It is generally believed that intelligent management for sewage treatment plants(STPs) is essential to the sustainable engineering of future smart cities.The core of management lies in the precise prediction of daily ...It is generally believed that intelligent management for sewage treatment plants(STPs) is essential to the sustainable engineering of future smart cities.The core of management lies in the precise prediction of daily volumes of sewage.The generation of sewage is the result of multiple factors from the whole social system.Characterized by strong process abstraction ability,data mining techniques have been viewed as promising prediction methods to realize intelligent STP management.However,existing data mining-based methods for this purpose just focus on a single factor such as an economical or meteorological factor and ignore their collaborative effects.To address this challenge,a deep learning-based intelligent management mechanism for STPs is proposed,to predict business volume.Specifically,the grey relation algorithm(GRA) and gated recursive unit network(GRU) are combined into a prediction model(GRAGRU).The GRA is utilized to select the factors that have a significant impact on the sewage business volume,and the GRU is set up to output the prediction results.We conducted a large number of experiments to verify the efficiency of the proposed GRA-GRU model.展开更多
Microplastics, plastic pieces of ≤5 mm in size, are ubiquitous in ther environment and can be found in both terrestrial and aquatic ecosystems. This manuscript reviews the literature on the fate of microplastics in w...Microplastics, plastic pieces of ≤5 mm in size, are ubiquitous in ther environment and can be found in both terrestrial and aquatic ecosystems. This manuscript reviews the literature on the fate of microplastics in wastewater treatment and briefly highlights novel developments in the removal of microplastics from aqueous systems.展开更多
Existing problems of sewage treatment plants in small towns were summarized firstly,and then the developing trend of construction of sewage treatment plants in small towns was discussed from the aspects of project dec...Existing problems of sewage treatment plants in small towns were summarized firstly,and then the developing trend of construction of sewage treatment plants in small towns was discussed from the aspects of project decision,site selection,design,processing technology and construction financing models. Finally,outlooks for its future development were proposed to provide reference for the construction of sewage treatment plants in small towns in future.展开更多
Concentrations of polychlorinated biphenyls (PCBs) have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high res...Concentrations of polychlorinated biphenyls (PCBs) have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high resolution gas chromatography/high resolution mass spectrometry method. The concentration of PCBs ranged from 65.6 to 157 ng/g dry weight (dw), with a mean value of 101 ng/g dw. The dioxin-like PCB WHO-TEQs (World Health Organization-Toxic Equivalents) of the sludge were lower than 1 pg /g dw. Consequently, all the concentrations of PCBs in sludge samples were below the upper limit for land application according to the Chinese legislation law for agriculture use. The PCB homologue profiles in sludge samples were dominated by tri-CBs and tetra- CBs. Similar distributions have been found in one of the Chinese PCB commercial products. The patterns of dioxin-like and indicator congeners observed in this study were quite similar in all samples. The predominant congener for dioxin-like and indicator PCBs were PCB-118 and PCB-28, respectively, while PCB-126 had the highest TEQ value.展开更多
Microplastic pollution has become a worldwide issue.The discharge of sewage treatment plants(STPs)or wastewater treatment plant(WWTPs)is an important way for microplastics to enter the environment.This study reviewed ...Microplastic pollution has become a worldwide issue.The discharge of sewage treatment plants(STPs)or wastewater treatment plant(WWTPs)is an important way for microplastics to enter the environment.This study reviewed the sources and occurrence characteristics(type,size,color and components)of microplastics in domestic and foreign sewage plants.It elaborated the removal principles of microplastics by primary,secondary and tertiary treatments.In addition,the removal effects of various treatment units and different processes on microplastics were summarized.In the future,the removal mechanism of microplastics in sewage treatment plants should be discussed in more depth,so as to further improve the removal rate of microplastics by optimizing and transforming traditional sewage treatment processes.Therefore,it is necessary to develop new technologies/processes specifically for the removal of microplastics and promote them to practical applications.展开更多
Iraq is one of the countries that is suffering from water shortage problems and, for this reason, wastewater treatment plants become a necessity to minimize this problem. In this study, the impact of A1-Hilla WWTP (w...Iraq is one of the countries that is suffering from water shortage problems and, for this reason, wastewater treatment plants become a necessity to minimize this problem. In this study, the impact of A1-Hilla WWTP (wastewater treatment plant) on the environment has been studied. This was achieved using SimaPro software package. This software is a powerful tool for analyzing the environmental impact on products during their whole life cycle. A huge amount of knowledge about the environment is built into the program and database, enabling to analyze a product with a minimum of specialized knowledge. The results of LCA (life cycle assessment) showed that the impact and damage on the environment by A1-Hilla WWTP was 41 bad points for each 1 m3 of treated wastewater. The most environmental impacts potentially were global warming, respiratory inorganics and non-renewable energy. The study also showed that most of the effects were the result of the use of cement, steel and electricity consumption.展开更多
Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution ...Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution and technology-specific emission inventory is still lacking to support mitigation strategies of MWWTPs.Here we develop a plant-level and technology-based MWWTP emission inventory for China covering 8703 plants and 19 treatment technology categories by compiling and harmonizing the most up-to-date facility-level databases.China's methane(CH_(4))and nitrous oxide(N_(2)O)emissions from MWWTPs in 2020 are estimated to be 150.6 Gg and 22.0 Gg,respectively,with the uncertainty range of-30%to 37%and-30%to 26%at 95%confidence interval.We find an emission inequality across cities,with the richest cities emitting two times more CH_(4)and N_(2)O per capita from municipal wastewater treatment than the poorest cities.The emitted CH_(4)and N_(2)O are dominated by Anaerobic/Anoxic/Oxic-,Sequencing Batch Reactor-,Oxidation Ditch-,and Anoxic/Oxic-based MWWTPs of less than 20 years old.Considering the relatively young age structure of China's MWWTPs,the committed emissions highlight the importance of reducing on-site GHG emissions by optimization of operating conditions and innovation management.The emission differences among our estimates,previous studies,and the Intergovernmental Panel on Climate Change guidelines are largely attributed to the uncertainties in emission factors,implying the urgent need for more plant-integrated measurements to improve the accuracy of emission accounting.展开更多
