In the present study,the nanofliud natural convection is investigated by the energy-conserving dissipative particle dynamics(eDPD)method,where the nanoparticles are considered at the single-particle level.The thermal ...In the present study,the nanofliud natural convection is investigated by the energy-conserving dissipative particle dynamics(eDPD)method,where the nanoparticles are considered at the single-particle level.The thermal expansion coefficientβand the viscosityμof the simulated system containing nanoparticles are calculated and found to be in close alignment with the previous simulation results.The single-particle hydrodynamics in e DPD enables simulations of nanofluid natural convection with higher Rayleigh numbers and greater nanoparticle volume fractions.Additionally,this approach is utilized to simulate the nanoparticle distribution during the enhanced heat transfer process in the nanofluid natural convection.The localized aggregation of nanoparticles enhances the heat transfer performance of the nanofluid under specific Rayleigh numbers and nanoparticles volume fractions.展开更多
Recycled moisture is an important indicator of the renewal capacity of regional water resources.Due to the existence of Yulong Snow Mountain,Lijiang in Yunnan Province,southeast of the Qinghai-Tibet Plateau,China,is t...Recycled moisture is an important indicator of the renewal capacity of regional water resources.Due to the existence of Yulong Snow Mountain,Lijiang in Yunnan Province,southeast of the Qinghai-Tibet Plateau,China,is the closest ocean glacier area to the equator in Eurasia.Daily precipitation samples were collected from 2017 to 2018 in Lijiang to quantify the effect of sub-cloud evaporation and recycled moisture on precipitation combined with the d-excess model during monsoon and non-monsoon periods.The results indicated that the d-excess values of precipitation fluctuated between–35.6‰and 16.0‰,with an arithmetic mean of 3.5‰.The local meteoric water line(LMWL)wasδD=7.91δ^(18)O+2.50,with a slope slightly lower than the global meteoric water line(GMWL).Subcloud evaporation was higher during the non-monsoon season than during the monsoon season.It tended to peak in March and was primarily influenced by the relative humidity.The source of the water vapour affected the proportion of recycled moisture.According to the results of the Hybrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT)model,the main sources of water vapour in Lijiang area during the monsoon period were the southwest and southeast monsoons.During the non-monsoon period,water vapour was transported by a southwesterly flow.The recycled moisture in Lijiang area between March and October 2017 was 10.62%.Large variations were observed between the monsoon and non-monsoon seasons,with values of 5.48%and 25.65%,respectively.These differences were primarily attributed to variations in the advection of water vapour.The recycled moisture has played a supplementary role in the precipitation of Lijiang area.展开更多
Characterization of the spatial and temporal variability of stable isotopes in surface water is essential for interpreting hydrological processes.In this study,we collected the water samples of river water,groundwater...Characterization of the spatial and temporal variability of stable isotopes in surface water is essential for interpreting hydrological processes.In this study,we collected the water samples of river water,groundwater,and reservoir water in the Burqin River Basin of the Altay Mountains,China in 2021,and characterized the oxygen and hydrogen isotope variations in different water bodies via instrumental analytics and modeling.Results showed significant seasonal variations in stable isotope ratios of oxygen and hydrogen(δ18O andδ2H,respectively)and significant differences inδ18O andδ2H among different water bodies.Higherδ18O andδ2H values were mainly found in river water,while groundwater and reservoir water had lower isotope ratios.River water and groundwater showed differentδ18O-δ2H relationships with the local meteoric water line,implying that river water and groundwater are controlled by evaporative enrichment and multi-source recharge processes.The evaporative enrichment experienced by reservoir water was less significant and largely influenced by topography,recharge sources,local moisture cycling,and anthropogenic factors.Higher deuterium excess(d-excess)value of 14.34‰for river water probably represented the isotopic signature of combined contributions from direct precipitation,snow and glacial meltwater,and groundwater recharge.The average annual d-excess values of groundwater(10.60‰)and reservoir water(11.49‰)were similar to the value of global precipitation(10.00‰).The findings contribute to understanding the hydroclimatic information reflected in the month-by-month variations in stable isotopes in different water bodies and provide a reference for the study of hydrological processes and climate change in the Altay Mountains,China.展开更多
Single-particle resonances in the continuum are crucial for studies of exotic nuclei.In this study,the Green’s function approach is employed to search for single-particle resonances based on the relativistic-mean-fie...Single-particle resonances in the continuum are crucial for studies of exotic nuclei.In this study,the Green’s function approach is employed to search for single-particle resonances based on the relativistic-mean-field model.Taking^(120)Sn as an example,we identify singleparticle resonances and determine the energies and widths directly by probing the extrema of the Green’s functions.In contrast to the results found by exploring for the extremum of the density of states proposed in our recent study[Chin.Phys.C,44:084105(2020)],which has proven to be very successful,the same resonances as well as very close energies and widths are obtained.By comparing the Green’s functions plotted in different coordinate space sizes,we also found that the results very slightly depend on the space size.These findings demonstrate that the approach by exploring for the extremum of the Green’s function is also very reliable and effective for identifying resonant states,regardless of whether they are wide or narrow.展开更多
Single-particle microbeam is uniquely capable of precisely delivering a preset number of charged particles to individual cells or sub-cellular targets to be determined in vitro, It is crucial to find a reference point...Single-particle microbeam is uniquely capable of precisely delivering a preset number of charged particles to individual cells or sub-cellular targets to be determined in vitro, It is crucial to find a reference point that relates the microbeam's location to the microscope's plane, and align individual targets at this reference point for cell irradiation. To choose an appropriate reference point, an approach based on analysing the intensity distribution of fluorescence in a thin scintillator excited by traversing particles is newly developed using the CAS-LIBB single-particle microbeam, which features decisive physical signification and sufficient resolution. As its bonus, this on-line analysis provides precise and fast response to the determination of beam profile and potentially optimizes the microbeam quality by further adjusting hardware setup.展开更多
