To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shan...To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.展开更多
This study investigates the use of dynamic a priori error information according to atmospheric moistness and the use of quality controls in temperature and water vapor profile retrievals from hyperspectral infrared ...This study investigates the use of dynamic a priori error information according to atmospheric moistness and the use of quality controls in temperature and water vapor profile retrievals from hyperspectral infrared （IR） sounders. Temperature and water vapor profiles are retrieved from Atmospheric InfraRed Sounder （AIRS） radiance measurements by applying a physical iterative method using regression retrieval as the first guess. Based on the dependency of first-guess errors on the degree of atmospheric moistness, the a priori first-guess errors classified by total precipitable water （TPW） are applied in the AIRS physical retrieval procedure. Compared to the retrieval results from a fixed a priori error, boundary layer moisture retrievals appear to be improved via TPW classification of a priori first-guess errors. Six quality control （QC） tests, which check non-converged or bad retrievals, large residuals, high terrain and desert areas, and large temperature and moisture deviations from the first guess regression retrieval, are also applied in the AIRS physical retrievals. Significantly large errors are found for the retrievals rejected by these six QCs, and the retrieval errors are substantially reduced via QC over land, which suggest the usefulness and high impact of the QCs, especially over land. In conclusion, the use of dynamic a priori error information according to atmospheric moistness, and the use of appropriate QCs dealing with the geographical information and the deviation from the first-guess as well as the conventional inverse performance are suggested to improve temperature and moisture retrievals and their applications.展开更多
The hourly and daily air quality concentration in the total air pollutant emission amount control zone is not sure to be continuously up to national ambient air quality standard, even though the total annual air pollu...The hourly and daily air quality concentration in the total air pollutant emission amount control zone is not sure to be continuously up to national ambient air quality standard, even though the total annual air pollutant emission is permitted under the total air pollutant emission amount control (TAPEAC) on the basis of A-value method. So the concept of the environmental quality guarantee ratio (EQGR) for TAPEAC is advanced in this paper and its quantitative formula is figured out for both hourly and daily EQGR. It is concluded that the EQGR is related with the yearly arrangement of A-value besides the pollutant type. According to the meteorological data in a lower area along Yangtze River in 2000, the yearly A-value trend is analyzed. Based on the data, the hourly EQGR of SO 2 and NO 2 is respectively 97.4% and 90.2%, and daily EQGR respectively 90.2% and 79.5%.展开更多
APEC conference was held in Beijing during November 3- 12,2014. Hohhot City and Baotou City fall into the peripheral key air pollution control cities in the ＂ Beijing- Tianjin- Hebei＂ region. Inner Mongolia governme...APEC conference was held in Beijing during November 3- 12,2014. Hohhot City and Baotou City fall into the peripheral key air pollution control cities in the ＂ Beijing- Tianjin- Hebei＂ region. Inner Mongolia government adopted powerful pollution control measures in the period of the conference. According to pollutant concentration data and meteorological data etc. in the course of the event and the same period of last year,the atmospheric pollution variations and control effect were discussed in this study. The results showed that during October 1- 25,2014,there were 16 days with air pollution in Hohhot City and 15 days with air pollution in Baotou City,respectively increasing by 8% and 34% compared with the same period of 2013,and the concentration of particulate matter was also higher than that of last year. During October 22- 24,2014,Hohhot and Baotou cities were polluted persistently. The variation features of hourly concentration of main pollutants PM（10） and PM2. 5were similar to those in the same period of 2013. That is,the pollutant concentration reached the maximum from 21：00 to 23：00,and the minimum appeared from 15： 00 to 19： 00 in the next day. In the course of the event,the concentration of particulate matter in the two cities stared to reduce greatly on October 26. From October 26 to November 13,there were no days with air pollution in Hohhot City,decreasing by 100% compared with the same period of 2013; there were five days with air pollution in Baotou City,and the numbers of days with slight,moderate and severe pollution reduced by 37%,100% and67% respectively compared with the same period of last year. The persistent air pollution from October 22 to the first 10 days of November was related to unfavorable meteorological conditions,and the meteorological condition in the same period of 2014 was even worse. In the course of the event,the Inner Mongolia Government adopted air pollution control measures around October 25 and began to adopt some powerful pollution control measures on November 1. As a result,air pollution in key cities has been controlled effectively. This event showed that urban atmospheric pollution problem can be resolved,and we should take an optimistic attitude towards this matter.展开更多