Effective monitoring and management of microbial risk factors in wastewater treatment plants(WWTPs)effluents require a comprehensive investigation of these risks.A global survey on microbial risk factors in WWTP efflu...Effective monitoring and management of microbial risk factors in wastewater treatment plants(WWTPs)effluents require a comprehensive investigation of these risks.A global survey on microbial risk factors in WWTP effluents could reveal important insights into their risk features.This study aims to explore the abundance and types of antibiotic resistance genes(ARGs),virulence factor genes(VFGs),the vector of ARG/VFG,and dominant pathogens in global WWTP effluents.We collected 113 metagenomes of WWTP effluents from the Sequence Read Archive of the National Center for Biotechnology Information and characterized the microbial risk factors.Our results showed that multidrug resistance was the dominant ARG type,while offensive virulence factors were the most abundant type of VFGs.The most dominant types of ARGs in the vector of plasmid and phage were both aminoglycoside resistance,which is concerning as aminoglycosides are often a last resort for treating multi-resistant infections.Acinetobacter baumannii was the most dominant pathogen,rather than Escherichia coli,and a weak negative correlation between Escherichia coli and two other dominant pathogens(Acinetobacter baumannii and Bacteroides uniformis)suggests that using Escherichia coli as a biological indicator for all pathogens in WWTP effluents may not be appropriate.The Getah virus was the most dominant virus found in global WWTP effluents.Our study presents a comprehensive global-scale investigation of microbial risk factors in WWTP effluents,providing valuable insights into the potential risks associated with WWTP effluents and contributing to the monitoring and control of these risks.展开更多
Dissolved organic matter(DOM)from each treatment process of wastewater treatment plants(WWTPs)contains abundant photosensitive substances,which could significantly affect the photodegradation of 17α-ethinylestradiol(...Dissolved organic matter(DOM)from each treatment process of wastewater treatment plants(WWTPs)contains abundant photosensitive substances,which could significantly affect the photodegradation of 17α-ethinylestradiol(EE2).Nevertheless,information about EE2 photodegradation behavior mediated by DOM from diverse WWTPs and the photosensitivity sources of such DOM are inadequate.This study explored the photodegradation behavior of EE2 mediated by four typical WWTPs’DOM solutions and investigated the photosensitivity sources of DOM in the anaerobic-anoxic-oxic(A2/O)process.The parallel factor analysis identified three varying fluorescing components of these DOM,tryptophan-like substances or protein-like substances,microbial humuslike substances,and humic-like components.The photodegradation rate constants of EE2 were positively associated with the humification degree of DOM(P<0.05).The triplet state substances were responsible for the degradation of EE2.DOM extracted from the A2/O process,especially in the secondary treatment process had the fastest EE2 photodegradation rate compared to that of the other three processes.Four types of components(water-soluble organic matter(WSOM),extracellular polymeric substance,humic acid,and fulvic acid)were separated from the A2/O process DOM.WSOM had the highest promotion effect on EE2 photodegradation.Fulvic acid-like components and humic acid-like organic compounds in WSOM were speculated to be important photosensitivity substances that can generate triplet state substances.This research explored the physicochemical properties and photosensitive sources of DOM in WWTPs,and explained the fate of estrogens photodegradation in natural waters.展开更多
Wastewater treatment plants(WWTPs)are important and energy-intensive municipal infrastructures.High energy consumption and relatively low operating performance are major challenges from the perspective of carbon neutr...Wastewater treatment plants(WWTPs)are important and energy-intensive municipal infrastructures.High energy consumption and relatively low operating performance are major challenges from the perspective of carbon neutrality.However,water-energy nexus analysis and models for WWTPs have rarely been reported to date.In this study,a cloud-model-based energy consumption analysis(CMECA)of a WWTP was conducted to explore the relationship between influent and energy consumption by clustering its influent’s parameters.The principal component analysis(PCA)and K-means clustering were applied to classify the influent condition using water quality and volume data.The energy consumption of the WWTP is divided into five standard evaluation levels,and its cloud digital characteristics(CDCs)were extracted according to bilateral constraints and golden ratio methods.Our results showed that the energy consumption distribution gradually dispersed and deviated from the Gaussian distribution with decreased water concentration and quantity.The days with high energy efficiency were extracted via the clustering method from the influent category of excessive energy consumption,represented by a compact-type energy consumption distribution curve to identify the influent conditions that affect the steady distribution of energy consumption.The local WWTP has high energy consumption with 0.3613 kW·h·m^(-3)despite low influent concentration and volumes,across four consumption levels from low(I)to relatively high(IV),showing an unsatisfactory operation and management level.The average oxygenation capacity,internal reflux ratio,and external reflux ratio during high energy efficiency days recognized by further clustering were obtained(0.2924-0.3703 kg O_(2)·m^(-3),1.9576-2.4787,and 0.6603-0.8361,respectively),which could be used as a guide for the days with low energy efficiency.Consequently,this study offers a water-energy nexus analysis method to identify influent conditions with operational management anomalies and can be used as an empirical reference for the optimized operation of WWTPs.展开更多
Plastic particles smaller than 5 mm are microplastics.They are among the significant pollutants that recently attracted attention.Great quantities of microplastics enter the sewage system daily and reach wastewater tr...Plastic particles smaller than 5 mm are microplastics.They are among the significant pollutants that recently attracted attention.Great quantities of microplastics enter the sewage system daily and reach wastewater treatment plants(WWTPs).As a result,WWTPs are potential microplastic sources.Hence,they create a pathway for microplastics to reach aquatic environments with treated wastewater discharge.Studies on microplastic characterization in WWTPs have gained momentum in academia.This study investigates the abundance,size,shape,color,polymer type,and removal efficiencies of microplastics in a municipal wastewater treatment plant(WWTP)in Denizli/Turkey.The results showed that the dominant microplastic shape in wastewater samples was fibers(41.78%–60.77%)in the 100–500μm(58.57%–80.07%)size range.Most of the microplastics were transparent-white(32.86%–58.93%).The dominant polymer types were polyethylene(54.05%)and polyethylene vinyl acetate(37.84%)in raw wastewater.Furthermore,the microplastic removal efficiencies of the Denizli Central WWTP as a whole and for individual treatment units were evaluated.Although the microplastic pollution removal efficiency of the Denizli Central WWTP was over 95%,the microplastic concentration discharged daily into the receiving environment was considerably high(1.28×1010 MP/d).Thus,Denizli Central WWTP effluents result in a high volume of emissions in terms of microplastic pollution with a significant daily discharge to theÇürüksu Stream.展开更多
Wastewater treatment plants(WWTPs)consume large amounts of energy and emit greenhouse gases to remove pollutants.This study proposes a framework for evaluating the energy neutrality potential(ENP)of WWTPs from an inte...Wastewater treatment plants(WWTPs)consume large amounts of energy and emit greenhouse gases to remove pollutants.This study proposes a framework for evaluating the energy neutrality potential(ENP)of WWTPs from an integrated perspective.Operational data of 970 WWTPs in the Yangtze River Economic Belt(YREB)were extracted from the China Urban Drainage Yearbook 2018.The potential chemical and thermal energies were estimated using combined heat and power(CHP)and water source heat pump,respectively.Two key performance indicators(KPIs)were then established:the energy self-sufficiency(ESS)indicator,which reflects the offset degree of energy recovery,and the comprehensive water–energy efficiency(CWEE)indicator,which characterizes the efficiency of water–energy conversion.For the qualitative results,98 WWTPs became the benchmark(i.e.,CWEE=1.000),while 112 WWTPs were fully self-sufficient(i.e.,ESS≥100%).Subsequently,four types of ENP were classified by setting the median values of the two KPIs as the critical value.The WWTPs with high ENP had high net thermal energy values and relatively loose discharge limits.The explanatory factor analysis of water quantity and quality verified the existence of scale economies.Sufficient carbon source and biodegradability condition were also significant factors.As the CWEE indicator was mostly sensitive to the input of CHP,future optimization shall focus on the moisture and organic content of sludge.This study proposes a novel framework for evaluating the ENP of WWTPs.The results can provide guidance for optimizing the energy efficiency and recovery of WWTPs.展开更多
