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Deliberation between PM1 and PM2.5 as air quality indicators based on comprehensive characterization of urban aerosols in Bangkok, Thailand
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作者 Issariya Vejpongsa Sirikalaya Suvachittanont +3 位作者 Natsucla Klinklan Thunyapat Thongyen Miklos Veres Wladyslaw W. Szymanski 《Particuology》 SCIE EI CAS CSCD 2017年第6期1-9,共9页
Urban ambient aerosols in the size range below 10 μm were measured and sampled for further evalua- tion (by Raman and Thermal-Optical analysis) of the collected material. The presented data shows that monitoring nu... Urban ambient aerosols in the size range below 10 μm were measured and sampled for further evalua- tion (by Raman and Thermal-Optical analysis) of the collected material. The presented data shows that monitoring number and/or surface area concentrations besides the mass concentration provides valu- able information for a meaningful assessment of the actual ambient air quality. The aim of the study was to characterize the urban aerosols using various instruments, methods, and sampling conditions, and to determine whether a split of the PMzs size fraction at PM1 may deliver a more sensible indication of the actual air quality than the current standard of monitoring PMzs. We found substantial differences relating to this split. PM2.5 data frequently include particles from both mechanical and combustion processes, PM1 measurements can be used to better distinguish particles derived from these two sources. We measured number concentrations of PM1 with PM2.5-1 concurrently with particle mass concentration and found that the typical average particle diameter by mass in the urban aerosols investigated was in the range of 120 nm; this corresponded well with the particle number size distributions measured in real time. Raman spectral analysis and thermal-optical evaluation of the sampled material also suggested that it would be sensible to split the measurement of the PM2.5 fraction into PM1 and PM2.s-1 size fractions, especially for analysis of carbonaceous aerosol components using the DRI thermal/optical reflectance carbon analysis system 展开更多
关键词 urban aerosol PM-ffactions Carbonaceous particles Raman spectroscopy Thermal-optical analysis
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Impact of Anthropogenic Aerosols on Summer Precipitation in the Beijing–Tianjin–Hebei Urban Agglomeration in China:Regional Climate Modeling Using WRF-Chem 被引量:1
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作者 Jun WANG Jinming FENG +1 位作者 Qizhong WU Zhongwei YAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2016年第6期753-766,共14页
The WRF model with chemistry (WRF-Chem) was employed to simulate the impacts of anthropogenic aerosols on summer precipitation over the Beijing-Tianjin-Hebei urban agglomeration in China. With the aid of a high-reso... The WRF model with chemistry (WRF-Chem) was employed to simulate the impacts of anthropogenic aerosols on summer precipitation over the Beijing-Tianjin-Hebei urban agglomeration in China. With the aid of a high-resolution gridded inventory of anthropogenic emissions of trace gases and aerosols, we conducted relatively long-term regional simulations, considering direct, semi-direct and indirect effects of the aerosols. Comparing the results of sensitivity experiments with and without emissions, it was found that anthropogenic aerosols tended to enhance