphene and modifying PEDOT:PSS with Zonyl, to get a PEDOT:PSS well-coated graphene film. Our results prove that both methods can be effective to solve the interface issue between graphene and PEDOT: PSS. Thereby it shows a positive application of the composited graphene/PEDOT:PSS film on graphene-based OSCs.展开更多
All-solution-processed organic solar cells(OSCs)(from the bottom electrode to the top electrode)are highly attractive thanks to their low cost,lightweight and high-throughput production.However,achieving highly effici...All-solution-processed organic solar cells(OSCs)(from the bottom electrode to the top electrode)are highly attractive thanks to their low cost,lightweight and high-throughput production.However,achieving highly efficient all-solution-processed OSCs remains a significant challenge.One of the key issues is the lack of high-quality solution-processed electrode systems that can replace indium tin oxide(ITO)and vacuum-deposited metal electrodes.In this paper,we comprehensively review recent advances in all-solution-processed osCs,and classified the devices as the top electrode materials,including silver nanowires(AgNWs),conducting polymers and composite conducting materials.The correlation between electrode materials,properties of electrodes,and device performance in all-solution-processed OSCs is elucidated.In addition,the critical roles of the active layer and interface layer are also discussed.Finally,the prospects and challenges of all-solution-processed OSCs are presented.展开更多
基金financially supported by the National Research Foundation of Korea(NRF)grant funded by the Korea government(nos.NRF-2020R1A5A1018153,NRF-2021R1A2C2010530,and 2022M3J1A106422611)The authors acknowledge King Saud University,Riyadh,Saudi Arabia,for funding this work through Researchers Supporting Project number(RSP2023R30).
文摘Traditional Korean Hanji paper and cotton fabric were introduced as flexible substrates in the fabrication of graphene-coated heaters.Silver nanowires and PEDOT:PSS were added to increase the electrical conductivity of the heaters,thereby enhancing their heating performance.The optimal concentrations of silver nanowires and PEDOT:PSS with respect to that of graphene were identified.These active materials were deposited on flexible Hanji/cotton and non-flexible alumina substrates using supersonic spraying.The proposed Hanji-and cotton-based heaters were light,wearable,stretchable,skin-friendly,and biodegradable.The unyielding alumina-based heater exhibited the highest heating temperature of 275°C at 13 V.Wearable heater bendability and stretchability were tested considering multiple bending and stretching cycles.Moreover,water boiling and fabric drying were successfully performed using the alumina-based heater.The supersonic spraying deposition technique was used to produce writable and patternable heaters.
基金National Natural Science Foundation of China (91333122,51402106,51372082,51172069,50972032,61204064 and 51202067)Ph.D. Programs Foundation of Ministry of Education of China (20110036110006,20120036120006,20130036110012)+1 种基金Par-Eu Scholars Programthe Fundamental Research Funds for the Central Universities
文摘The interface between graphene and organic layers is a key factor responsible for the performance of graphene-based organic solar cells(OSCs). In this paper, we focus on coating PEDOT:PSS onto the surface of graphene. We demonstrate two approaches, applying UV/Ozone treatment on graphene and modifying PEDOT:PSS with Zonyl, to get a PEDOT:PSS well-coated graphene film. Our results prove that both methods can be effective to solve the interface issue between graphene and PEDOT: PSS. Thereby it shows a positive application of the composited graphene/PEDOT:PSS film on graphene-based OSCs.
基金the National Natural Science Foundation of China(52103221,52172048,22205130,52063010)Shandong Provincial Natural Science Foundation(ZR2021QB179,ZR2021QB024,ZR2021ZD06)+2 种基金Guangdong Natural Science Foundation of China(2023A1515012323,2023A1515010943,2022A1515110643)the National Key Research and Development Program of China(2022YFB4200400)funded by M0STthe Fundamental Research Funds of Shandong University.
文摘All-solution-processed organic solar cells(OSCs)(from the bottom electrode to the top electrode)are highly attractive thanks to their low cost,lightweight and high-throughput production.However,achieving highly efficient all-solution-processed OSCs remains a significant challenge.One of the key issues is the lack of high-quality solution-processed electrode systems that can replace indium tin oxide(ITO)and vacuum-deposited metal electrodes.In this paper,we comprehensively review recent advances in all-solution-processed osCs,and classified the devices as the top electrode materials,including silver nanowires(AgNWs),conducting polymers and composite conducting materials.The correlation between electrode materials,properties of electrodes,and device performance in all-solution-processed OSCs is elucidated.In addition,the critical roles of the active layer and interface layer are also discussed.Finally,the prospects and challenges of all-solution-processed OSCs are presented.