Small RNAs(sRNAs)are key players in the regulation of bacterial gene expression.However,the distribution and regulatory functions of sRNA in pig farm wastewater treatment plants(WWTPs)remains unknown.In this study,the...Small RNAs(sRNAs)are key players in the regulation of bacterial gene expression.However,the distribution and regulatory functions of sRNA in pig farm wastewater treatment plants(WWTPs)remains unknown.In this study,the wastewaters in anoxic and oxic tanks of the WWTPs were collected.The profiles of the community structure,mRNA expression,and sRNA expression of bacteria in pig farm wastewater were investigated using transcriptome sequencing and qPCR.This study demonstrated that there was a higher abundance of sRNA in the pig farm WWTPs and 52 sRNAs were detected.The sRNAs were mainly present in Proteobacteria and Firmicutes,including the potential human pathogenic bacteria(HPB)(Escherichia,Shigella,Bordetella and Morganella),crop pathogen(Pectobacterium)and denitrifying bacteria(Zobellella).And the sRNAs were involved in the bacterial functional activities such as translation,transcription,drug resistance,membrane transport and amino acid metabolism.In addition,most sRNAs had a higher abundance in anoxic tanks which contained a higher abundance of the genes associated with infectious diseases and drug resistance than that in oxic tanks.The results presented here show that in pig farm WWTPs,sRNA played an important role in bacterial function activities,especially the infectious diseases,drug resistance and denitrification,which can provide a new point of penetration for improving the pig farm WWTPs.展开更多
To assess the potential endocrine disruptive effects through multiple nuclear receptors (NRs), especially non-steroidal NRs, in municipal wastewater, we examined the agonistic activities on four NRs (estrogen recep...To assess the potential endocrine disruptive effects through multiple nuclear receptors (NRs), especially non-steroidal NRs, in municipal wastewater, we examined the agonistic activities on four NRs (estrogen receptor α, thyroid hormone receptor α, retinoic acid receptor ct and retinoid X receptor α) of untreated and treated wastewater from municipal wastewater treatment plants (WWTPs) in Japan using a yeast two-hybrid assay. Investigation of the influent and effluent of seven WWTPs revealed that agonistic activities against steroidal and non-steroidal NRs were always detected in the influents and partially remained in the effluents. Further investigation of four WWTPs employing conventional activated sludge, pseudo-anoxic-oxic, anoxic-oxic and anaerobic-anoxic-oxic processes revealed that the ability to reduce the agonistic activity against each of the four NRs varies depending on the treatment process. These results indicated that municipal wastewater in Japan commonly contains endocrine disrupting chemicals that exert agonistic activities on steroidal and non-steroidal NRs, and that some of these chemicals are released into the natural aquatic environment. Although the results obtained in yeast assays suggested that measured levels of non-steroidal NR agonists in the effluent of WWTPs were not likely to cause any biological effect, further study is required to assess their possible risks in detail.展开更多
The concentration and distribution of nonylphe-nol polyethoxylates(NPEOs represents the mixture,and NPnEO represents the monomer)and its metabolites in the influent and effluent of four municipal sewage treatment plan...The concentration and distribution of nonylphe-nol polyethoxylates(NPEOs represents the mixture,and NPnEO represents the monomer)and its metabolites in the influent and effluent of four municipal sewage treatment plants(STPs)in the north of China were measured.Moreover,the concentration and distribution of the above chemicals in the sludge of two STPs were also determined,and the transfer and fate of NPEOs in the sewage treatment process were discussed primarily by analyzing the distribu-tion of the products in the effluent and the sludge.The results showed that NPEOs and its metabolites existed in all the samples of the influent,effluent,and sludge.NPEOs were degraded in the sewage treatment process with the removal efficiency in the range of 23.38%-77.11%,or an average of 52.86%.However,the large analogs of NPnEO were only degraded to small ones,whose degradation rate was rather slow,and consequently the degradation was not complete.Hence,the concentrations of some small metabolites,such as nonylphenol(NP),nonylphenol monoethoxylate(NP1EO),and nonylphenol diethoxylate(NP2EO)were elevated in the effluent.These small metabolites are more toxic than the large NPnEO analogs,and some of them were reported to exhibit environmental endocrine disrupting activity.From this point of view,the process of sewage treatment does not reduce but elevate the risk of NPEOs,which becomes the main source of these small NPnEO in the environment.The sludge exhibited good adsorption ability for NPEOs,especially for the small analogs,which led to the high level of NPEOs in the sludge.Hence,reasonable disposal of the surplus sludge to avoid re-pollution is very important.展开更多
Most of the monitoring data on the occurrence of antibiotics in sewage treatment plants(STPs)have been reported from Europe,North America and some countries in Northeast Asia,while very limited data can be found in So...Most of the monitoring data on the occurrence of antibiotics in sewage treatment plants(STPs)have been reported from Europe,North America and some countries in Northeast Asia,while very limited data can be found in Southeast Asian countries.As a pioneering research in Sri Lanka,we collected 24 h composite wastewater samples at the influent and effluent of two municipal STPs for consecutive 7 days to investigate occurrence,consumption and removal efficiency of seventeen antibiotics.The STP was located in Colombo and Hikkaduwa,respectively,representing two kinds of communities(i.e.local and tourists)in Sri Lanka.The targeted antibiotics were extracted by solid-phase extraction method and detected on an Agilent HPLCMSMS(1290/6470QQQ).Results illustrated that the majority of the antibiotics can be always detected from both STPs,except for chlorotetracycine(CTC),doxycycline(DOX)and florfenicol(FF).Fluoroquinolones(FQs)were detected at highest concentrations with ciprofloxacin(CIP)being the dominant compound.Concentrations of CIP in the influent samples were in the range of 433 e6010 ng/L.The consumption of antibiotics was estimated on the basis of influent mass load and catchment population data.We found difference in consumption patterns between the two served areas.Compared to local people in Colombo,tourists in Hikkaduwa appeared to take more antibiotics during the study period with the estimated daily dose of 0.25 g per 1000 persons.Moreover,macrolides accounted for a larger portion than FQs in Hikkaduwa,with azithromycin(AZM)being the most prevalent antibacterial agent.After comparison with an official report by Medical Supplies Division of Sri Lanka,we conjected that AZM was not commonly used among local people and it was mainly introduced by foreign arrivals.As for the removal efficiency,the activated sludge system of Colombo exhibited better elimination and more stable performance than the constructed wetland process of Hikkaduwa.展开更多
