为认识西北地区的云水资源(Cloud Water Resource,简称CWR)特征以及科学规划人工增雨开发空中水资源作业布局,利用2000—2019年中国1°×1°CWR观测诊断评估数据集,采用线性拟合和经验正交函数分解(EOF)等方法,统计分析了...为认识西北地区的云水资源(Cloud Water Resource,简称CWR)特征以及科学规划人工增雨开发空中水资源作业布局,利用2000—2019年中国1°×1°CWR观测诊断评估数据集,采用线性拟合和经验正交函数分解(EOF)等方法,统计分析了西北地区CWR的分布及演变气候特征。结果表明:(1)从全区整体看,CWR的相关物理量(状态量、平流量、总量和降水效率)主要表现为夏季最高,春、秋季次之,冬季最低的季节变化特征。其中,春季CWR总量约为1736亿t(折合柱水量约为51.2 mm),仅次于夏季;春季水凝物降水效率为48.7%,相较于秋季,春季的CWR开发潜力更大。(2)从区域内1°×1°网格的计算结果得到空间分布,受地势与环流的影响,近20年CWR年总量及水汽年总量、水凝物年总量的多年平均空间分布呈“两高一低”的特征,高值位于西风急流区与季风影响边缘区,低值区主要位于高原气候区。(3)近20年,西北地区格点的CWR年总量平均以23.6 mm/a速率增加,其中春季的增加趋势最显著,增速为8.5 mm/a。季节分布上,CWR夏季最多,春、秋季次之,冬季最少;水凝物降水效率夏季高,秋、春季较低,冬季最低。(4)CWR年总量的EOF分解第一模态(EOF1)贡献率为78.2%,分布特征为区域东部较高,在2008年出现年际转折,开始转变为CWR东部多、西部少的分布格局。(5)在西北地区典型区域中,天山区域年平均及格点平均后的CWR年总量以及水凝物降水效率均高于祁连山区,年际变化上祁连山区的CWR在增多,天山区的在减少。展开更多
Carbon nitrides with two-dimensional layered structures and high theoretical capacities are attractive as anode materials for sodium-ion batteries while their low crystallinity and insufficient structural stability st...Carbon nitrides with two-dimensional layered structures and high theoretical capacities are attractive as anode materials for sodium-ion batteries while their low crystallinity and insufficient structural stability strongly restrict their practical applications.Coupling carbon nitrides with conductive carbon may relieve these issues.However,little is known about the influence of nitrogen(N)configurations on the interactions between carbon and C_(3)N_(4),which is fundamentally critical for guiding the precise design of advanced C_(3)N_(4)-related electrodes.Herein,highly crystalline C_(3)N_(4)(poly(triazine imide),PTI)based all-carbon composites were developed by molten salt strategy.More importantly,the vital role of pyrrolic-N for enhancing charge transfer and boosting Na+storage of C_(3)N_(4)-based composites,which was confirmed by both theoretical and experimental evidence,was spot-highlighted for the first time.By elaborately controlling the salt composition,the composite with high pyrrolic-N and minimized graphitic-N content was obtained.Profiting from the formation of highly crystalline PTI and electrochemically favorable pyrrolic-N configurations,the composite delivered an unusual reverse growth and record-level cycling stability even after 5000 cycles along with high reversible capacity and outstanding full-cell capacity retention.This work broadens the energy storage applications of C_(3)N_(4) and provides new prospects for the design of advanced all-carbon electrodes.展开更多
The ultra-long electromagnetic wave remote sensing technique developed by Peking University is one of new future techniques, which can detect the submarine geological information from the depth of 20 to 10000 m below ...The ultra-long electromagnetic wave remote sensing technique developed by Peking University is one of new future techniques, which can detect the submarine geological information from the depth of 20 to 10000 m below the surface by receiving natural ultra-long electromagnetic waves (n Hz to n 100 Hz). The new remote sensor is composed of three parts: a main instrument with a portable computer, an antenna with an amplifier and an external power.展开更多
Using Ti powder as reagent,ultra-long TiO2 nanofibers were prepared via hydrothermal method in NaOH solution.The samples were char-acterized respectively by means of field emission scanning electron microscopy (FESEM)...Using Ti powder as reagent,ultra-long TiO2 nanofibers were prepared via hydrothermal method in NaOH solution.The samples were char-acterized respectively by means of field emission scanning electron microscopy (FESEM),transmission electron microscopy (TEM) with selected area electron diffraction (SAED),and X-ray diffraction (XRD).The diameter and the length of the ultra-long TiO2 nanofiber were ~100 nm and >200μm,respectively.The ultra-long TiO2 nanofibers were anatase after heat treatment at 450 ?C for 1 h.Moreover,the optical properties of the products were investigated by UV-visible light absorption spectrum.Furthermore,methyl orange was used as a target molecule to estimate the photocatalytic activity of the specimens.Under the same testing conditions,the photocatalytic activity of the ultra-long TiO2 nanofibers was higher than that of P25.Direct electrical pathway and improved light-harvesting efficiency were crucial for the superior photocatalytic activity of the ultra-long TiO2 nanofibers.展开更多
A stability of a nonlinear ultra-long wave and its solution are discussed in this paper by employing Burger model which is subject to heat resource. It is of interest noted that the wave solution can be described by a...A stability of a nonlinear ultra-long wave and its solution are discussed in this paper by employing Burger model which is subject to heat resource. It is of interest noted that the wave solution can be described by an equation of KDV or MKDV and that conditions for the existence of the solution are related to characteristic divergences. In addition, a wave velocity expression for nonlinear ultra-long waves and some diagnostic correlations among wave parameters have been obtained.展开更多