summer precipitation over the metropolitan areas. Domain-averaged rainfall was increased throughout the day, except for the time around noon. Aerosols shifted the precipitation probability distribution from light or moderate to extreme rain. Further analysis showed that the anthropogenic aerosol radiative forcing had a cooling effect at the land surface, but a warming effect in the atmosphere. However, enhanced convective strength and updrafts accompanied by water vapor increases and cyclone-like wind shear anomalies were found in the urban areas. These responses may originate from cloud microphysical effects of aerosols on convection, which were identified as the primary cause for the summer rainfall enhancement. 展开更多
关键词 anthropogenic aerosols summer precipitation urban agglomeration regional climate
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High Contribution of Sea Salt Aerosols on Atmospheric Particles Measured at an Urban Tropical Location in Reunion Island
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作者 Chatrapatty Bhugwant Miloud Bessafi +3 位作者 Olivier Favez Laura Chiappini Bruno Sieja Eva Leoz-Garziandia 《Journal of Environmental Protection》 2013年第8期828-842,共15页
PM10 was monitored during 2008-2011 period at LUT and BON, two urban tropical stations close to each other at Saint-Pierre city, in Reunion Island (south-western Indian Ocean). During the study period, notable PM10 co... PM10 was monitored during 2008-2011 period at LUT and BON, two urban tropical stations close to each other at Saint-Pierre city, in Reunion Island (south-western Indian Ocean). During the study period, notable PM10 concentrations are observed at BON close to the coasts. At LUT, a more inland site, the daily PM10 concentration range between 13 and 70 μg/m3. Importantly, the limit value for the protection of the human health is systematically exceeded at BON while it is never exceeded at LUT. Also, the quality objective (QO: 30 μg/m3, on annual average) and the limit value for the human health protection (LV: 40 μg/m3, on annual average) are exceeded at BON each year during 2008-2011, while at LUT no regulatory values are exceeded. Nitrogen dioxide, an atmospheric tracer of anthropogenic activities was also monitored at LUT and BON. The mean diurnal NO2 variation is of the same level and order of magnitude and exhibits a similar pattern at both stations suggesting that distinct sources influence the PM10 at LUT and at BON. Chemical analysis was performed on daily filters sampled in September-November 2011 at the two stations to determine the sea salt contribution on PM10 across Saint-Pierre city. It showed that the sea salt contribution to the PM10 is 55% at BON in September 2011. The sea salt particles are therefore the main cause for the exceedances of the regulatory values of PM10 recorded at BON. The results importantly suggest that the notable PM10 concentrations measured at this urban marine site might have some but minor impact on human health. 展开更多
关键词 PM10 Nitrogen Dioxide ANTHROPOGENIC Sea Salt aerosolS Chemical Characterization REGULATORY Values Human Health Lung Cancer urban TROPICAL
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西安市城市气溶胶污染岛长时间序列特征分析
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作者 李芮 陈健 +1 位作者 陆嘉栋 祝善友 《生态与农村环境学报》 CAS CSCD 北大核心 2024年第4期490-498,共9页