Municipal wastewater consists of a downstream collection of flushed sewage(without solid waste),other household runoffs,industrial runoffs,hospital runoffs and agricultural runoffs through an underground pipe before t...Municipal wastewater consists of a downstream collection of flushed sewage(without solid waste),other household runoffs,industrial runoffs,hospital runoffs and agricultural runoffs through an underground pipe before treatment.A runoff collection system called the wastewater treatment plant(WWTPs)treats such wastewater before release into environment following specific regulatory standards.This years-long practice has been improved upon by adding end-to-end pipe technologies with a view to enhancing the quality of effluent released.However,effluents released into the environment from design/application of WWTPs appear to contain emerging contaminants of both biotic and abiotic nature.The observation of chemical contaminants,antibiotic resistant bacteria(ARB),antibiotic resistant genes(ARGs)and diverse pathogenic bacteria genera in wastewater works release further affirm the abundance of such emerging contaminants.As a result,the government and water regulatory organizations in various part of the world are considering the removal of water reuse act from recycling policy/process.Current global debate is focused on questions about sustenance of any improved additional treatment level;effect of energy consumption by added treatment stage and its impact on the environmental wellness as contaminants borne wastewater is consistently released.Technological advancement/research suggests implementation of newer innovative infrastructural systems(NIIS)such as Mobbing Bed Biofilm Rector(MBBR),for wastewater effluent management which involve addition of newer wastewater treatment stages.This review addressed current pitfalls including wastewater microbiota of high epidemiological/public health relevance and affirms the need for such improvement which requires modification of ongoing institutional framework with a view to encourage implementation of NIIS for an improved effluent release.Exploiting the advances of microbial biofilming and the potentials of microbial biofueling as discussed in various section promises a future of robust environmental system,stable operational standard,release of quality effluent and sustainable management of wastewater works.Application of the aforementioned would enhance qualityWWTPs release and in-defacto reduces spread of ARB/ARGs as well as impacts both the environment wellness and public health.展开更多
To improve nitrogen removal performance of wastewater treatment plants (WWTPs), it is essential to understand the behavior of nitrogen cycling communities, which comprise various microorganisms. This study character...To improve nitrogen removal performance of wastewater treatment plants (WWTPs), it is essential to understand the behavior of nitrogen cycling communities, which comprise various microorganisms. This study characterized the quantity and diversity of nitrogen cycling genes in various processes of municipal WWTPs by employing two molecular-based methods:most probable number-polymerase chain reaction (MPN-PCR) and DNA microarray. MPN-PCR analysis revealed that gene quantities were not statistically different among processes, suggesting that conventional actwated sludge processes (CAS) are similar to nitrogen removal processes in their ability to retain an adequate population of nitrogen cycling microorganisms. Furthermore, most processes in the WWTPs that were researched shared a pattern:the nitS and the bacterial amoA genes were more abundant than the nirK and archaeal amoA genes, respectivelv. DNA microarray analysis revealed that several kinds of nitrification and denitrification genes were detected in both CAS and anaerobic-oxic processes (AO), whereas limited genes were detected in nitrogen removal processes. Results of this study suggest that CAS maintains a diverse community of nitrogen cycling microorganisms; moreover, the microbial communities in nitrogen removal processes may be specific.展开更多
N-nitrosodimethylamine (NDMA) and several other N-nitrosamines have been detected as disinfection by-products in drinking waters in many countries around the world. An ultra-performance liquid chromatography- tandem...N-nitrosodimethylamine (NDMA) and several other N-nitrosamines have been detected as disinfection by-products in drinking waters in many countries around the world. An ultra-performance liquid chromatography- tandem mass spectrometry method with solid phase extraction sample preparation was developed to study the occurrence of N-nitrosamines in several water treatment plants and distribution systems in China. Isotope labeled N-nitrosodi-n-propylamine-dl4 (NDPA-dl4) was selected as the internal standard for quantification. The solid phase extraction procedures including pH, enrichment process and MS/MS parameters including capillary voltage, cone gas flow, cone voltage, collision energy were optimized to give average recoveries of 26% to 112% for nine N- nitrosamine species. The instrument detection limits were estimated to range from 0.5 to 5μg.L-1 for the nine N- nitrosamine species. NDMA and several other N-nitrosa- mines were found at fairly high concentrations in several water treatment plants and distribution systems. NDMA was found in all locations, and the highest concentrations in cities B, G, T, and W were 3.0, 35.7, 21.3, and 19.7 ng. L 1, respectively. A wide range of N-nitrosamines concentrations and species were observed in different locations. Higher concentrations of N-nitrosamines were detected in distribution systems that were further away from the treatment plants, suggesting that the contact time between the residual disinfectant and natural organic matter may play an important role in the formation of these compounds.展开更多
The water quality and energy consumption of wastewater treatment plants(WWTPs)in Taihu Basin were evaluated on the basis of the operation data from 204 municipal WWTPs in the basin by using various statistical methods...The water quality and energy consumption of wastewater treatment plants(WWTPs)in Taihu Basin were evaluated on the basis of the operation data from 204 municipal WWTPs in the basin by using various statistical methods.The influent ammonia nitrogen(NH3-N)and total nitrogen(TN)of WWTPs in Taihu Basin showed normal distribution,whereas chemical oxygen demand(COD),biochemical oxygen demand(BOD5),suspended solid(SS),and total phosphorus(TP)showed positively skewed distribution.The influent BOD5/COD was 0.4%-0.6%,only 39.2%SS/BOD5 exceeded the standard by 36.3%,the average BOD5/TN was 3.82,and the probability of influent BOD5/TP>20 was 82.8%.The average energy consumption of WWTPs in Taihu Basin in 2017 was 0.458 kWh/m^3.The specific energy consumption of WWTPs with a daily treatment capacity of more than 5×10^4 m^3 in Taihu Basin was stable at 0.33 kWh/m^3.A power function relationship was observed between the reduction in COD and NH3-N and the specific energy consumption of pollutant reduction,and the higher the pollutant reduction is,the lower the specific energy consumption of pollutant reduction presents.In addition,a linear relationship existed between the energy consumption of WWTPs and the specific energy consumption of influent volume and pollutant reduction.Therefore,upgrading and operation with less energy consumption of WWTPs is imperative and the suggestions for Taihu WWTPs based on stringent discharge standard are proposed in detail.展开更多
基金Project(KJZD-M202000801) supported by the Major Project of Chongqing Municipal Education Commission,ChinaProject(2016YFE0205600) supported by the National Key Research&Development Program of China+1 种基金Project(CXQT19023) supported by the Chongqing University Innovation Group Project,ChinaProjects(KFJJ2018069,1853061,1856033) supported by the Key Platform Opening Project of Chongqing Technology and Business University,China。
文摘It is generally believed that intelligent management for sewage treatment plants(STPs) is essential to the sustainable engineering of future smart cities.The core of management lies in the precise prediction of daily volumes of sewage.The generation of sewage is the result of multiple factors from the whole social system.Characterized by strong process abstraction ability,data mining techniques have been viewed as promising prediction methods to realize intelligent STP management.However,existing data mining-based methods for this purpose just focus on a single factor such as an economical or meteorological factor and ignore their collaborative effects.To address this challenge,a deep learning-based intelligent management mechanism for STPs is proposed,to predict business volume.Specifically,the grey relation algorithm(GRA) and gated recursive unit network(GRU) are combined into a prediction model(GRAGRU).The GRA is utilized to select the factors that have a significant impact on the sewage business volume,and the GRU is set up to output the prediction results.We conducted a large number of experiments to verify the efficiency of the proposed GRA-GRU model.