We develop a new electrospinning method to prepare ultra-long ordered La1-xSrxMnO3 (LSMO) nanowires. The length is up to several centimeters and is only limited by the size of the collector. The well-ordered straigh...We develop a new electrospinning method to prepare ultra-long ordered La1-xSrxMnO3 (LSMO) nanowires. The length is up to several centimeters and is only limited by the size of the collector. The well-ordered straight-line structure ensures the transport measurement, which is impossible to be carried out for the random nanowires fabricated by the traditional electrospinning method. Magnetic and transport measurements indicate that the physical properties of the LSMO nanowires depend sensitively on the doping concentration. At the optimum doping, the LSMO wires are ferromagnetic at room temperature with a metal-insulator transition temperature close to room temperature. Magnetic force microscopy studies are also performed to provide a microscopic view of these ultra-long nanowires.展开更多
Recently, an effective exciton diffusion length L exceeding 100μm has been reported for organic- inorganic halide perovskites owing to both the high mobility and ultra-long lifetime of the excitons; however, the orig...Recently, an effective exciton diffusion length L exceeding 100μm has been reported for organic- inorganic halide perovskites owing to both the high mobility and ultra-long lifetime of the excitons; however, the origin of ultra-long L is still unclear in nature. In some photoelectric materials, reverse intersystem crossing (RISC) from the triplet to the singlet state can enhance the quantum yield of pho- toluminescence greatly. In this study, our theoretical investigation indicated that the energy difference △E_st between the singlet state and the triplet state of CH_3NH_3Pbl_3 was less than 0.1 eV, which represents one crucial prerequisite for the occurrence of RISC. Meanwhile, the experimental results showed that the photoluminescence lifetime increased with the increasing temperature, a typical feature of RISC. Based on this study, we put forward the hypothesis that the ultra-long lifetime of excitons in organic-inorganic halide perovskite might be caused by the RISC process. This may provide a new insight into the important photophysical properties of such novel photovoltaic materials.展开更多
In the novel approach to the diagnostic tests of continuous welded rail (CWR) track by the use of the tamping machine, the fundamental statement related to the recording of the curvature with a definite value of the...In the novel approach to the diagnostic tests of continuous welded rail (CWR) track by the use of the tamping machine, the fundamental statement related to the recording of the curvature with a definite value of the lateral displacement being subjected to verification, can provide a basis for the determination of the longitudinal axial force in the rail. An attempt has also been made to define an alternative factor which by means of the measured signals, could be used for the determination of the axial forces in the rail sections. A power engineering approach has been adopted to this concept. Within the framework of the experimental investigations, measurements were carried out in the track test section. The investigations were based on stretching the rail sections by stretchers and on lateral displacements of the track by the tamping machine. The operation of the measuring apparatus was also tested in the experimental railway track section while carrying out the geometrical adjustments by the tamping machine. As a result of next series of the investigation carried out in 2006-2007, the authors worked out a procedure of estimating the longitudinal forces in rails of CWR track.展开更多
基金supported by the National Natural Science Foundation of China(51904059)Applied Basic Research Program of Liaoning(2022JH2/101300200)+1 种基金Guangdong Basic and Applied Basic Research Foundation(2022A1515140188)Fundamental Research Funds for the Central Universities(N_(2)002005,N_(2)125004,N_(2)225044)。
文摘Carbon nitrides with two-dimensional layered structures and high theoretical capacities are attractive as anode materials for sodium-ion batteries while their low crystallinity and insufficient structural stability strongly restrict their practical applications.Coupling carbon nitrides with conductive carbon may relieve these issues.However,little is known about the influence of nitrogen(N)configurations on the interactions between carbon and C_(3)N_(4),which is fundamentally critical for guiding the precise design of advanced C_(3)N_(4)-related electrodes.Herein,highly crystalline C_(3)N_(4)(poly(triazine imide),PTI)based all-carbon composites were developed by molten salt strategy.More importantly,the vital role of pyrrolic-N for enhancing charge transfer and boosting Na+storage of C_(3)N_(4)-based composites,which was confirmed by both theoretical and experimental evidence,was spot-highlighted for the first time.By elaborately controlling the salt composition,the composite with high pyrrolic-N and minimized graphitic-N content was obtained.Profiting from the formation of highly crystalline PTI and electrochemically favorable pyrrolic-N configurations,the composite delivered an unusual reverse growth and record-level cycling stability even after 5000 cycles along with high reversible capacity and outstanding full-cell capacity retention.This work broadens the energy storage applications of C_(3)N_(4) and provides new prospects for the design of advanced all-carbon electrodes.