城市气溶胶污染岛(UAPI)对人体健康、城市热环境、城市气候、大气辐射传输等有重要影响。该研究利用西安市2016—2019年城郊多个站点的PM_(2.5)数据定量化计算UAPI强度,分析PM_(2.5)和UAPI强度的日变化和年变化规律,并使用经验模态分解... 城市气溶胶污染岛(UAPI)对人体健康、城市热环境、城市气候、大气辐射传输等有重要影响。该研究利用西安市2016—2019年城郊多个站点的PM_(2.5)数据定量化计算UAPI强度,分析PM_(2.5)和UAPI强度的日变化和年变化规律,并使用经验模态分解方法(EMD)对UAPI强度的长时间序列多尺度特征进行分析。结果表明,西安市具有明显的城市气溶胶污染岛效应,UAPI强度大于10μg·m^(-3)的比例达87.63%。在日内变化上,UAPI强度呈现夜晚高、白天低的特点;在年内变化上,呈现冬春高、夏秋低的“U”型分布特征;在年际变化上,2016—2019年UAPI效应呈逐年减弱的变化特征。利用EMD分解可以很好地揭示UAPI强度的多尺度特征,如IMF2、IMF4、IMF6分别体现了UAPI强度以周、月、年为周期的变化特征。对比PM_(2.5)和UAPI强度的时间序列,该方法可以较好地排除跨区域传输污染和大区域二次污染等对UAPI强度的影响。 展开更多
关键词 PM_(2.5) 城市气溶胶污染岛 城乡差异 经验模态分解
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Black Carbon Particles in the Urban Atmosphere in Beijing 被引量:11
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作者 王庚辰 白建辉 +1 位作者 孔琴心 Alexander EMILENKO 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2005年第5期640-646,共7页
A study of the concentration of black carbon particles and its variation in the urban atmosphere has been carried out since 1996 in the Beijing area. The measurements were done in the late autumn and early winter each... A study of the concentration of black carbon particles and its variation in the urban atmosphere has been carried out since 1996 in the Beijing area. The measurements were done in the late autumn and early winter each year, the period before and after domestic heating activities begin. The results show the presence of black carbon particles at the high level that vary over a large range in the urban atmosphere in Beijing. The mean value of daily average concentration for the whole observation period of 1996-2004 is 20.0 μgm^-3. An evident decrease of black carbon particle concentration in the Beijing area is observed after 2000, and the daily average concentration of black carbon particles is estimated to be 16.0 μgm^-3 with a variation range of 2.10-50.50 μgm^-3 for the period of 2000-2004. The observation method and main variation behavior characteristics of black carbon particles in the urban atmosphere in the Beijing area are given and discussed. 展开更多
关键词 black carbon particles urban atmosphere aerosolS BEIJING
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Characteristics of air particulate matter and their sources in urban and rural area of Beijing, China 被引量:8
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作者 YANG Shao jin, DONG Jin quan, CHENG Bing ru (Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100080, China) 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2000年第4期402-409,共8页
During October 1993 and March 1996, the samples of fine and coarse air particulate matter have been collected at representative urban and rural site of Beijing with the Gent Stacked Filter Unit Sampler. Instrumental n... During October 1993 and March 1996, the samples of fine and coarse air particulate matter have been collected at representative urban and rural site of Beijing with the Gent Stacked Filter Unit Sampler. Instrumental neutron activation analysis (INAA) and proton induced X ray emission (PIXE) method were used to determine the elemental composition of the particulate matter. Average elemental concentrations and enrichment factors were calculated for the fine and coarse size fractions. Based on the particulate matter data obtained at urban and rural site together with the chemical constituents of the aerosol from the different sources are discussed. The results show that the relative particulate mass and elemental concentrations of crustal and pollutant elements in the air particulate matter collected over the urban are