The data, measured by a three-wavelength Integrating Nephelometer over Lanzhou City during the winters of 2001/2002 and 2002/2003 respectively, have been analyzed for investigating the scattering properties of atmos...The data, measured by a three-wavelength Integrating Nephelometer over Lanzhou City during the winters of 2001/2002 and 2002/2003 respectively, have been analyzed for investigating the scattering properties of atmospheric aerosols and exploring their relationship and the status of air pollution. The aerosol particle volume distribution is inverted with the measured spectral scattering coe?cients. The results show that the daily variation of the aerosol scattering coe?cients is in a tri-peak shape. The average ratio of backscattering coe?cient to total scattering coe?cient at 550 nm is 0.158; there exists an excellent correlation between the scattering coe?cients and the concentration of PM10. The average ratio of the concentration of PM10 to the scattering coe?cients is 0.37 g m?2, which is contingent on the optical parameters of aerosol particles such as the size distribution, etc.; an algorithm is developed for inverting the volume distribution of aerosol particles by using the histogram and Monte-Carlo techniques, and the test results show that the inversion is reasonable.展开更多
Smoothing by spectral dispersion (SSD) leads to considerable improvement on laser-irradiation uniformity in far field for fusion lasers. Phase modulation in time and spectral angular dispersion (SAD) across the be...Smoothing by spectral dispersion (SSD) leads to considerable improvement on laser-irradiation uniformity in far field for fusion lasers. Phase modulation in time and spectral angular dispersion (SAD) across the beam introduced by SSD will affect the stimulated rotational Raman scattering (SRRS) gain in the near field. This paper focuses on the influence of SAD on SRRS gain under different laser conditions. Results show that the SAD will aggravate the generation of SRRS when the laser initial additional phase is constant. On the contrary, the SAD can reduce the SRRS gain if appropriate SSD parameters are adopted when the laser initial additional phase is variable. SSD has a certain application prospect in SRRS suppression.展开更多
In pH 7.2 Na2HPO4-NaH2PO4 buffer solution and in the (GABF) was combined with human factor B (BF) specifically, presence of PEG-6000, goat-anti-human factor B and aggregated to form immune complex particles that e...In pH 7.2 Na2HPO4-NaH2PO4 buffer solution and in the (GABF) was combined with human factor B (BF) specifically, presence of PEG-6000, goat-anti-human factor B and aggregated to form immune complex particles that exhibited a resonance scattering (RS) peak at 400 nm. The laser scattering indicated that the average diameter of immune complex particles was 1320 nm. BF in the concentration range of 0.04 to 9.60 μg/mL was proportional to the resonance scattering intensity at 400 nm. Its regression equation was A/=33.61C + 1.4, with a correlation coefficient of 0.9969, and a detection limit of 0.01 μg/mL BF. This label-free resonance scattering spectral (RSS) method has been applied to the determination of BF in serum samples, and the results were in agreement with that of the immunoturbity.展开更多
In pH 7.2 Na2HPO4-NaH2PO4 buffer solution, polyphenoloxidase (PPO) could catalyze the oxidization of do- pamine (DA) to form polymer particles in dark-red color, which exhibited a strong resonance scattering (RS...In pH 7.2 Na2HPO4-NaH2PO4 buffer solution, polyphenoloxidase (PPO) could catalyze the oxidization of do- pamine (DA) to form polymer particles in dark-red color, which exhibited a strong resonance scattering (RS) peak at 780 nm. In the chosen conditions, as the PPO activity increased, the RS intensity at 780 nm increased linearly. The increased RS intensity (△I780nm) was linear to the PPO activity in the range of 0.10--6.0 U·mL^- 1, with a regression equation of △I780 nm = 96.6C+ 15.1, a relative coefficient of 0.9987 and a detection limit of 0.06 U·mL^-1 PPO. The proposed method was applied to detecting PPO activity in potato sample with satisfactory results.展开更多
The 5 nm AuPd nanoalloy in mole ratio of Au:Pd=32 : 1 was prepared, using sodium citrate as the stabilizing agent and NaBH4 as the reductant. The AuPd nanoalloy was modified by the aptamer to prepare an aptamer- Au...The 5 nm AuPd nanoalloy in mole ratio of Au:Pd=32 : 1 was prepared, using sodium citrate as the stabilizing agent and NaBH4 as the reductant. The AuPd nanoalloy was modified by the aptamer to prepare an aptamer- AuPd (AptAuPd) probe for resonance scattering (RS) detection of 5.(Y-1250 nmol/L Hg2+. The AptAuPd-Hg2+ aptamer reaction solution was filtrated by membrane, and the AptAuPd in the filtrate exhibited strong catalytic ef- fect on the slow NiP particle reaction between NiCI2 and NaHzPO2, and the NiP particles showed a RS peak at 508 nm. The RS intensity decreased when Hg2+ concentration increased. The decreased RS intensity was linear to Hg2+ concentration in the range of 0.5--1250 nmol/L. The RS assays were used to determine Hg2+ in real samples, with good results.展开更多
基金the National Natural Science Foundation of China(Grant Nos.49875027,40275039).