文摘Microplastics, plastic pieces of ≤5 mm in size, are ubiquitous in ther environment and can be found in both terrestrial and aquatic ecosystems. This manuscript reviews the literature on the fate of microplastics in wastewater treatment and briefly highlights novel developments in the removal of microplastics from aqueous systems.
文摘Existing problems of sewage treatment plants in small towns were summarized firstly,and then the developing trend of construction of sewage treatment plants in small towns was discussed from the aspects of project decision,site selection,design,processing technology and construction financing models. Finally,outlooks for its future development were proposed to provide reference for the construction of sewage treatment plants in small towns in future.
基金supported by the Key Project of Chinese Academy of Sciences (No. KZCX2-YW-420)the National Basic Research Program (973) of China (No.2009CB421606)the National Natural Science Foundation of China (No. 20621703)
文摘Concentrations of polychlorinated biphenyls (PCBs) have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high resolution gas chromatography/high resolution mass spectrometry method. The concentration of PCBs ranged from 65.6 to 157 ng/g dry weight (dw), with a mean value of 101 ng/g dw. The dioxin-like PCB WHO-TEQs (World Health Organization-Toxic Equivalents) of the sludge were lower than 1 pg /g dw. Consequently, all the concentrations of PCBs in sludge samples were below the upper limit for land application according to the Chinese legislation law for agriculture use. The PCB homologue profiles in sludge samples were dominated by tri-CBs and tetra- CBs. Similar distributions have been found in one of the Chinese PCB commercial products. The patterns of dioxin-like and indicator congeners observed in this study were quite similar in all samples. The predominant congener for dioxin-like and indicator PCBs were PCB-118 and PCB-28, respectively, while PCB-126 had the highest TEQ value.
基金Supported by Project of National Natural Science Foundation of China(42007317)Project of Guangdong Basic and Applied Basic Research Foundation(2019A1515110272)+1 种基金Outstanding Young Teachers'Scientific Research Ability Improvement Program Funding Project of Zhaoqing University(YQ202105)Innovation and Entrepreneurship Training Program for College Students(202210580015).
文摘Microplastic pollution has become a worldwide issue.The discharge of sewage treatment plants(STPs)or wastewater treatment plant(WWTPs)is an important way for microplastics to enter the environment.This study reviewed the sources and occurrence characteristics(type,size,color and components)of microplastics in domestic and foreign sewage plants.It elaborated the removal principles of microplastics by primary,secondary and tertiary treatments.In addition,the removal effects of various treatment units and different processes on microplastics were summarized.In the future,the removal mechanism of microplastics in sewage treatment plants should be discussed in more depth,so as to further improve the removal rate of microplastics by optimizing and transforming traditional sewage treatment processes.Therefore,it is necessary to develop new technologies/processes specifically for the removal of microplastics and promote them to practical applications.
文摘Iraq is one of the countries that is suffering from water shortage problems and, for this reason, wastewater treatment plants become a necessity to minimize this problem. In this study, the impact of A1-Hilla WWTP (wastewater treatment plant) on the environment has been studied. This was achieved using SimaPro software package. This software is a powerful tool for analyzing the environmental impact on products during their whole life cycle. A huge amount of knowledge about the environment is built into the program and database, enabling to analyze a product with a minimum of specialized knowledge. The results of LCA (life cycle assessment) showed that the impact and damage on the environment by A1-Hilla WWTP was 41 bad points for each 1 m3 of treated wastewater. The most environmental impacts potentially were global warming, respiratory inorganics and non-renewable energy. The study also showed that most of the effects were the result of the use of cement, steel and electricity consumption.
基金supported by the Shenzhen Science and Technology Innovation Commission(No.RCBS20210609103731062,No.WDZC20220810110301001)Guangdong Basic and Applied Basic Research Foundation(No.2021A1515110887)H.L.acknowledge additional support from the Shenzhen Overseas High-Level Talent Project.
文摘Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution and technology-specific emission inventory is still lacking to support mitigation strategies of MWWTPs.Here we develop a plant-level and technology-based MWWTP emission inventory for China covering 8703 plants and 19 treatment technology categories by compiling and harmonizing the most up-to-date facility-level databases.China's methane(CH_(4))and nitrous oxide(N_(2)O)emissions from MWWTPs in 2020 are estimated to be 150.6 Gg and 22.0 Gg,respectively,with the uncertainty range of-30%to 37%and-30%to 26%at 95%confidence interval.We find an emission inequality across cities,with the richest cities emitting two times more CH_(4)and N_(2)O per capita from municipal wastewater treatment than the poorest cities.The emitted CH_(4)and N_(2)O are dominated by Anaerobic/Anoxic/Oxic-,Sequencing Batch Reactor-,Oxidation Ditch-,and Anoxic/Oxic-based MWWTPs of less than 20 years old.Considering the relatively young age structure of China's MWWTPs,the committed emissions highlight the importance of reducing on-site GHG emissions by optimization of operating conditions and innovation management.The emission differences among our estimates,previous studies,and the Intergovernmental Panel on Climate Change guidelines are largely attributed to the uncertainties in emission factors,implying the urgent need for more plant-integrated measurements to improve the accuracy of emission accounting.