For pollution research with regard to urban surface runoff, most sampling strategies to date have focused on differences in land usage. With single land-use sampling, total surface runoff pollution effect cannot be ev...For pollution research with regard to urban surface runoff, most sampling strategies to date have focused on differences in land usage. With single land-use sampling, total surface runoff pollution effect cannot be evaluated unless every land usage spot is monitored. Through a new sampling strategy known as mixed stormwater sampling for a street community at discharge outlet adjacent to river, this study assessed the total urban surface runoff pollution effect caused by a variety of land uses and the pollutants washed off from the rain pipe system in the Futian River watershed in Shenzhen City of China. The water quality monitoring indices were COD （chemical oxygen demand）, TSS （total suspend solid）, TP （total phosphorus）, TN （total nitrogen） and BOD （biochemical oxygen demand）. The sums of total pollution loads discharged into the river for the four indices of COD, TSS, TN, and TP over all seven rainfall events were very different. The mathematical model for simulating total pollution loads was established from discharge outlet mixed stormwater sampling of total pollution loads on the basis of four parameters： rainfall intensity, total land area, impervious land area, and pervious land area. In order to treat surface runoff pollution, the values of MFF30 （mass first flush ratio） and FF30 （first 30% of runoff volume） can be considered as split-flow control criteria to obtain more effective and economical design of structural BMPs （best management practices） facilities.展开更多
The total emission control method based on atmospheric environmental capacity is the most effective in air pollution mitigation. The atmospheric environmental capacities of SO2 on representative days over Lanzhou are ...The total emission control method based on atmospheric environmental capacity is the most effective in air pollution mitigation. The atmospheric environmental capacities of SO2 on representative days over Lanzhou are estimated using the numerical models RAMS, HYPACT and a linear programming model, according to the national ambient air quality standard of China （NAAQSCHN）. The results show that the fields of meteorological elements and SO2 simulated by the models agree reasonably well with observations. The atmospheric environmental capacity of SO2 over Lanzhou is around 111.7 × 10^3 kg d^-1, and in order to meet the air quality level Ⅱ of the NAAQSCHN, SO2 emissions need to be reduced by 20%.展开更多
A method of quantification of perfluorinated compounds(PFCs)from atmospheric particulate matter(APM)is described.A single step pretreatment method,selective pressurized liquid extraction(SPLE),was developed to reduce ...A method of quantification of perfluorinated compounds(PFCs)from atmospheric particulate matter(APM)is described.A single step pretreatment method,selective pressurized liquid extraction(SPLE),was developed to reduce the high matrix background and avoid contamination from commonly used multiple sample pretreatment steps.An effective sorbent was selected to purify the PFCs during SPLE,followed by liquid chromatography-tandem mass spectrometry(LC–MS/MS),for quantification of PFCs.Conditions affecting the SPLE efficiency,including temperature,static extraction time,and number of extraction cycles used,were studied.The optimum conditions were found to be 120℃,10 min,and 3 cycles,respectively.LC-MS/MS method was developed to obtain the optimal sensitivity specific to PFCs.The method detection limits(MDLs)were 0.006 to 0.48 ng/g for the PFCs studied and the linear response range was from 0.1 to 100 ng/g.To ensure accurate values were obtained,each step of the experiment was evaluated and controlled to prevent contamination.The optimized method was tested by performing spiking experiments in natural particulate matter matrices and good rates of recovery and reproducibility were obtained for all target compounds.Finally,the method was successfully used to measure 16 PFCs in the APM samples collected in Beijing over five years from 2015 to 2019.It is observed that some PFCs follow the trend of total PFC changes,and can be attributed to the environment influencing events and policy enforcement,while others don't seem to change as much with time of the year or from year to year.展开更多
文摘To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.