higher than rural and winter heating period are higher than in ordinary season. Beijing atmosphere is polluted by aerosols from regional and faraway sources. It was noticed that the toxic or harmful elements such as As, Sb, Pb, Cu, Ni, S and Zn were mainly enriched in fine particles with diameter less than 2 μm. A receptor model was used to assess the relative contribution of major air pollution sources at receptor sites in Beijing. Trace elements were used as the markers for the above assessment. Factor analysis method was used to identify possible emission sources of air particles. The major sources of dust soil, coal burning, motor vehicle emission, industry emission and refuse incineration were identified. 展开更多
关键词 atmospheric particulate matter urban RURAL SOURCE aerosol
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Validation of MODIS C6 AOD Products Retrieved by the Dark Target Method in the Beijing–Tianjin–Hebei Urban Agglomeration,China 被引量:1
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作者 Jie ZHANG Jinyuan Xin +6 位作者 Wenyu ZHANG Shigong WANG Lili WANG Wei XIE Guojie XIAO Hela PAN Lingbin KONG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2017年第8期993-1002,共10页
The quality of the MODIS C6 3-km and 10-km aerosol optical depth(AOD) products retrieved by the Dark Target(DT)method is discussed using ground-based observations in the Beijing–Tianjin–Hebei region from 1 Augus... The quality of the MODIS C6 3-km and 10-km aerosol optical depth(AOD) products retrieved by the Dark Target(DT)method is discussed using ground-based observations in the Beijing–Tianjin–Hebei region from 1 August 2007 to 31 July2008. Good consistency exists between the 3-km and 10-km products and ground-based observations. The retrieval accuracy of the two products both show distinctive seasonality. The percentage falling within the expected error(EE) is largest in the winter, moderate in the spring and autumn, and smallest in the summer. A worse overestimation appears in the spring and summer(27%–66%). However, the 3-km and 10-km products over different surfaces still exhibit obvious deviations. The 10-km product performs better in the large cities, while the 3-km product has advantages in the suburbs. In urban areas, the percentage falling within EE of the 3-km AOD product(18%–59%) is lower than that for the 10-km AOD product(31%–69%). However, in suburban areas, the percentage falling within EE of the 3-km AOD product(61%–84%) is higher than for the 10 km AOD product(54%–83%).The percentages falling within EE differ considerably when the AOD is greater than1.5(73% and 63% for the 3-km and 10-km products, respectively). On the whole, the 3-km(10-km) AOD product performs better in suburban(urban) areas. 展开更多
关键词 aerosol urban agglomeration MODIS AOD
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Contrasting Characteristics of the Surface Energy Balance between the Urban and Rural Areas of Beijing 被引量:9
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作者 WANG Linlin GAO Zhiqiu +4 位作者 MIAO Shiguang GUO Xiaofeng SUN Ting Maofeng LIU Dan LI 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2015年第4期505-514,共10页