基金supported by the National Natural Science Foundation of China(Nos.52170156,52250056,and 52293442)the Shenzhen Science and Technology Program(No.KQTD20190929172630447)。
文摘Effective monitoring and management of microbial risk factors in wastewater treatment plants(WWTPs)effluents require a comprehensive investigation of these risks.A global survey on microbial risk factors in WWTP effluents could reveal important insights into their risk features.This study aims to explore the abundance and types of antibiotic resistance genes(ARGs),virulence factor genes(VFGs),the vector of ARG/VFG,and dominant pathogens in global WWTP effluents.We collected 113 metagenomes of WWTP effluents from the Sequence Read Archive of the National Center for Biotechnology Information and characterized the microbial risk factors.Our results showed that multidrug resistance was the dominant ARG type,while offensive virulence factors were the most abundant type of VFGs.The most dominant types of ARGs in the vector of plasmid and phage were both aminoglycoside resistance,which is concerning as aminoglycosides are often a last resort for treating multi-resistant infections.Acinetobacter baumannii was the most dominant pathogen,rather than Escherichia coli,and a weak negative correlation between Escherichia coli and two other dominant pathogens(Acinetobacter baumannii and Bacteroides uniformis)suggests that using Escherichia coli as a biological indicator for all pathogens in WWTP effluents may not be appropriate.The Getah virus was the most dominant virus found in global WWTP effluents.Our study presents a comprehensive global-scale investigation of microbial risk factors in WWTP effluents,providing valuable insights into the potential risks associated with WWTP effluents and contributing to the monitoring and control of these risks.
基金This research was supported by the National Natural Science Foundation of China(Grant Nos.21866017 and 42067056)the Yunnan Fundamental Research Projects(China)(202101BE070001-013 and 202201AU070157)the Foundation for Distinguished Young Talents of Yunnan Province(China)(202101AV070006).
文摘Dissolved organic matter(DOM)from each treatment process of wastewater treatment plants(WWTPs)contains abundant photosensitive substances,which could significantly affect the photodegradation of 17α-ethinylestradiol(EE2).Nevertheless,information about EE2 photodegradation behavior mediated by DOM from diverse WWTPs and the photosensitivity sources of such DOM are inadequate.This study explored the photodegradation behavior of EE2 mediated by four typical WWTPs’DOM solutions and investigated the photosensitivity sources of DOM in the anaerobic-anoxic-oxic(A2/O)process.The parallel factor analysis identified three varying fluorescing components of these DOM,tryptophan-like substances or protein-like substances,microbial humuslike substances,and humic-like components.The photodegradation rate constants of EE2 were positively associated with the humification degree of DOM(P<0.05).The triplet state substances were responsible for the degradation of EE2.DOM extracted from the A2/O process,especially in the secondary treatment process had the fastest EE2 photodegradation rate compared to that of the other three processes.Four types of components(water-soluble organic matter(WSOM),extracellular polymeric substance,humic acid,and fulvic acid)were separated from the A2/O process DOM.WSOM had the highest promotion effect on EE2 photodegradation.Fulvic acid-like components and humic acid-like organic compounds in WSOM were speculated to be important photosensitivity substances that can generate triplet state substances.This research explored the physicochemical properties and photosensitive sources of DOM in WWTPs,and explained the fate of estrogens photodegradation in natural waters.
基金the financial support from the National Key Research and Development Program of China(2019YFD1100204)the National Natural Science Foundation of China(52091545)+2 种基金the State Key Laboratory of Urban Water Resource and Environment,Harbin Institute of Technology(2021TS03)The Important Projects in the Scientific Innovation of CECEP(cecep-zdkj-2020-009)the Open Project of Key Laboratory of Environmental Biotechnology,Chinese Academy of Sciences(kf2018002).
文摘Wastewater treatment plants(WWTPs)are important and energy-intensive municipal infrastructures.High energy consumption and relatively low operating performance are major challenges from the perspective of carbon neutrality.However,water-energy nexus analysis and models for WWTPs have rarely been reported to date.In this study,a cloud-model-based energy consumption analysis(CMECA)of a WWTP was conducted to explore the relationship between influent and energy consumption by clustering its influent’s parameters.The principal component analysis(PCA)and K-means clustering were applied to classify the influent condition using water quality and volume data.The energy consumption of the WWTP is divided into five standard evaluation levels,and its cloud digital characteristics(CDCs)were extracted according to bilateral constraints and golden ratio methods.Our results showed that the energy consumption distribution gradually dispersed and deviated from the Gaussian distribution with decreased water concentration and quantity.The days with high energy efficiency were extracted via the clustering method from the influent category of excessive energy consumption,represented by a compact-type energy consumption distribution curve to identify the influent conditions that affect the steady distribution of energy consumption.The local WWTP has high energy consumption with 0.3613 kW·h·m^(-3)despite low influent concentration and volumes,across four consumption levels from low(I)to relatively high(IV),showing an unsatisfactory operation and management level.The average oxygenation capacity,internal reflux ratio,and external reflux ratio during high energy efficiency days recognized by further clustering were obtained(0.2924-0.3703 kg O_(2)·m^(-3),1.9576-2.4787,and 0.6603-0.8361,respectively),which could be used as a guide for the days with low energy efficiency.Consequently,this study offers a water-energy nexus analysis method to identify influent conditions with operational management anomalies and can be used as an empirical reference for the optimized operation of WWTPs.
基金supported by the Pamukkale University Scientific Research Project(Turkey)(No.2019FEBE009).
文摘Plastic particles smaller than 5 mm are microplastics.They are among the significant pollutants that recently attracted attention.Great quantities of microplastics enter the sewage system daily and reach wastewater treatment plants(WWTPs).As a result,WWTPs are potential microplastic sources.Hence,they create a pathway for microplastics to reach aquatic environments with treated wastewater discharge.Studies on microplastic characterization in WWTPs have gained momentum in academia.This study investigates the abundance,size,shape,color,polymer type,and removal efficiencies of microplastics in a municipal wastewater treatment plant(WWTP)in Denizli/Turkey.The results showed that the dominant microplastic shape in wastewater samples was fibers(41.78%–60.77%)in the 100–500μm(58.57%–80.07%)size range.Most of the microplastics were transparent-white(32.86%–58.93%).The dominant polymer types were polyethylene(54.05%)and polyethylene vinyl acetate(37.84%)in raw wastewater.Furthermore,the microplastic removal efficiencies of the Denizli Central WWTP as a whole and for individual treatment units were evaluated.Although the microplastic pollution removal efficiency of the Denizli Central WWTP was over 95%,the microplastic concentration discharged daily into the receiving environment was considerably high(1.28×1010 MP/d).Thus,Denizli Central WWTP effluents result in a high volume of emissions in terms of microplastic pollution with a significant daily discharge to theÇürüksu Stream.
基金supported by the Foundation of Key Laboratory of Yangtze River Water Environment,Ministry of Education(Tongji University),China(No.YRWEF 202007)supported by the Science and Technology Commission of Shanghai Municipality Foundation(Nos.17DZ1202100,21230712200).