The Experiments, methods and results of obtaining micron beam in the Microbeam Facility of the Institute of Plasma Physics were discussed in this paper. The H+2 beam was accelerated by the Van de GraafF electrostatic ...The Experiments, methods and results of obtaining micron beam in the Microbeam Facility of the Institute of Plasma Physics were discussed in this paper. The H+2 beam was accelerated by the Van de GraafF electrostatic accelerator, and the collimator at the end of the beam line is a 60 μm thick stainless steel chip. And as a result, particle tracks on the solid track probes (CR39 film) etched in the solution of NaOH showed that the beam can go through the collimator with a small aperure (2000, 300, 55, 30, or 10 μm) and 3.5 μm thick vacuum film (Mylar). Besides the CR39 method, the beam was measured by an energy spectrum detector after the 10 μm diameter aperture and the 3.5 μm thick vacuum film too.展开更多
Single-particle microbeam as a powerful tool can open a research field to find answers to many enigmas in radiobiology. A single-particle microbeam facility has been constructed at the Key Laboratory of Ion Beam Bioen...Single-particle microbeam as a powerful tool can open a research field to find answers to many enigmas in radiobiology. A single-particle microbeam facility has been constructed at the Key Laboratory of Ion Beam Bioengineering (LIBB), Chinese Academy of Sciences (CAS), China. However there has been less research activities in this field concerning the original process of the interaction between low-energy ions and complicated organisms. To address this challenge, an in situ multi-dimensional quantitative fluorescence microscopy system combined with the CAS-LIBB single-particle microbeam II endstation is proposed. In this article, the rationale, logistics and development of many aspects of the proposed system are discussed.展开更多
We study the level structures of N = 7 - 9 isotones and their mirror nuclei in the framework of the single-particle potential model. Considering the limitation of the conventional potential-model calculation, the isos...We study the level structures of N = 7 - 9 isotones and their mirror nuclei in the framework of the single-particle potential model. Considering the limitation of the conventional potential-model calculation, the isospindependent 12 coupling is newly introduced in the average potential. The modified model gives a unified description for the structures of all studied nuclei. Galculations self-consistently produce the s-d level inversion in N = 9 isotones and their mirror nuclei. Meanwhile, the s-p level inversion in the mirror nuclei ^11Be and ^11N is reproduced. The study confirms the neutron halo structures in ^11Be(2s1/2), ^11Be(1p1/2), ^12B(2s1/2), ^14B(2s1/2), ^13C(2sl/2), ^15C(2s1/2) and the proton halo structure in ^17F(2s1/2). The agreement between theory and experiment indicates that the inclusion of the i2 coupling is a feasible way to explain the abnormal structures of exotic light nuclei.展开更多
The focusing and the stable transport of an intense elliptic sheet electron beam in a uniform magnetic field are investigated thoroughly by using the macroscopic cold-fluid model and the single-particle orbit theory.T...The focusing and the stable transport of an intense elliptic sheet electron beam in a uniform magnetic field are investigated thoroughly by using the macroscopic cold-fluid model and the single-particle orbit theory.The results indicate that the envelopes and the tilted angles of the sheet electron beam obtained by the two theories are consistent.The single-particle orbit theory is more accurate due to its treatment of the space-charge fields in a rectangular drift tube.The macroscopic cold-fluid model describes the collective transport process in order to provide detailed information about the beam dynamics,such as beam shape,density,and velocity profile.The tilt of the elliptic sheet beam in a uniform magnetic field is carefully studied and demonstrated.The results presented in this paper provide two complete theories for systemically discussing the transport of the sheet beam and are useful for understanding and guiding the practical engineering design of electron optics systems in high power vacuum electronic devices.展开更多
The proposed multi-dimensional quantitative fluorescence microscopy for the CASLIBB single-particle microbeam II endstation is a CCD-based imaging system. We systematically analyse the theoretical and the practical co...The proposed multi-dimensional quantitative fluorescence microscopy for the CASLIBB single-particle microbeam II endstation is a CCD-based imaging system. We systematically analyse the theoretical and the practical considerations pertinent to choosing the right CCD camera and unveiling the principles underlying multifarious parameters. Therefore, this analysis can be a valuable tool in scrutinizing each parameter and clarifying proper usage of a scientific CCD camera.展开更多
We have studied the structural and atomic transport properties of liquid f-shell Yb in the temperature range 1123 K–1473 K. Pair interactions between atoms are derived using a local pseudopotential. The potential par...We have studied the structural and atomic transport properties of liquid f-shell Yb in the temperature range 1123 K–1473 K. Pair interactions between atoms are derived using a local pseudopotential. The potential parameters are fitted to the phonon dispersion curve at room temperature. The local pseudopotential used in the present study is computationally more efficient with only three parameters, and it is found to be transferable to the liquid phase without changing the parameters.Since the various computed properties agree with reported theoretical and experimental findings, the adopted fitting scheme is justified. As a significant outcome of the study, we find that(i) the melting in Yb is governed by the Lindemann's law,(ii)the mass transport mechanism obeys the Arrhenius law,(iii) the role of the three-particle correlation function in deriving the velocity autocorrelation function is small,(iv) the mean-square atomic displacement is more sensitive to the choice of interaction potential than the other bulk properties, and(v) liquid Yb does not show liquid–liquid phase transition within the studied temperature range. Further, due to the good description of the structural and mass transport properties, we propose that Yb remains divalent at reduced density.展开更多
