A two‐step photocatalytic water splitting system,termed a“Z‐scheme system”,was achieved using Zn‐doped g‐C3N4for H2evolution and BiVO4for O2evolution with Fe2+/Fe3+as a shuttle redox mediator.H2and O2were evalua...A two‐step photocatalytic water splitting system,termed a“Z‐scheme system”,was achieved using Zn‐doped g‐C3N4for H2evolution and BiVO4for O2evolution with Fe2+/Fe3+as a shuttle redox mediator.H2and O2were evaluated simultaneously when the doping amount of zinc was10%.Moreover,Zn‐doped(10%)g‐C3N4synthesized by an impregnation method showed superior active ability to form the Z‐scheme with BiVO4than by in‐situ synthesis.X‐ray diffraction,UV‐Vis spectroscopy,scanning electron microscopy,and X‐ray photoelectron spectroscopy were used to characterize the samples.It was determined that more Zn?N bonds could be formed on the surface of g‐C3N4by impregnation,which could facilitate charge transfer.展开更多
AIM To investigate the role of bloodtransfusion in TT viral infection(TTV).METHODS We retrospectively studied serumsamples from 192 transfusion recipients whounderwent cardiovascular surgery and bloodtransfusion betwe...AIM To investigate the role of bloodtransfusion in TT viral infection(TTV).METHODS We retrospectively studied serumsamples from 192 transfusion recipients whounderwent cardiovascular surgery and bloodtransfusion between July 1991 and June 1992.Allpatients had a follow-up every other week for atleast 6 months after transfusion.Eightyrecipients received blood before screeningdonors for hepatitis C antibody(anti-HCV),and112 recipients received screened blood.Recipients with alanine aminotransferase level】2.5 times the upper normal limit were testedfor serological markers for viral hepatitis A,B,C,G,Epstein-Barr virus and cytomegalovirus.TTV infection was defined by the positivity forserum TTV DNA using the polymerase chainreaction method.RESULTS Eleven and three patients,whoreceived anti-HCV unscreened and screened'blood,respectively,had serum ALT levels】90 IU/L.Five patients(HCV and TTV:1;HCV,HGV,and TTV:1;TTV:2;and CMV and TTV:1)were positive for TTV DNA,and four of them hadsero-conversion of TTV DNA.CONCLUSION TTV can be transmitted viablood transfusion.Two recipients infected byTTV alone may be associated with the hepatitis.However,whether TTV was the causal agentremains unsettled,and further studies arenecessary to define the role of TTV infection inchronic hepatitis.展开更多
The tracking, telemetry and command （TT＆C） mission is extremely reliable for its characters of small time horizon and high redundancy. The combined forcing and failure biasing （CFFB） method that is usually used f...The tracking, telemetry and command （TT＆C） mission is extremely reliable for its characters of small time horizon and high redundancy. The combined forcing and failure biasing （CFFB） method that is usually used for simulating the unreliability of the highly dependable mission system seems not so efficient for the TT＆C mission. The concept about the importance of failure transition is proposed based on the logical relationship between TT＆C mission and its involved resources. Then, the importance is used for readjusting the transition rate of the failure transition when using the forcing and failure biasing during the simulation. Examples show that the improved CFFB method can evidently increase the occurrence of the TT＆C mission failure event and decrease the sample variance. More redundancy of the TT＆C mission leads to the improved CFFB method more efficient.展开更多