文摘The data, measured by a three-wavelength Integrating Nephelometer over Lanzhou City during the winters of 2001/2002 and 2002/2003 respectively, have been analyzed for investigating the scattering properties of atmospheric aerosols and exploring their relationship and the status of air pollution. The aerosol particle volume distribution is inverted with the measured spectral scattering coe?cients. The results show that the daily variation of the aerosol scattering coe?cients is in a tri-peak shape. The average ratio of backscattering coe?cient to total scattering coe?cient at 550 nm is 0.158; there exists an excellent correlation between the scattering coe?cients and the concentration of PM10. The average ratio of the concentration of PM10 to the scattering coe?cients is 0.37 g m?2, which is contingent on the optical parameters of aerosol particles such as the size distribution, etc.; an algorithm is developed for inverting the volume distribution of aerosol particles by using the histogram and Monte-Carlo techniques, and the test results show that the inversion is reasonable.
基金Project supported by the State Key Program of the National Natural Science Foundation of China(Grant No.61138005)the National Natural Science Foundation of China(Grant No.61008004)
文摘Smoothing by spectral dispersion (SSD) leads to considerable improvement on laser-irradiation uniformity in far field for fusion lasers. Phase modulation in time and spectral angular dispersion (SAD) across the beam introduced by SSD will affect the stimulated rotational Raman scattering (SRRS) gain in the near field. This paper focuses on the influence of SAD on SRRS gain under different laser conditions. Results show that the SAD will aggravate the generation of SRRS when the laser initial additional phase is constant. On the contrary, the SAD can reduce the SRRS gain if appropriate SSD parameters are adopted when the laser initial additional phase is variable. SSD has a certain application prospect in SRRS suppression.
基金Acknowledgement This work was supported by the National Natural Science Foundation of China (Nos. 21165005, 21075023), the fund of State Key Laboratory Cultivation Base for the Chemistry and Molecular Engineering of Medicinal Resources, Ministry of Science and Technology of China (CMEMR2011-10).
文摘In pH 7.2 Na2HPO4-NaH2PO4 buffer solution and in the (GABF) was combined with human factor B (BF) specifically, presence of PEG-6000, goat-anti-human factor B and aggregated to form immune complex particles that exhibited a resonance scattering (RS) peak at 400 nm. The laser scattering indicated that the average diameter of immune complex particles was 1320 nm. BF in the concentration range of 0.04 to 9.60 μg/mL was proportional to the resonance scattering intensity at 400 nm. Its regression equation was A/=33.61C + 1.4, with a correlation coefficient of 0.9969, and a detection limit of 0.01 μg/mL BF. This label-free resonance scattering spectral (RSS) method has been applied to the determination of BF in serum samples, and the results were in agreement with that of the immunoturbity.
基金Project supported by the National Natural Science Foundation of China (Nos. 20865002, 20965002, 21075023), the Natural Science Foundation ot Guangxi (Nos. 0991021 z, 0832260) and the Research Funds of Key Laboratory of Ecology of Rare and Endangered Species and Environmental Protection (Guangxi Normal University), Ministry of Education.
文摘In pH 7.2 Na2HPO4-NaH2PO4 buffer solution, polyphenoloxidase (PPO) could catalyze the oxidization of do- pamine (DA) to form polymer particles in dark-red color, which exhibited a strong resonance scattering (RS) peak at 780 nm. In the chosen conditions, as the PPO activity increased, the RS intensity at 780 nm increased linearly. The increased RS intensity (△I780nm) was linear to the PPO activity in the range of 0.10--6.0 U·mL^- 1, with a regression equation of △I780 nm = 96.6C+ 15.1, a relative coefficient of 0.9987 and a detection limit of 0.06 U·mL^-1 PPO. The proposed method was applied to detecting PPO activity in potato sample with satisfactory results.
基金Project supported by the National Natural Science Founclation of china (Nos. 21075023, 20965002, 20865002), Natural Science Foundation of Guangxi (No. 0991021z), the Research Funds of Guangxi Water Conservancy, the Research Funds of Key Laboratory of Ecology of Rare and En- dangered Species and Environmental Protection, Ministry of Education (No. 10012019) and the Research Funds of Guangxi Education Office.
文摘The 5 nm AuPd nanoalloy in mole ratio of Au:Pd=32 : 1 was prepared, using sodium citrate as the stabilizing agent and NaBH4 as the reductant. The AuPd nanoalloy was modified by the aptamer to prepare an aptamer- AuPd (AptAuPd) probe for resonance scattering (RS) detection of 5.(Y-1250 nmol/L Hg2+. The AptAuPd-Hg2+ aptamer reaction solution was filtrated by membrane, and the AptAuPd in the filtrate exhibited strong catalytic ef- fect on the slow NiP particle reaction between NiCI2 and NaHzPO2, and the NiP particles showed a RS peak at 508 nm. The RS intensity decreased when Hg2+ concentration increased. The decreased RS intensity was linear to Hg2+ concentration in the range of 0.5--1250 nmol/L. The RS assays were used to determine Hg2+ in real samples, with good results.