Modern chromatography is increasingly focused on miniaturization and integration. Compared to conventional liquid chromatography, microfluidic chip liquid chromatography(microchip-LC) has the potential due to its zero...Modern chromatography is increasingly focused on miniaturization and integration. Compared to conventional liquid chromatography, microfluidic chip liquid chromatography(microchip-LC) has the potential due to its zero-dead volume connection and ease of integration. Nano-sized packings have the potential to significantly enhance separation performance in microchip-LC. However, their application has been hindered by packing difficulties. This study presents a method for packing nano-sized silica particles into a microchannel as the stationary phase. The microchip-LC packed column was prepared by combining the weir and the porous silica single-particle as frit to retain the packing particles. A surface tensionbased single-particle picking technique was established to insert porous single-particle frit into glass microchannels. Additionally, we developed a slurry packing method that utilizes air pressure to inject nano-sized packing into the microchannel. Pressure-driven chromatographic separation was performed using this nano-packed column integrated into a glass microchip. The mixture of four PAHs was successfully separated within just 8 min using a 5 mm separation channel length, achieving high theoretical plates(10~6plates/m). Overall, these findings demonstrate the potential of utilizing nano-sized packings for enhancing chromatographic performance in microchip systems.展开更多
The single-particle Schrödinger fluid model is designed mainly to calculate the moments of inertia of the axially symmetric deformed nuclei by assuming that each nucleon in the nucleus is moving in a single-parti...The single-particle Schrödinger fluid model is designed mainly to calculate the moments of inertia of the axially symmetric deformed nuclei by assuming that each nucleon in the nucleus is moving in a single-particle potential which is deformed with time t, through its parametric dependence on a classical shape variable α(t). Also, the Nilsson model is designed for the calculations of the single-particle energy levels, the magnetic dipole moments, and the electric quadrupole moments of axially symmetric deformed nuclei by assuming that all the nucleons are moving in the field of an anisotropic oscillator potential. On the other hand, the nuclear superfluidity model is designed for the calculations of the nuclear moments of inertia and the electric quadrupole moments of deformed nuclei which have no axes of symmetry by assuming that the nucleons are moving in a quadruple deformed potential. Furthermore, the cranked Nilsson model is designed for the calculations of the total nuclear energy and the quadrupole moments of deformed nuclei which have no axes of symmetry by modifying the Nilsson potential to include second and fourth order oscillations. Accordingly, to investigate whether the six p-shell isotopes <sup>6</sup>Li, <sup>7</sup>Li, <sup>8</sup>Li, <sup>9</sup>Li, <sup>10</sup>Li, and <sup>11</sup>Li have axes of symmetry or not, we applied the four mentioned models to each nucleus by calculating their moments of inertia, their magnetic dipole moments, and their electric quadrupole moments by varying the deformation parameter β and the non-axiality parameter γ in wide ranges of values for this reason. Hence for the assumption that these isotopes are deformed and have axes of symmetry, we applied the single-particle Schrödinger fluid model and the Nilsson model. On the other hand, for the assumption that these isotopes are deformed and have no axes of symmetry, we applied the cranked Nilsson model and the nuclear super fluidity model. As a result of our calculations, we can conclude that the nucleus <sup>6</sup>Li may be assumed to be deformed and has an axis of symmetry.展开更多
Strength and deformation behaviors of rockfill materials,key factors for determining the stability of dams,pertain strongly to the grain crushing characteristics.In this study,single-particle crushing tests were carri...Strength and deformation behaviors of rockfill materials,key factors for determining the stability of dams,pertain strongly to the grain crushing characteristics.In this study,single-particle crushing tests were carried out on rockfill materials with nominal particle diameters of 2.5 mm,5 mm and 10 mm to investigate the particle size effect on the single-particle strength and the relationship between the characteristic stress and probability of non-failure.Test data were found to be described by the Weibull distribution with the Weibull modulus of 3.24.Assemblies with uniform nominal grains were then subjected to one-dimensional compression tests at eight levels of vertical stress with a maximum of 100 MPa.The yield stress in one-dimensional compression tests increased with decreasing the particle size,which could be estimated from the single-particle crushing tests.The void ratio-vertical stress curve could be predicted by an exponential function.The particle size distribution curve increased obviously with applied stresses less than 16 MPa and gradually reached the ultimate fractal grading.The relative breakage index became constant with stress up to 64 MPa and was obtained from the ultimate grading at the fractal dimension(a?2:7).A hyperbolical function was also found useful for describing the relationship between the relative breakage index and input work during one-dimensional compression tests.展开更多
The tensor parts of Skyrme interactions are constrained from the collective charge-exchange spin-dipole and Gamow-Teller excitation energies in 90Zr and 208Pb,together with the isotopic dependence of energy splitting ...The tensor parts of Skyrme interactions are constrained from the collective charge-exchange spin-dipole and Gamow-Teller excitation energies in 90Zr and 208Pb,together with the isotopic dependence of energy splitting between proton h11=2 and g7=2 single-particle orbits along the Z=50 isotopes.With the optimized tensor interactions,the binding energies of spherical or weakly deformed nuclei with A=54-228 are studied systematically.The present results show that the global effect of tensor interaction is attractive and systematically increases the binding energies of all these nuclei and makes the nuclei more bound.The root mean squared deviation of the calculated binding energies from the experimental values is significantly improved by the optimized tensor interactions,and the contribution of the tensor interaction to the binding energy is estimated.展开更多
The center of the stability island of super-heavy nuclei(SHN)is the subject of intense experimental and theoretical investigations and has potential technological applications.^(298)^(114) Fl lies in the Z=114 isotopi...The center of the stability island of super-heavy nuclei(SHN)is the subject of intense experimental and theoretical investigations and has potential technological applications.^(298)^(114) Fl lies in the Z=114 isotopic chain as a persuasive candidate of the spherical double-magic nucleus in SHN,and in this study,the calculations of nuclear binding energies,one-nucleon and two-nucleon separation energies,a-decay energies,and the corresponding halflives provide strong evidence for this point.These calculations within an improved Weizsacker-Skyrme nuclear mass model(WS*)were performed and compared with the calculations of the finite-range droplet model(FRDM2012)and experimental data for Z=114 isotopes and N=184 isotones.Concurrently,the corresponding single-particle levels in a Woods-Saxon potential well with a spin-orbit term are calculated,which can be used as a powerful indicator to identify the shell effects existing in114298Fl.Both the study of the properties of the isotopic chain and microphysical quantities provide a vital signal that ^(298)^(114) Fl is a spherical double-magic nucleus and also the center of the SHN.展开更多