文摘The ultra-long electromagnetic wave remote sensing technique developed by Peking University is one of new future techniques, which can detect the submarine geological information from the depth of 20 to 10000 m below the surface by receiving natural ultra-long electromagnetic waves (n Hz to n 100 Hz). The new remote sensor is composed of three parts: a main instrument with a portable computer, an antenna with an amplifier and an external power.
基金supported by Peak of Six Major Human Resources Plan of Jiangsu Province and Jiangsu Key Technology R&D Program (BE2009130)
文摘Using Ti powder as reagent,ultra-long TiO2 nanofibers were prepared via hydrothermal method in NaOH solution.The samples were char-acterized respectively by means of field emission scanning electron microscopy (FESEM),transmission electron microscopy (TEM) with selected area electron diffraction (SAED),and X-ray diffraction (XRD).The diameter and the length of the ultra-long TiO2 nanofiber were ~100 nm and >200μm,respectively.The ultra-long TiO2 nanofibers were anatase after heat treatment at 450 ?C for 1 h.Moreover,the optical properties of the products were investigated by UV-visible light absorption spectrum.Furthermore,methyl orange was used as a target molecule to estimate the photocatalytic activity of the specimens.Under the same testing conditions,the photocatalytic activity of the ultra-long TiO2 nanofibers was higher than that of P25.Direct electrical pathway and improved light-harvesting efficiency were crucial for the superior photocatalytic activity of the ultra-long TiO2 nanofibers.
文摘A stability of a nonlinear ultra-long wave and its solution are discussed in this paper by employing Burger model which is subject to heat resource. It is of interest noted that the wave solution can be described by an equation of KDV or MKDV and that conditions for the existence of the solution are related to characteristic divergences. In addition, a wave velocity expression for nonlinear ultra-long waves and some diagnostic correlations among wave parameters have been obtained.
基金Supported by the National Basic Research Program of China under Grant Nos 2016YFA0300700,2013CB932901 and2014CB921104the National Natural Science Foundation of China under Grant Nos 11274071 and 11504053the Shanghai Municipal Natural Science Foundation under Grant No 11ZR140260
文摘We develop a new electrospinning method to prepare ultra-long ordered La1-xSrxMnO3 (LSMO) nanowires. The length is up to several centimeters and is only limited by the size of the collector. The well-ordered straight-line structure ensures the transport measurement, which is impossible to be carried out for the random nanowires fabricated by the traditional electrospinning method. Magnetic and transport measurements indicate that the physical properties of the LSMO nanowires depend sensitively on the doping concentration. At the optimum doping, the LSMO wires are ferromagnetic at room temperature with a metal-insulator transition temperature close to room temperature. Magnetic force microscopy studies are also performed to provide a microscopic view of these ultra-long nanowires.
基金The financial supports of the National Natural Science Foundation of China (grant nos. 21373042, 21677029 and 51402036)the Fundamental Research Funds for the Central Universities (grant no. DUT15YQ109)
文摘Recently, an effective exciton diffusion length L exceeding 100μm has been reported for organic- inorganic halide perovskites owing to both the high mobility and ultra-long lifetime of the excitons; however, the origin of ultra-long L is still unclear in nature. In some photoelectric materials, reverse intersystem crossing (RISC) from the triplet to the singlet state can enhance the quantum yield of pho- toluminescence greatly. In this study, our theoretical investigation indicated that the energy difference △E_st between the singlet state and the triplet state of CH_3NH_3Pbl_3 was less than 0.1 eV, which represents one crucial prerequisite for the occurrence of RISC. Meanwhile, the experimental results showed that the photoluminescence lifetime increased with the increasing temperature, a typical feature of RISC. Based on this study, we put forward the hypothesis that the ultra-long lifetime of excitons in organic-inorganic halide perovskite might be caused by the RISC process. This may provide a new insight into the important photophysical properties of such novel photovoltaic materials.
文摘In the novel approach to the diagnostic tests of continuous welded rail (CWR) track by the use of the tamping machine, the fundamental statement related to the recording of the curvature with a definite value of the lateral displacement being subjected to verification, can provide a basis for the determination of the longitudinal axial force in the rail. An attempt has also been made to define an alternative factor which by means of the measured signals, could be used for the determination of the axial forces in the rail sections. A power engineering approach has been adopted to this concept. Within the framework of the experimental investigations, measurements were carried out in the track test section. The investigations were based on stretching the rail sections by stretchers and on lateral displacements of the track by the tamping machine. The operation of the measuring apparatus was also tested in the experimental railway track section while carrying out the geometrical adjustments by the tamping machine. As a result of next series of the investigation carried out in 2006-2007, the authors worked out a procedure of estimating the longitudinal forces in rails of CWR track.