Graphite‐like carbon nitride(g‐C3N4)‐based compounds have attracted considerable attention because of their excellent photocatalytic performance.In this work,a novel direct Z‐scheme system constructed from two‐di...Graphite‐like carbon nitride(g‐C3N4)‐based compounds have attracted considerable attention because of their excellent photocatalytic performance.In this work,a novel direct Z‐scheme system constructed from two‐dimensional(2D)g‐C3N4nanoplates and zero‐dimensional(0D)MoS2quantum dots(QDs)was prepared through the combination of a hydrothermal process and microemulsion preparation.The morphologies,structures,and optical properties of the as‐prepared photocatalysts were characterized by X‐ray diffraction,X‐ray photoelectron spectroscopy,atomic force microscopy,transmission electron microscopy,and UV‐vis diffuse reflectance spectroscopy.In addition,the photocatalytic performances of the prepared2D/0D hybrid composites were evaluated based on the photodegradation of rhodamine B under visible‐light irradiation.The results demonstrated that the introduction of MoS2QDs to g‐C3N4greatly enhanced the photocatalytic efficiency.For the optimum7%MoS2QD/g‐C3N4photocatalyst,the degradation rate constant was8.8times greater than that of pure g‐C3N4under visible‐light irradiation.Photocurrent and electrochemical impedance spectroscopy results further demonstrated that the MoS2QD/g‐C3N4composites exhibited higher photocurrent density and lower chargetransfer resistance than those of the pure g‐C3N4or MoS2QDs.Active species trapping,terephthalic acid photoluminescence,and nitro blue tetrazolium transformation experiments were performed to investigate the evolution of reactive oxygen species,including hydroxyl radicals and superoxide radicals.The possible enhanced photocatalytic mechanism was attributed to a direct Z‐scheme system,which not only can increase the separation efficiency of photogenerated electron‐hole pairs but also possesses excellent oxidation and reduction ability for high photocatalytic performances.This work provides an effective synthesis approach and insight to help develop other C3N4‐based direct Z‐scheme photocatalytic systems for environmental purification and energy conversion.展开更多
The whole airspace phased array telemetry,track and command(TT&C)system is regarded as the development tendency of next generation TT&C system,and the distribution of the antenna units and the beamforming tech...The whole airspace phased array telemetry,track and command(TT&C)system is regarded as the development tendency of next generation TT&C system,and the distribution of the antenna units and the beamforming technology have sparked wide interest in this field.A method for antenna distribution is proposed based on the linear subarrays technology.A symmetrical truncated cone conformal array is composed of the linear subarrays placed on the generatrix.The impact of truncated cone bottom radius and elevation angle on beamforming are studied and simulated.Simulation results verify the system design.展开更多
With the sharp increase of China＇s in-orbit spacecraft and the constraint TT＆C resources, a mathematical model for optimal TT＆C resource allocation is proposed, and the TT＆C facility remote monitoring function is ...With the sharp increase of China＇s in-orbit spacecraft and the constraint TT＆C resources, a mathematical model for optimal TT＆C resource allocation is proposed, and the TT＆C facility remote monitoring function is designed to achieve the multitask operation pattern under the unified management of the network management center. With this pattern, the TT＆C network management and the spacecraft management are separated, which is quite different from the previous pattern. Further, a novel spacecraft TT＆C technique based on spacecraft control language is developed, and the telecommanding pattern is designed to address the spacecraft operation problems. The engineering application shows that this pattern fundamentally improves the TT＆C network capability, increases the resource efficiency, and satisfies the efficient, accurate, and flexible operation of spacecraft.展开更多
For a mesoscopic L-C circuit,besides the Louisell's quantization scheme in which electric charge q andelectric current I are respectively quantized as the coordinate operator Q and momentum operator P,in this pape...For a mesoscopic L-C circuit,besides the Louisell's quantization scheme in which electric charge q andelectric current I are respectively quantized as the coordinate operator Q and momentum operator P,in this paperwe propose a new quantization scheme in the context of number-phase quantization through the standard Lagrangianformalism.The comparison between this number-phase quantization with the Josephson junction's Cooper pair number-phase-difference quantization scheme is made.展开更多