Lipid-based nanomedicines(LBNMs),including liposomes,lipid nanoparticles(LNPs)and extracellular vesicles(EVs),are recognized as one of the most clinically acceptable nano-formulations.However,the bench-to-bedside tran...Lipid-based nanomedicines(LBNMs),including liposomes,lipid nanoparticles(LNPs)and extracellular vesicles(EVs),are recognized as one of the most clinically acceptable nano-formulations.However,the bench-to-bedside translation efficiency is far from satisfactory,mainly due to the lack of in-depth understanding of their physical and biochemical attributes at the single-particle level.In this review,we first give a brief introduction of LBNMs,highlighting some milestones and related scientific and clinical achievements in the past several decades,as well as the grand challenges in the characterization of LBNMs.Next,we present an overview of each category of LB-NMs as well as the core properties that largely dictate their biological characteristics and clinical performance,such as size distribution,particle concentration,morphology,drug encapsulation and surface properties.Then,the recent applications of several analytical techniques including electron microscopy,atomic force microscopy,fluorescence microscopy,Raman microscopy,nanoparticle tracking analysis,tunable resistive pulse sensing and flow cytometry on the single-particle characterization of LBNMs are thoroughly discussed.Particularly,the com-parative advantages of the newly developed nano-flow cytometry that enables quantitative analysis of both the physical and biochemical characteristics of LBNMs smaller than 40 nm with high throughput and statistical ro-bustness are emphasized.The overall aim of this review article is to illustrate the importance,challenges and achievements associated with single-particle characterization of LBNMs.展开更多
Energies, widths and wave functions of the single-particle resonant continuum are determined by solvingscattering states of the Dirac equation with proper asymptotic conditions for the continuous spectrum in the relat...Energies, widths and wave functions of the single-particle resonant continuum are determined by solvingscattering states of the Dirac equation with proper asymptotic conditions for the continuous spectrum in the relativisticmean-field theory. The relativistic regular and irregular Coulomb wave functions are calculated numerically. Theresonance states in the continuum for some closed- or sub-closed-shell nucleus in Sn-isotopes, such as 1 14Sn, 1 16Sn, 1 18Sn,and 120Sn are calculated. Results show that the S-matrix method is a reliable and straightforward way in determiningenergies and widths of resonant states.展开更多
Brake wear is an important but unregulated vehicle-related source of atmospheric particulate matter(PM).The single-particle spectral fingerprints of brake wear particles(BWPs)provide essential information for understa...Brake wear is an important but unregulated vehicle-related source of atmospheric particulate matter(PM).The single-particle spectral fingerprints of brake wear particles(BWPs)provide essential information for understanding their formation mechanism and atmospheric contributions.Herein,we obtained the single-particle mass spectra of BWPs by combining a brake dynamometer with an online single particle aerosol mass spectrometer and quantified real-world BWP emissions through a tunnel observation in Tianjin,China.The pure BWPs mainly include three distinct types of particles,namely,Bacontaining particles,mineral particles,and carbon-containing particles,accounting for 44.2%,43.4%,and 10.3%of the total BWP number concentration,respectively.The diversified mass spectra indicate complex BWP formation pathways,such as mechanical,phase transition,and chemical processes.Notably,the mass spectra of Ba-containing particles are unique,which allows them to serve as an excellent indicator for estimating ambient BWP concentrations.By evaluating this indicator,we find that approximately 4.0%of the PM in the tunnel could be attributable to brake wear;the real-world fleet-average emission factor of 0.28 mg km1 veh1 is consistent with the estimation obtained using the receptor model.The results presented herein can be used to inform assessments of the environmental and health impacts of BWPs to formulate effective emissions control policies.展开更多
The progress of a microbeam facility in the Institute of Plasma Physics was discussed in this paper. This kind of equipment can supply single-particle beam which may be implanted into cells in micrometer-radius and me...The progress of a microbeam facility in the Institute of Plasma Physics was discussed in this paper. This kind of equipment can supply single-particle beam which may be implanted into cells in micrometer-radius and measured by a new outstanding detector among global microbeam systems. Measurements by some plain targets showed that the highest current after the accelerator tube can be larger than 20 /μA, the H_2^+ current before the second bending magnet is near 0.9 /μA, the current after the second bending magnet is near 0.8 μA, and the current of the beam line (after a 2-mm diameter aperture) is near 0.25 nA which is enough for the single-particle microbeam experiment. It took scientists 3 months to do their microbeam experiment after setting up the accelerator beam line and get the microbeam from this equipment. Two pre-collimators were installed between the 2-mm diameter aperture and the collimator to survey the beam. Tracks on the CR39 film etched in the solution of NaOH showed that the beam can go through the collimator including a 10 μm diameter aperture and the 3.5 μm thick vacuum sealing film (Mylar). A new method, which is called optimization of the beam quality, was put forward in this paper, in order to get smaller diameter of beam-spot in microbeam system.展开更多
基金Project supported by the National Natural Science Foundation of China(Nos.11872283 and 2002212)the Sailing Program of Shanghai,China(No.20YF1432800)。
文摘In the present study,the nanofliud natural convection is investigated by the energy-conserving dissipative particle dynamics(eDPD)method,where the nanoparticles are considered at the single-particle level.The thermal expansion coefficientβand the viscosityμof the simulated system containing nanoparticles are calculated and found to be in close alignment with the previous simulation results.The single-particle hydrodynamics in e DPD enables simulations of nanofluid natural convection with higher Rayleigh numbers and greater nanoparticle volume fractions.Additionally,this approach is utilized to simulate the nanoparticle distribution during the enhanced heat transfer process in the nanofluid natural convection.The localized aggregation of nanoparticles enhances the heat transfer performance of the nanofluid under specific Rayleigh numbers and nanoparticles volume fractions.