A direct comparison of urban and rural surface energy balances, as well as a variety of other variables including incoming shortwave/longwave radiation and aerosol optical depth, is conducted for the Beijing metropoli... A direct comparison of urban and rural surface energy balances, as well as a variety of other variables including incoming shortwave/longwave radiation and aerosol optical depth, is conducted for the Beijing metropolitan area. The results indicate that, overall, the urban area receives a smaller amount of incoming shortwave radiation but a larger amount of incoming longwave radiation. However, comparisons in the aerosol optical depth and cloud fraction at the two locations suggest that neither aerosol optical depth nor cloud fraction alone can explain the difference in the incoming shortwave radiation. The urban–rural differences in the incoming longwave radiation are unlikely to be caused by the presence of more abundant greenhouse gases over the urban area, as suggested by some previous studies, given that water vapor is the most dominant greenhouse gas and precipitable water is found to be less in urban areas. The higher incoming longwave radiation observed over the urban area is mostly likely due to the higher temperatures of the ambient air. The urban area is also found to always produce higher sensible heat fluxes and lower latent heat fluxes in the growing season. Furthermore, the urban area is associated with a larger amount of available energy(the sum of sensible and latent heat fluxes) than the rural area, except in May and October when evapotranspiration in the rural area significantly exceeds that in the urban area. This study provides observational evidence of urban–rural contrasts in relevant energy-balance components that plausibly arise from urban–rural differences in atmospheric and land-surface conditions. 展开更多
关键词 aerosol load cloud evapotranspiration surface energy balance urbanization
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Simultaneous Monitoring of Nitrogen Dioxide and Aerosol Concentrations with Dual Path Differential Optical Absorption Spectroscopy 被引量:1
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作者 Hayato Saito Yutaro Goto +9 位作者 Yusaku Mabuchi Ilham Alimuddin Gerry Bagtasa Naohiro Manago Hitoshi Irie Ippei Harada Toshihiko Ishibashi Kazunori Yashiro Shumpei Kameyama Hiroaki Kuze 《Open Journal of Air Pollution》 2014年第1期20-32,共13页
Differential optical absorption spectroscopy (DOAS) is a useful technique for measuring nitrogen dioxide (NO2) and aerosol, the most important species in urban environmental pollution. This paper reports on the result... Differential optical absorption spectroscopy (DOAS) is a useful technique for measuring nitrogen dioxide (NO2) and aerosol, the most important species in urban environmental pollution. This paper reports on the results of our dual path DOAS measurements recently conducted in Chiba City, Japan, using xenon flashlights equipped on tall constructions as aviation obstruction lights. Because of the proximity of the southern DOAS path to an industrial area, it is found that the level of air pollution generally increases with the dominance of westerly winds, from the plausible source area to the observation light path. This situation is consistent with the result of wind lidar measurement covering a sector of ±28? with the observation range of approximately 2.8 km. In spite of the fact that the two DOAS paths, having path lengths of 5.5 and 3.5 km each, are located in separated regions of Chiba City, the observed temporal behavior was similar for both nitrogen dioxide and aerosol, though the southern path tends to exhibit slightly higher pollution levels than the northern counterpart. Additionally it is confirmed that size information of aerosol particles can be derived from the DOAS data through the analysis of the wavelength dependence of the aerosol optical thickness, which shows fairly good correlation with the mass ratio between PM2.5 and suspended particulate matter (SPM) obtained from the in-situ sampling station measurement. Thus, the DOAS approach can also be utilized for obtaining information on PM2.5 that is considered to be more harmful to human health than SPM. 展开更多
