Linear and nonlinear characteristics of time-resolved photoluminescence modulation by terahertz pulse

The linear and nonlinear characteristics of time-resolved photoluminescence （PL） of n-type bulk semiconductor GaAs modulated with terahertz （THz） pulse are studied by using an ensemble Monte Carlo （EMC） method. In this paper the center energy valley （Г valley） electron concentration changes with the pulse delay time, sampling time and the outfield are mainly discussed. The results show that the sampling time and the THz field should exceed certain thresholds to effectively excite photoluminescence quenching （PLQ）. Adopting a direct current （DC） field makes the sampling time threshold shortened and the linear range of THz field-modulation PL expanded. Moreover, controlling the sampling time and the outfield intensity can improve the linear quality： with forward time, the larger outfield is used; with backward time, the smaller outfield is used. This study can provide a theoretical basis of THz field linear modulation in a larger range for new light emitting devices.

Simultaneous field-free molecular orientation and planar delocalization by THz laser pulses[Invited]

This study shows the unexpected and counterintuitive possibility of simultaneously orienting a molecule while delocalizing its molecular axis in a plane in field-free conditions.The corresponding quantum states are characterized,and different control strategies using shaped terahertz(THz)laser pulses are proposed to reach such states at zero and nonzero temperatures.The robustness against temperature effects of a simple control procedure combining a laser and a THz pulse is shown.Such control strategies can be applied not only to linear molecules but also to symmetric top molecules.

Intense terahertz generation from photoconductive antennas

In this paper,we review the past and recent works on generating intense terahertz(THz)pulses from photoconductive antennas(PCAs).We will focus on two types of large-aperture photoconductive antenna(LAPCA)that can generate high-intensity THz pulses(a)those with large-aperture dipoles and(b)those with interdigitated electrodes.We will first describe the principles of THz generation from PCAs.The critical parameters for improving the peak intensity of THz radiation from LAPCAs are summarized.We will then describe the saturation and limitation process of LAPCAs along with the advantages and disadvantages of working with widebandgap semiconductor substrates.Then,we will explain the evolution of LAPCA with interdigitated electrodes,which allows one to reduce the photoconductive gap size,and thus obtain higher bias fields while applying lower voltages.We will also describe recent achievements in intense THz pulses generated by interdigitated LAPCAs based on wide-bandgap semiconductors driven by ampli-fied lasers.Finally,we will discuss the future perspectives of THz pulse generation using LAPCAs.