Currently, TT&C of spacecraft is performed by a ground system. Because more and more spacecrafts are launched into orbits, it is difficult for the ground system to meet the TT&C requirements of the spacecrafts...Currently, TT&C of spacecraft is performed by a ground system. Because more and more spacecrafts are launched into orbits, it is difficult for the ground system to meet the TT&C requirements of the spacecrafts. To explore a new, effective and economical TT&C mode is absolutely necessary. A method is proposed to use SGBM mode in TT&C spacecrafts in low earth orbits, here. Firstly, the principle of the mode is discussed; secondly, the system to simulate the mode is designed; thirdly, the relative issues to use the mode are indicated; fourthly, the experimental results (simulation) to apply the mode to TT&C spacecrafts are analyzed; and finally dawn is the main conclusion of the method.展开更多
基金supported by the National Natural Science Foundation of China (21773153)~~
文摘A two‐step photocatalytic water splitting system,termed a“Z‐scheme system”,was achieved using Zn‐doped g‐C3N4for H2evolution and BiVO4for O2evolution with Fe2+/Fe3+as a shuttle redox mediator.H2and O2were evaluated simultaneously when the doping amount of zinc was10%.Moreover,Zn‐doped(10%)g‐C3N4synthesized by an impregnation method showed superior active ability to form the Z‐scheme with BiVO4than by in‐situ synthesis.X‐ray diffraction,UV‐Vis spectroscopy,scanning electron microscopy,and X‐ray photoelectron spectroscopy were used to characterize the samples.It was determined that more Zn?N bonds could be formed on the surface of g‐C3N4by impregnation,which could facilitate charge transfer.
文摘AIM To investigate the role of bloodtransfusion in TT viral infection(TTV).METHODS We retrospectively studied serumsamples from 192 transfusion recipients whounderwent cardiovascular surgery and bloodtransfusion between July 1991 and June 1992.Allpatients had a follow-up every other week for atleast 6 months after transfusion.Eightyrecipients received blood before screeningdonors for hepatitis C antibody(anti-HCV),and112 recipients received screened blood.Recipients with alanine aminotransferase level】2.5 times the upper normal limit were testedfor serological markers for viral hepatitis A,B,C,G,Epstein-Barr virus and cytomegalovirus.TTV infection was defined by the positivity forserum TTV DNA using the polymerase chainreaction method.RESULTS Eleven and three patients,whoreceived anti-HCV unscreened and screened'blood,respectively,had serum ALT levels】90 IU/L.Five patients(HCV and TTV:1;HCV,HGV,and TTV:1;TTV:2;and CMV and TTV:1)were positive for TTV DNA,and four of them hadsero-conversion of TTV DNA.CONCLUSION TTV can be transmitted viablood transfusion.Two recipients infected byTTV alone may be associated with the hepatitis.However,whether TTV was the causal agentremains unsettled,and further studies arenecessary to define the role of TTV infection inchronic hepatitis.
基金supported by the National Natural Science Foundation of China (71071159)
文摘The tracking, telemetry and command （TT＆C） mission is extremely reliable for its characters of small time horizon and high redundancy. The combined forcing and failure biasing （CFFB） method that is usually used for simulating the unreliability of the highly dependable mission system seems not so efficient for the TT＆C mission. The concept about the importance of failure transition is proposed based on the logical relationship between TT＆C mission and its involved resources. Then, the importance is used for readjusting the transition rate of the failure transition when using the forcing and failure biasing during the simulation. Examples show that the improved CFFB method can evidently increase the occurrence of the TT＆C mission failure event and decrease the sample variance. More redundancy of the TT＆C mission leads to the improved CFFB method more efficient.