关键词 Differential Optical Absorption Spectroscopy (DOAS) WIND Lidar urban Air POLLUTION Nitrogen Dioxide aerosol PM2.5 SPM
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Applications of Satellite Data for Aerosol Optical Depth (AOD) Retrievals and Validation with AERONET Data
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作者 Sunil Bhaskaran Neal Phillip +1 位作者 Atiqur Rahman Javed Mallick 《Atmospheric and Climate Sciences》 2011年第2期61-67,共7页
An understanding of the amount and type of aerosols present in the atmosphere is required for the atmospheric correction of satellite imagery. A sensitivity analysis of the atmospheric inputs to the MOD09 software has... An understanding of the amount and type of aerosols present in the atmosphere is required for the atmospheric correction of satellite imagery. A sensitivity analysis of the atmospheric inputs to the MOD09 software has shown that uncertainty in the estimation of Aerosol Optical Depth (AOD) has the greatest impact on the accuracy of atmospheric correction of MODIS data. The MOD09 software used for the generation of surface reflectance products estimates the AOD of the atmosphere at the time of image acquisition. AOD measurements retrieved from MODIS were compared with near-simultaneous AErosol RObotic NETwork (AERONET) data over three sites in Australia, using time-series of MODIS surface reflectance products. The results of the study provide an important independent validation of ACRES MODIS Surface Reflectance Products. This procedure may be applied to long time series MODIS data for estimating the accuracy of MOD09 retrieved AOD. 展开更多
关键词 aerosol Optical DEPTH MODIS DATA urban Area
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城市污水厂病毒气溶胶逸散特征研究现状与未来展望
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作者 王莹 韩云平 +4 位作者 李琳 李衍博 李慧丽 颜昌仁 李彩侠 《化工进展》 EI CAS CSCD 北大核心 2023年第S01期439-446,共8页
近年来,大规模病毒传染性疾病的频繁爆发已引起全世界关于气载致病微生物的重点关注,尤其是不同人为源病毒气溶胶的产生及逸散过程。本文通过综述近年来污水处理厂病毒气溶胶的逸散浓度、主要种群及关键逸散点源,重点分析了病毒气溶胶... 近年来,大规模病毒传染性疾病的频繁爆发已引起全世界关于气载致病微生物的重点关注,尤其是不同人为源病毒气溶胶的产生及逸散过程。本文通过综述近年来污水处理厂病毒气溶胶的逸散浓度、主要种群及关键逸散点源,重点分析了病毒气溶胶与生物气溶胶逸散之间的相互关系及影响因素,探究了目前污水厂病毒气溶胶研究中存在的关键问题,并对未来研究趋势及方向进行了展望。结果发现,病毒气溶胶中的主要组分为诺如病毒和人腺病毒,其浓度存在较为明显的工艺单元及季节差异。污水污泥、污水厂的处理规模、运行状况及其所处的环境条件均是影响城市污水厂病毒气溶胶逸散的主要因素。同时,通过综述已有研究发现,目前针对城市污水厂病毒气溶胶的产生机制、扩散规律以及潜在风险评估还缺乏深入研究,也缺乏针对污水厂实际应用的有效控制措施,未来应在这些方面加强关注。 展开更多
关键词 污水处理厂 病毒 气溶胶 曝气 污染
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南京夏季气溶胶吸湿增长因子和云凝结核的观测研究 被引量:21
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作者 李琦 银燕 +5 位作者 顾雪松 袁亮 孔少飞 江琪 陈魁 李力 《中国环境科学》 EI CAS CSCD 北大核心 2015年第2期337-346,共10页
为了更加全面地研究长三角地区气溶胶的理化特性,尤其是吸湿和活化特性,于2013年8月在南京市区对气溶胶的吸湿增长因子(GF)和云凝结核(CCN)展开相关观测研究.使用串联电迁移率颗粒物吸湿粒径分析仪(H-TDMA)观测32~350nm气溶胶在... 为了更加全面地研究长三角地区气溶胶的理化特性,尤其是吸湿和活化特性,于2013年8月在南京市区对气溶胶的吸湿增长因子(GF)和云凝结核(CCN)展开相关观测研究.使用串联电迁移率颗粒物吸湿粒径分析仪(H-TDMA)观测32~350nm气溶胶在相对湿度为90%条件下的吸湿性参数,使用云凝结核计数器(CCNC)观测过饱和度在0.2%~0.8%的CCN数浓度.结果表明,不同气溶胶粒子的吸湿增长行为均表现出较为明显的双峰分布,即一个强吸湿模态和一个弱吸湿模态,且吸湿性在不同粒径(爱根核模态和积聚模态)上存在较为明显的不同,不溶性物质和二次气溶胶所占比重较大,并且在稳定的天气条件下,气溶胶的混合状态表现为由外混向内混发展的过程.观测期间该区域CCN的平均数浓度为13776(0.6%)cm-3,比沿海区、山区、干旱地区及清洁城市地区要高很多.其日变化表现为中午时刻出现峰值,影响因素主要与光化学反应有关.同时25日出现的轻雾过程对CCN有较为明显的清除作用.通过吸湿性参数计算得到的CCN数浓度和实际观测得到的CCN数浓度进行了闭合实验,结果显示出较好的相关性,表明将未饱和条件下观测得到的吸湿性参数带入到K?hler方程中,即可预测过饱和条件下气溶胶的活化能力. 展开更多