基金supported by GOES-R Algorithm Working Group Program and GOES-R High Impact Weather Project (Grant No NA10NES4400013)supported by the Korea Meteorological Administration Research and Development Program under Grant CATER 2006-2103the BK21 Project of the Korean Government
文摘This study investigates the use of dynamic a priori error information according to atmospheric moistness and the use of quality controls in temperature and water vapor profile retrievals from hyperspectral infrared （IR） sounders. Temperature and water vapor profiles are retrieved from Atmospheric InfraRed Sounder （AIRS） radiance measurements by applying a physical iterative method using regression retrieval as the first guess. Based on the dependency of first-guess errors on the degree of atmospheric moistness, the a priori first-guess errors classified by total precipitable water （TPW） are applied in the AIRS physical retrieval procedure. Compared to the retrieval results from a fixed a priori error, boundary layer moisture retrievals appear to be improved via TPW classification of a priori first-guess errors. Six quality control （QC） tests, which check non-converged or bad retrievals, large residuals, high terrain and desert areas, and large temperature and moisture deviations from the first guess regression retrieval, are also applied in the AIRS physical retrievals. Significantly large errors are found for the retrievals rejected by these six QCs, and the retrieval errors are substantially reduced via QC over land, which suggest the usefulness and high impact of the QCs, especially over land. In conclusion, the use of dynamic a priori error information according to atmospheric moistness, and the use of appropriate QCs dealing with the geographical information and the deviation from the first-guess as well as the conventional inverse performance are suggested to improve temperature and moisture retrievals and their applications.
文摘The hourly and daily air quality concentration in the total air pollutant emission amount control zone is not sure to be continuously up to national ambient air quality standard, even though the total annual air pollutant emission is permitted under the total air pollutant emission amount control (TAPEAC) on the basis of A-value method. So the concept of the environmental quality guarantee ratio (EQGR) for TAPEAC is advanced in this paper and its quantitative formula is figured out for both hourly and daily EQGR. It is concluded that the EQGR is related with the yearly arrangement of A-value besides the pollutant type. According to the meteorological data in a lower area along Yangtze River in 2000, the yearly A-value trend is analyzed. Based on the data, the hourly EQGR of SO 2 and NO 2 is respectively 97.4% and 90.2%, and daily EQGR respectively 90.2% and 79.5%.
基金Supported by the Small-scale Service Construction Program of China Meteorological Administration(Construction of Environmental Meteorological Early Warning Service System in Beijing-Tianjin-Hebei Region,Changjiang River Delta and Zhujiang River Dalta)Expert Forecaster Innovation Panel of Dust Storm and Haze in Inner MongoliaSci-tech Innovation Program of Inner Mongolia Meteorological Bureau(nmqxkjcx201411)
文摘APEC conference was held in Beijing during November 3- 12,2014. Hohhot City and Baotou City fall into the peripheral key air pollution control cities in the ＂ Beijing- Tianjin- Hebei＂ region. Inner Mongolia government adopted powerful pollution control measures in the period of the conference. According to pollutant concentration data and meteorological data etc. in the course of the event and the same period of last year,the atmospheric pollution variations and control effect were discussed in this study. The results showed that during October 1- 25,2014,there were 16 days with air pollution in Hohhot City and 15 days with air pollution in Baotou City,respectively increasing by 8% and 34% compared with the same period of 2013,and the concentration of particulate matter was also higher than that of last year. During October 22- 24,2014,Hohhot and Baotou cities were polluted persistently. The variation features of hourly concentration of main pollutants PM（10） and PM2. 5were similar to those in the same period of 2013. That is,the pollutant concentration reached the maximum from 21：00 to 23：00,and the minimum appeared from 15： 00 to 19： 00 in the next day. In the course of the event,the concentration of particulate matter in the two cities stared to reduce greatly on October 26. From October 26 to November 13,there were no days with air pollution in Hohhot City,decreasing by 100% compared with the same period of 2013; there were five days with air pollution in Baotou City,and the numbers of days with slight,moderate and severe pollution reduced by 37%,100% and67% respectively compared with the same period of last year. The persistent air pollution from October 22 to the first 10 days of November was related to unfavorable meteorological conditions,and the meteorological condition in the same period of 2014 was even worse. In the course of the event,the Inner Mongolia Government adopted air pollution control measures around October 25 and began to adopt some powerful pollution control measures on November 1. As a result,air pollution in key cities has been controlled effectively. This event showed that urban atmospheric pollution problem can be resolved,and we should take an optimistic attitude towards this matter.