基金supported by National Natural Science Foundation of China(51672113)Six Talent Peaks Project in Jiangsu Province(2015-XCL-026)+3 种基金Natural Science Foundation of Jiangsu Province(BK20171299)State Key Laboratory of Photocatalysis on Energy and Environment(SKLPEE-KF201705),Fuzhou UniversityState Key Laboratory of Advanced Technology for Materials Synthesis and Processing(2016-KF-10),Wuhan University of Technologythe Qing Lan Project Foundation of Jiangsu Province~~
文摘Graphite‐like carbon nitride(g‐C3N4)‐based compounds have attracted considerable attention because of their excellent photocatalytic performance.In this work,a novel direct Z‐scheme system constructed from two‐dimensional(2D)g‐C3N4nanoplates and zero‐dimensional(0D)MoS2quantum dots(QDs)was prepared through the combination of a hydrothermal process and microemulsion preparation.The morphologies,structures,and optical properties of the as‐prepared photocatalysts were characterized by X‐ray diffraction,X‐ray photoelectron spectroscopy,atomic force microscopy,transmission electron microscopy,and UV‐vis diffuse reflectance spectroscopy.In addition,the photocatalytic performances of the prepared2D/0D hybrid composites were evaluated based on the photodegradation of rhodamine B under visible‐light irradiation.The results demonstrated that the introduction of MoS2QDs to g‐C3N4greatly enhanced the photocatalytic efficiency.For the optimum7%MoS2QD/g‐C3N4photocatalyst,the degradation rate constant was8.8times greater than that of pure g‐C3N4under visible‐light irradiation.Photocurrent and electrochemical impedance spectroscopy results further demonstrated that the MoS2QD/g‐C3N4composites exhibited higher photocurrent density and lower chargetransfer resistance than those of the pure g‐C3N4or MoS2QDs.Active species trapping,terephthalic acid photoluminescence,and nitro blue tetrazolium transformation experiments were performed to investigate the evolution of reactive oxygen species,including hydroxyl radicals and superoxide radicals.The possible enhanced photocatalytic mechanism was attributed to a direct Z‐scheme system,which not only can increase the separation efficiency of photogenerated electron‐hole pairs but also possesses excellent oxidation and reduction ability for high photocatalytic performances.This work provides an effective synthesis approach and insight to help develop other C3N4‐based direct Z‐scheme photocatalytic systems for environmental purification and energy conversion.
文摘The whole airspace phased array telemetry,track and command(TT&C)system is regarded as the development tendency of next generation TT&C system,and the distribution of the antenna units and the beamforming technology have sparked wide interest in this field.A method for antenna distribution is proposed based on the linear subarrays technology.A symmetrical truncated cone conformal array is composed of the linear subarrays placed on the generatrix.The impact of truncated cone bottom radius and elevation angle on beamforming are studied and simulated.Simulation results verify the system design.
基金supported by the China Postdotoral Science Foundation (20060401004).
文摘With the sharp increase of China＇s in-orbit spacecraft and the constraint TT＆C resources, a mathematical model for optimal TT＆C resource allocation is proposed, and the TT＆C facility remote monitoring function is designed to achieve the multitask operation pattern under the unified management of the network management center. With this pattern, the TT＆C network management and the spacecraft management are separated, which is quite different from the previous pattern. Further, a novel spacecraft TT＆C technique based on spacecraft control language is developed, and the telecommanding pattern is designed to address the spacecraft operation problems. The engineering application shows that this pattern fundamentally improves the TT＆C network capability, increases the resource efficiency, and satisfies the efficient, accurate, and flexible operation of spacecraft.
基金The project supported by the President Foundation of the Chinese Academy of Sciences
文摘For a mesoscopic L-C circuit,besides the Louisell's quantization scheme in which electric charge q andelectric current I are respectively quantized as the coordinate operator Q and momentum operator P,in this paperwe propose a new quantization scheme in the context of number-phase quantization through the standard Lagrangianformalism.The comparison between this number-phase quantization with the Josephson junction's Cooper pair number-phase-difference quantization scheme is made.
文摘Currently, TT&C of spacecraft is performed by a ground system. Because more and more spacecrafts are launched into orbits, it is difficult for the ground system to meet the TT&C requirements of the spacecrafts. To explore a new, effective and economical TT&C mode is absolutely necessary. A method is proposed to use SGBM mode in TT&C spacecrafts in low earth orbits, here. Firstly, the principle of the mode is discussed; secondly, the system to simulate the mode is designed; thirdly, the relative issues to use the mode are indicated; fourthly, the experimental results (simulation) to apply the mode to TT&C spacecrafts are analyzed; and finally dawn is the main conclusion of the method.