关键词 南京市 城市气溶胶 吸湿增长 云凝结核
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中国北方气溶胶散射和PM_(10)浓度特征 被引量:33
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作者 延昊 矫梅燕 +2 位作者 赵琳娜 张志刚 牛若芸 《高原气象》 CSCD 北大核心 2008年第4期852-858,共7页
利用积分浊度计和PM10浓度监测仪,对中国北方2005年观测的气溶胶散射系数σsp与可吸入颗粒物PM10质量浓度的分析表明,张北站σsp年均值为130 Mm-1,民勤站σsp年均值为116 Mm-1;四季中都是冬季均值最高,张北站sσp为301.6 Mm-1,民勤站σs... 利用积分浊度计和PM10浓度监测仪,对中国北方2005年观测的气溶胶散射系数σsp与可吸入颗粒物PM10质量浓度的分析表明,张北站σsp年均值为130 Mm-1,民勤站σsp年均值为116 Mm-1;四季中都是冬季均值最高,张北站sσp为301.6 Mm-1,民勤站σsp为170.9 Mm-1,这说明张北站的气溶胶散射情况比民勤站显著。而PM10浓度反映了不同的变化规律,张北站PM10年均值为53μg.m-3,民勤站PM10年均值为130μg.m-3;四季中都是春季均值最高,张北站PM10为82.2μg.m-3,民勤站PM10为190.1μg.m-3,这说明民勤站的PM10污染比张北站严重很多。张北站的质量散射效率α年均值为2.4 m2.g-1,民勤站的α年均值为1.1 m2.g-1,这与张北站全年主要受城市污染型气溶胶的影响,而民勤站全年主要受沙尘气溶胶的影响有密切关系。α具有反映中国北方两种典型气溶胶的能力。 展开更多
关键词 中国北方 积分浊度计 可吸入颗粒物 沙尘气溶胶 城市污染型气溶胶
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从雾的气候变化看城市发展对雾的影响 被引量:37
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作者 石春娥 杨军 +2 位作者 邱明燕 谢伟 张浩 《气候与环境研究》 CSCD 北大核心 2008年第3期327-336,共10页
利用安徽省78个测站近半个世纪的资料分析了安徽雾的年代际变化特征,并着重讨论了城市发展对雾的影响。安徽省雾的年代际变化趋势分布不均匀,以1980年为中心的10年是安徽年均雾日数最高的10年,以后呈减少趋势。根据两类城市年雾日数演... 利用安徽省78个测站近半个世纪的资料分析了安徽雾的年代际变化特征,并着重讨论了城市发展对雾的影响。安徽省雾的年代际变化趋势分布不均匀,以1980年为中心的10年是安徽年均雾日数最高的10年,以后呈减少趋势。根据两类城市年雾日数演变趋势,揭示城市在不同的发展阶段对雾的影响不同。最近30年,城市雾的消散时间明显推后,平均持续时间增加,雾内能见度下降。1985年之后,全省平均雾日数和合肥地区北京时间8时雾内能见距离与全省煤耗量之间存在显著的反相关。城市雾发生率下降的原因可能是城市热岛加强和大气气溶胶粒子增多共同作用的结果。 展开更多
关键词 年代际变化 城市发展 城市气候 大气气溶胶
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城市大气气溶胶的物理化学特性及其对人体健康的影响 被引量:63
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作者 任丽新 游荣高 +2 位作者 吕位秀 张文 王秀玲 《气候与环境研究》 CSCD 1999年第1期67-73,共7页
根据在北京、重庆、上海等城市大气气溶胶的观测结果和气溶胶中有机化学成分的有关资料,分析城市地区大气气溶胶的浓度、尺度谱分布、日变化规律及其化学成分的谱分布特征,并与干净地区的结果作比较,进而探讨了大气气溶胶对人体健康... 根据在北京、重庆、上海等城市大气气溶胶的观测结果和气溶胶中有机化学成分的有关资料,分析城市地区大气气溶胶的浓度、尺度谱分布、日变化规律及其化学成分的谱分布特征,并与干净地区的结果作比较,进而探讨了大气气溶胶对人体健康的影响。 展开更多
关键词 城市 大气气溶胶 人体健康
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城市气溶胶对太阳辐射的影响及其在边界层温度变化中的反映 被引量:21
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作者 王海啸 黄建国 陈长和 《气象学报》 CSCD 北大核心 1993年第4期457-464,共8页
本文利用冬季观测的兰州市区、邻近山顶以及郊区皋兰县的辐射资料和温度廓线资料,分析了兰州城市气溶胶对太阳辐射影响;并用二流近似累加法计算了低层大气吸收太阳辐射的加热率,其结果与低层大气上部的实际增温在数值上比较接近。分析... 本文利用冬季观测的兰州市区、邻近山顶以及郊区皋兰县的辐射资料和温度廓线资料,分析了兰州城市气溶胶对太阳辐射影响;并用二流近似累加法计算了低层大气吸收太阳辐射的加热率,其结果与低层大气上部的实际增温在数值上比较接近。分析了城市气溶胶短波辐射效应对边界层温度廓线分布的影响。表明城市烟雾层削弱了地面热通量但增加了低层大气中上部的增温,从而增加了城市低层大气的稳定度。 展开更多
关键词 城市 气溶胶 边界层 温度 太阳辐射
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Quantitative relationship between visibility and mass concentration of PM2.5 in Beijing 被引量:31
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作者 WANG Jing-li ZHANG Yuan-hang +4 位作者 SHAO Min LIU Xu-lin ZENG Li-min CHENG Cong-lan XU Xiao-feng 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2006年第3期475-481,共7页