文摘Wastewater treatment plants(WWTPs)consume large amounts of energy and emit greenhouse gases to remove pollutants.This study proposes a framework for evaluating the energy neutrality potential(ENP)of WWTPs from an integrated perspective.Operational data of 970 WWTPs in the Yangtze River Economic Belt(YREB)were extracted from the China Urban Drainage Yearbook 2018.The potential chemical and thermal energies were estimated using combined heat and power(CHP)and water source heat pump,respectively.Two key performance indicators(KPIs)were then established:the energy self-sufficiency(ESS)indicator,which reflects the offset degree of energy recovery,and the comprehensive water–energy efficiency(CWEE)indicator,which characterizes the efficiency of water–energy conversion.For the qualitative results,98 WWTPs became the benchmark(i.e.,CWEE=1.000),while 112 WWTPs were fully self-sufficient(i.e.,ESS≥100%).Subsequently,four types of ENP were classified by setting the median values of the two KPIs as the critical value.The WWTPs with high ENP had high net thermal energy values and relatively loose discharge limits.The explanatory factor analysis of water quantity and quality verified the existence of scale economies.Sufficient carbon source and biodegradability condition were also significant factors.As the CWEE indicator was mostly sensitive to the input of CHP,future optimization shall focus on the moisture and organic content of sludge.This study proposes a novel framework for evaluating the ENP of WWTPs.The results can provide guidance for optimizing the energy efficiency and recovery of WWTPs.
基金financially supported by the Guangdong Technological Innovation Strategy of Special Funds(Key Areas of Research and Development Program,No.2018B020205003)
文摘Small RNAs(sRNAs)are key players in the regulation of bacterial gene expression.However,the distribution and regulatory functions of sRNA in pig farm wastewater treatment plants(WWTPs)remains unknown.In this study,the wastewaters in anoxic and oxic tanks of the WWTPs were collected.The profiles of the community structure,mRNA expression,and sRNA expression of bacteria in pig farm wastewater were investigated using transcriptome sequencing and qPCR.This study demonstrated that there was a higher abundance of sRNA in the pig farm WWTPs and 52 sRNAs were detected.The sRNAs were mainly present in Proteobacteria and Firmicutes,including the potential human pathogenic bacteria(HPB)(Escherichia,Shigella,Bordetella and Morganella),crop pathogen(Pectobacterium)and denitrifying bacteria(Zobellella).And the sRNAs were involved in the bacterial functional activities such as translation,transcription,drug resistance,membrane transport and amino acid metabolism.In addition,most sRNAs had a higher abundance in anoxic tanks which contained a higher abundance of the genes associated with infectious diseases and drug resistance than that in oxic tanks.The results presented here show that in pig farm WWTPs,sRNA played an important role in bacterial function activities,especially the infectious diseases,drug resistance and denitrification,which can provide a new point of penetration for improving the pig farm WWTPs.
基金supported in part by the Environment Research and Technology Development Fund (C-0802) of the Ministry of the Environment,Japanthe Grant-in-Aid for Young Scientists (B) 20760362 from the Ministry of Education,Culture,Sports,Science and Technology,Japan
文摘To assess the potential endocrine disruptive effects through multiple nuclear receptors (NRs), especially non-steroidal NRs, in municipal wastewater, we examined the agonistic activities on four NRs (estrogen receptor α, thyroid hormone receptor α, retinoic acid receptor ct and retinoid X receptor α) of untreated and treated wastewater from municipal wastewater treatment plants (WWTPs) in Japan using a yeast two-hybrid assay. Investigation of the influent and effluent of seven WWTPs revealed that agonistic activities against steroidal and non-steroidal NRs were always detected in the influents and partially remained in the effluents. Further investigation of four WWTPs employing conventional activated sludge, pseudo-anoxic-oxic, anoxic-oxic and anaerobic-anoxic-oxic processes revealed that the ability to reduce the agonistic activity against each of the four NRs varies depending on the treatment process. These results indicated that municipal wastewater in Japan commonly contains endocrine disrupting chemicals that exert agonistic activities on steroidal and non-steroidal NRs, and that some of these chemicals are released into the natural aquatic environment. Although the results obtained in yeast assays suggested that measured levels of non-steroidal NR agonists in the effluent of WWTPs were not likely to cause any biological effect, further study is required to assess their possible risks in detail.
基金This work was supported by Kurita Water Environ-ment Foundation of Japan(14701)the National Natural Science Foundation of China(Grant No.20277022).
文摘The concentration and distribution of nonylphe-nol polyethoxylates(NPEOs represents the mixture,and NPnEO represents the monomer)and its metabolites in the influent and effluent of four municipal sewage treatment plants(STPs)in the north of China were measured.Moreover,the concentration and distribution of the above chemicals in the sludge of two STPs were also determined,and the transfer and fate of NPEOs in the sewage treatment process were discussed primarily by analyzing the distribu-tion of the products in the effluent and the sludge.The results showed that NPEOs and its metabolites existed in all the samples of the influent,effluent,and sludge.NPEOs were degraded in the sewage treatment process with the removal efficiency in the range of 23.38%-77.11%,or an average of 52.86%.However,the large analogs of NPnEO were only degraded to small ones,whose degradation rate was rather slow,and consequently the degradation was not complete.Hence,the concentrations of some small metabolites,such as nonylphenol(NP),nonylphenol monoethoxylate(NP1EO),and nonylphenol diethoxylate(NP2EO)were elevated in the effluent.These small metabolites are more toxic than the large NPnEO analogs,and some of them were reported to exhibit environmental endocrine disrupting activity.From this point of view,the process of sewage treatment does not reduce but elevate the risk of NPEOs,which becomes the main source of these small NPnEO in the environment.The sludge exhibited good adsorption ability for NPEOs,especially for the small analogs,which led to the high level of NPEOs in the sludge.Hence,reasonable disposal of the surplus sludge to avoid re-pollution is very important.
基金This work was funded by the International Partnership Program of the Chinese Academy of Sciences,(Grant No.132744KYSB20170002)UCAS scholarship for international students.The authors want to acknowledge the generous support from the National Water Supply and Drainage Board(Sewerage division),Sri Lanka and to Mr.S.M.Samaraweera for the assistance in wastewater sampling.