基金Under the auspices of National Natural Science Foundation of China (No.42101044,42077188,52109007)。
文摘Recycled moisture is an important indicator of the renewal capacity of regional water resources.Due to the existence of Yulong Snow Mountain,Lijiang in Yunnan Province,southeast of the Qinghai-Tibet Plateau,China,is the closest ocean glacier area to the equator in Eurasia.Daily precipitation samples were collected from 2017 to 2018 in Lijiang to quantify the effect of sub-cloud evaporation and recycled moisture on precipitation combined with the d-excess model during monsoon and non-monsoon periods.The results indicated that the d-excess values of precipitation fluctuated between–35.6‰and 16.0‰,with an arithmetic mean of 3.5‰.The local meteoric water line(LMWL)wasδD=7.91δ^(18)O+2.50,with a slope slightly lower than the global meteoric water line(GMWL).Subcloud evaporation was higher during the non-monsoon season than during the monsoon season.It tended to peak in March and was primarily influenced by the relative humidity.The source of the water vapour affected the proportion of recycled moisture.According to the results of the Hybrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT)model,the main sources of water vapour in Lijiang area during the monsoon period were the southwest and southeast monsoons.During the non-monsoon period,water vapour was transported by a southwesterly flow.The recycled moisture in Lijiang area between March and October 2017 was 10.62%.Large variations were observed between the monsoon and non-monsoon seasons,with values of 5.48%and 25.65%,respectively.These differences were primarily attributed to variations in the advection of water vapour.The recycled moisture has played a supplementary role in the precipitation of Lijiang area.
基金This work was funded by the Science and Technology Program of Gansu Province(23ZDFA017,22ZD6FA005)the Third Xinjiang Scientific Expedition Program(2022xjkk0802).
文摘Characterization of the spatial and temporal variability of stable isotopes in surface water is essential for interpreting hydrological processes.In this study,we collected the water samples of river water,groundwater,and reservoir water in the Burqin River Basin of the Altay Mountains,China in 2021,and characterized the oxygen and hydrogen isotope variations in different water bodies via instrumental analytics and modeling.Results showed significant seasonal variations in stable isotope ratios of oxygen and hydrogen(δ18O andδ2H,respectively)and significant differences inδ18O andδ2H among different water bodies.Higherδ18O andδ2H values were mainly found in river water,while groundwater and reservoir water had lower isotope ratios.River water and groundwater showed differentδ18O-δ2H relationships with the local meteoric water line,implying that river water and groundwater are controlled by evaporative enrichment and multi-source recharge processes.The evaporative enrichment experienced by reservoir water was less significant and largely influenced by topography,recharge sources,local moisture cycling,and anthropogenic factors.Higher deuterium excess(d-excess)value of 14.34‰for river water probably represented the isotopic signature of combined contributions from direct precipitation,snow and glacial meltwater,and groundwater recharge.The average annual d-excess values of groundwater(10.60‰)and reservoir water(11.49‰)were similar to the value of global precipitation(10.00‰).The findings contribute to understanding the hydroclimatic information reflected in the month-by-month variations in stable isotopes in different water bodies and provide a reference for the study of hydrological processes and climate change in the Altay Mountains,China.
基金supported by the National Natural Science Foundation of China(No.U2032141)the Natural Science Foundation of Henan Province(No.202300410479,No.202300410480)+1 种基金the Foundation of Fundamental Research for Young Teachers of Zhengzhou University(No.JC202041041)the Physics Research and Development Program of Zhengzhou University(No.32410217).
文摘Single-particle resonances in the continuum are crucial for studies of exotic nuclei.In this study,the Green’s function approach is employed to search for single-particle resonances based on the relativistic-mean-field model.Taking^(120)Sn as an example,we identify singleparticle resonances and determine the energies and widths directly by probing the extrema of the Green’s functions.In contrast to the results found by exploring for the extremum of the density of states proposed in our recent study[Chin.Phys.C,44:084105(2020)],which has proven to be very successful,the same resonances as well as very close energies and widths are obtained.By comparing the Green’s functions plotted in different coordinate space sizes,we also found that the results very slightly depend on the space size.These findings demonstrate that the approach by exploring for the extremum of the Green’s function is also very reliable and effective for identifying resonant states,regardless of whether they are wide or narrow.
文摘Single-particle microbeam is uniquely capable of precisely delivering a preset number of charged particles to individual cells or sub-cellular targets to be determined in vitro, It is crucial to find a reference point that relates the microbeam's location to the microscope's plane, and align individual targets at this reference point for cell irradiation. To choose an appropriate reference point, an approach based on analysing the intensity distribution of fluorescence in a thin scintillator excited by traversing particles is newly developed using the CAS-LIBB single-particle microbeam, which features decisive physical signification and sufficient resolution. As its bonus, this on-line analysis provides precise and fast response to the determination of beam profile and potentially optimizes the microbeam quality by further adjusting hardware setup.