The pollution of particulate matter less than 2.5μm (PM2.5) is a serious environmental problem in Beijing. The annual average concentration of PM2.5 in 2001 from seasonal monitor results was more than 6 times that ... The pollution of particulate matter less than 2.5μm (PM2.5) is a serious environmental problem in Beijing. The annual average concentration of PM2.5 in 2001 from seasonal monitor results was more than 6 times that of the U,S, national ambient air quality standards proposed by U.S. EPA. The major contributors to mass of PM2.5 were organics, crustal elements and sulfate. The chemical composition of PM2.5 varied largely with season, but was similar at different monitor stations in the same season. The fine particles (PM2.5) cause atmospheric visibility deterioration through light extinction, The mass concentrations of PM2.5 were anti-correlated to the visibility, the best fits between atmospheric visibility and the mass concentrations of PM2.5 were somehow different: power in spring, exponential in summer, logarithmic in autumn, power or exponential in winter. As in each season the meteorological parameters such as air temperature and relative humidity change from day to day, probably the reason of above correlations between PM2.5 and visibility obtained at different seasons come from the differences in chemical compositions of PM2.5. 展开更多
关键词 PM2.5 atmospheric urban aerosol air pollution meteorological factor VISIBILITY
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用MODIS反演北京城市地区地表反照率精度以及算法改进 被引量:7
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作者 王开存 王建凯 +1 位作者 王普才 陈洪滨 《大气科学》 CSCD 北大核心 2008年第1期67-74,共8页
MODIS(MODerate-resolution Imaging Spectroradiometer)地表反照率的精度在乡村地区已经得到了检验,但是至今没有在城市地区的有关研究。地表反照率的精度在很大程度上取决于大气订正的精度,作者利用2002年以来的北京AERONET(国际气溶... MODIS(MODerate-resolution Imaging Spectroradiometer)地表反照率的精度在乡村地区已经得到了检验,但是至今没有在城市地区的有关研究。地表反照率的精度在很大程度上取决于大气订正的精度,作者利用2002年以来的北京AERONET(国际气溶胶检测网络)站点Cimel气溶胶观测资料对反射率进行大气订正,通过对比来评价MODIS地表反照率算法中大气订正的精度。结果发现,MODIS大气订正在蓝光波段具有明显的过度订正现象,MODIS大气订正后地表反射率平均偏低0.03。MODIS地表反照率在冬季有约75%的缺测,这是因为冬季严重的空气污染使得MODIS云检测得到晴空观测较少。MODIS使用三参数双向反射率函数(BRDF)要求16天以内至少有3次以上的晴空观测(MODIS算法中要求7次)。通过分析MODIS反演得到的三参数,发现虽然它们的绝对值具有明显的季节变化,但是它们的比值是十分稳定的,这样使BRDF函数降低到只需要一个参数,有效降低了对晴空观测次数的要求,这一思想可以应用到热带等晴空日数较少的地区。 展开更多
关键词 地表反照率 城市地区 气溶胶 双向反射率函数 北京
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采暖期前后兰州城市气溶胶光学特性变化特征 被引量:14
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作者 张婕 刘海文 +1 位作者 肖国杰 冯婉 《干旱气象》 2012年第2期178-181,248,共5页
利用兰州市2003~2004年采暖期前后,大气气溶胶散射系数和光学厚度(AOD)观测资料,结合同期的环境质量常规监测资料,分析了该地区大气气溶胶性质变化特征及其与空气污染的关系。结果表明:兰州市总散射系数和后向散射系数采暖期具有明显的... 利用兰州市2003~2004年采暖期前后,大气气溶胶散射系数和光学厚度(AOD)观测资料,结合同期的环境质量常规监测资料,分析了该地区大气气溶胶性质变化特征及其与空气污染的关系。结果表明:兰州市总散射系数和后向散射系数采暖期具有明显的3峰变化,非采暖期呈双峰变化。采暖期和非采暖期绿光通道总散射系数最大值与最小值之比分别为1.66和3.51;采暖期光学厚度远大于非采暖期,光学厚度和总散射系数具有较好的相关性,相关系数为0.483;气溶胶的后向散射比日间变化随季节不同而改变;AOD与空气污染指数(API)、可吸入颗粒物(PM10)的变化在大多数情况下具有很好的相关性,AOD与PM10变化趋势基本相同,但其浓度值采暖期要高于非采暖期,而且两者之间的比值采暖期要大于非采暖期。 展开更多
关键词 城市气溶胶 采暖期 非采暖期 光学特性 空气污染
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南京细颗粒物对城市热岛强度的影响 被引量:15
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作者 吴昊 王体健 +5 位作者 方欢 马亚平 韩永秋 黄澍 姚宇昂 史均清 《大气科学学报》 CSCD 北大核心 2014年第4期425-431,共7页
随着城市化和工业化进程的加快,南京城市热岛效应显著,细颗粒物污染加剧,对大气环境、气候变化和人体健康产生重要影响。本文基于观测资料,分析了南京市不同颗粒物浓度水平下城市热岛强度的变化特征;利用光学特性模型OPAC(optical prope... 随着城市化和工业化进程的加快,南京城市热岛效应显著,细颗粒物污染加剧,对大气环境、气候变化和人体健康产生重要影响。本文基于观测资料,分析了南京市不同颗粒物浓度水平下城市热岛强度的变化特征;利用光学特性模型OPAC(optical properties of aerosols and clouds model)和辐射传输模型TUV(troposphere ultraviolet-visible model)估计了气溶胶的光学厚度及辐射强迫;定量分析了细颗粒物对城市热岛强度的影响及其可能机制。结果表明:南京城市热岛强度范围为-0.5~1.3K,冬季强于夏季。细颗粒物质量浓度范围为32~135μg/m3,冬季高于夏季,城区和郊区差别不大;当大气中细颗粒物质量浓度较高时,城市热岛强度相对较弱;南京城郊气溶胶光学厚度变化范围为0.28~1.01,在地面产生的辐射强迫达-3.88^-4.72 W·m-2;由于城区和郊区下垫面、人为热、细颗粒物浓度水平的差异,造成城郊近地面降温的不同,导致细颗粒物对城市热岛强度的削弱,夏季减弱0.1 K,冬季减弱0.2 K。 展开更多
关键词 城市热岛 气溶胶 细颗粒物 辐射强迫 南京
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