基金supported by the Key Project of Chinese Ministry of Education(No.108177)the National Natural Science Foundation of China(No.50679049)
文摘For pollution research with regard to urban surface runoff, most sampling strategies to date have focused on differences in land usage. With single land-use sampling, total surface runoff pollution effect cannot be evaluated unless every land usage spot is monitored. Through a new sampling strategy known as mixed stormwater sampling for a street community at discharge outlet adjacent to river, this study assessed the total urban surface runoff pollution effect caused by a variety of land uses and the pollutants washed off from the rain pipe system in the Futian River watershed in Shenzhen City of China. The water quality monitoring indices were COD （chemical oxygen demand）, TSS （total suspend solid）, TP （total phosphorus）, TN （total nitrogen） and BOD （biochemical oxygen demand）. The sums of total pollution loads discharged into the river for the four indices of COD, TSS, TN, and TP over all seven rainfall events were very different. The mathematical model for simulating total pollution loads was established from discharge outlet mixed stormwater sampling of total pollution loads on the basis of four parameters： rainfall intensity, total land area, impervious land area, and pervious land area. In order to treat surface runoff pollution, the values of MFF30 （mass first flush ratio） and FF30 （first 30% of runoff volume） can be considered as split-flow control criteria to obtain more effective and economical design of structural BMPs （best management practices） facilities.
基金the National Natural Science Foundation of China （Grant No. 40305020）.
文摘The total emission control method based on atmospheric environmental capacity is the most effective in air pollution mitigation. The atmospheric environmental capacities of SO2 on representative days over Lanzhou are estimated using the numerical models RAMS, HYPACT and a linear programming model, according to the national ambient air quality standard of China （NAAQSCHN）. The results show that the fields of meteorological elements and SO2 simulated by the models agree reasonably well with observations. The atmospheric environmental capacity of SO2 over Lanzhou is around 111.7 × 10^3 kg d^-1, and in order to meet the air quality level Ⅱ of the NAAQSCHN, SO2 emissions need to be reduced by 20%.
基金supported by the NQI Project of National key R&D Program of China (No.2016YFF0201102)the project for the“Development of analytical method and certified reference materials for tracing air pollutant source” (No.21AKY1514)from the National Institute of Metrology,Beijing,China。
文摘A method of quantification of perfluorinated compounds(PFCs)from atmospheric particulate matter(APM)is described.A single step pretreatment method,selective pressurized liquid extraction(SPLE),was developed to reduce the high matrix background and avoid contamination from commonly used multiple sample pretreatment steps.An effective sorbent was selected to purify the PFCs during SPLE,followed by liquid chromatography-tandem mass spectrometry(LC–MS/MS),for quantification of PFCs.Conditions affecting the SPLE efficiency,including temperature,static extraction time,and number of extraction cycles used,were studied.The optimum conditions were found to be 120℃,10 min,and 3 cycles,respectively.LC-MS/MS method was developed to obtain the optimal sensitivity specific to PFCs.The method detection limits(MDLs)were 0.006 to 0.48 ng/g for the PFCs studied and the linear response range was from 0.1 to 100 ng/g.To ensure accurate values were obtained,each step of the experiment was evaluated and controlled to prevent contamination.The optimized method was tested by performing spiking experiments in natural particulate matter matrices and good rates of recovery and reproducibility were obtained for all target compounds.Finally,the method was successfully used to measure 16 PFCs in the APM samples collected in Beijing over five years from 2015 to 2019.It is observed that some PFCs follow the trend of total PFC changes,and can be attributed to the environment influencing events and policy enforcement,while others don't seem to change as much with time of the year or from year to year.