基金The project supported by the National Science Foundation of in Anhui Province,China(No.01046201)
文摘The Experiments, methods and results of obtaining micron beam in the Microbeam Facility of the Institute of Plasma Physics were discussed in this paper. The H+2 beam was accelerated by the Van de GraafF electrostatic accelerator, and the collimator at the end of the beam line is a 60 μm thick stainless steel chip. And as a result, particle tracks on the solid track probes (CR39 film) etched in the solution of NaOH showed that the beam can go through the collimator with a small aperure (2000, 300, 55, 30, or 10 μm) and 3.5 μm thick vacuum film (Mylar). Besides the CR39 method, the beam was measured by an energy spectrum detector after the 10 μm diameter aperture and the 3.5 μm thick vacuum film too.
文摘Single-particle microbeam as a powerful tool can open a research field to find answers to many enigmas in radiobiology. A single-particle microbeam facility has been constructed at the Key Laboratory of Ion Beam Bioengineering (LIBB), Chinese Academy of Sciences (CAS), China. However there has been less research activities in this field concerning the original process of the interaction between low-energy ions and complicated organisms. To address this challenge, an in situ multi-dimensional quantitative fluorescence microscopy system combined with the CAS-LIBB single-particle microbeam II endstation is proposed. In this article, the rationale, logistics and development of many aspects of the proposed system are discussed.
基金National Natural Science Foundation of China under Grant Nos.10535010 and 10775068the State Key Basic Research Program under Grant No.2007CB815004+1 种基金the CAS Knowledge Innovation Project under Grant No.KJCX2-SW-N02the Research Fund of High Education under Grant No.20010284036
文摘We study the level structures of N = 7 - 9 isotones and their mirror nuclei in the framework of the single-particle potential model. Considering the limitation of the conventional potential-model calculation, the isospindependent 12 coupling is newly introduced in the average potential. The modified model gives a unified description for the structures of all studied nuclei. Galculations self-consistently produce the s-d level inversion in N = 9 isotones and their mirror nuclei. Meanwhile, the s-p level inversion in the mirror nuclei ^11Be and ^11N is reproduced. The study confirms the neutron halo structures in ^11Be(2s1/2), ^11Be(1p1/2), ^12B(2s1/2), ^14B(2s1/2), ^13C(2sl/2), ^15C(2s1/2) and the proton halo structure in ^17F(2s1/2). The agreement between theory and experiment indicates that the inclusion of the i2 coupling is a feasible way to explain the abnormal structures of exotic light nuclei.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 60501019,10775139 and 60971073)
文摘The focusing and the stable transport of an intense elliptic sheet electron beam in a uniform magnetic field are investigated thoroughly by using the macroscopic cold-fluid model and the single-particle orbit theory.The results indicate that the envelopes and the tilted angles of the sheet electron beam obtained by the two theories are consistent.The single-particle orbit theory is more accurate due to its treatment of the space-charge fields in a rectangular drift tube.The macroscopic cold-fluid model describes the collective transport process in order to provide detailed information about the beam dynamics,such as beam shape,density,and velocity profile.The tilt of the elliptic sheet beam in a uniform magnetic field is carefully studied and demonstrated.The results presented in this paper provide two complete theories for systemically discussing the transport of the sheet beam and are useful for understanding and guiding the practical engineering design of electron optics systems in high power vacuum electronic devices.
基金supported by the the National Major Technologies R&D Programme of China during the 10th Five-Year Plan Period(No.2001BA302B)the National Science Foundation for Distinguished Young Scholars(No.10225526)+1 种基金the Knowledge Innovation Programme of the Chinese Academy of Sciences(No.KSCX2-SW-324)the Foundation for University Key Teacher by the Ministry of Education(No.2005jq1135).
文摘The proposed multi-dimensional quantitative fluorescence microscopy for the CASLIBB single-particle microbeam II endstation is a CCD-based imaging system. We systematically analyse the theoretical and the practical considerations pertinent to choosing the right CCD camera and unveiling the principles underlying multifarious parameters. Therefore, this analysis can be a valuable tool in scrutinizing each parameter and clarifying proper usage of a scientific CCD camera.
文摘We have studied the structural and atomic transport properties of liquid f-shell Yb in the temperature range 1123 K–1473 K. Pair interactions between atoms are derived using a local pseudopotential. The potential parameters are fitted to the phonon dispersion curve at room temperature. The local pseudopotential used in the present study is computationally more efficient with only three parameters, and it is found to be transferable to the liquid phase without changing the parameters.Since the various computed properties agree with reported theoretical and experimental findings, the adopted fitting scheme is justified. As a significant outcome of the study, we find that(i) the melting in Yb is governed by the Lindemann's law,(ii)the mass transport mechanism obeys the Arrhenius law,(iii) the role of the three-particle correlation function in deriving the velocity autocorrelation function is small,(iv) the mean-square atomic displacement is more sensitive to the choice of interaction potential than the other bulk properties, and(v) liquid Yb does not show liquid–liquid phase transition within the studied temperature range. Further, due to the good description of the structural and mass transport properties, we propose that Yb remains divalent at reduced density.