文摘Most of the monitoring data on the occurrence of antibiotics in sewage treatment plants(STPs)have been reported from Europe,North America and some countries in Northeast Asia,while very limited data can be found in Southeast Asian countries.As a pioneering research in Sri Lanka,we collected 24 h composite wastewater samples at the influent and effluent of two municipal STPs for consecutive 7 days to investigate occurrence,consumption and removal efficiency of seventeen antibiotics.The STP was located in Colombo and Hikkaduwa,respectively,representing two kinds of communities(i.e.local and tourists)in Sri Lanka.The targeted antibiotics were extracted by solid-phase extraction method and detected on an Agilent HPLCMSMS(1290/6470QQQ).Results illustrated that the majority of the antibiotics can be always detected from both STPs,except for chlorotetracycine(CTC),doxycycline(DOX)and florfenicol(FF).Fluoroquinolones(FQs)were detected at highest concentrations with ciprofloxacin(CIP)being the dominant compound.Concentrations of CIP in the influent samples were in the range of 433 e6010 ng/L.The consumption of antibiotics was estimated on the basis of influent mass load and catchment population data.We found difference in consumption patterns between the two served areas.Compared to local people in Colombo,tourists in Hikkaduwa appeared to take more antibiotics during the study period with the estimated daily dose of 0.25 g per 1000 persons.Moreover,macrolides accounted for a larger portion than FQs in Hikkaduwa,with azithromycin(AZM)being the most prevalent antibacterial agent.After comparison with an official report by Medical Supplies Division of Sri Lanka,we conjected that AZM was not commonly used among local people and it was mainly introduced by foreign arrivals.As for the removal efficiency,the activated sludge system of Colombo exhibited better elimination and more stable performance than the constructed wetland process of Hikkaduwa.
文摘Municipal wastewater consists of a downstream collection of flushed sewage(without solid waste),other household runoffs,industrial runoffs,hospital runoffs and agricultural runoffs through an underground pipe before treatment.A runoff collection system called the wastewater treatment plant(WWTPs)treats such wastewater before release into environment following specific regulatory standards.This years-long practice has been improved upon by adding end-to-end pipe technologies with a view to enhancing the quality of effluent released.However,effluents released into the environment from design/application of WWTPs appear to contain emerging contaminants of both biotic and abiotic nature.The observation of chemical contaminants,antibiotic resistant bacteria(ARB),antibiotic resistant genes(ARGs)and diverse pathogenic bacteria genera in wastewater works release further affirm the abundance of such emerging contaminants.As a result,the government and water regulatory organizations in various part of the world are considering the removal of water reuse act from recycling policy/process.Current global debate is focused on questions about sustenance of any improved additional treatment level;effect of energy consumption by added treatment stage and its impact on the environmental wellness as contaminants borne wastewater is consistently released.Technological advancement/research suggests implementation of newer innovative infrastructural systems(NIIS)such as Mobbing Bed Biofilm Rector(MBBR),for wastewater effluent management which involve addition of newer wastewater treatment stages.This review addressed current pitfalls including wastewater microbiota of high epidemiological/public health relevance and affirms the need for such improvement which requires modification of ongoing institutional framework with a view to encourage implementation of NIIS for an improved effluent release.Exploiting the advances of microbial biofilming and the potentials of microbial biofueling as discussed in various section promises a future of robust environmental system,stable operational standard,release of quality effluent and sustainable management of wastewater works.Application of the aforementioned would enhance qualityWWTPs release and in-defacto reduces spread of ARB/ARGs as well as impacts both the environment wellness and public health.
文摘To improve nitrogen removal performance of wastewater treatment plants (WWTPs), it is essential to understand the behavior of nitrogen cycling communities, which comprise various microorganisms. This study characterized the quantity and diversity of nitrogen cycling genes in various processes of municipal WWTPs by employing two molecular-based methods:most probable number-polymerase chain reaction (MPN-PCR) and DNA microarray. MPN-PCR analysis revealed that gene quantities were not statistically different among processes, suggesting that conventional actwated sludge processes (CAS) are similar to nitrogen removal processes in their ability to retain an adequate population of nitrogen cycling microorganisms. Furthermore, most processes in the WWTPs that were researched shared a pattern:the nitS and the bacterial amoA genes were more abundant than the nirK and archaeal amoA genes, respectivelv. DNA microarray analysis revealed that several kinds of nitrification and denitrification genes were detected in both CAS and anaerobic-oxic processes (AO), whereas limited genes were detected in nitrogen removal processes. Results of this study suggest that CAS maintains a diverse community of nitrogen cycling microorganisms; moreover, the microbial communities in nitrogen removal processes may be specific.
文摘N-nitrosodimethylamine (NDMA) and several other N-nitrosamines have been detected as disinfection by-products in drinking waters in many countries around the world. An ultra-performance liquid chromatography- tandem mass spectrometry method with solid phase extraction sample preparation was developed to study the occurrence of N-nitrosamines in several water treatment plants and distribution systems in China. Isotope labeled N-nitrosodi-n-propylamine-dl4 (NDPA-dl4) was selected as the internal standard for quantification. The solid phase extraction procedures including pH, enrichment process and MS/MS parameters including capillary voltage, cone gas flow, cone voltage, collision energy were optimized to give average recoveries of 26% to 112% for nine N- nitrosamine species. The instrument detection limits were estimated to range from 0.5 to 5μg.L-1 for the nine N- nitrosamine species. NDMA and several other N-nitrosa- mines were found at fairly high concentrations in several water treatment plants and distribution systems. NDMA was found in all locations, and the highest concentrations in cities B, G, T, and W were 3.0, 35.7, 21.3, and 19.7 ng. L 1, respectively. A wide range of N-nitrosamines concentrations and species were observed in different locations. Higher concentrations of N-nitrosamines were detected in distribution systems that were further away from the treatment plants, suggesting that the contact time between the residual disinfectant and natural organic matter may play an important role in the formation of these compounds.
文摘The water quality and energy consumption of wastewater treatment plants(WWTPs)in Taihu Basin were evaluated on the basis of the operation data from 204 municipal WWTPs in the basin by using various statistical methods.The influent ammonia nitrogen(NH3-N)and total nitrogen(TN)of WWTPs in Taihu Basin showed normal distribution,whereas chemical oxygen demand(COD),biochemical oxygen demand(BOD5),suspended solid(SS),and total phosphorus(TP)showed positively skewed distribution.The influent BOD5/COD was 0.4%-0.6%,only 39.2%SS/BOD5 exceeded the standard by 36.3%,the average BOD5/TN was 3.82,and the probability of influent BOD5/TP>20 was 82.8%.The average energy consumption of WWTPs in Taihu Basin in 2017 was 0.458 kWh/m^3.The specific energy consumption of WWTPs with a daily treatment capacity of more than 5×10^4 m^3 in Taihu Basin was stable at 0.33 kWh/m^3.A power function relationship was observed between the reduction in COD and NH3-N and the specific energy consumption of pollutant reduction,and the higher the pollutant reduction is,the lower the specific energy consumption of pollutant reduction presents.In addition,a linear relationship existed between the energy consumption of WWTPs and the specific energy consumption of influent volume and pollutant reduction.Therefore,upgrading and operation with less energy consumption of WWTPs is imperative and the suggestions for Taihu WWTPs based on stringent discharge standard are proposed in detail.