基金supported by the National Natural Science Foundation of China (No.21936001)the Beijing Outstanding Young Scientist Program (No.BJJWZYJH01201910005017)。
文摘Modern chromatography is increasingly focused on miniaturization and integration. Compared to conventional liquid chromatography, microfluidic chip liquid chromatography(microchip-LC) has the potential due to its zero-dead volume connection and ease of integration. Nano-sized packings have the potential to significantly enhance separation performance in microchip-LC. However, their application has been hindered by packing difficulties. This study presents a method for packing nano-sized silica particles into a microchannel as the stationary phase. The microchip-LC packed column was prepared by combining the weir and the porous silica single-particle as frit to retain the packing particles. A surface tensionbased single-particle picking technique was established to insert porous single-particle frit into glass microchannels. Additionally, we developed a slurry packing method that utilizes air pressure to inject nano-sized packing into the microchannel. Pressure-driven chromatographic separation was performed using this nano-packed column integrated into a glass microchip. The mixture of four PAHs was successfully separated within just 8 min using a 5 mm separation channel length, achieving high theoretical plates(10~6plates/m). Overall, these findings demonstrate the potential of utilizing nano-sized packings for enhancing chromatographic performance in microchip systems.
文摘The single-particle Schrödinger fluid model is designed mainly to calculate the moments of inertia of the axially symmetric deformed nuclei by assuming that each nucleon in the nucleus is moving in a single-particle potential which is deformed with time t, through its parametric dependence on a classical shape variable α(t). Also, the Nilsson model is designed for the calculations of the single-particle energy levels, the magnetic dipole moments, and the electric quadrupole moments of axially symmetric deformed nuclei by assuming that all the nucleons are moving in the field of an anisotropic oscillator potential. On the other hand, the nuclear superfluidity model is designed for the calculations of the nuclear moments of inertia and the electric quadrupole moments of deformed nuclei which have no axes of symmetry by assuming that the nucleons are moving in a quadruple deformed potential. Furthermore, the cranked Nilsson model is designed for the calculations of the total nuclear energy and the quadrupole moments of deformed nuclei which have no axes of symmetry by modifying the Nilsson potential to include second and fourth order oscillations. Accordingly, to investigate whether the six p-shell isotopes <sup>6</sup>Li, <sup>7</sup>Li, <sup>8</sup>Li, <sup>9</sup>Li, <sup>10</sup>Li, and <sup>11</sup>Li have axes of symmetry or not, we applied the four mentioned models to each nucleus by calculating their moments of inertia, their magnetic dipole moments, and their electric quadrupole moments by varying the deformation parameter β and the non-axiality parameter γ in wide ranges of values for this reason. Hence for the assumption that these isotopes are deformed and have axes of symmetry, we applied the single-particle Schrödinger fluid model and the Nilsson model. On the other hand, for the assumption that these isotopes are deformed and have no axes of symmetry, we applied the cranked Nilsson model and the nuclear super fluidity model. As a result of our calculations, we can conclude that the nucleus <sup>6</sup>Li may be assumed to be deformed and has an axis of symmetry.
基金financial support from the 111 Project (Grant No. B13024)the National Science Foundation of China (Grant Nos. 51509024, 51678094 and 51578096)+2 种基金the Fundamental Research Funds for the Central Universities (Grant No. 106112017CDJQJ208848)the Special Financial Grant from the China Postdoctoral Science Foundation (Grant No. 2017T100681)the State Key Laboratory for Geo Mechanics and Deep Underground Engineering, China University of Mining and Technology (Grant No. SKLGDUEK1810)
文摘Strength and deformation behaviors of rockfill materials,key factors for determining the stability of dams,pertain strongly to the grain crushing characteristics.In this study,single-particle crushing tests were carried out on rockfill materials with nominal particle diameters of 2.5 mm,5 mm and 10 mm to investigate the particle size effect on the single-particle strength and the relationship between the characteristic stress and probability of non-failure.Test data were found to be described by the Weibull distribution with the Weibull modulus of 3.24.Assemblies with uniform nominal grains were then subjected to one-dimensional compression tests at eight levels of vertical stress with a maximum of 100 MPa.The yield stress in one-dimensional compression tests increased with decreasing the particle size,which could be estimated from the single-particle crushing tests.The void ratio-vertical stress curve could be predicted by an exponential function.The particle size distribution curve increased obviously with applied stresses less than 16 MPa and gradually reached the ultimate fractal grading.The relative breakage index became constant with stress up to 64 MPa and was obtained from the ultimate grading at the fractal dimension(a?2:7).A hyperbolical function was also found useful for describing the relationship between the relative breakage index and input work during one-dimensional compression tests.
基金supported by the National Natural Science Foundation of China(Nos.11575120 and 11822504)JSPS KAKENHI(No.JP19K03858)
文摘The tensor parts of Skyrme interactions are constrained from the collective charge-exchange spin-dipole and Gamow-Teller excitation energies in 90Zr and 208Pb,together with the isotopic dependence of energy splitting between proton h11=2 and g7=2 single-particle orbits along the Z=50 isotopes.With the optimized tensor interactions,the binding energies of spherical or weakly deformed nuclei with A=54-228 are studied systematically.The present results show that the global effect of tensor interaction is attractive and systematically increases the binding energies of all these nuclei and makes the nuclei more bound.The root mean squared deviation of the calculated binding energies from the experimental values is significantly improved by the optimized tensor interactions,and the contribution of the tensor interaction to the binding energy is estimated.
基金supported by the National Natural Science Foundation of China(Nos.10775061,11175054,11675066,11665019,and11947229)the China Postdoctoral Science Foundation(No.2019M663853)+1 种基金the Fundamental Research Funds for the Central Universities(Nos.lzujbky-2017-ot04 and lzujbky-2020-it01)Feitian Scholar Project of Gansu Province。
文摘The center of the stability island of super-heavy nuclei(SHN)is the subject of intense experimental and theoretical investigations and has potential technological applications.^(298)^(114) Fl lies in the Z=114 isotopic chain as a persuasive candidate of the spherical double-magic nucleus in SHN,and in this study,the calculations of nuclear binding energies,one-nucleon and two-nucleon separation energies,a-decay energies,and the corresponding halflives provide strong evidence for this point.These calculations within an improved Weizsacker-Skyrme nuclear mass model(WS*)were performed and compared with the calculations of the finite-range droplet model(FRDM2012)and experimental data for Z=114 isotopes and N=184 isotones.Concurrently,the corresponding single-particle levels in a Woods-Saxon potential well with a spin-orbit term are calculated,which can be used as a powerful indicator to identify the shell effects existing in114298Fl.Both the study of the properties of the isotopic chain and microphysical quantities provide a vital signal that ^(298)^(114) Fl is a spherical double-magic nucleus and also the center of the SHN.
基金We are grateful to the National Natural Science Foundation of China(21934004,21627811)the National Key R&D Program of China(2021YFA0909400)the Natural Science Foundation of Fujian Province(2022J01329)for financial support.
文摘Lipid-based nanomedicines(LBNMs),including liposomes,lipid nanoparticles(LNPs)and extracellular vesicles(EVs),are recognized as one of the most clinically acceptable nano-formulations.However,the bench-to-bedside translation efficiency is far from satisfactory,mainly due to the lack of in-depth understanding of their physical and biochemical attributes at the single-particle level.In this review,we first give a brief introduction of LBNMs,highlighting some milestones and related scientific and clinical achievements in the past several decades,as well as the grand challenges in the characterization of LBNMs.Next,we present an overview of each category of LB-NMs as well as the core properties that largely dictate their biological characteristics and clinical performance,such as size distribution,particle concentration,morphology,drug encapsulation and surface properties.Then,the recent applications of several analytical techniques including electron microscopy,atomic force microscopy,fluorescence microscopy,Raman microscopy,nanoparticle tracking analysis,tunable resistive pulse sensing and flow cytometry on the single-particle characterization of LBNMs are thoroughly discussed.Particularly,the com-parative advantages of the newly developed nano-flow cytometry that enables quantitative analysis of both the physical and biochemical characteristics of LBNMs smaller than 40 nm with high throughput and statistical ro-bustness are emphasized.The overall aim of this review article is to illustrate the importance,challenges and achievements associated with single-particle characterization of LBNMs.
基金The project supported by National Natural Science Foundation of China under Grant Nos. 10075080, 19847002, 19835010 and Major State Basic Research Development Program under Grant No. G20000774
文摘Energies, widths and wave functions of the single-particle resonant continuum are determined by solvingscattering states of the Dirac equation with proper asymptotic conditions for the continuous spectrum in the relativisticmean-field theory. The relativistic regular and irregular Coulomb wave functions are calculated numerically. Theresonance states in the continuum for some closed- or sub-closed-shell nucleus in Sn-isotopes, such as 1 14Sn, 1 16Sn, 1 18Sn,and 120Sn are calculated. Results show that the S-matrix method is a reliable and straightforward way in determiningenergies and widths of resonant states.
基金supported by the National key research and development program of China(2022YFE0135000)the Tianjin Science and Technology Plan Project(19YFZCSF00960)+2 种基金the National Natural Science Foundation of China(42177084,42175123,42107114,42107125)the Natural Science Foundation of Tianjin(20JCYBJC01270)the Fundamental Research Funds for the Central Universities(63221411).
文摘Brake wear is an important but unregulated vehicle-related source of atmospheric particulate matter(PM).The single-particle spectral fingerprints of brake wear particles(BWPs)provide essential information for understanding their formation mechanism and atmospheric contributions.Herein,we obtained the single-particle mass spectra of BWPs by combining a brake dynamometer with an online single particle aerosol mass spectrometer and quantified real-world BWP emissions through a tunnel observation in Tianjin,China.The pure BWPs mainly include three distinct types of particles,namely,Bacontaining particles,mineral particles,and carbon-containing particles,accounting for 44.2%,43.4%,and 10.3%of the total BWP number concentration,respectively.The diversified mass spectra indicate complex BWP formation pathways,such as mechanical,phase transition,and chemical processes.Notably,the mass spectra of Ba-containing particles are unique,which allows them to serve as an excellent indicator for estimating ambient BWP concentrations.By evaluating this indicator,we find that approximately 4.0%of the PM in the tunnel could be attributable to brake wear;the real-world fleet-average emission factor of 0.28 mg km1 veh1 is consistent with the estimation obtained using the receptor model.The results presented herein can be used to inform assessments of the environmental and health impacts of BWPs to formulate effective emissions control policies.
基金The project supported by the Natural Science Foundation Committee in Anhui Province, China (No. 01046201)
文摘The progress of a microbeam facility in the Institute of Plasma Physics was discussed in this paper. This kind of equipment can supply single-particle beam which may be implanted into cells in micrometer-radius and measured by a new outstanding detector among global microbeam systems. Measurements by some plain targets showed that the highest current after the accelerator tube can be larger than 20 /μA, the H_2^+ current before the second bending magnet is near 0.9 /μA, the current after the second bending magnet is near 0.8 μA, and the current of the beam line (after a 2-mm diameter aperture) is near 0.25 nA which is enough for the single-particle microbeam experiment. It took scientists 3 months to do their microbeam experiment after setting up the accelerator beam line and get the microbeam from this equipment. Two pre-collimators were installed between the 2-mm diameter aperture and the collimator to survey the beam. Tracks on the CR39 film etched in the solution of NaOH showed that the beam can go through the collimator including a 10 μm diameter aperture and the 3.5 μm thick vacuum sealing film (Mylar). A new method, which is called optimization of the beam quality, was put forward in this paper, in order to get smaller diameter of beam-spot in microbeam system.